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Publications authored/co-authored by staff of the Nuclear Data Section
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Extension of recommended cross section database for production of therapeutic isotopes |
F. Tarkanyi, A. Hermanne, A. V. Ignatyuk, F. Ditroi, S. Takacs, R. Capote Noy, J. Radioanal. Nucl. Chem. 333 (2024) pp. 717-804. doi:10.1007/s10967-023-09283-8 |
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Extension of evaluated cross section database for charged particle monitor reactions |
F. Tarkanyi, A. Hermanne, A. V. Ignatyuk, F. Ditroi, S. Takacs, R. Capote-Noy, J. Radioanal. Nucl. Chem. 333 (2024) pp. 4243-4331. doi:10.1007/s10967-024-09513-7 |
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Examination of static fission properties of 236U and233Th using Cassinian oval parametrization within the macroscopic?microscopic approach |
P. Jachimowicz, R. Capote and M. Kowal, Eur. Phys. J. A 60 (2024) 160. doi:10.1140/epja/s10050-024-01381-9 |
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Benchmarking of Stainless Steel Cube Neutron Leakage in Research Center Rez [Abstract] |
Michal Kostal,..., Roberto Capote, et al., Nucl. Sci. Eng. 198 (2024) pp. 399-410. doi:10.1080/00295639.2023.2206770 |
Abstract Integral experiments covering neutron leakage from geometrically simple assemblies with a 252Cf
source inside are very valuable tools usable in the validation of transport cross-section data since geometric
uncertainties play a much smaller role in simple geometric assemblies than in complex assemblies as for
example reactor pressure vessel geometry. Since 252Cf spontaneous fission is a standard neutron source, the
uncertainties connected with the source neutron spectrum can be even neglected. The paper refers to validation
efforts of neutron leakage from an ~50 � 50 � 50-cm stainless steel block in the Research Center Rez. Both the
neutron leakage flux at a distance of 1 m from the center of the cubical assembly using stilbene spectrometry and
activation rates at different positions of the assembly were evaluated. In addition to experiments, main sources of
uncertainty were identified and evaluated. The results of the stilbene measurements are consistent with the
activation measurement results. | |
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Broomstick experiment with copper in VR-1 reactor [Abstract] |
Michal Kostal,..., Roberto Capote, et al., Ann. Nucl. Energy 211 (2024) 110993. |
Abstract Copper is an important structural material used in nuclear technology, often used as a cover for spent fuel
canisters or planned to be used in fusion devices. Despite its significance, there is a lack of integral experiments
useful for validating and improving the evaluations of copper nuclear data. To address this gap, a neutron
leakage experiment was conducted a few years ago using a point 252Cf(s.f.) neutron source placed inside a large
block of copper. In this work a pencil beam transmission-attenuation experiment (a broomstick) employing
various thicknesses (5?20 cm) of copper blocks (cylinders of 6 cm in diameter) was undertaken to expand the
dataset of available experiments for copper in the fast neutron energy range (1?10 MeV). This type of experiment
has the highest sensitivity to the total cross sections, and sensitivities are different from other integral experiments,
making it a complementary measurement to already existing integral data. The measurement was performed
using stilbene scintillation spectrometry. Measured transmission shows that the current INDEN
evaluation, proposed to be adopted for ENDF/B-VIII.1 and JEFF-4 libraries, exhibits excellent agreement with
experimental data. The JEFF-3.3 evaluation displays significant discrepancies, consistent with previous results
from integral experiments involving copper. In the case of JENDL-5, discrepancies were found in the energy
region 1.7?4.9 MeV. | |
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High-energy neutron emission in thermal neutron-induced fission of 235U |
Martin Schulc,...,Roberto Capote, et al., Phys. Rev. C 109 (2024) 054616. doi:10.1103/PhysRevC.109.054616 |
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Measurement of spectrum averaged cross sections in LR-0 benchmark
reference neutron field [Abstract] |
Michal Kostal,..., Roberto Capote, et al., Ann. Nucl. Energy 206 (2024) 110616. doi:10.1016/j.anucene.2024.110616 |
Abstract The measured and evaluated excitation functions are fundamental quantities that affect the accuracy of all
calculations in nuclear applications. Some cross sections, such as 14N(n,p)14C, have added value for special
applications, as these reactions may be responsible for possible contamination in industrial processes such as
spent fuel reprocessing. For the validation of the evaluated cross sections, we can rely on the comparison of the
calculated spectrum averaged cross sections (SACS) for the given neutron spectrum with the measured SACS
value. The benchmark reference neutron field has been identified, characterized, and well validated in the LR-
0 special core. A very large set of SACS measurements in the LR-0 reference field is measured with low uncertainty,
making it an excellent set for deconvolution codes? validation. The impact of the gamma-induced reaction
on the production yield of neutron-induced reactions was investigated for most of the benchmarked reactions.
Gamma competition was found to contribute at most 1 % for the 197Au(n,2n) reaction, while being substantially
lower for other target isotopes and neutron-induced activation reactions. | |
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Looking for integral references for the fission cross sections in actinides above 1 MeV [Abstract] |
Ignacio Duran, Roberto Capote and Georg Schnabel, EPJ Web of Conferences 294 (2024) 04001. doi:10.1016/j.nds.2024.01.004 |
Abstract One of the most important sources of systematic uncertainties in the evaluation of measured cross sections is the absolute normalization of every dataset, which were often performed by measuring simultaneously the reference cross-section of the standard isotope. In other experiments the shape of the cross-section spectrum is normalized using as reference the integral value in a certain energy interval taken from an evaluated library. The choice of the energy interval used as reference has been often left up to the experimentalist criteria, leading to inconsistent normalizations and hardly assessable uncertainties. In this work the experimental datasets of the (n,f) cross section of many actinides are reviewed looking for the best suited energy interval to be recommended for renormalization purposes. Using standard integration intervals, wide enough to get very low statistical uncertainties, should improve the normalization of every experimental dataset, reducing so the associated total uncertainty when making the evaluation. A common integration range from 8 to 10 MeV is proposed for the whole set of actinides needed in fission applications. This energy range, which falls between the second and the third fission-chance thresholds, is characterized by a flat behaviour of the fission cross sections. | |
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Monte Carlo evaluation of the semiclassical multi-step direct reaction series [Abstract] |
Brett V. Carlson, Emanuel V. Chimanski and Roberto Capote, EPJ Web of Conferences 292 (2024) 04004. doi:10.1051/epjconf/202429204004 |
Abstract We show how the multi-step direct reaction series can be evaluated
using Monte Carlo methods. Nucleon-nucleon collisions occur according to the
random selection of a nucleon?s attenuation factor along its classical trajectory.
The particles and hole excited in a collision are selected from a local Fermi
distribution. We assume that the particles continue to propagate and possibly
collide again before leaving the nucleus. We assume that holes collide in place,
to possibly produce other particles and holes. | |
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Microscopic modeling of direct pre-equilibrium emission: impact on exclusive and inclusive (n,xn) and fission channels [Abstract] |
M. Dupuis, R. Capote, et al., EPJ Web of Conferences 292 (2024) 04003. doi:10.1051/epjconf/202429204003 |
Abstract We report on a microscopic modeling of the first order of multistep
direct emission based on one phonon excitations, given by the QRPA model,
and an effective in-medium nucleon nucleon interaction, described within the
JLM folding model. The results of our coupled channels framework for deformed
target are illustrated in the case of low energy discrete state excitations
in 152Sm. Pre-equilibrium predictions and their impact on inclusive and exclusive
(n,xn) cross sections and fission cross sections are discussed for actinides.
We discuss the importance of i) collective excitations to describe the neutron
emission spectra and of ii) spin distribution of the residual nucleus formed after
the neutron pre-equilibrium emission, that is a key ingredient to model the
residual nucleus decay. | |
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Activation cross-sections of proton-induced nuclear reactions on natural zinc in the energy range of 4-30 MeV [Abstract] |
M.U. Khandaker, H. Haba, A. R. Usman, M. Mahmoud, N. Otuka, S.K.I. Ali, Radiat. Phys. Chem. 226 (2025) 112272. doi:10.1016/j.radphyschem.2024.112272 |
Abstract In the present work, the excitation functions for the proton-induced nuclear reactions on natural zinc were measured in the energy range of 4?30 MeV using the well-established stacked-foil activation procedure. The activation products were measured based on their characteristic gamma lines using HPGe gamma-ray spectrometry. The radioactivities determined were used for the calculation of cross-sections of the radionuclides of interest, i.e., 61Cu, 62,65,69mZn, 57Co and 66,67,68Ga. The cross-sections have also been compared with the available literature data and the theoretical prediction of the TALYS code via its latest TENDL-2023 library as well as the prediction of EMPIRE-3.2.2 model code. The results show a reasonable agreement when compared with the available literature data. This work, however, shows that the theoretical data extracted from the TENDL-2023 library and EMPIRE-3.2.2 default calculation significantly underestimate the experimental cross-sections of 57Co nuclide while they overestimate those of 69mZn. The present result has potential applications to improve the predicting capability of the model codes as well as to serve as additional data for the nuclear reaction cross-section database. | |
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Isomer production studied with simultaneous decay curve analysis for alpha-particle induced reactions on natural platinum up to 29 MeV [Abstract] |
N. Otuka, S. Takács, M. Aikawa, S. Ebata, H. Haba, Eur. Phys. J. A 60 (2024) 195. doi:10.1140/epja/s10050-024-01383-7 |
Abstract The isomeric ratios of 198Au, 197Hg and 195Hg produced by alpha-particle induced reactions on natural platinum were investigated experimentally up to 29 MeV by using the standard stacked foil activation technique and gamma-ray spectrometry. The isomeric ratios of 197Hg and 195Hg determined by the conventional activation cross section formula showed strong cooling time dependence. The time dependence was resolved by adjusting the isomeric transition branching ratios for the two isotopes within a simultaneous decay curve analysis framework. Our analysis suggests 94.5 � 0.7% and 48.9 � 1.8% as the isomeric transition branching ratios of 197mHg (24 h) and 195mHg (42 h), respectively. The isomeric ratios and independent production cross sections of 198Au, 197Hg, 195Hg and some other Hg, Au and Pt isotopes were also measured down to 6 MeV with these corrected isomeric transition branching ratios, and compared with predictions of statistical and pre-equilibrium models by TALYS-2.0 to discuss spin cutoff parameter dependence. We found the measured isomeric ratios are better predicted if we reduce the spin cutoff parameter to half or less from that estimated with the rigid body moment of inertia. | |
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X4Pro - universal, fully relational EXFOR database [Abstract] |
V. Zerkin, EPJ Web of Conferences 284 (2023) 14015. doi:10.1051/epjconf/202328414015 |
Abstract EXFOR library contains experimental reaction data compiled by the Nuclear Reaction Data
Centers (NRDC) since 1970 and presenting data from more than 25,000 experiments in the EXFOR format
with associated dictionaries and documentation. The IAEA-NDS provides nuclear data services primarily
through computer systems built on relational databases and retrieval software. X4Pro is an extended EXFOR
relational database designed for programmatic access to whole EXFOR content and distributed as local
SQLite database with demo-codes in Python and Fortran. | |
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Excitation functions of helion-induced nuclear reactions on natural copper up to 55 MeV [Abstract] |
M.U. Khandaker, K. Nagatsu, K. Minegishi, M.R. Zhang, M. Mahmoud, S.K.I. Ali, N. Otuka doi:10.1016/j.radphyschem.2024.111999 |
Abstract Excitation functions for the natCu(3He,x)66,67Ga,62,65Zn,61,64Cu and 56,57,58,60Co nuclear reactions were measured from the respective threshold up to 55 MeV incident energy by using the conventional stacked foil activation technique combined with HPGe gamma-ray spectrometry. Independent cross-sections for the natCu(3He,x)62Zn and 61,64Cu reactions are reported here for the first time in the energy region of 35-53 MeV. Measured data were critically compared with the relevant earlier experimental data and also with the theoretical data obtained from the model calculations. Present results confirmed some of the previous experimental data, whereas only a partial agreement was found with the evaluated data in the TENDL-2023 library and data calculated by Empire-3.2 code. Such discrepancies indicate that the nuclear reaction sub-models and parameters adopted in the codes were insufficient to accurately characterize the reactions under investigation. The measured cross-sections were used to infer the physical thick target yields for the reaction products under investigation. The measured data are useful for reducing the existing discrepancies in the literature, improving the nuclear reaction model codes, and enriching the experimental database for various other applications including medical isotope production, thin layer activation analysis, etc. | |
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Activation cross sections of 7Li-induced reactions on natCu for
monitor reactions [Abstract] |
M. Aikawa, S. Goto, D. Gantumur, D. Ichinkhorloo, N. Ukon, N. Otuka, S. Tak?cs, H. Haba, Nucl. Instrum. Meth. B 554 (2024) 165441. doi:10.1016/j.nimb.2024.165441 |
Abstract Activation cross sections of 7Li-induced reactions on natCu were measured in order to investigate suitability of
some reactions for monitoring experimental parameters. Cross sections producing 69,68Ge, 67,66Ga and 69m,65Zn were determined. Physical thick target yields were experimentally measured and compared with those calculated
using the measured cross sections. The measured cross sections were verified by the agreements between the
directly measured thick target yields and the thick target yields deduced from the measured cross sections. The
7Li-induced reactions on natCu for the production of 67,66Ga and 65Zn are suggested as monitor reactions. | |
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Distribution of Tritium in the Near Surface of Candidate Structural Materials for Fusion Reactors. Type 304L Stainless Steel, Inconel, Hastelloy, Eurofer-97, Oxide Dispersion-Strengthened Alloy 14YWT [Abstract] |
J. O Callaghan,...K. Heinola, IEEE Trans. Plasma Sci. (2024). doi:10.1109/TPS.2024.3396645 |
Abstract Five different candidate structural materials for fusion have undergone pure tritium gas soaking at room temperature and at 310-mbar(a) pressure. The tritium uptake on the surface and in the bulk of the alloys has been analyzed using surface leaching, chemical etching, and thermal desorption. The nickel-based alloys: Inconel-X-750 and Hastelloy-X, absorbed the least amount of total tritium compared with austenitic stainless steel AISI 304L, reduced activation ferritic-martensitic (RAFM) Eurofer-97, and advanced nanoferritic alloy 14YWT. Microstructural analyses using electron backscatter diffraction (EBSD) indicate that the number of grains and mean grain size is not a dominant factor in near surface tritium uptake. The quantity of iron dissolved in the surface oxide appears to be the major factor in encouraging tritium absorption. | |
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Solubility of Hydrogen in a WMoTaNbV High-Entropy Alloy |
A. Liski,..., K. Heinola, Materials 17 (2024) 2574. doi:10.3390/ma17112574 |
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Characterization of a HPGe detector response for
activation cross section measurements: regression
method versus Monte Carlo method [Abstract] |
V. Semkova, N. Otuka and A.J. Plompen, J. Nucl. Sci. Technol. 61 No. 2 (2024) pp. 151-160. doi:https://doi.org/10.1080/00223131.2023.2278598 |
Abstract The full energy peak efficiencies and covariances of a high purity germanium (HPGe) detector
studied by the regression method and Monte Carlo method were compared. The impact of the
obtained results on the neutron activation cross-sections measured relative to monitor crosssections
was studied. In the regression method, the efficiencies measured for a set of calibration
point sources were analysed by the least-squares analysis. In the Monte Carlo method, the
efficiencies for the calibration point sources were calculated by MCNP. The covariances of the
efficiencies determined by the regression method were calculated analytically. Perturbation
analysis was performed to estimate the covariances of the efficiencies calculated by the Monte
Carlo method. Positive correlations higher than 0.8 were found in the uncertainties of the MCNP
data for point-like sources. In the case of the regression method, the correlation coefficient
contains both positive and negative terms. The efficiencies and their covariances for finite sample
geometry were also estimated by both methods to take into account sample effects such as
geometrical effect, and gamma-ray self-absorption, and found considerable differences in the
cross-sections and their uncertainties for reaction products quantified with low energy gammas.
The efficiencies and covariances were clearly affected by the properties of the sample. | |
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The IAEA electronic stopping power database: Modernization, review, and analysis of the existing experimental data |
C.C. Montanari, P. Dimitriou, L. Marian, A.M.P Mendez, J.P. Peralta, F. Bivort-Haiek, Nucl. Instrum. Methods Phys. Res. B 551 (2024) 165336. doi:10.1016/j.nimb.2024.165336 |
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Evaluated and recommended cross-section data for production of
radionuclides with emerging interest in nuclear medicine imaging. Part 1:
Positron emission tomography (PET) |
A. Hermanne, F.T. Tarkanyi, A.V. Ignatyuk, S. Takacs and R. Capote, Nucl. Instrum. Methods Phys. Res. B 535 (2023) pp. 149-192. doi:10.1016/j.nimb.2022.11.002 |
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Normalization of ToF (n,f) Measurements in Fissile Targets: Microscopic cross-section
integrals |
I. Duran, R. Capote and P. Cabanelas, Nucl. Data Sheets 193 (2024) pp. 95-104. doi:10.1016/j.nds.2024.01.004 |
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Evaluated and recommended cross section data for production of
radionuclides with emerging interest in nuclear medicine imaging. Part 2:
Single photon emission computed tomography (SPECT) |
A. Hermanne, F.T. Tarkanyi, A.V. Ignatyuk, S. Takacs and R. Capote, Nucl. Instrum. Methods Phys. Res. B 544 (2023) 165119. doi:10.1016/j.nimb.2023.165119 |
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Optical potentials for the rare-isotope beam era |
C. Hebborn, J.W. Holt, F.M. Nunes, M.C. Atkinson, G. Potel, W.H. Dickhoff, R.B. Baker, G. Blanchon, M. Burrows, C. Barbieri, R. Capote, P. Danielewicz, M. Dupuis,, Ch. Elster. J.E. Escher, L. Hlophe, A. Idini, H. Jayatissa. B.P. Kay, K. Kravvaris, J.J. Manfredi, A. Mercenne, B. Morillon, G.
Perdikakis, G.H. Sargsyan, C.D. Pruitt, I.J. Thompson, M. Vorabbi, T.R. Whitehead, J. Phys. G: Nucl. Part. Phys. 50 (2023) 060501. doi:10.1088/1361-6471/acc348 |
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Benchmarking of Stainless Steel Cube Neutron Leakage in Research Center Rez |
Michal Kostal, Zdenek Matej, Martin Schulc, Evzen Losa, Jan Simon, Evzen Novak, Frantisek Cvachovec, Vaclav Prenosil, Filip Mravec, Tomas Czakoj, Vojtech Rypar, Andrej Trkov, Roberto Capote, Nucl. Sci. Eng. 198 (2024) pp. 399-410. doi:10.1080/00295639.2023.2206770 |
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Dispersive optical model analysis of nucleon scattering on 90Zr |
X. Zhao, W. Du, R. Capote, E.Sh. Soukhovitskii, Phys. Rev. C 107 (2023) 064606. doi:10.1103/PhysRevC.107.064606 |
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Progress in the Evaluation and Validation of n+56,57Fe Cross Sections |
A. Trkov, R. Capote, D. Bernard, R. Beyer, Y. Danon, A. Daskalakis, A. Junghans, M. Kostal, P. Leconte, M. Schulc, S. Simakov, EPJ Web of Conferences 284 (2023) 12002. doi:10.1051/epjconf/202328412002 |
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Measurement of partial (n, n'gamma) reaction cross-sections on highly radioactive
nuclei of interest for energy production |
Francois Claeys, Philippe Dessagne, Maelle Kerveno, Cyrille De Saint Jean, Catalin Borcea, Marian Boromiza, Roberto Capote, Nicolas Dari Bako, Marc Dupuis, Greg Henning, Stephane Hilaire, Alexandru Negret, Gilles Noguere, Markus Nyman, Adina Olacel, Arjan Plompen, EPJ Web of Conferences 284 (2023) 01014. doi:10.1051/epjconf/202328401014 |
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GRAPhEME: performances, achievements (@EC-JRC/GELINA) and future (@GANIL/SPIRAL2/NFS) |
Maelle Kerveno, Catalin Borcea, Marian Boromiza, Roberto Capote, Francois Claeys, Nicolas Dari Bako, Cyrille De Saint Jean, Philippe Dessagne, Jean Claude Drohe, Marc Dupuis, Greg Henning, Stephane Hilaire, Toshihiko Kawano, Alexandru Negret, Markus Nyman, Adina Olacel, Carlos Paradela, Arjan Plompen, Ruud Wynants, EPJ Web of Conferences 284 (2023) 01005. doi:10.1051/epjconf/202328401005 |
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Measurement of 183W(n, n'gamma) and (n, 2ngamma) cross-sections (preliminary) |
Greg Henning, Kerveno Maelle, Philippe Dessagne, Francois Claeys, Nicolas Dari Bako, Marc Dupuis, Stephane Hilaire, Pascal Romain, Cyrille de Saint Jean, Roberto Capote, Marian Boromiza, Adina Olacel, Alexandru Negret, Catalin Borcea, Arjan Plompen, Carlos Paradela Dobarro, Markus Nyman, Jean-Claude Drohe, Ruud Wynants, EPJ Web of Conferences 284 (2023) 01046. doi:10.1051/epjconf/202328401046 |
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Using the Monte-Carlo method to analyze experimental data and produce uncertainties
and covariances. |
Greg Henning, Maelle Kerveno, Philippe Dessagne, Francois Claeys, Nicolas Dari Bako, Marc Dupuis, Stephane Hilaire, Pascal Romain, Cyrille de Saint Jean, Roberto Capote, Marian Boromiza, Adina Olacel, Alexandru Negret, Catalin Borcea, Arjan Plompen, Carlos Paradela Dobarro, Markus Nyman, Jean-Claude Drohe, Ruud Wynants, EPJ Web of Conferences 284 (2023) 01045. doi:10.1051/epjconf/202328401045 |
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Database work for the new cross section standards evaluation |
A. Carlson, R. Capote, D. Neudecker, V. Pronyaev, G. Schnabel, EPJ Web of Conferences 284 (2023) 14006. doi:10.1051/epjconf/202328414006 |
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From 232Th(n, n'gamma) cross sections to level production and total neutron inelastic
scattering cross sections |
Nicolas Dari Bako, Maelle Kerveno, Philippe Dessagne, Catalin Borcea, Marian Boromiza, Roberto Capote, Francois Claeys, Marc Dupuis, Greg Henning, Alexandru Negret, Markus Nyman, Adina Olacel, Eliot Party, Arjan Plompen, EPJ Web of Conferences 284 (2023) 08005. doi:10.1051/epjconf/202328408005 |
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Spectral averaged cross sections as a probe to a high energy tail of 235U PFNS |
Martin Schulc, Michal Kostal, Roberto Capote, Jan Simon, Tomas Czakoj, Evzen Novak, EPJ Web of Conferences 284 (2023) 04021. doi:10.1051/epjconf/202328404021 |
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On the need for precise nuclear structure data for high quality (n, n'gamma) cross section measurements |
Greg Henning, Maelle Kerveno, Philippe Dessagne, Francois Claeys, Nicolas Dari Bako, Marc Dupuis, Stephane Hilaire, Pascal Romain, Cyrille de Saint Jean, Roberto Capote, Marian Boromiza, Adina Olacel, Alexandru Negret, Catalin Borcea, Arjan Plompen, Carlos Paradela Dobarro, Markus Nyman, EPJ Web of Conferences 284 (2023) 01022. doi:/10.1051/epjconf/202328401022 |
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Experimental spectrum averaged cross sections (SACS) in 252Cf(sf) neutron field and its impact on the evaluation of neutron standards |
R. Capote, G. Schnabel, A.D. Carlson, V.G. Pronyaev, G. Noguere, D. Neudecker, EPJ Web of Conferences 281 (2023) 00027. doi:10.1051/epjconf/202328100027 |
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Cassini-oval description of the multidimensional potential energy surface for 236U: Role of octupole deformation and calculation of the most probable fission path |
K. Okada, T. Wada, R. Capote, N. Carjan, Phys. Rev. C 107 (2023) 034608. doi:10.1103/PhysRevC.107.034608 |
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Manhattan Project 1940s research on the prompt fission neutron spectrum |
M.B. Chadwick and R. Capote, Front. Phys. 11 (2023) 1105593. doi:10.3389/fphy.2023.1105593 |
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FENDL: A library for fusion research and applications [Abstract] |
G.Schnabel, D.L. Aldama, T. Bohm, U. Fischer, S. Kunieda, A. Trkov, C. Konno, R. Capote, A.J. Koning, S. Breidokaite, T. Eade, M. Fabbri, D. Flammini, L. Isolan, I. Kodeli, M. Kostal, S. Kwon, D. Laghi, D. Leichtle, S. Nakayama, M. Ohta, L.W. Packer, Y. Qiu, S. Sato, M. Sawan, M. Schulc, G.
Stankunas, M. Sumini, A. Valentine, R. Villari, A. Zohar, Nucl. Data Sheets 193 (2024) pp.1-78. doi:10.1016/j.nds.2024.01.001 |
Abstract The Fusion Evaluated Nuclear Data Library (FENDL) is a comprehensive and validated collection of nuclear cross section data coordinated by the International Atomic Energy Agency (IAEA) Nuclear Data Section (NDS). FENDL assembles the best nuclear data for fusion applications selected from available nuclear data libraries and has been under development for decades. FENDL contains sub-libraries for incident neutron, proton, and deuteron cross sections including general purpose and activation files used for particle transport and nuclide inventory calculations.
In this work, we describe the history, selection of evaluations for the various sub-libraries (neutron, proton, deuteron) with the focus on transport and reactor dosimetry applications, the processing of the nuclear data for application codes (e.g. MCNP), and the development of the TENDL-2017 library which is the currently recommended activation library for FENDL. We briefly describe the IAEA IRDFF library as the recommended library for dosimetry fusion applications. We also present work on validation of the neutron sub-library using a variety of fusion relevant computational and experimental benchmarks using the MCNP transport code and ACE-formatted cross section libraries. A variety of cross section libraries are used for the validation work including FENDL-2.1, FENDL-3.1d, FENDL-3.2, ENDF/B-VIII.0, and JEFF-3.2 with the emphasis on the FENDL libraries.
The results of the validation using computational benchmarks showed generally good agreement among the tested neutron cross section libraries for neutron flux, nuclear heating, and primary displacement damage (dpa). Gas production (H/He) in structural materials showed substantial differences to the reference FENDL-2.1 library. The results of the experimental validation showed that the performance of FENDL-3.2b is at least as good and in most cases better than FENDL-2.1.
Future work will consider improved evaluations developed by the International Nuclear Data Evaluation Network (INDEN) for materials such as O, Cu, W, Li, B, and F. Additionally, work will need to be done to investigate differences in gas production in structural materials. Covariance matrices will need to be developed or updated as availability of consistent and comprehensive uncertainty information will be needed as fusion technology and facility construction matures. Finally, additional validation work for high energy neutrons, protons and deuterons, as well as validation work for the activation library will be needed. | |
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Global comparison between experimentally measured isomeric yield ratios and nuclear model calculations [Abstract] |
S. Cannarozzo, S. Pomp, A. Al-Adili, A. Gook, A. Solders, A. Koning, Eur. J. Phys. A59 No. 12 (2023) 295. doi:10.1140/epja/s10050-023-01202-5 |
Abstract The level density steers transition probabilities between different states in the decay and de-excitation of excited nuclei. Reliable level density modelling is, therefore, key in describing, e.g., de-excitation of fission fragments, with implications on neutron and gamma-rays multiplicities, and also manifested in the population of isomeric states. We test six currently used level density models and the spin distribution in the level density by comparing calculations with measured isomeric yield ratios. The model calculations are performed with the TALYS code and experimental data for nuclear reactions populating spin isomers are retrieved from the EXFOR database. On average, calculations are in agreement with measured data. However, we find that the population of the high-spin state in an isomeric pair is clearly favoured in all of the six studied level density models. Further studies are then performed on the three used phenomenological level density models, to investigate the significance of their effect. We find that a significant reduction of the spin width distribution improves the agreement between calculated and experimentally observed isomeric yield ratios. This result is independent of the incident particle in the nuclear reaction. The needed reduction of the spin width distribution to comply with empirical data has, e.g., implications for studies in angular momentum generation in fission using isomeric yield rations, calculations of anti-neutrino spectra from nuclear reactors, as well as neutron and gamma-ray multiplicities in nuclear reactor calculations. | |
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Templates of Expected Measurement Uncertainties for (n,xn) Cross Sections [Abstract] |
Jeffrey R. Vanhoy, Robert C. Haight, Sally F. Hicks, Michal Herman, Arjan Koning, Keegan J. Kelly, Matthew Devlin, Ian Thompson, EPJ Nucl. Sci. Technol. 9 (2023) 31. doi:/10.1051/epjn/2023019 |
Abstract A template is provided for evaluating experimental uncertainties for neutron elastic and inelastic scattering cross sections and gamma-ray production cross sections from (n, xn) measurements at laboratories with monoenergetic or white neutron sources. A typical range of uncertainties is presented for experiments detecting the scattered neutrons or the resulting de-excitation gamma rays based on a survey of available data and input from many experimentalists and theorists with extensive knowledge in the field. Models commonly used to evaluate the resulting cross-sections are also discussed. Suggestions are made regarding what experimental and uncertainty information is needed for data evaluations and should be included when reporting experimental (n, xn) cross sections. Uncertainty values and correlations are recommended if these values cannot be estimated for past data from the literature. | |
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Templates of Expected Measurement Uncertainties [Abstract] |
Denise Neudecker, Amanda M. Lewis, Eric F. Matthews, Jeffrey Vanhoy, Robert C. Haight, Donald L. Smith, Patrick Talou, Stephen Croft, Allan D. Carlson, Bruce Pierson, Anton Wallner, Ali Al-Adili, Lee Bernstein, Roberto Capote, Matthew Devlin, Manfred Drosg, Dana L. Duke, Sean Finch, Michal W. Herman, Keegan J. Kelly, Arjan Koning, Amy E. Lovell, Paola Marini, Kristina Montoya, Gustavo P.A. Nobre, Mark Paris, Boris Pritychenko, Henrik Sjöstrand, Lucas Snyder, Vladimir Sobes, Andreas Solders, Julien Taieb, EPJ Nucl. Sci. Technol. 9 (2023) 35. doi:/10.1051/epjn/2023014 |
Abstract The covariance committee of CSEWG (Cross Section Evaluation Working Group) established templates of expected measurement uncertainties for neutron-induced total, (n,gamma), neutron-induced charged-particle, and (n,xn) reaction cross sections as well as prompt fission neutron spectra, average prompt and total fission neutron multiplicities, and fission yields. Templates provide a list of what uncertainty sources are expected for each measurement type and observable, and suggest typical ranges of these uncertainties and correlations based on a survey of experimental data, associated literature, and feedback from experimenters. Information needed to faithfully include the experimental data in the nuclear-data evaluation process is also provided. These templates could assist (a) experimenters and EXFOR compilers in delivering more complete uncertainties and measurement information relevant for evaluations of new experimental data, and (b) evaluators in achieving a more comprehensive uncertainty quantification for evaluation purposes. This effort might ultimately lead to more realistic evaluated covariances for nuclear-data applications. In this topical issue, we cover the templates coming out of this CSEWG effort?typically, one observable per paper. This paper here prefaces this topical issue by introducing the concept and mathematical framework of templates, discussing potential use cases, and giving an example of how they can be applied (estimating missing experimental uncertainties of 235U(n,f) average prompt fission neutron multiplicities), and their impact on nuclear-data evaluations. | |
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TALYS: modeling of nuclear reactions [Abstract] |
Arjan Koning, Stephane Hilaire and Stephane Goriely, Eur. J. of Phys. A59 (2023) 131. doi:10.1140/epja/s10050-023-01034-3 |
Abstract TALYS is a software package for the simulation of nuclear reactions below 200 MeV. It is used worldwide for the analysis and prediction of nuclear reactions and is based on state-of-art nuclear structure and nuclear reaction models. A general overview of the implemented physics and capabilities of TALYS is given. The general nuclear reaction mechanisms described are the optical model, direct reactions, compound nucleus model, pre-equilibrium reactions and fission. The most important nuclear structure models are those for masses, discrete levels, level densities, photon strength functions and fission barriers. A wide variety of nuclear reactions simulated with TALYS will be demonstrated, ranging from low-energy neutron cross sections, astrophysics, high-energy charged particle reactions and other reactions. TALYS is a nuclear reaction software which aims to give a complete description of nuclear reaction observables, and to be an important link between fundamental nuclear physics and applications. | |
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Compilation of isomeric ratios of light particle-induced nuclear reactions [Abstract] |
A. Rodrigo, N. Otuka, S. Takacs and A.J Koning, At. Nucl. Data Tables 153 (2023) 101583. doi:10.1016/j.adt.2023.101583 |
Abstract Experimental isomeric ratios of light (A
4) particle-induced nuclear reactions were compiled for the product nuclides having metastable states with half-lives longer than 0.1 s. The experimental isomeric ratio data were taken from the EXFOR library and reviewed. When an experiment reports isomer production cross sections instead of isomeric ratios, the cross sections taken from the EXFOR library were converted to the isomeric ratios by us. During compilation, questionable data (e.g., preliminary data compiled in EXFOR in parallel with their final data, sum of isomer production cross sections larger than the total production cross sections) were excluded. As an application of the new compilation, goodness-of-fit was studied for the isomeric ratios predicted by the reaction model code TALYS-1.96. A text file and plots of the compiled isomer production cross sections and isomeric ratios are provided as supplemental materials. | |
|
STEK: A potential fast spectrum benchmark for fission product cross sections [Abstract] |
Steven van der Marck and Arjan Koning, Front. Energy Res. 11 (2023) 1085857. doi:/10.3389/fenrg.2023.1085857 |
Abstract The reactivity worth of many fission product samples was measured in fast spectrum conditions in the STEK facility during the early 1970s. These results were then used to improve and validate nuclear data evaluations for fission products, but in the last 2 decades STEK has not been used: the nuclear data evaluations for fission products in the current versions of libraries like ENDF/B or JEFF have not been tested against STEK results. Here we argue that the STEK data are still valuable, because there is no other data set that can replace them, and the interest in fast spectrum conditions is picking up strongly of late. It should be considered to evaluate whether a benchmark can be defined for the International Reactor Physics Experiments Handbook. | |
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Second Report of the Nuclear Data Charge Subcommittee of the Nuclear Science Advisory Committee |
L. Bernstein, A. Koning, et al., Lawrence Livermore Report LLNL-TR-845408 (2023). |
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CollisionDB: A New Database of Atomic and Molecular Collisional Processes with an Interactive API [Abstract] |
C. Hill, Dipti, K.Heinola, M. Hanicinec, Atoms 12 No. 4 (2024) 20. doi:/10.3390/atoms12040020 |
Abstract The Atomic and Molecular Data Unit of the International Atomic Energy Agency has developed a new database, CollisionDB, to provide an open, free, robust and long-term repository of data on plasma collisional processes. The database contains data on cross sections and rate coefficients for collisions of electrons, photons and heavy particles with atomic and molecular species. A fundamental requirement for this database is the implementation of standardized metadata, which provide an unambiguous description of the collisional data available in peer-reviewed sources. CollisionDB offers both a browser-based search interface and an application programming interface (API) that allows users to filter, process and compare collisional datasets. For this purpose, a Python package PyCollisionDB has been developed to access the CollisionDB API. Here, we present an overview of the technical developments, including data schemas, standards and user interface underlying the CollisionDB application, with particular emphasis on the API developed to support the integration of data into modeling and other codes. | |
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Atomic and Molecular Databases Open Science for a sustainable world [Abstract] |
M.L. Dubernet, C. Hill, et al., Proc. Int. Astronomical Union 18 S371 (2024) 72. doi:10.1017/S1743921323000261 |
Abstract The building of online atomic and molecular databases for astrophysics and for other research fields started with the beginning of the internet. These databases have encompassed different forms: databases of individual research groups exposing their own data, databases providing collected data from the refereed literature, databases providing evaluated compilations, databases providing repositories for individuals to deposit their data, and so on. They were, and are, the replacement for literature compilations with the goal of providing more complete and in particular easily accessible data services to the users communities. Such initiatives involve not only scientific work on the data, but also the characterization of data, which comes with the ?standardization? of metadata and of the relations between metadata, as recently developed in different communities. This contribution aims at providing a representative overview of the atomic and molecular databases ecosystem, which is available to the astrophysical community and addresses different issues linked to the use and management of data and databases. The information provided in this paper is related to the keynote lecture ?Atomic and Molecular Databases: Open Science for better science and a sustainable world? whose slides can be found at DOI : doi.org/10.5281/zenodo.6979352 on the Zenodo repository connected to the ?cb5-labastro? Zenodo Community (https://zenodo.org/communities/cb5-labastro).
| |
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Recommended electron-impact excitation and ionization cross sections for Be II [Abstract] |
Dipti, I. Bray, D. V. Fursa, C. Hill, Yu. Ralchenko, At. Data and Nucl. Data Tables 156 (2024) 101634. doi:10.1016/j.adt.2023.101634 |
Abstract An overview of the current status of electron-impact excitation and ionization cross sections for Be II is given and the recommended data sets for use in plasma modeling are presented. Accurate cross sections between the lowest 14 atomic terms of
configurations are calculated with the convergent close-coupling (CCC) method and compared with the available experimental and theoretical results. The recommended electron-impact excitation and ionization cross sections are represented by analytical fitting functions that preserve correct asymptotic behavior. Uncertainties in the recommended data sets are determined by assessing the accuracy of the target structures, the convergence in the subsequent collisional calculations, and the fitting method. They are well within 15 % for most of the transitions. The fitting coefficients for 91 excitation cross sections and 14 ionization cross sections are provided for use in plasma modeling simulations. | |
|
2022 Review of Data-Driven Plasma Science [Abstract] |
R. Anirudh, C. Hill, et al., IEEE Transactions on Plasma Science 51 (2023) pp. 1750-1838. doi:10.1109/TPS.2023.3268170 |
Abstract Data-driven science and technology offer transformative tools and methods to science. This review article highlights the latest development and progress in the interdisciplinary field of data-driven plasma science (DDPS), i.e., plasma science whose progress is driven strongly by data and data analyses. Plasma is considered to be the most ubiquitous form of observable matter in the universe. Data associated with plasmas can, therefore, cover extremely large spatial and temporal scales, and often provide essential information for other scientific disciplines. Thanks to the latest technological developments, plasma experiments, observations, and computation now produce a large amount of data that can no longer be analyzed or interpreted manually. This trend now necessitates a highly sophisticated use of high-performance computers for data analyses, making artificial intelligence and machine learning vital components of DDPS. This article contains seven primary sections, in addition to the introduction and summary. Following an overview of fundamental data-driven science, five other sections cover widely studied topics of plasma science and technologies, i.e., basic plasma physics and laboratory experiments, magnetic confinement fusion, inertial confinement fusion and high-energy-density physics, space and astronomical plasmas, and plasma technologies for industrial and other applications. The final Section before the summary discusses plasma-related databases that could significantly contribute to DDPS. Each primary Section starts with a brief introduction to the topic, discusses the state-of-the-art developments in the use of data and/or data-scientific approaches, and presents the summary and outlook. Despite the recent impressive signs of progress, the DDPS is still in its infancy. This article attempts to offer a broad perspective on the development of this field and identify where further innovations are required. | |
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Templates of expected measurement uncertainties for neutron-induced capture and charged-particle production cross section observables [Abstract] |
Amanda M. Lewis, Denise Neudecker, Allan D. Carlson, Donald L. Smith, Ian Thompson, Anton Wallner, Devin P. Barry, Lee A. Bernstein, Robert C. Block, Stephen Croft, Yaron Danon, Manfred Drosg, Robert C. Haight, Michal W. Herman, Hye Young Lee, Naohiko Otuka, Henrik Sjöstrand, Vladimir Sobes, EPJ Nuclear Sci. Technol. 9 (2023) 33 doi:10.1051/epjn/2023015 |
Abstract This paper provides a template of expected uncertainties and correlations for measurements of neutron-induced capture and charged-particle production cross sections. Measurements performed in-beam include total absorption spectroscopy, total energy detection, gamma-ray spectroscopy, and direct charged-particle detection. Offline measurements include activation analysis and accelerator mass spectrometry. The information needed for proper use of the datasets in resonance region and high energy region evaluations is described, and recommended uncertainties are provided when specific values are not available for a dataset. | |
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Templates of expected measurement uncertainties for total neutron cross-section observables [Abstract] |
Amanda M. Lewis, Allan D. Carlson, Donald L. Smith, Devin P. Barry, Robert C. Block, Stephen Croft, Yaron Danon, Manfred Drosg, Michal W. Herman, Denise Neudecker, Naohiko Otuka, Henrik Sjöstrand, Vladimir Sobes, EPJ Nuclear Sci. Technol. 9 (2023) 34 doi:10.1051/epjn/2023015 |
Abstract This paper provides a template of expected uncertainties and correlations for measurements of total neutron cross-section observables by transmission. Measurements with time-of-flight and monoenergetic neutron sources are covered. The information required for evaluations in the resonance region and high energy region is detailed, along with the template of uncertainties and correlations that can be used in the absence of other information. | |
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Nuclear physics midterm plan at Legnaro National Laboratories (LNL) [Abstract] |
M. Ballan, A. Koning, et al., Eur. Physical J. Plus 138 (2023) 709. doi:10.1140/epjp/s13360-023-04249-x |
Abstract The next years will see the completion of the radioactive ion beam facility SPES (Selective Production of Exotic Species) and the upgrade of the accelerators complex at Istituto Nazionale di Fisica Nucleare ? Legnaro National Laboratories (LNL) opening up new possibilities in the fields of nuclear structure, nuclear dynamics, nuclear astrophysics, and applications. The nuclear physics community has organised a workshop to discuss the new physics opportunities that will be possible in the near future by employing state-of-the-art detection systems. A detailed discussion of the outcome from the workshop is presented in this report. | |
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EXFOR-based simultaneous evaluation for fast neutron-induced fission cross section of thorium-232 [Abstract] |
Vidya Devi, Naohiko Otuka, S. Ganesan, J. Nucl. Sci. Technol. 61 (2024) pp. 44-56. doi:10.1080/00223131.2023.2256715 |
Abstract The 232Th neutron-induced fission cross section was evaluated from 500 keV to 200 MeV. The experimental 232Th fission cross sections and their ratios to the 235,238U fission cross sections in the EXFOR library were reviewed and analysed by using the least-squares method. The newly published 232Th/235U fission cross-section ratios from the time-of-flight measurements at the CERN n_TOF and CSNS Back-n facilities were compiled in EXFOR. Additional simultaneous evaluation was performed by including the experimental 233,238U and 239,240,241Pu fission cross sections and their ratios. The new evaluation provides the 232Th fission cross section systematically lower than the JENDL-5 cross section. The reduction is 4% in the plateau region between 2 and 6 MeV and more significant in the subthreshold fission region. The present evaluation reduces the 232Th fission cross section averaged over the 252Cf spontaneous fission neutron spectrum from the JENDL-5 evaluation by 4%, which is closer to the other general purpose libraries but underestimates Grundl et al.'s measurement by 11%. | |
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EXFOR-based simultaneous evaluation for neutron-induced fission cross section of plutonium-242 [Abstract] |
Riko Okuyama, Naohiko Otuka, Go Chiba, Osamu Iwamoto, J. Nucl. Sci. Technol. 61 (2024) pp. 57-67. doi:10.1080/00223131.2023.2267070 |
Abstract The 242Pu neutron-induced fission cross section was evaluated from 100 keV to 200 MeV. The experimental 242Pu and 235U fission cross sections and their ratios in the EXFOR library were reviewed and analysed by the least-squares method. Additional simultaneous evaluation was performed by including the experimental database of the 233,238U and 239,240,241Pu fission cross sections and their ratios developed for JENDL-5 evaluation. The 242Pu fission cross sections from our evaluation and JENDL-5 evaluation are close to each other below 1 MeV while they systematically differ from each other above 10 MeV. The cross section from our evaluation is systematically lower than the JENDL-4.0 cross section in the prompt fission neutron spectrum peak region (~5% lower around 1 MeV). The newly evaluated 242Pu fission cross section was verified against the cross section measured in the 252Cf spontaneous fission neutron field and criticalities of small-sized LANL fast systems and demonstrated better performance than the JENDL-4.0 cross section on the same level with the JENDL-5 cross section. | |
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Developing a New Web Service for Experimental Nuclear Reaction Database (EXFOR) Using RESTful API and JSON [Abstract] |
S. Okumura, G. Schnabel and A. Koning, EPJ Web of Conferences |
Abstract Efficient data mining from the Experimental Nuclear Reaction
Database (EXFOR) has a potential for utilization of modern computational
analysis techniques to find trends, shortcomings and hidden patterns in the
database, which in turn helps improve our knowledge of nuclear physics. To
facilitate the data mining, we have developed two EXFOR parsing computer
programs (EXFOR Parser) to convert the data in the database stored in the EXFOR
format into the widely adopted JSON format. The converted JSON data
are used for further processing to extract individual physical observables and
generate tabulated data (x, y, dx, dy) where all units of measurement are standardized.
Furthermore, we have developed REST APIs and an open web system
for easy access and quick visualizations of these converted datasets. | |
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Prompt-fission observable and fission yield calculations for actinides by TALYS [Abstract] |
K. Fujio, s. Okumura, et al., EPJ Web of Conferences |
Abstract The nuclear reaction code TALYS adopts the Hauser-Feshbach statistical decay
theory, to de-excite fission fragments. This involves the evaporation of prompt
fission neutrons and gamma-rays. TALYS incorporates a database of primary fission
fragment distribution which consists of primary fission fragment yield and data
for excitation energy distribution of fission fragments. We conducted a sensitivity
study on three parameters in TALYS and fitted them in order to reproduce
experimental and evaluated data, in thermal neutron-induced fission of 235U.
Moreover, we demonstrate a large-scale calculation of average prompt neutron
and gamma-ray multiplicities for 243 selected actinide isotopes. | |
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The difference between charge polarizations of fission fragments deduced by the static theoretical model and in the current data library [Abstract] |
S. Ebata, S. Okumura, C. Ishizuka and S. Chiba, Int. J. Mod. Phys. E 32 (2023) 2350030. doi:10.1142/S0218301323500301 |
Abstract In this paper, we propose a theoretical method to deduce the charge polarization (CP) and most probable charge for fission fragments for the selected range of mass numbers based on a quantum many-body framework, namely, a constrained Skyrme Hartree?Fock+BCS model. We investigate the CP on the low energy neutron-induced fission of 235U as a representative reaction. We have found that the calculated CP has a noticeable dip that is clearly affected by the spherical shell structure around 132Sn and deformed one around A=144 and a peak for their counterparts, which are common features to those of widely-used Wahl?s systematics, but otherwise, our CP values converge to zero. Especially, we could not see a deep valley and a big hump in the region of symmetric fission at A=
112 and 124 present in Wahl?s systematics. The gradient of our CP near the symmetric fission is negative concerning the mass number of fission fragments, which is consistent with other previous theoretical studies; however, that is the opposite of the gradient in Wahl?s systematics. This paper shows the difference between the charge distribution of fission fragments, which has been used practically so far, in comparison with the calculation by microscopic nuclear theory. | |
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Charge polarization calculated with a microscopic model for the fission fragments of U-236 [Abstract] |
S. Ebata, S. Okumura, C. Ishizuka and S. Chiba, EPJ Web of Conferences 284 (2023) 04008. doi:10.1051/epjconf/202328404008 |
Abstract We investigated theoretical methods to estimate the charge polarization of the fission fragments. The
method is based on the microscopic mean-field model with the nucleon degree of freedom, and is represented
in the three-dimensional coordinate space for dealing with any nuclear deformation. We employed the Skyrme
effective interaction for the calculations and uranium-236 as a target nucleus. We reported static and dynamic
methods in which the potential energy surface of the fissioning nucleus concerning the quadrupole and octupole
deformations are used. Although the static method deduced the charge polarization which indicates the nuclei
with the magic number and the octupole deformation, the quantities are not consistent with the existing data
library (Wahl?s systematics). The dynamic method with the iso-energy initial condition on the potential energy
surface showed the finite charge polarization of light and heavy fission fragments which is consistent with the
data library. Furthermore, it indicates that the charge polarization has energy dependence of the initial states of
the dynamic method. | |
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Consideration of memory of spin and parity in the fissioning compound nucleus by applying the Hauser-Feshbach fission fragment decay model to photonuclear reactions [Abstract] |
T. Kawano, A. E. Lovell, S. Okumura, H. Sasaki, I. Stetcu, and P. Talou, Phys. Rev. C 107 (2023) 044608. doi:10.1103/PhysRevC.107.044608 |
Abstract Prompt and beta-delayed fission observables, such as the average number of prompt and delayed neutrons, the
independent and cumulative fission product yields, and the prompt gamma-ray energy spectra for the photonuclear
reactions on 235,238U and 239Pu, are calculated with the Hauser-Feshbach fission fragment decay (HF3D) model
and compared with available experimental data. In the analysis of neutron-induced fission reactions to the case of
photo-induced fission, an excellent reproduction of the delayed neutron yields supports a traditional assumption
that the photo fission might be similar to the neutron-induced fission at the same excitation energies regardless
of the spin and parity of the fissioning systems. | |
|
TALYS calculations of prompt fission observables and independent
fission product yields for the neutron-induced fission of 235U [Abstract] |
K.Fujio, A.Al-Adili, F.Nordstrom, J.-F.Lemaitre, S.Okumura, S.Chiba, A.Koning, Eur. Phys. J. A 59 (2023) 178. doi:10.1140/epja/s10050-023-01095-4 |
Abstract The TALYS nuclear reaction code?s Hauser-
Feshbach statistical decay model has been adapted in order
to calculate prompt fission neutron and gamma-ray observables
by iterating over deexciting fission fragments. Several fission
fragment generators such as GEF, HF3D, and SPY
were employed to provide TALYS with databases. These
databases contain standardized tables with fission fragment
yields, mean excitation energies and their widths, and average
total kinetic energy, as a function of charge and mass
number of primary fission fragments. The resulting calculations,
including prompt particle multiplicities, spectra, average
energies, and independent fission product yields, were
compared with experimental and evaluated data. This work
first outlines the new methodology implemented in TALYS
and examines the effects of three important parameters on
the final evaporation data. Furthermore, the neutron-induced
fission of 235U is investigated in detail as a function of incident
energy. The results from TALYS, with input from GEF
and HF3D, were compared with available experimental data
and the results of the stand-alone GEF code. The proposed
methodology contributes to an improved capability to model
the fission process. | |
|
Irradiation Damage Independent Deuterium Retention in WMoTaNbV [Abstract] |
A. Liski, K. Heinola, et al., Materials 15 (2022) 7296. doi:10.3390/ma15207296 |
Abstract High entropy alloys are a promising new class of metal alloys with outstanding radiation resistance and thermal stability. The interaction with hydrogen might, however, have desired (H storage) or undesired effects, such as hydrogen-induced embrittlement or tritium retention in the fusion reactor wall. High entropy alloy WMoTaNbV and bulk W samples were used to study the quantity of irradiation-induced trapping sites and properties of D retention by employing thermal desorption spectrometry, secondary ion mass spectrometry, and elastic recoil detection analysis. The D implantation was not found to create additional hydrogen traps in WMoTaNbV as it does in W, while 90 at% of implanted D is retained in WMoTaNbV, in contrast to 35 at% in W. Implantation created damage predicted by SRIM is 0.24 dpa in WMoTaNbV, calculated with a density of 6.044�1022
atoms/cm3
. The depth of the maximum damage was 90 nm. An effective trapping energy for D in WMoTaNbV was found to be about 1.7 eV, and the D emission temperature was close to 700 �C. | |
|
Hydrogen isotope exchange experiments in high entropy alloy WMoTaNbV [Abstract] |
T. Vuoriheimo, K. Heinola, et al., Nucl. Mater. Energy 34 (2023) 101348. doi:10.1016/j.nme.2022.101348 |
Abstract Plasma-facing components in future fusion reactors must endure high temperatures as well as high fluxes and fluences of high energy particles. Currently tungsten has been chosen as the primary plasma-facing material due to its good thermal conductivity, low erosion rate and low fuel retention. Materials with even better properties are still being investigated to be used in reactor regions with demanding plasma conditions. High entropy alloys (HEA) are a new class of metallic alloys and their exploitation in fusion applications has not been widely studied. In this work, the hydrogen isotope exchange effect in an equiatomic HEA containing W, Mo, Ta, Nb, and V was studied. Deuterium was implanted into HEA samples with 30 keV/D energy and the HEA and reference samples were annealed in H2 atmosphere and in vacuum at various temperatures up to 400 C, respectively. The near-surface D concentration profiles were measured with ERDA and the isotope exchange was observed to remove over 90 % of the trapped deuterium from the implantation region at temperatures above 200 C. TDS was used to measure retention deeper in the bulk in which the reduction of trapped deuterium was significantly lower. High total retention of H was found in the bulk after H2 atmosphere annealing which indicates permeation and deep trapping of H in the material. | |
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Deuterium retention in tungsten studied by sequential implantations at ELM-relevant energies [Abstract] |
T. Vuoriheimo, K. Heinola, et al., Nucl. Mater. Energy 34 (2023) 101392. doi:10.1016/j.nme.2023.101392 |
Abstract Plasma edge-localized modes (ELMs) can cause considerable fuel retention in fusion reactor vessel walls by implanting plasma particles with high energies and fluxes. The effect of deuterium ions implanted into tungsten with ELM-relevant energies was studied in laboratory conditions using ion beams. Deuterium implantations were done at room temperature with low fluxes with energies and fluences corresponding to JET and ITER estimates in a single ELM event for both inter-ELM and intra-ELM conditions at the divertor during high power operation. Deuterium implantations with 100 eV/D correspond to an inter-ELM phase, whereas implantations with 5 keV/D or 20 keV/D were used to mimic intra-ELM phases at JET and ITER, respectively. Resulted deuterium retention from these single energy implantations was compared with sequential implantations of low energy ? high energy sequences as well as high energy ? low energy sequences. Retention was measured by ERDA to obtain the amount of deuterium at the irradiated depth as well as the depth profiles for each implantation. High energy ? low energy sequential implantations showed increased retention profile around the implantation-induced damage maximum. In low energy ? high energy sequential implantations the observed retention was increased throughout the analyzed depth. | |
|
The HITRAN2020 molecular spectroscopic database [Abstract] |
I.E. Gordon, C. Hill, et al., J. Quantitative Spectroscopy and Radiative Transfer 277 (2022) 107949. doi:10.1016/j.jqsrt.2021.107949 |
Abstract The HITRAN database is a compilation of molecular spectroscopic parameters. It was established in the early 1970s and is used by various computer codes to predict and simulate the transmission and emission of light in gaseous media (with an emphasis on terrestrial and planetary atmospheres). The HITRAN compilation is composed of five major components: the line-by-line spectroscopic parameters required for high-resolution radiative-transfer codes, experimental infrared absorption cross-sections (for molecules where it is not yet feasible for representation in a line-by-line form), collision-induced absorption data, aerosol indices of refraction, and general tables (including partition sums) that apply globally to the data. This paper describes the contents of the 2020 quadrennial edition of HITRAN. The HITRAN2020 edition takes advantage of recent experimental and theoretical data that were meticulously validated, in particular, against laboratory and atmospheric spectra. The new edition replaces the previous HITRAN edition of 2016 (including its updates during the intervening years).
All five components of HITRAN have undergone major updates. In particular, the extent of the updates in the HITRAN2020 edition range from updating a few lines of specific molecules to complete replacements of the lists, and also the introduction of additional isotopologues and new (to HITRAN) molecules: SO, CH
F, GeH
, CS
, CH
I and NF
. Many new vibrational bands were added, extending the spectral coverage and completeness of the line lists. Also, the accuracy of the parameters for major atmospheric absorbers has been increased substantially, often featuring sub-percent uncertainties. Broadening parameters associated with the ambient pressure of water vapor were introduced to HITRAN for the first time and are now available for several molecules.
The HITRAN2020 edition continues to take advantage of the relational structure and efficient interface available at www.hitran.org and the HITRAN Application Programming Interface (HAPI). The functionality of both tools has been extended for the new edition. | |
|
2022 Review of Data-Driven Plasma Science [Abstract] |
R. Anirudh, C. Hill, et al., IEEE Transactions on Plasma Science 51 No. 7 (2023) pp. 1750-1838. doi:10.1109/TPS.2023.3268170 |
Abstract Data-driven science and technology offer transformative tools and methods to science. This review article highlights the latest development and progress in the interdisciplinary field of data-driven plasma science (DDPS), i.e., plasma science whose progress is driven strongly by data and data analyses. Plasma is considered to be the most ubiquitous form of observable matter in the universe. Data associated with plasmas can, therefore, cover extremely large spatial and temporal scales, and often provide essential information for other scientific disciplines. Thanks to the latest technological developments, plasma experiments, observations, and computation now produce a large amount of data that can no longer be analyzed or interpreted manually. This trend now necessitates a highly sophisticated use of high-performance computers for data analyses, making artificial intelligence and machine learning vital components of DDPS. This article contains seven primary sections, in addition to the introduction and summary. Following an overview of fundamental data-driven science, five other sections cover widely studied topics of plasma science and technologies, i.e., basic plasma physics and laboratory experiments, magnetic confinement fusion, inertial confinement fusion and high-energy-density physics, space and astronomical plasmas, and plasma technologies for industrial and other applications. The final Section before the summary discusses plasma-related databases that could significantly contribute to DDPS. Each primary Section starts with a brief introduction to the topic, discusses the state-of-the-art developments in the use of data and/or data-scientific approaches, and presents the summary and outlook. Despite the recent impressive signs of progress, the DDPS is still in its infancy. This article attempts to offer a broad perspective on the development of this field and identify where further innovations are required. | |
|
LiDB: Database of molecular radiative lifetimes for plasma processes [Abstract] |
Alec Owens, Christian Hill, et al., Plasma Sources Sci. Technol. 32 (2023) 085015. doi:10.1088/1361-6595/aceeb0 |
Abstract LiDB is a newly developed database of molecular vibrational and vibronic state radiative lifetimes. It has been created with the aim of enabling radiative effects to be properly captured in low-temperature plasma models. Datasets have been generated for 36 molecules using comprehensive and highly accurate molecular line lists from the ExoMol spectroscopic database. The main data output of LiDB is radiative lifetimes at vibrational state resolution. Partial lifetimes, which give information on the dominant decay channels in a molecule, are also provided. LiDB is freely available to the scientific community and is hosted at www.exomol.com/lidb. Users can dynamically view molecular datasets or use a specially-designed application programming interface to make data requests. LiDB will continue to expand in the future by adding more molecules, important isotopologues, and neutral and singly-charged atomic species. | |
|
Atomic collisional data for neutral beam modeling in fusion plasmas [Abstract] |
C. Hill, et al., Nucl. Fusion 63 (2023) 125001. doi:10.1088/1741-4326/acf5da |
Abstract The injection of energetic neutral particles into the plasma of magnetic confinement fusion reactors is a widely-accepted method for heating such plasmas; various types of neutral beam are also used for diagnostic purposes. Accurate atomic data are required to properly model beam penetration into the plasma and to interpret photoemission spectra from both the beam particles themselves (e.g. beam emission spectroscopy) and from plasma impurities with which they interact (e.g. charge exchange recombination spectroscopy). This paper reviews and compares theoretical methods for calculating ionization, excitation and charge exchange cross sections applied to several important processes relevant to neutral hydrogen beams, including H + Be4+ and H + H+. In particular, a new cross section for the proton-impact ionization of H (1s) is recommended which is significantly larger than that previously accepted at fusion-relevant energies. Coefficients for an empirical fit function to this cross section and to that of the first excited states of H are provided and uncertainties estimated. The propagation of uncertainties in this cross section in modeling codes under JET-like conditions has been studied and the newly-recommended values determined to have a significant effect on the predicted beam attenuation. In addition to accurate calculations of collisional atomic data, the use of these data in codes modeling beam penetration and photoemission for fusion-relevant plasma density and temperature profiles is discussed. In particular, the discrepancies in the modeling of impurities are reported. The present paper originates from a Coordinated Research Project (CRP) on the topic of fundamental atomic data for neutral beam modeling that the International Atomic Energy Agency (IAEA) ran from 2017 to 2022; this project brought together ten research groups in the fields of fusion plasma modeling and collisional cross section calculations. Data calculated during the CRP is summarized in an appendix and is available online in the IAEA s atomic database, CollisionDB. | |
|
Production of 11C, 13N and 15O in proton-induced nuclear reactions up to 200 MeV |
T. Rodriguez-Gonzalez, R. Capote, et al., Nucl. Data Sheets 187 (2023) pp. 579-596. doi:10.1016/j.nds.2023.01.004 |
|
Simultaneous evaluation of uranium and plutonium fast neutron fission cross sections up to 200 MeV for JENDL-5 and its updates [Abstract] |
N. Otuka, O. Iwamoto, EPJ Web Conf. 284 (2023) 08011. doi:10.1051/epjconf/202328408011 |
Abstract Simultaneous evaluation of 233,235,238U and 239,240,241Pu fission cross sections for fast neutrons up to 200 MeV was performed for the JENDL-5 library. Experimental covariances were estimated for each experimental dataset of cross sections or cross section ratios extracted from the EXFOR library, and they were stored in an experimental database dedicated to the new evaluation. The cross sections were expressed by Schmittroth?s roof functions, and the values on defined incident energy grids were adjusted by the least-squares method to reproduce the experimental cross sections and their ratios. The newly evaluated cross sections were validated using the spectrum averaged cross sections measured in the 252Cf spontaneous fission neutron standard field. The evaluation adopted by the JENDL-5 library was further updated by addition of two datasets and deletion of one dataset. | |
|
Activation cross-sections for short-lived reaction products on hafnium isotopes induced by 1 - 20 MeV neutrons [Abstract] |
V. Semkova, A. Demerdjiev, A. Moens, N. Otuka, A. Plompen, D. Tonev, EPJ Web Conf. 284 (2023) 01038. doi:10.1051/epjconf/202328401038 |
Abstract Results of new activation cross-section measurements for production of 178m1Hf (T1/2 = 4.0 s) and 179m1Hf (T1/2 = 18.67 s) are presented for the following reactions: 178Hf(n,n')178m1Hf, 179Hf(n,2n)178m1Hf, 180Hf(n,3n)178m1Hf, 179Hf(n,n')179m1Hf, and 180Hf(n,2n)179m1Hf. The irradiations were carried out at the 7-MV Van de Graaff accelerator at EC-JRC, Geel. Neutrons in the 1-3 MeV energy range were produced via the 3H(p,n)3He reaction. Deuteron beam and a deuterium gas target were used to produce 5 and 6 MeV neutrons. For the production of quasi-monoenergetic neutrons between 16 and 19.5 MeV the 3H(d,n)4He reactions was employed. Both samples with natural composition and isotopic enrichment were employed to differentiate reactions leading to the same product. An automated pneumatic system was used for the sample irradiation, transport and radioactivity measurements. The radioactivity of the samples was determined by standard gamma-spectrometry using HPGe detector. The results obtained in the present work are compared with the data from other authors and TENDL-2017 evaluation. | |
|
Overview of the dissemination of n_TOF experimental data and resonance parameters [Abstract] |
E. Dupont, N. Otuka, D. Rochman, G. Nogu�re, O. Aberle, V. Alcayne, S. Altieri, S. Amaducci, J. Andrzejewski et al., EPJ Web Conf. 284 (2023) 18001. doi:10.1051/epjconf/202328418001 |
Abstract The n_TOF neutron time-of-flight facility at CERN is used for nuclear data measurements. The n_TOF Collaboration works closely with the Nuclear Reaction Data Centres (NRDC) network to disseminate the experimental data through the international EXFOR library. In addition, the Collaboration helps integrate the results in the evaluated library projects. The present contribution describes the dissemination status of n_TOF results, their impact on evaluated libraries and ongoing efforts to provide n_TOF resonance parameters in ENDF-6 format for further use by evaluation projects. | |
|
Overview of Validation Experiments Focused on Silicon in LR-0 |
T. Czakoj, R. Capote, et al., J. Nucl. Sci. Eng. Radiat. Sci. 7(2021) 021502. doi:10.1115/1.4048480 |
|
First Report of the Nuclear Data Charge Subcommittee of the Nuclear Science Advisory Committee |
L. Bernstein, A. Koning, et al., DOE Report (2022). |
|
Covariances from model variation: Application to quantities for astrophysics |
D.A. Rochman, A. Koning, S. Goriely, Proceedings of the 5th International Workshop on Nuclear Data Covariances (CW2022), September 26-30, 2020 (2022). |
|
Characterization of the neutron flux on the surface of a liquid water target intended for 18F production |
M. Kostal, R. Capote, et al., Radiat. Phys. Chem 184 (2021) 109475. doi:10.1016/j.radphyschem.2021.109475 |
|
Modeling photon-induced reactions on 233,238U actinide targets |
M. Sin, R. Capote, M.W. Herman, A. Trkov and B.V. Carlson, Phys. Rev. C 103 (2021) 054605. doi:10.1103/PhysRevC.103.054605 |
|
Development of a Reference Database for Beta-Delayed Neutron Emission |
P. Dimitriou, M. Verpelli, et al., Nucl. Data Sheets 173 (2021) 144-238. doi:10.1016/j.nds.2021.04.006 |
|
Newly Evaluated Neutron Reaction Data on Chromium Isotopes |
G.P.A. Nobre, R. Capote, et al., Nucl. Data Sheets 173 (2021) 1-41.
doi:10.1016/j.nds.2021.04.002 |
|
Nucleon scattering analysis with a lane-consistent dispersive optical potential for Hf,W and Ta isotopes |
X. Zhao, R. Capote, et al., J. Phys. G: Nucl. Part. Phys. 48 (2021) 075101. doi:10.1088/1361-6471/abe280 |
|
Measurement of 182,184,186W (n, n ?) Cross Sections and What We Can Learn From it. |
G. Henning, R. Capote, et al., EPJ Web of Conferences 247 (2021) 09003. doi:10.1051/epjconf/202124709003 |
|
An impact of Jacques Raynal on nuclear data evaluation |
R. Capote and J.M. Quesada, Eur. Phys. J. A (2021) 57:210. doi:10.1140/epja/s10050-021-00486-9 |
|
What can we learn from(n,x n gama) cross sections about reaction mechanism and nuclear structure? |
M. Kerveno, R. Capote, et al., EPJ Web of Conferences 239 (2020) 01023. doi:10.1051/epjconf/202023901023 |
|
Spectrum averaged cross section measurements of lutetium using standard 252Cf neutron source |
M. Schulc, R. Capote, et al., Appl. Radiat. Isot. 188 (2022) 110378. doi:10.1016/j.apradiso.2022.110378 |
|
Measurement of very high threshold reactions using 252Cf source |
M. Schulc, R. Capote, et al., Appl. Radiat. Isot. 166 (2020) 109355. |
|
Validation of IRDFF-II library in VR-1 reactor field using thin targets |
M. Kostal, R. Capote, et al., Ann. Nucl. Energy 158 (2021) 108268. doi:10.1016/j.anucene.2021.108268 |
|
Impact of reactor neutron spectrum on measured spectrum averaged cross sections |
M. Kostal, R. Capote, et al.,Ann. Nucl. Energy 179 (2022) 109418. doi:10.1016/j.anucene.2022.109418 |
|
EXFOR-based simultaneous evaluation of neutron-induced uranium and plutonium fission cross sections for JENDL-5 : Inputs and outputs [Abstract] |
Naohiko Otuka, Osamu Iwamoto, JAEA-Data/Code 2022-005 (2022). doi:10.11484/jaea-data-code-2022-005 |
Abstract The neutron-induced fission cross sections were simultaneously evaluated for the JENDL-5 library for 233,235U and 239,241Pu from 10 keV to 200 MeV and for 238U and 240Pu from 100 keV to 200 MeV. Evaluation was performed by least-squares fitting of Schmittroth?s roof function to the logarithms of the experimental cross sections and cross section ratios in the EXFOR library. A simultaneous evaluation code SOK was used with its extension to data in arbitrary unit. This report describes (1) construction of the experimental database, (2) selection of data points from TUD-KRI collaboration, (3) comparison with the evaluated cross sections in recent major libraries, and (4) impact of of the 235U datasets published in 1970s. | |
|
EXFOR-based simultaneous evaluation of neutron-induced uranium and plutonium fission cross sections for JENDL-5 [Abstract] |
Naohiko Otuka, Osamu Iwamoto, J. Nucl. Sci. Technol. 59 (2022) pp. 1004-1036. doi:10.1080/00223131.2022.2030259 |
Abstract The neutron-induced fission cross sections were simultaneously evaluated for the JENDL-5 library for
233,235U and 239,241Pu from 10 keV to 200 MeV and for 238U and 240Pu from 100 keV to 200 MeV.
Evaluation was performed by least-squares fitting of Schmittroth?s roof function to the logarithms of the experimental
cross sections and cross section ratios in the EXFOR library. A simultaneous evaluation code SOK was used with its extension
to data in arbitrary unit. The outputs of the code were adopted as the evaluated cross sections without any further corrections.
The newly obtained evaluated cross sections were compared with the evaluated cross sections in the JENDL-4.0 library and the IAEA
Neutron Data Standards 2017. The evaluated cross sections were also validated against the californium-252 spontaneous
fission neutron spectrum averaged cross sections, SS (coupled thermal/fast uranium and boron carbide spherical assembly)
neutron spectrum averaged cross sections, and small-sized LANL fast system criticalities. The changes in the obtained
evaluated cross sections from those in the JENDL-4.0 library are within 4% (241Pu), 3% (233U, 240Pu), or 2%
(235U, 239Pu). The newly evaluated 235U,
238U and 239Pu cross sections agree with the IAEA Neutron Data Standards 2017 within 2% with some exceptions. | |
|
Evaluation of the Prompt Fission Gamma Properties for Neutron Induced Fission of 235,238U and 239Pu
|
I. Stetcu, M.B. Chadwick, T. Kawano, P. Talou, R. Capote and A. Trkov, Nucl. Data Sheets 163 (2020) 261-279. doi:10.1016/j.nds.2019.12.007 |
|
Corrigendum to: "Evaluation of the Neutron Data Standards" [Nucl. Data Sheets 148, p. 143 (2018)] |
A.D. Carlson, R. Capote, et al., Nucl. Data Sheets 163 (2020) 280-281. doi:1www.elsevier.com/locate/nds https://doi.org/10.1016/ |
|
HPRL - International cooperation to identify and monitor priority nuclear data
needs for nuclear applications
|
E. Dupont, R. Capote, EPJ Web of Conferences 239 (2020) 15005. doi:10.1051/epjconf/202023915005 |
|
Multiband coupling and nuclear softness in optical model calculations for
even-even and odd-A actinides
|
D. Martyanov, E. Soukhovitskii, R. Capote, J.M. Quesada and S. Chiba, EPJ Web of Conferences 239 92020) 03003. doi:10.1051/epjconf/202023903003 |
|
Measurement of the α ratio and (n, γ) cross section of 235U from 0.2 to 200 eV at n_TOF
|
J. Balibrea-Correa, R. Capote, et al., Phys. Rev. C 102 (2020) 044615. doi:10.1103/PhysRevC.102.044615 |
|
Infrastructure for the new paradigm of nuclear reaction evaluation |
M. Herman, R. Capote, et al., Ann. Nucl. Energy 163 (2021) 108494. doi:10.1016/j.anucene.2021.108494 |
|
WPEC Subgroup 44 computational Inter-comparison exercise on correlations in nuclear data libraries [Abstract] |
V. Sobes, R. Capote, et al., Ann. Nucl. Energy 164 (2021) 108605. doi:10.1016/j.anucene.2021.108605 |
Abstract There is a long-standing controversy on nuclear data uncertainty assessment for general purpose nuclear
data libraries. On the one hand, nuclear data users would like the libraries to predict uncertainties for
selected integral quantities consistent with the integral experimental uncertainties, while on the other
hand, doing so could make evaluations dependent on selected integral datasets breaking the general
applicability of the library to any existing or future applications. This article studies the hypothesis that
certain correlations between nuclear data, which come from the immutable nature of the reactor physics
in the integral experiment used as benchmarks, and can be estimated almost independently of the choice
of selected integral experiments, nuclear data library, or evaluation methodology. This article reports the
findings of an international computational inter-comparison study carried out under the auspices of the
Working Party on International Nuclear Data Evaluation Co-operation. The participants represented 5 different
organizations, on three different continents and used different initial nuclear data libraries and different
calculation methodologies. This study focused on estimating the correlation coefficients between
fission, capture and nu-bar for Pu-239 which would arise in the final evaluated nuclear data library if a
plutonium metal fast-neutron-spectrum critical experiment with typical integral-measurement uncertainty
of 100 pcm was used in the validation and feedback to compile the nuclear data library. The additional
knowledge of the correlation coefficients can effectively reduce the propagated uncertainty on
criticality experiments from the extended library. This exercise helped to improve understanding the different
approaches used, to identify weaknesses and provide indications where further work is required to
develop a scientifically rigorous method. This article does not aim at recommending these methods as
standards. It aims at honoring the effort of Massimo Salvatores, who was instrumental in pushing studies
that should lead to development of uncertainty estimation and by participating in them. | |
|
Progress on the reevaluation and validation of the n+233U neutron cross
sections |
M.T. Pigni, R. Capote, A. Trkov, Ann. Nucl. Energy 163 (2021) 108595. doi:10.1016/j.anucene.2021.108595 |
|
Modeling photon-induced reactions on 233-238U actinide targets [Abstract] |
M. Sin, R. Capote, M.W. Herman, A. Trkov and B.V. Carlson, Phys. Rev. c 103 (2021) 054605. doi:10.1103/PhysRevC.103.054605 |
Abstract Comprehensive calculations of photon-induced reactions on 233-238U targets for incident photon energies from
3 up to 30 MeV are undertaken with the statistical model code EMPIRE-3.2 Malta. Results are compared with the
experimental data from EXFOR and with the current evaluations. The differences and the similarities between
the models and parameters used in calculations of photon- and neutron-induced reactions on the same nuclei are
discussed with focus on fission. The role of the extended optical model for fission that includes partial damping
in the continuum in improving the description of the measured data is pointed out. | |
|
Which nuclear data can be validated with LLNL pulsed-sphere experiments? [Abstract] |
D. Neudecker, R. Capote, et al., Ann. Nucl. Energy 159 (2021) 108345. doi:10.1016/j.anucene.2021.108345 |
Abstract It is shown here that 14-MeV D+T LLNL pulsed-sphere experiments bring complementary information
into the process of validating nuclear data compared to experiments that are traditionally used for this
purpose?such as critical assemblies. To be more specific, the 14-MeV D+T LLNL pulsed-sphere
neutron-leakage spectra enable to validate scattering and fission nuclear data up to 15 MeV (compared
to approximately up to 5 MeV when using criticality experiments) and employ to this end simple compound
targets containing only few isotopes. Sensitivity profiles of the spectra to nuclear data are calculated
in order to understand in detail which isotopes, observables, and energy ranges of nuclear data
contribute significantly to their simulation. These profiles are presented for a few selected spheres containing
16O, 12C, 56Fe, and 239Pu. It is shown that the neutron-leakage spectra of spheres containing light
elements are mostly sensitive to elastic- and inelastic-scattering cross sections on discrete levels and corresponding
angular distributions. Spheres of structural materials are sensitive to elastic- and inelastic scattering
cross sections, including scattering on discrete levels and the continuum, and double differential
cross sections. Actinide spheres are also strongly sensitive to the fission observables, in particular
to the total-fission neutron spectrum. Thin spheres (in which neutrons experience on average less
than one scatter) are mostly sensitive to data near the elastic peak, in the energy range from 12-15 MeV,
while thicker ones can be sensitive to data at lower incident-neutron energies due to multiple-scattering
effects. This information is brought together with simulations of 71 pulsed-sphere neutron-leakage spectra
using the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear-data libraries. This analysis highlights ENDF/BVIII.
0 data that could be further investigated for potential shortcomings (6Li, 12C, 16O, 24-26Mg, 27Al,
48Ti, 56Fe, and 208Pb) or are likely reliable (1,2H, 7Li, 9Be, 14N, 235,238U, and 239Pu) as indicated by validating
with LLNL pulsed-sphere experiments. | |
|
Measurement of238U(n, n'gamma) cross section data and their impact on reaction models |
M. Kerveno, R. Capote, et al., Phys. Rev. C 104 (2021) 044605. doi:10.1103/PhysRevC.104.044605 |
|
The effect of heavy reflector on neutronic parameters of core |
M. Kostal, R. Capote, et al., Ann. Nucl. En. 168 (2022) 108898. doi:10.1016/j.anucene.2021.108898 |
|
Production cross sections of samarium-153 and -145 via alpha-particle-induced reactions on natural neodymium [Abstract] |
M. Aikawa, M. Sakaguci, N. Ukon, Y. Komori, H. Haba, N. Otuka, S, Takács, Appl. Radiat. Isot. 187 (2022) 110345. doi:10.1016/j.apradiso.2022.110345 |
Abstract Production cross sections of 153,145Sm via alpha-particle-induced reactions on natNd were measured up to 23
MeV. The stacked-foil activation technique and high-resolution gamma-ray spectrometry were adopted for the measurement. The obtained cross sections were compared with the literature data and the TENDL-2019 and TENDL-2021 values. Physical thick target yields of the two radionuclides were derived from the measured cross sections | |
|
Nuclear data uncertainty in iterative neutron spectrum unfolding
[Abstract] |
Katsumi Aoki, Tadahiro Kin, Naohiko Otuka, J. Nucl. Sci. Technol. 59 (2022) pp. 907-914. doi:10.1080/00223131.2021.2018370 |
Abstract We developed an algorithm for propagating the uncertainty of dosimetry cross sections to that of the neutron spectrum obtained through multiple-foil activation and unfolding process. The algorithm derives the uncertainty of the solution spectrum as the standard deviation of a set of
solution spectra obtained by unfolding with numerous sets of dosimetry cross sections, which are randomly generated from the evaluated cross sections and their covariances in a data library. We simulated a multiple-foil activation experiment in a C(d,n) neutron field by PHITS code for some dosimetry reactions to test the algorithm. The GRAVEL code analyzed production amounts to unfold neutron spectrum and then our new algorithm derived the uncertainties of the resultant neutron spectrum originated in the nuclear data uncertainty. Further, we found the uncertainty of the solution spectrum becomes smaller if we ignore the off-diagonal elements of the covariance matrices of the dosimetry cross sections. | |
|
EXFOR-NSR PDF database: a system for nuclear knowledge preservation and data curation |
V.V. Zerkin, B. Pritychenko, J. Totans, L. Vrapcenjak, A. Rodionov, G.I. Shulyak J. Instrum. 17 (2022) P03012. doi:10.1088/1748-0221/17/03/P03012 |
|
Iterative Bayesian Monte Carlo for nuclear data evaluation |
E. Alhassan, D. Rochman, A. Vasiliev, M. Hursin, A.J.Koning, H. Ferroukhi, Nucl. Sci. Tech. 33(2022) 50. doi:10.1007/s41365-022-01034-w |
|
Impact of H in H2O thermal scattering data on criticality calculation: uncertainty and adjustment |
D.A. Rochman, A. Vasiliev, H. Ferroukhi, A. Koning, J.-Ch. Sublet, EPJ Nucl. Sci. Technol. 8 (2022) 3. doi:10.1051/epjn/2021028 |
|
Advanced breakup-nucleon enhancement of deuteron-induced reaction cross sections |
M. Avrigeanu, D. Rochman, A.J. Koning, U. Fischer, D. Leichtle, C. Costache, V. Avrigeanu, Eur. J. Phys. A58 (2022) 3. doi:10.1140/epja/s10050-021-00659-6 |
|
Radioisotope products and the Medicine of the future: an IAEA perspective |
A. Jalilian, A. Korde, V. Starovoitova, J.Jr. Osso, A. Koning, N. Pessoa Barradas, C. Horak, M. Denecke, Bull. Sci. Cent. Expert Eval. Med. Prod. (2022) 539.163:615.31:615.849. doi:10.30895/1991-2919-2022-423 |
|
Comparative study of deuterium retention and vacancy content of self-ion irradiated tungsten
|
A. Hollingsworth, K. Heinola, et al., J. Nucl. Mat. 558 (2022) 153373. doi:10.1016/j.jnucmat.2021.153373 |
|
Nuclear data evaluation with Bayesian networks |
G. Schnabel, R. Capote, A. Koning, D. Brown, Arxiv preprint arxiv:2110.10322 (2021) |
|
Development and application of marginal likelihood optimization for integral parameter adjustment |
D. Siefman, M. Hursin, G. Schnabel, H. Sjoestrand, Ann. Nucl. En. 159 (2021). |
|
Application of JADE V&V capabilities to the new FENDL v3.2 beta release |
D. Laghi, M. Fabbri, L. Isolan, M. Sumini, G. Schnabel, A. Trkov, Nucl. Fusion 61 (2011) 116073. doi:10.1088/1741-4326/ac121a |
|
Data on erosion and hydrogen fuel retention in Beryllium plasma-facing materials |
G. De Temmerman, C. Hill, et al., Nucl. Mater. En. 27 (2021) 100994. |
|
Vibrational excitation and dissociation of deuterium molecule by electron impact |
V. Laporta, R. Agnello, G. Fubiani, I.Furno, C. Hill, D. Reiter, F. Taccogna, Plasma Phys. Control. Fusion 63 (2021) 085006. |
|
Re-investigation of the infrared spectrum of the NCN radical by laser magnetic resonance spectroscopy |
H. Ganser, C. Hill, J. H. George, J. M. Brown, M. Jackson, J. Mol. Spectrosc. 382 (2021) 111547 |
|
Data on erosion and hydrogen fuel retention in Beryllium plasma-facing materials |
G. De Temmerman, K. Heinola, et al., Nucl. Mater. Energy 27 (2021) 100994. doi:10.1016/j.nme.2021.100994 |
|
Comparison of JET inner wall erosion in the first three ITER-Like Wall campaigns |
S. Krat, K. Heinola, et al., Nucl. Mater. Energy 29 (2021) 101072. doi:10.1016/j.nme.2021.101072 |
|
Comparative study of deuterium retention and vacancy content of self-ion irradiated tungsten |
A. Hollingsworth, K. Heinola, et al., J. Nucl. Mat. 558 (2021) 153373. doi:10.1016/j.jnucmat.2021.153373 |
|
Evaluation of tritium retention in plasma-facing components during JET tritium operations |
A. Widdowson, K. Heinola, et al., Phys. Scripta 96 (2021) 124075. doi:10.1088/1402-4896/ac3b30 |
|
Molecular dynamics simulations of hydrogen isotope exchange in tungsten vacancies |
O. Lindblom, T. Ahlgren, K. Heinola, Nucl. Mater. Energy 29 (2021) 101099. doi:10.1016/j.nme.2021.101099 |
|
Investigating High-Energy Proton-Induced Reactions on Spherical Nuclei: Implications for the Pre-Equilibrium Exciton Model |
Morgan B. Fox, Arjan J. Koning, et l., Phys. Rev. C 103 (2021) 034601. |
|
Conception and software implementation of a nuclear data evaluation pipeline |
G. Schnabel, H. Sjoestrand, J. Hansson, D. Rochman, A. Koning, and R. Capote, Nucl. Data Sheets 173 (2021) 239-284. |
|
Measurement and Modeling of Proton-Induced Reactions on Arsenic from 35 to 200 MeV |
Morgan B. Fox, Arjan J. Koning, et al., Phys. Rev. C 104 (2021) 064615. |
|
New Development in TALYS - Fission Fragment Statistical Decay Model |
K. Fujio, S. Okumura, and A. Koning, Proceedings of the 2021 Symposium on Nuclear Data (2021). |
|
Improved modelling of alpha-particle emission in nucleon induced reactions |
A.Yu. Konobeyev, D. Leichtle, A.J. Koning, KIT Scientific Working Papers 176 (2021). |
|
Uranium-235 neutron capture cross section at keV energies |
Naohiko Otuka, Tsuneo Nakagawa, Keiichi Shibata, J. Nucl. Sci. Technol. 44 (2007) pp. 815-818. doi:10.1080/18811248.2007.9711318 |
|
Fast-neutron induced reaction cross section measurement of tin with dual monitor foils and covariance analysis
[Abstract] |
R.Pachuau, N.Otuka, C.V.Midhun, A.Gandhi, A.Mazumdar, H.Krishnamoorthy, A.Reza, V.Vatsa, S.V.Suryanarayana, B.K.Nayak, L.S.Danu, T.Patel, S.Bishnoi, I.Pasha, A.Kumar, V.Nanal, Eur. Phys. J. A 57 (2021) p.268. doi:10.1140/epja/s10050-021-00578-6 |
Abstract The fast-neutron induced elemental cross sections have been measured relative to the
197Au(n,2n)196Au and 27Al(n,α)24Na monitor cross sections at
14.5 � 0.2 MeV by using a natural Sn sample and the activation technique for production of 111Sn,
117Snm, 123Snm, 111In (cumulative),
116Inm1+m2, 117Inm, 117Ing (cumulative),
and 118Inm1+m2. The off-diagonal weighted mean of the elemental cross sections
were determined by constructing the covariance between the cross sections obtained with the two
monitor cross sections. From the measured elemental cross sections, the respective isotopic cross
sections were also determined for the 112Sn(n,2n)111Sn, 124Sn(n,2n)123Snm,
112Sn(n,x)111In and 118Sn(n,p)118Inm1+m2 reactions.
The comparison of the measured elemental and isotopic cross sections with those in the EXFOR, JEFF-3.1/A,
JENDL/AD-2017 and TENDL-2019 libraries as well as those predicted by TALYS-1.9 is discussed. | |
|
Activation cross section measurement of alpha-particle induced reactions on natural neodymium [Abstract] |
M. Sakaguchi, M. Aikawa, N. Ukon, Y. Komori, H. Haba, N. Otuka, S. Tak�cs, Appl. Radiat. Isot. 176 (2021) 109826. doi:10.1016/j.apradiso.2021.109826 |
Abstract Excitation functions of alpha-particle induced reactions on natNd up to 50 MeV were measured at the RIKEN AVF cyclotron. To derive cross sections activation method, stacked target technique and gamma-ray spectrometry were adopted. Formations of 153,145Sm, 151,150,149,148m,148g,144,143Pm, and 149,147Nd were investigated. The results were compared with the previous experimental data and the TENDL-2019 data. Discrepancies among most of them were found. | |
|
Erratum to "Uncertainty propagation in activation cross section measurements" [Radiat. Phys. Chem. 140 (2017) 502-510] |
N. Otuka, B. Lalremruata, M.U. Khandaker, A.R. Usman, L.R.M. Punte, Radiat. Phys. Chem. 184 (2021) 109440. doi:10.1016/j.radphyschem.2021.109440 |
|
Completeness of neutron-, photo-induced and spontaneous fission yields data |
B. Pritychenko, O. Schwerer, J. Totans, V. Zerkin and O. Gritzay, EPJ Web of Conferences 239 (2020) 09003. doi:10.1051/epjconf/202023909003 |
|
Extension of the Hauser-Feshbach fission fragment decay model to multichance fission |
A. E. Lovell, T. Kawano, S. Okumura, et al., Phys. Rev. C 103 (2020) 014615. doi:10.1103/PhysRevC.103.014615 |
|
Evaluation of fission product yields and associated covariance matrices |
K. Tsubakihara, S. Okumura, et al., Nucl. Sci. Technol. 58 (2020) pp. 151-165. doi:10.1080/00223131.2020.1813643 |
|
The fission yield calculations with Langevin model, Hauser-Feshbach statistical decay, and beta decay |
Shin Okumura, Toshihiko Kawano and Satoshi Chiba, EPJ Web of Conferences 239 (2020) 03005. doi:10.1051/epjconf/202023903005 |
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Completeness Check of Experimental Fission Product Yield Data in EXFOR Database |
Shin Okumura, EPJ Web of Conferences 242 (2020) 02002. doi:10.1051/epjconf/202024202002 |
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Vibrational excitation and dissociation of deuterium molecule by electron impact |
V. Laporta, C. Hill, et al., Plasma Phys. Control. Fusion (2021). |
|
Ratio of spectral averaged cross sections measured in standard 252Cf(sf) and 235U(nth,f) neutron fields |
M. Schulc, R. Capote, et al., EPJ WEb Conf 239 (2020) 19004. doi:10.1051/epjconf/202023919004 |
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A reference neutron field for measurement of spectrum averaged cross
sections |
M. Kostal, R. Capote, et al., Ann. Nucl. En. 140 (2020) 107119. doi:10.1016/j.anucene.2019.107119 |
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Results of the Collaborative International Evaluated Library Organisation (CIELO) Project |
M. Fleming, R. Capote, et al., EPJ WEb Conf. 239 (2020) 15003. doi:10.1051/epjconf/202023915003 |
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Upgrade of IAEA recommended data of selected nuclear reactions for production of
PET and SPECT isotopes |
A. Hermanne, R. Capote, et al., ArXiv |
|
Testing of various neutron filters in reference neutron field in LR-0 reactor
for nuclear data validation and verification |
M. Kostal, R. Capote, et al., Appl. Radiat. Isot. 169 (2020) 109566. doi:10.1016/j.apradiso.2020.109566 |
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Dispersive optical model description of nucleon scattering on Pb and Bi isotopes |
Xiuniao Zhao, R. Capote, et al., Phys. Rev. C 101 (2020) 064618. doi:10.1103/PhysRevC.101.064618 |
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Comprehensive validation of silicon cross sections |
T. Czakoj, R. Capote, et al., Nucl. Eng. Technol. 52 (2020) 2717-2724. doi:10.1016/j.net.2020.05.019 |
|
Excitation function of natCu(3He,x)65Zn nuclear reaction for 3He beam monitoring purpose [Abstract] |
M.U. Khandaker, K. Nagatsu, H. Obata, K. Minegishi, M.R. Zhang, S.K.I. Ali, N. Otuka, EPJ Web Conf. 230 (2020) 20009. doi:10.1051/epjconf/202023920009 |
Abstract The excitation function of the natCu(3He,x)65Zn nuclear reaction was measured from its threshold up to 53 MeV incident energy relative to the natTi(3He,x)48V monitor reaction by using the conventional stacked foil activation technique combined with HPGe γ-ray spectrometry. Our result is systematically higher than the IAEA recommendation, and more experimental works are desired especially above 25 MeV. | |
|
Erratum: Nucleon scattering on actinides using a dispersive optical model with extended couplings
[Phys. Rev. C 94, 064605 (2016)] |
E.Sh. Soukhovitski, R. Capote, J.M. Quesada, S. Chiba and D.S. Martyanov, Phys. Rev. C 102 (2020) 059901. doi:10.1103/PhysRevC.102.059901 |
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Progress in international collaboration on EXFOR library [Abstract] |
N. Otuka, B. Pritychenko, M. Fleming, Y. Jin, G. Pikulina, R. Suzuki, V. Devi, M. Mikhailiukova, S. Okumura, N. Soppera, T. Tada, S. Takács, S. Taova, V.V. Varlamov, J.M. Wang, S.C. Yang, V. Zerkin, EPJ Web Conf. 239 (2020) 15001. doi:10.1051/epjconf/202023915001 |
Abstract The EXFOR library has served as the unique repository of experimental cross section and other nuclear reaction data for 50 years. The Nuclear Reaction Data Centres (NRDC) have compiled data sets from more than 22000 experimental works for the EXFOR library. Our collaboration and effort on improvement of EXFOR coverage are described in this paper, as well as tools for digitization of numerical data from graph images developed by us for EXFOR compilation. | |
|
Uncertainties of calculated coincidence-summing correction factors in gamma-ray spectrometry [Abstract] |
V. Semkova, N. Otuka, A.J.M. Plompen, EPJ Web Conf. 239 (2020) 12003. doi:10.1051/epjconf/202023912003 |
Abstract Uncertainty propagation to the γ-γ coincidence-summing correction factor from the covariances of the nuclear data and detection efficiencies have been formulated. The method was applied in the uncertainty analysis of the coincidence-summing correction factors in the γ-ray spectrometry of the 134Cs point source using a p-type coaxial HPGe detector. | |
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Completeness of experimental fission product yields in EXFOR database [Abstract] |
T. Fukuda, S. Okumura, N. Otuka, EPJ Web Conf. 239 (2020) 05013. doi:10.1051/epjconf/202023905013 |
Abstract The Nuclear Reaction Data Centres (NRDC) collaborate on worldwide compilation and dissemination of experimental nuclear reaction data by developing and maintaining the EXFOR database. With the growing interests in the fission product yields of various projectiles and a wide range of energies, several evaluation activities are ongoing. In line with these activities, the IAEA conducted completeness check of fission product yield data in EXFOR against two experimental datasets developed by the ENDF and UKFY library evaluators. The present status and statistics of these datasets as well as the result of the EXFOR completeness review are presented. | |
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Covariance analysis on the thermal neutron capture cross sections using an Am-Be neutron source [Abstract] |
P. Panikkath, N. Otuka, P. Mohanakrishnan, EPJ Web Conf. 239 (2020) 01027. doi:10.1051/epjconf/202023901027 |
Abstract We measured the thermal cross sections of 71Ga(n,γ)72Ga using an Am-Be neutron source having strength of 4 � 107 neutrons/sec using the two monitor reactions 197Au(n,γ)198Au and 55Mn(n,γ)56Mn, and obtained 4.07�0.27 b and 3.97�0.31 b as the values measured relative to Au and Mn neutron captures, respectively. We constructed their covariance matrix by taking into account the correlation of parameters which are not independent in derivation of these two thermal cross sections (e.g., Ga sample weight, decay data of 72Ga, detector efficiency of γ-ray emitted from M72Ga). The off-diagonal weighted mean of the two cross sections 4.04�0.27 b was derived from the two thermal cross sections and their covariance matrix. | |
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Referencing Sources of Molecular Spectroscopic Data in the Era of Data Science: Application to the HITRAN and AMBDAS Databases [Abstract] |
F.M. Skinner, C. Hill, et al., Atoms 8 2 (2020) 16. doi:10.3390/atoms8020016 |
Abstract The application described has been designed to create bibliographic entries in large databases with diverse sources automatically, which reduces both the frequency of mistakes and the workload for the administrators. This new system uniquely identifies each reference from its digital object identifier (DOI) and retrieves the corresponding bibliographic information from any of several online services, including the SAO/NASA Astrophysics Data Systems (ADS) and CrossRef APIs. Once parsed into a relational database, the software is able to produce bibliographies in any of several formats, including HTML and BibTeX, for use on websites or printed articles. The application is provided free-of-charge for general use by any scientific database. The power of this application is demonstrated when used to populate reference data for the HITRAN and AMBDAS databases as test cases. HITRAN contains data that is provided by researchers and collaborators throughout the spectroscopic community. These contributors are accredited for their contributions through the bibliography produced alongside the data returned by an online search in HITRAN. Prior to the work presented here, HITRAN and AMBDAS created these bibliographies manually, which is a tedious, time-consuming and error-prone process. The complete code for the new referencing system can be found on the HITRANonline GitHub website. | |
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A Decade with VAMDC: Results and Ambitions [Abstract] |
D. Albert, C. Hill, et al., Atoms 8 4 (2020) 76. doi:10.3390/atoms8040076 |
Abstract This paper presents an overview of the current status of the Virtual Atomic and Molecular Data Centre (VAMDC) e-infrastructure, including the current status of the VAMDC-connected (or to be connected) databases, updates on the latest technological development within the infrastructure and a presentation of some application tools that make use of the VAMDC e-infrastructure. We analyse the past 10 years of VAMDC development and operation, and assess their impact both on the field of atomic and molecular (A&M) physics itself and on heterogeneous data management in international cooperation. The highly sophisticated VAMDC infrastructure and the related databases developed over this long term make them a perfect resource of sustainable data for future applications in many fields of research. However, we also discuss the current limitations that prevent VAMDC from becoming the main publishing platform and the main source of A&M data for user communities, and present possible solutions under investigation by the consortium. Several user application examples are presented, illustrating the benefits of VAMDC in current research applications, which often need the A&M data from more than one database. Finally, we present our vision for the future of VAMDC. | |
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The 2020 release of the ExoMol database: Molecular line lists for exoplanet and other hot atmospheres [Abstract] |
J. Tennyson, C. Hill, et al., J. Quant. Spectrosc. Radiat. Transfer 255 (2020) 107228. doi:10.1016/j.jqsrt.2020.107228 |
Abstract The ExoMol database (www.exomol.com) provides molecular data for spectroscopic studies of hot atmospheres. While the data are intended for studies of exoplanets and other astronomical bodies, the dataset is widely applicable. The basic form of the database is extensive line lists; these are supplemented with partition functions, state lifetimes, cooling functions, Lande g-factors, temperature-dependent cross sections, opacities, pressure broadening parameters, k-coefficients and dipoles. This paper presents the latest release of the database which has been expanded to consider 80 molecules and 190 isotopologues totaling over 700 billion transitions. While the spectroscopic data are concentrated at infrared and visible wavelengths, ultraviolet transitions are being increasingly considered in response to requests from observers. The core of the database comes from the ExoMol project which primarily uses theoretical methods, albeit usually fine-tuned to reproduce laboratory spectra, to generate very extensive line lists for studies of hot bodies. The data have recently been supplemented by line lists derived from direct laboratory observations, albeit usually with the use of ab initiotransition intensities. A major push in the new release is towards accurate characterisation of transition frequencies for use in high resolution studies of exoplanets and other bodies. | |
|
Comparison of erosion and deposition in JET divertor during first three ITER-like wall campaigns, |
S. Krat, K. Heinola, et al., Phys. Scripta T171 (2020) 014059. doi:10.1088/1402-4896/ab5c11 |
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Improvements to sink strength theory used in multi-scale rate equation simulations of defects in solids |
Tommy Ahlgren and Kalle Heinola, Materials 13 2621 (2020) doi:10.3390/ma13112621 |
|
Why trust nuclear data evaluations with Bayesian networks |
G. Schnabel, R. Capote and D.L. Aldama, EPJ Web of Conferences 284 (2023) 12004. doi:10.1051/epjconf/202328412004 |
|
Data assimilation of post-irradiation examination data for fission yields from GEF [Abstract] |
D. Siefman, G. Schnabel, et al., EPJ Nuclear Sci. Technol. 6 (2020) 52. doi:10.1051/epjn/2020015 |
Abstract Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel which can exceed engineering target accuracies. Herein, we present a new framework that extends data assimilation methods to burnup simulations by using post-irradiation examination experiments. The adjusted fission yields lowered the bias and reduced the uncertainty of the simulations. Our approach adjusts the model parameters of the code GEF. We compare the BFMC and MOCABA approaches to data assimilation, focusing especially on the effects of the non-normality of GEF?s fission yields. In the application that we present, the best data assimilation framework decreased the average bias of the simulations from 26% to 14%. The average relative standard deviation decreased from 21% to 14%. The GEF fission yields after data assimilation agreed better with those in JEFF3.3. For Pu-239 thermal fission, the average relative difference from JEFF3.3 was 16% before data assimilation and after it was 12%. For the standard deviations of the fission yields, GEF?s were 100% larger than JEFF3.3?s before data assimilation and after were only 4% larger. The inconsistency of the integral data had an important effect on MOCABA, as shown with the Marginal Likelihood Optimization method. When the method was not applied, MOCABA?s adjusted fission yields worsened the bias of the simulations by 30%. BFMC showed that it inherently accounted for this inconsistency. Applying Marginal Likelihood Optimization with BFMC gave a 2% lower bias compared to not applying it, but the results were more poorly converged. | |
|
Strangeness production in the new version of the Liège Intra-Nuclear Cascade model [Abstract] |
J. Hirtz, G. Schnabel, et al., Phys. Rev. C 101 (2020) 014608. |
Abstract The capabilities of the new version of the Liege intranuclear cascade model (labeled INCL++6 from now on) are presented in detail. This new version of INCL is able to handle strange particles, such as kaons and the Λ and Σ hyperons, and the associated reactions and also allows extending nucleon-nucleon collisions up to about 15-20 GeV incident energy. Compared to the previous version, new observables can be studied, e.g., kaon, hyperon, and hypernuclei production cross sections (with the use of a suitable de-excitation code) as well as aspects of kaon-induced spallation reactions. The main purpose of this paper is to present the specific ingredients of the new INCL version and its new features, notably the newly implemented variance reduction scheme. We also compare, for some illustrative strangeness production cases, theoretical results calculated using this version of INCL with experimental data. | |
|
Production of Hypernuclei and Strange Particles in Spallation Reactions at a Few GeV Using an Intranuclear Cascade Approach |
Jean-Christophe David, Georg Schnabel, et al., Proc. Int. Conf. Few-Body Problems in Physics, Recent Progress in Few-Body Physics FB22 2018 (2020) pp. 959-963. |
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Unrecognized Sources of Uncertainties (USU) in Experimental Nuclear Data [Abstract] |
R. Capote, G. Schnabel, A.D. Carlson, et al., Nucl. Data Sheets 163 (2020) pp.191-227. doi:10.1016/j.nds.2019.12.004 |
Abstract Evaluated nuclear data uncertainties reported in the literature or archived in data libraries are often perceived as unrealistic, most often because they are thought to be too small. The impact of this issue in applied nuclear science has been discussed widely in recent years. Commonly suggested causes are: poor estimates of specific error components, neglect of uncertainty correlations, and overlooked known error sources. However, instances have been reported where very careful, objective assessments of all known error sources have been made with realistic error magnitudes and correlations provided, yet the resulting evaluated uncertainties still appear to be inconsistent with observed scatter of predicted mean values. These discrepancies might be attributed to significant unrecognized sources of uncertainty (USU) that limit the accuracy to which these physical quantities can be determined.
The objective of our work has been to develop qualitative and quantitative procedures for revealing and including USU estimates in nuclear data evaluations involving experimental input data. This paper identifies several specific clues that can be explored by evaluators in identifying the existence of USU. It then describes numerical procedures we have introduced to generate quantitative estimates of USU magnitudes. Key requirements for these procedures to be viable are that sufficient numbers of data points be available, for statistical reasons, and that additional supporting information about the measurements be provided by the experimenters. Several realistic examples are described here to illustrate these procedures and demonstrate their outcomes and limitations. Our work strongly supports the view that USU is an important issue in nuclear data evaluation, with significant consequences for applications, and that this topic warrants further investigation by the nuclear science community. | |
|
How to search on EXFOR [Abstract] |
N. Otuka, N. Soppera, J. Phys. Conf. Ser. 1555 (2020) 012009 doi:10.1088/1742-6596/1555/1/012009 |
Abstract The experimental nuclear reaction data compiled in the EXFOR library are loaded to databases and accessed by users. The EXFOR library covers not only the cross section but also various other nuclear reaction quantities such as fission yield and thick target yield. It is not always trivial to find an appropriate set of keywords extracting the data sets of interest neither too many or too few. Sometimes users are too specific in their queries, and find nothing in the database. This article presents some examples of EXFOR retrievals for better access to the databases. | |
|
Bayesian updating for data adjustments and multi-level uncertainty propagation within Total Monte Carlo |
E. Alhasssan, D. Rochman, P. Helgesson, H. Sjostrand, A. Vasiliev, and A.J. Koning, Ann. Nucl. En. 139 (2020) 107239. |
|
A statistical analysis of evaluated neutron resonances with TARES for JEFF-3.3, JENDL-4.0, ENDF/B-VIII.0 and TENDL-2019 |
D. Rochman, A.J. Koning, J.-Ch. Sublet, Nucl. Data Sheets 163 (2020) 163. |
|
Excitation functions of deuteron-induced nuclear reactions on erbium in the energy range of 4-24 MeV [Abstract] |
M.U. Khandaker, H. Haba, Y. Komori, N. Otuka, Nucl. Instrum.Meth. B 470 (2020) pp. 1-9. doi:j.nimb.2020.02.035 |
Abstract Excitation functions for the natEr(d,x)163,165,166,167,168,170Tm and natEr(d,x)171Er nuclear reactions were measured from the respective thresholds up to 24 MeV by using a stacked-foil activation technique combined with HPGe γ-ray spectrometry. Measured data show a partial agreement when compared with the available literature data, theoretical data extracted from the TENDL-2019 library, and predicted data by the model code EMPIRE-3.2.2. Estimated physical thick target yields of the reaction products show close values to the directly measured ones available in the literature. The deduced yield curves indicate that a typical irradiation (Ed = 15 MeV, Id = 100 μA, tirr = 72 h) of enriched 167Er target by a low energy deuteron cyclotron is suitable to obtain more than a hundred GBq activity of 167Tm with negligible impurity from 168Tm. Measured data of 170Er(d,p)171Er reaction have great significance to improve the predicting capability of the model code. | |
|
Effect of surface temperature on fuel retention and structure of Be-containing co-deposited layers |
A. Hakola, K. Heinola, Phys. Scripta T171 (2020) 014038. doi:10.1088/1402-4896/ab4be8 |
|
Deposition in the tungsten divertor during the 2011-2016 campaigns in JET with ITER-Like Wall |
N. Catarino, A. Widdowson, A. Baron-Wiechec, J. P. Coad, K. Heinola, M. Rubel, N. P. Barradas and E. Alves, Phys. Scripta T171 (2020) 014044. doi:10.1088/1402-4896/ab4df7 |
|
Fuel inventory and material migration of JET main chamber plasma facing components compared over three operational period |
A. Widdowson, K. Heinola, et al., Phys. Scripta T171 (2020) 014051. doi:10.1088/1402-4896/ab5350 |
|
Hydrogen isotope exchange mechanism in tungsten studied by ERDA |
T. Vuoriheimo, P. Jalkanen, A. Liski, K. Mizohata, T. Ahlgren, K. Heinola and J. Raisanen, Phys. Scripta T171 (2020) 014056. doi:10.1088/1402-4896/ab57ad |
|
Deposition of impurity metals during campaigns with the JET ITER-Like Wall |
A. Widdowson, K. Heinola, et al., Nucl. Mat. Energy 19 (2019) 218. doi:10.1016/j.nme.2018.12.024 |
|
Investigation of deuterium trapping and release in the JET divertor during the third ILW campaign using TDS |
J.Likonen, K. Heinola, A. De Backer, A. Baron-Wiechec, N. Catarino, I. Jepu, C. F. Ayres, P. Coad, G. F. Matthews and A. Widdowson, Nucl. Mat. Energy 19 (2019) 300. doi:10.1016/j.nme.2019.03.012 |
|
Modelling of the effect of ELMs on fuel recycling at the bulk W divertor target of JET |
K. Heinola, T. Ahlgren, S. Brezinsek, T. Vuoriheimo, S. Wiesen, Nucl. Mat. Energy 19 (2019) 397. doi:10.1016/j.nme.2019.03.013 |
|
Erosion, screening, and migration of Tungsten in the JET divertor |
S. Brezinsek, K. Heinola, et al., Nucl. Fusion 59 (2019) 096035. doi:10.1088/1741-4326/ab2aef |
|
Ion beam analysis of fusion plasma-facing materials and components |
M. Mayer, K. Heinola, et al., Nucl. Fusion 60 (2019) 025001. doi:10.1088/1741-4326/ab5817 |
|
Production cross sections of thulium radioisotopes for alpha-particle induced reactions on holmium [Abstract] |
A.R. Usman, M.U. Khandaker, H. Haba, N. Otuka, M. Murakami, Nucl. Instrum. Meth. B 469 (2020) pp. 42-48. doi:10.1016/j.nimb.2020.02.036 |
Abstract The production cross sections of 165?168Tm radioisotopes produced in α-particle induced reactions on 165Ho were measured from 49.6 MeV down to the respective thresholds using the stacked-foil activation technique and HPGe gamma-ray spectrometry. The measured excitation functions were compared with previous measurements as well as the TENDL-2019 library. We also calculated the thick target yields for all the assessed radioisotopes by integration of the measured excitation functions and found that they show good agreement with the directly measured thick target yields except for 168Tm production. | |
|
Ab initio modelling of molecular IR spectra of astrophysical interest: application to CH4 |
R. Warmbier, B.J. Braams, et al., Astron. Astrophys. 495 (2009) 655-661. doi:10.1051/0004-6361:200810983 |
|
A reference neutron field for measurement of spectrum averaged cross
sections [Abstract] |
M. Kostal, R. Capote, et al., Ann. Nucl. Energy in press. doi:10.1016/j.anucene.2019.107119 |
Abstract A new reactor neutron reference field is proposed, which can be used for measurements of spectrum
averaged cross sections (SACS). The reference field is identified in the center of a dry irradiation channel
surrounded by six 3.3% enriched fuel assemblies assembled in the zero-power LR-0 reactor with negligible
burn-up. The neutron field can be defined as a reference one, because of the well-defined neutron
spectrum and neutron flux, well-characterized criticality and core power distribution, and reproducibility
of results. Extensive experimental validation was undertaken. A new reference field can be used for the
measurement of reaction rates and SACS used in nuclear data validation. It is shown that above 6 MeV the
spectrum is undistinguishable from the thermal-neutron induced 235U prompt fission neutron spectrum
(PFNS). Thus, when a reaction has threshold over this limit, the SACS in the thermal-neutron induced 235U
fission neutron field can be derived from reaction rates obtained in this reference neutron field. A comprehensive
set of SACS measurements with uncertainties below 5% in the reference field is presented. | |
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IRDFF-II: A New Neutron Metrology Library [Abstract] |
A. Trkov, R. Capote, et al., Nucl. Data Sheets 163 (2019) 1-108. |
Abstract High quality nuclear data is the most fundamental underpinning for all neutron metrology applications.
This paper describes the release of version II of the International Reactor Dosimetry and Fusion
File (IRDFF-II) that contains a consistent set of nuclear data for fission and fusion neutron metrology
applications up to 60 MeV neutron energy. The library is intended to support: a) applications in
research reactors; b) safety and regulatory applications in the nuclear power generation in commercial
fission reactors; and c) material damage studies in support of the research and development of
advanced fusion concepts. The paper describes the contents of the library, documents the thorough
verification process used in its preparation, and provides an extensive set of validation data gathered
from a wide range of neutron benchmark fields. The new IRDFF-II library includes 119 metrology
reactions, four cover material reactions to support self-shielding corrections, five metrology metrics
used by the dosimetry community, and cumulative fission products yields for seven fission products in
three different neutron energy regions. In support of characterizing the measurement of the residual
nuclei from the dosimetry reactions and the fission product decay modes, the present document
lists the recommended decay data, particle emission energies and probabilities for 68 activation
products. It also includes neutron spectral characterization data for 29 neutron benchmark fields
for the validation of the library contents. Additional six reference fields were assessed (four from
plutonium critical assemblies, two measured fields for thermal-neutron induced fission on 233U and
239Pu targets) but not used for validation due to systematic discrepancies in C/E reaction rate values
or lack of reaction-rate experimental data. Another ten analytical functions are included that can be
useful for calculating average cross sections, average energy, thermal spectrum average cross sections
and resonance integrals. The IRDFF-II library and comprehensive documentation is available online
at www-nds.iaea.org/IRDFF/. Evaluated cross sections can be compared with experimental data
and other evaluations at www-nds.iaea.org/exfor/endf.htm. The new library is expected to become
the international reference in neutron metrology for multiple applications. | |
|
7Li(p, n)7Be cross section from threshold to 1960 keV and precise measurement of the 197Au(n,gamma) spectrum-averaged cross section at 30 keV |
Guido Mart?n-Hern?ndez, Pierfrancesco Mastinu, Elizabeth Musacchio Gonz?lez, Roberto Capote, Hector Lubi?n, and Miguel Macias, Phys. Rev. C 99 (2019) 034616. |
|
International Co-operation in Nuclear Data Evaluation: An Extended Summary of the Collaborative International Evaluated
Library Organisation (CIELO) Pilot Project |
M.R. Chadwick, R. Capote, et al., Nucl. Science NEA No. 7498 (2019). |
|
Analysis of neutron bound states of 208Pb by a dispersive optical model potential [Abstract] |
Xiuniao Zhao, Weili Sun, E.Sh. Soukhovitski, D.S. Martyanov, J.M. Quesada and R. Capote, J. Phys. G: Nucl. Part. Phys. 46 (2019) 055103. |
Abstract A Lane-consistent dispersive spherical optical model potential (DOMP) was
derived in EPJ Web of Conferences 146, 12010 (2017) to describe the nucleon
scattering on 208Pb by fitting scattering data at positive energies. The real part
of this dispersive potential, representing the shell-model potential, is used to
calculate the energies of the bound single-particle states of the target nucleus.
The effect of dispersive correction terms on the calculation of the bound-state
energies is discussed. A set of re-adjusted optical potential parameters, in
particular of the spin?orbit potential, is fitted to measured energies of the
bound single-particle states of 208Pb. Derived 208Pb root mean square radius
shows good agreement with the measured data. This new set of optical model
parameters is also shown to improve the agreement with the polarization
scattering data for proton induced reactions on 208Pb. | |
|
Recommended nuclear data for medical radioisotope production:
diagnostic gamma emitters [Abstract] |
F.T. Tarkanyi, R. Capote, et al., J. Radioanal. Nucl. Chem. 319 (2019) 487-531. doi:10.1007/s10967-018-6142-4 |
Abstract An extensive series of evaluations have been performed as part of an IAEA coordinated research project to study a set of
nuclear reactions that produce the diagnostic gamma-ray emitting radionuclides 51Cr, 99mTc, 111In, 123I and 201Tl. Recommended
cross-section data in the form of excitation functions have been derived, along with quantifications of their
uncertainties. These evaluations involved the compilation of all previously published values and newly measured experimental
data, followed by critical assessments and selection of those experimental datasets and accompanying uncertainties
judged to be fully valid and statistically consistent for model-independent least-squares fitting by means of Pade�
approximations. Integral yields as a function of the energy were also calculated on the basis of the recommended cross
sections deduced from these various fits. All evaluated numerical results and their corresponding uncertainties are available
online at www-nds.iaea.org/medical/gamma_emitters.html and also on the medical portal of the International Atomic
Energy Agency/Nuclear Data Section (IAEA-NDS) www-nds.iaea.org/medportal/. | |
|
Description of analyzing power and (p,n) reaction by a global dispersive coupled-channel optical model potential |
W.L. Sun, L.J. Hao, E.Sh. Soukhovitskii, R. Capote and J.M. Quesada, Proc. 7. China-Japan Joint Nucl. Phys. Symp. CP1235 (2010) 43. |
|
Neutron cross-sections for next generations reactors: New data from n_TOF |
N. Colonna, R. Capote, et al., Appl. Radiat. Isot. 68 (2010) 643-646. |
|
Template for estimating uncertainties of measured
neutron-induced fission cross-sections |
D. Neudecker, B. Hejnal, F. Tovesson, M.C. White, D.L. Smith, D. Vaughan and R. Capote, EPJ Nucl. Sci. Technol. 4 (2018) 21. doi:10.1051/epjn/2018026 |
|
Assessment of Novel Techniques for Nuclear Data Evaluation |
P. Helgesson, D. Neudecker, H. Sjoestrand, M. Grosskopf, D.L. Smith and R. Capote, Reactor Dosimetry: 16th International Symposium, ASTM STP1608 (2018) 105-116. doi:10.1520/STP160820170087 |
|
Predicting Spectrum Averaged Cross Sections in Prompt Fission Neutron Fields |
R. Capote and A. Trkov, Reactor Dosimetry: 16th International Symposium, ASTM STP1608 (2018) 117-123. doi:10.1520/STP160820170114 |
|
Results of a New Evaluation of the Neutron Standards |
A.D. Carlson, et al., Reactor Dosimetry: 16th International Symposium, ASTM STP1608 (2018) 91-104. doi:10.1520/STP160820170069 |
|
Deposition of impurity metals during campaigns with the JET ITER-Like Wall |
A. Widdowson, J. P. Coad, E. Alves, A. Baron-Wiechec, N. Catarino, V. Corregidor, K. Heinola,
S. Krat, C. Makepeace, G. F. Matthews, M. Mayer, K. Mizohata, M. Sertoli, Nucl. Mat. Energy 19 (2019) 218.
doi:10.1016/j.nme.2018.12.024 |
|
Investigation of deuterium trapping and release in the JET divertor during the third ILW campaign using TDS |
J.Likonen, K. Heinola, A. De Backer, A. Baron-Wiechec, N. Catarino, I. Jepu, C. F. Ayres, P. Coad, G. F. Matthews and A. Widdowson, Nucl. Mat. Energy 19 (2019) 300. doi:10.1016/j.nme.2019.03.012 |
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Modelling of the effect of ELMs on fuel recycling at the bulk W divertor target of JET |
K. Heinola, T. Ahlgren, S. Brezinsek, T. Vuoriheimo, S. Wiesen, Nucl. Mat. Energy 19 (2019) 397. doi:10.1016/j.nme.2019.03.013 |
|
Erosion, screening, and migration of Tungsten in the JET divertor |
S. Brezinsek, A. Kirschner, M. Mayer, A. Baron-Wiechec, I. Borodkina, D. Borodin, I. Coffey,
J. W. Coenen, N. d. Harder, A. Eksaeva, C. Guillemaut, K. Heinola, A. Huber, V. Huber, M.
Imrisek, S. Jachmich, E. Pawelec, S. Krat, G. Sergienko, G. Matthews, A. Meigs, S. Wiesen
and A. Widdowson, Nucl. Fusion 59 (2019) 096035.
doi:10.1088/1741-4326/ab2aef |
|
Ion beam analysis of fusion plasma-facing materials and components |
M. Mayer, S. Moller, M. Rubel, A. Widdowson, S. Charisopoulos, T. Ahlgren, E. Alves, G.
Apostolopoulos, N. Barradas, S. Donnelly, S. Fazinic, K. Heinola, O. Kakuee, H. Khodja,
A. Kimura, A. Lagogiannis, M. Li, S. Markelj, M. Mudrinic, P. Petersson, I. Portnykh, D.
Primetzhofer, P. Reichart, D. Ridikas, T. Silva, S. Gonzalez de Vicente and Y. Wang, Nucl. Fusion 60 (2019) 025001.
doi:10.1088/1741-4326/ab5817 |
|
IAEA Photonuclear Data Library 2019 [Abstract] |
R. Capote, et al., Nucl. Data Sheets 163 (2020) 109-162. doi:10.1016/j.nds.2019.12.002 |
Abstract Photo-induced reaction cross section data are of importance for a variety of current or emerging
applications, such as radiation shielding design and radiation transport analyses, calculations
of absorbed dose in the human body during radiotherapy, physics and technology of ssion reactors
(in
uence of photo-reactions on neutron balance) and fusion reactors (plasma diagnostics and
shielding), activation analyses, safeguards and inspection technologies, nuclear waste transmutation,
medical isotope production and astrophysical applications.
To address these data needs the IAEA Photonuclear Data library was produced in 2000, containing
evaluated photo-induced cross sections and neutron spectra for 164 nuclides which were deemed
relevant for the applications.
Since the release of the IAEA Photonuclear Data Library however, new experimental data as
well as new methods to assess the reliability of experimental cross sections have become available.
Theoretical models and input parameters used to evaluate photo-induced reactions have improved
signicantly over the years. In addition, new measurements of partial photoneutron cross sections
using mono-energetic photon beams and advanced neutron detection systems have been performed
allowing for the validation of the evaluations and assessments of the experimental data. Furthermore,
technological advances have led to the construction of new and more powerful gamma-beam facilities,
therefore new data needs are emerging.
We report our coordinated eorts to address these data needs and present the results of the
new evaluations of more than 200 nuclides included in the new updated IAEA Photonuclear Data
Library, where the photon energy goes up to 200 MeV. We discuss the new assessment method and
make recommendations to the user community in cases where the experimental data are discrepant
and the assessments disagree. In addition, in the absence of experimental data, we present model
predictions for photo-induced reaction cross section on nuclides of potential interest to medical
radioisotope production. | |
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Applying a Template of Expected Uncertainties to Updating 239Pu(n,f) Cross-section Covariances in the Neutron Data Standards Database [Abstract] |
D. Neudecker, R. Capote, et al., Nucl. Data Sheets163 (2019) pp. 228-248. |
Abstract Templates of uncertainties expected in specific measurement types were recently developed. One
aim of these templates is to help evaluators in identifying (1) missing or suspiciously low uncertainties
and (2) missing correlations between uncertainties of the same and different experiments,
when estimating covariances for experimental data employed in their evaluations. These templates
also provide realistic estimates of standard deviations and correlations for a particular uncertainty
source and measurement type that can be used by evaluators in situations where they are not supplied
by the experimenters. This information allows for a more comprehensive uncertainty analysis
across all measurements considered in an evaluation and, thus, more realistic evaluated covariances.
Here, we extend a template that is applicable to uncertainties expected in neutron-induced fission,
(n,f), cross-section measurements. It is applied to improving covariances of 239Pu(n,f) cross-section
measurements in the database underlying the Neutron Data Standards evaluations. This particular
example was chosen since this evaluation is primarily based on experimental information. Also,
some uncertainties of individual 239Pu(n,f) cross-section experiments in this database were suspected
to be underestimated. The evaluated uncertainties obtained after updating the covariances
in the database by means of the template indeed do increase compared to their original values.
Even more importantly, the evaluated mean values change noticeably. These modified cross sections
impact application calculations significantly, as is demonstrated by employing them in simulations
of the effective neutron multiplication factor for a few selected critical assemblies. However, this
updated evaluated 239Pu(n,f) cross section should not be interpreted as the final one that should
replace values of the current Neutron Data Standards project. Evaluations for the Neutron Data
Standards of the 239Pu(n,f) cross section must be linked to many other observables included in the
associated database, most notably to cross sections for 235U(n,f), but also to those for 10B(n,alpha), 6Li(n,t), 238U(n,f), and 238U(n,gamma), because of included measurements of the 239Pu(n,f) cross section
that appear as ratios to these reactions. Some of these other reactions are correlated to further
observables in the database. Hence, updating uncertainties of data sets of any of these observables
can potentially impact the 239Pu(n,f) cross section. Uncertainties for all measurements of these
linked physical observables have to be updated before a comprehensive evaluation of the 239Pu(n,f)
cross section and its corresponding uncertainties can be provided. | |
|
Quasiparticle nature of excited states in random-phase approximation |
E.V. Chimanski, B.V. Carlson, R. Capote, and A.J. Koning, Phys. Rev. C 99 (2019) 014305. doi:10.1103/PhysRevC.99.014305 |
|
7Li(p, n)7Be cross section from threshold to 1960 keV and precise measurement of the 197Au(n, gamma) spectrum-averaged cross section at 30 keV |
R. Capote, et al., Phys. Rev. C 99 (2019) 034616. doi:10.1103/PhysRevC.99.034616 |
|
Analysis of neutron bound states of 208Pb by a dispersive optical model potential |
R. Capote, et al., J. Phys. G: Nucl. Part. Phys. 46 (2019) 055103. doi:10.1088/1361-6471/ab0010 |
|
Recommended nuclear data for medical radioisotope production: diagnostic gamma emitters |
R. Capote, et al., J. Radioanal. Nucl. Chem. 319 (2019) 487-531. doi:0.1007/s10967-018-6142-4 |
|
Recommended nuclear data for medical radioisotope production: diagnostic positron emitters |
R. Capote, et al., J. Radioanal. Nucl. Chem. 319 (2019) 533-666. doi:10.1007/s10967-018-6380-5 |
|
Recommended Nuclear Data for the Production of Selected Therapeutic Radionuclides [Abstract] |
R. Capote, et al., Nucl. Data Sheets 155 (2019) 56-74. |
Abstract Increasing interest in the treatment of human disease by means of targeted radionuclide-based
therapies requires an accurate understanding of achievable yields and quantification of realisable
degrees of purity. Important studies within a more extensive Coordinated Research Project of
the International Atomic Energy Agency (IAEA CRP) have included in-depth assessments and
evaluations of all available measured cross-section data for ten nuclear reactions leading to the
formation of 131Cs, 131Ba, 225Ac, 225Ra, 227Th, 227Ac, 230U and 230Pa for various on-going and
proposed therapeutic applications in nuclear medicine. Equivalent studies were also undertaken of
possible reactions to produce the 178W/low-spin 178mTa generator system that has been clinically
applied in diagnosis by means of SPECT - these particular cross-section studies and recommendations
are included in this paper for completeness. All available measured data have been critically reviewed
and assessed to produce statistically consistent datasets. Selected datasets have been fitted by a
least-squares method with Pad�e approximations of variable order to evaluate the production cross
sections and corresponding uncertainties. New measurements have been made in some instances,
and reported data have been adjusted to accommodate new nuclear decay or monitor reaction data
which altered the original reported quantities adversely. Insufficient measured data are available
in many cases to permit a reliable evaluation of cross sections, and these instances are discussed.
Recommended therapeutic radionuclide production reaction data and their uncertainties are available
on the Web page of the IAEA Nuclear Data Section at www-nds.iaea.org/radionuclides/ and also at
the IAEA medical portal www-nds.iaea.org/medportal/ . | |
|
A reference neutron field for measurement of spectrum averaged cross
sections |
R. Capote, et al., Ann. Nucl. Energy (2019) 107119. doi:10.1016/j.anucene.2019.107119 |
|
Recommended Nuclear Data for the Production of Selected Therapeutic Radionuclides |
R. Capote, et al., Nucl. Data Sheets 155 92019) 56-74. |
|
TENDL-based evaluation and adjustment of p+111Cd between 1 and 100 MeV, [Abstract] |
E. Alhassan D. Rochman, A. Vasiliev, A.J. Koning, H. Ferroukhi,, Appl. Radiat. Isot. 198 (2023) 110832. doi:10.1016/j.apradiso.2023.110832 |
Abstract Proton induced reaction data are needed in the optimization of various radioisotope production routes, among others. In this work, the evaluation of proton-induced reactions on 111Cd between 1 and 100 MeV using the TALYS code system within an iterative Bayesian Monte Carlo (iBMC) framework, is presented. The method involves the simultaneous variation of a large number of nuclear reaction models included in the TALYS code system as well as their parameters. Each random TALYS calculation yields a vector of calculated values of cross section observables as well as the angular distributions, among others, which were compared with corresponding vectors of carefully selected differential experimental data for reaction channels where data were available. The random nuclear data file with the maximum likelihood function value obtained from combining the individuals computed for the considered reaction channels was chosen as the parent vector and the starting point for the generation of a further set of random TALYS calculations. This was repeated multiple times until a targeted convergence of 5% was reached. The final evaluated file was compared with available experimental data from the EXFOR database as well as with the evaluations from the TENDL-2021 and JENDL5.0 libraries, and found to compare favorably. | |
|
The gamma-ray strength function for Thallium isotopes relevant to the 205Pb-205Tl chronometry |
H. Utsunomiya , T. Renstroem, G.M. Tveten, S. Goriely, T. Ari-izumi, D. Filipescu, J. Kaur, W. Luo, S. Miyamoto, T. Glodariu, Y.-W. Lui, S. Miyamoto, A-C. Larsen, S. Hilaire, S. Peru, and A.J.Koning, Phys. Rev. C 99 (2019) 024609. |
|
Correlation nubar-sigma for U-Pu in the thermal and resonance neutron range via integral information |
D. Rochman, A. Vasiliev, H. Ferroukhi, S. Pelloni, E. Bauge, and A.J. Koning, Eur. Phys. J. Plus 134 (2019) 453. |
|
Gamma-ray strength function for Barium isotopes |
H. Utsunomiya , T. Renstroem, G.M. Tveten, S. Goriely, T. Ari-izumi, V.W. Ingeberg, B.V. Kheswa, Y.-W. Lui, S. Miyamoto, S. Hilaire, S. Peru, and A.J.Koning, Phys. Rev. C 100 (2019) 034605. |
|
Our future nuclear data needs |
L.A. Bernstein, D.A. Brown, A.J. Koning, B.T. Rearden, C.E. Romano, A.A. Sonzogni, A.S. Voyles and W. Younes, Annu. Rev. Nucl. Part. Sci. 69 (2019). |
|
Compilation of experimental nuclear reaction data measured in Kazakhstan and Uzbekistan for the EXFOR Library [Abstract] |
N.Kenzhebayev, T.K.Zholdybayev, F.Kh.Ergashev, N.Otuka Bull. Russ. Acad. Sci. Ser. Phys.83(2019)pp. 1429-1432. doi:10.3103/S1062873819110121 |
Abstract Compilation of the nuclear reaction data measured in Kazakhstan and Uzbekistan was started by researchers from these countries as well as the International Atomic Energy Agency in 2013. This paper describes a brief history of compilation of data measured in these countries before and after formation of our group, and also reports the achievements and plans of our compilation activity. | |
|
Nuclear Reaction Data Center Network; International and Asia [Abstract] |
K. Kato, N. Otuka, AIP Conf. Ser. 1109 (2009) pp.157-164. doi:10.1063/1.3122248 |
Abstract The activities of the Nuclear Reaction Data Centre at Hokkaido University and International Network of Nuclear Reaction Data Centre (NRDC) are explained. Finally, collaboration in the nuclear data activities among Asian countries are proposed. | |
|
Measurement of thermal neutron capture cross section of 71Ga with dual monitor foils and covariance analysis [Abstract] |
P. Panikkath, N. Otuka, Y. Iwamoto and P. Mohanakrishnan, Eur. Phys. J. A 55 (2019) p.91. doi:10.1140/epja/i2019-12768-4 |
Abstract The thermal neutron cross section of 71Ga(n,γ)72Ga reaction was measured with respect to the 197Au(n,γ)198Au and 55Mn(n,γ)56Mn monitor reactions using neutrons from an Am-Be source placed inside a concrete bunker. A covariance analysis was performed to obtain the off-diagonal weighted mean
of the results determined with the two monitor reactions. The thermal neutron cross section obtained in the present study is 4.05±0.27 b. The present result is lower than the data measured under neutron fields having broad neutron spectra in general, but more consistent with the thermal neutron cross sections extrapolated from the cross sections measured under monoenergetic neutron fields according to the 1/v law.
The current status of the 71Ga(n,γ)72Ga reaction cross section in the nuclear databases is briefly
reviewed in the relation with the Maxwellian spectrum averaged cross section for s-process calculation. | |
|
IAEA CIELO evaluation of neutron-induced reactions on 235U and 238U targets |
R. Capote, A. Trkov, M. Sin, M.T. Pigni, V.G. Pronyaev, J. Balibrea, D. Bernard, D. Cano-Ott, Y. Danon, A. Daskalakis, T. Goricanec, M.W. Herman, B. Kiedrowski, S. Kopecky, E. Mendoza, D. Neudecker, L. Leal, G. Noguere, P. Schillebeeckx, I. Sirakov, E.S. Soukhovitskii, I. Stetcu, P. Talou, Nucl. Data Sheets 148 (2018)pp. 254-292. doi:10.1016/j.nds.2018.02.005 |
|
Evaluation of neutron reactions on iron isotopes for CIELO and ENDF/B-VIII.0 |
M. Herman, A. Trkov, R. Capote, G.P.A. Nobre, D.A. Brown, R. Arcilla, Y. Danon, A. Plompen, S.F. Mughabghab, Q. Jing, Ge Zhigang, Liu Tingjin, Lu Hanlin, Ruo Xichao, L.Leal, B.V. Carlson, T. Kawano, M. Sin, S.P. Simakov, K.Guber, Nucl. Data Sheets 148 (2018) pp. 214-253. doi:10.1016/j.nds.2018.02.004 |
|
Neutron-induced damage simulations: Beyond defect production cross-section, displacement per atom and iron-based metrics [Abstract] |
J.-Ch. Sublet et al., Eur. Phys. J. Plus 134 (2019) 350. doi:10.1140/epjp/i2019-12758-y |
Abstract Nuclear interactions can be the source of atomic displacement and post-short-term cascade
annealing defects in irradiated structural materials. Such quantities are derived from, or can be correlated
to, nuclear kinematic simulations of primary atomic energy distributions spectra and the quantification of
the numbers of secondary defects produced per primary as a function of the available recoils, residual and
emitted, energies. Recoils kinematics of neutral, residual, charged and multi-particle emissions are now
more rigorously treated based on modern, complete and enhanced nuclear data parsed in state of the art
processing tools. Defect production metrics are the starting point in this complex problem of correlating and
simulating the behaviour of materials under irradiation, as direct measurements are extremely improbable.
The multi-scale dimensions (nuclear-atomic-molecular-material) of the simulation process is tackled from
the Fermi gradation to provide the atomic- and meso-scale dimensions with better metrics relying upon a
deeper understanding and modelling capabilities of the nuclear level. Detailed, segregated primary knockon-
atom metrics are now available as the starting point of further simulation processes of isolated and
clustered defects in material lattices. This allows more materials, incident energy ranges and particles, and
irradiations conditions to be explored, with sufficient data to adequately cover both standard applications
and novel ones, such as advanced-fission, accelerators, nuclear medicine, space and fusion. This paper
reviews the theory, describes the latest methodologies and metrics, and provides recommendations for
standard and novel approaches. | |
|
ENDF/B-VIII.0 : The 8th major release of the nuclear reaction data library with CIELO-project cross sections, new standards and thermal scattering data |
D.A. Brown, M.B. Chadwick, R. Capote, A.C. Kahler, A. Trkov, M. W.Herman, A.A. Sonzogni, Y. Danon, A.D. Carlson, M. Dunn, D.L. Smith, G.M. Hale, G. Arbanas, R. Arcilla, C.R. Bates, B. Beck, B. Becker, F. Brown, R.J. Casperson, J. Conlin, D.E. Cullen, M.-A. Descalle, R. Firestone, T. Gaines, K.H. Guber, A.I. Hawari, J. Holmes, T.D. Johnson, T. Kawano, B.C. Kiedrowski, A.J. Koning, S. Kopecky, L. Leal, J.P. Lestone, C. Lubitz, J.I. Marquez Damian, C.M. Mattoon, E.A. McCutchan, S. Mughabghab, P. Navratil, D. Neudecker, G.P.A. Nobre, G. Noguere, M. Paris, M.T. Pigni, A.J. Plompen, B. Pritychenko, V.G. Pronyaev, D. Roubtsov, D. Rochman, P. Romano, P. Schillebeeckx, S. Simakov, M. Sin, I. Sirakov, B. Sleaford, V. Sobes, E.S. Soukhovitskii, I. Stetcu, P. Talou, I. Thompson, S. Van Der Marck, L. Welser-Sherrill, D. Wiarda, M. White, J.L. Wormald, R.Q. Wright, M. Zerkle, G. Zerovnik, Y.Zhu, Nucl. Data Sheets 148 (2018) pp. 1-142. doi:10.1016/j.nds.2018.02.001 |
|
Evaluation of the neutron data standards |
A.D. Carlson, V.G. Pronyaev, R. Capote, G.M. Hale, Z.-P. Chen, I. Duran, F.-J. Hambsch, S. Kunieda,W. Mannhart, B. Marcinkevicius, R.O. Nelson, D. Neudecker, G. Noguere, M. Paris, S.P. Simakov, P. Schillebeeckx, D.L. Smith, X. Tao, A. Trkov, A. Wallner, W. Wang Nucl. Data Sheets 148 (2018) pp. 143-188. doi:10.1016/j.nds.2018.02.002 |
|
Rod insertion method analysis - a methodology update and comparison to boron dilution method |
V. Merljak, M. Kromar, A. Trkov, Ann. Nucl. En. 113 (2018) pp. 96-104. doi:ISSN 0306-4549 |
|
How inelastic scattering stimulates nonlinear reactor core parameter behaviour |
D. Rochman, A. Vasiliev, H. Ferroukhi, H. Dokhane, A.J. Koning, Ann. Nucl. En. 112 (2018) pp. 236-244. doi:10.1016/j.anucene.2017.10.018 |
|
Monte Carlo nuclear data adjustment via integral information
|
D. Rochman, E. Bauge, A. Vasiliev, H. Ferroukhi, S. Pelloni, A.J. Koning and J.C. Sublet, Eur. Phys. Journ. Plus 133 (2018) 537. doi:epjp/i2018-12361-x |
|
Iron NRT- and arc-displacement cross sections and their covariances |
S.P. Simakov, U. Fischer, A.J. Koning, A.Yu. Konobeyev, D.A. Rochman, Nucl. Mat. En. 15 (2018) pp. 244-248. doi:10.1016/j.nme.2018.05.006 |
|
Photoneutron cross sections for Ni isotopes: Toward understanding (n,gamma) cross sections relevant to weak s-process nucleosynthesis |
H. Utsunomiya , T. Renstroem, G.M. Tveten, S. Goriely, S. Katayama, T. Ari-izumi, D. Takenaka, D. Symochko, B.V. Keshwa, V.W. Ingeberg, T. Glodariu, Y.-W. Lui, S. Miyamoto, A-C. Larsen, J.E. Midtboe, A. Goergen, S. Siem, L. Crespo Campo, M. Guttormsen, S. Hilaire, S. Peru, and A.J.Koning, Phys. Rev. C 98 (2018) 054619. doi:10.1103/PhysRevC.98.054619 |
|
TENDL: Complete Nuclear Data Library for Innovative Nuclear Science and Technology
|
A.J. Koning, D. Rochman, J.-Ch. Sublet, N. Dzysiuk, M. Fleming, and S. van der Marck, Nucl. Data Sheets 155 (2019) 1. doi:10.1016/j.nds.2019.01.002 |
|
The experimental nuclear reaction data (EXFOR): Extended computer database and Web retrieval system [Abstract] |
V. Zerkin, B. Pritychenko, Nucl. Instrum. Meth. A 888 (2018) pp.31-43. doi:10.1016/j.nima.2018.01.045 |
Abstract The EXchange FORmat (EXFOR) experimental nuclear reaction database and the associated Web interface provide access to the wealth of low- and intermediate-energy nuclear reaction physics data. This resource is based on numerical data sets and bibliographical information of approx.
22,000 experiments since the beginning of nuclear science. The principles of the computer database organization, its extended contents and Web applications development are described. New capabilities for the data sets uploads, renormalization, covariance matrix, and inverse reaction calculations are presented.
The EXFOR database, updated monthly, provides an essential support for nuclear data evaluation, application development, and research activities. It is publicly available at the websites of the International Atomic Energy Agency Nuclear Data Section, http://www-nds.iaea.org/exfor, the U.S. National Nuclear Data Center, http://www.nndc.bnl.gov/exfor, and the mirror sites in China, India and Russian Federation. | |
|
Energy dependence of the neutron capture cross section on 70Zn near the inelastic scattering threshold [Abstract] |
R.Pachuau, B.Lalremruata, N.Otuka, S.V.Suryanarayana, L.R.M.Punte, L.R.Hlondo, V.V.Desai, B.Satheesh, S.Kailas, S.Ganesan, B.K.Nayak, A.Saxena, Phys. Rev. C 97 (2018) 064617 doi:10.1103/PhysRevC.97.064617 |
Abstract The 70Zn(n,?)71Znm (T1/2=3.96 h) cross section has been measured at 0.40 � 0.15 MeV and 0.70 � 0.10 MeV using a 7Li(p,n)7Be neutron source. The energy of proton energy of neutron energy spectrum code was used to calculate the neutron energy spectrum, and the 197Au(n,?)198Au reaction was used as monitor reaction. Detailed uncertainty analysis has been performed, and the newly measured cross sections are reported with their uncertainties and correlation coefficients. The energy dependence seen in the cross sections measured in the
present work and in the previous work at higher energies has been compared with the theoretical model prediction with various level density models and ?-ray strength functions. Model code dependence of the prediction is also discussed. | |
|
Erratum to "Uncertainty propagation in activation cross section measurements" [Radiat. Phys. Chem. 140 (2017) 502-510] |
N. Otuka, B. Lalremruata, M.U. Khandaker, A.R. Usman, L.R.M. Punte, Radiat. Phys. Chem. 149 (2018) p. 151. doi:10.1016/j.radphyschem.2018.04.017 |
|
CIELO Collaboration Summary Results: International Evaluations of Neutron Reactions on Uranium, Plutonium, Iron, Oxygen and Hydrogen [Abstract] |
M.B.Chadwick, R.Capote, A.Trkov, M.W.Herman, D.A.Brown, G.M.Hale, A.C.Kahler, P.Talou, A.J.Plompen, P.Schillebeeckx, M.T.Pigni, L.Leal, Y.Danon, A.D.Carlson, P.Romain, B.Morillon, E.Bauge, F.-J.Hambsch, S.Kopecky, G.Giorginis, T.Kawano, J.Lestone, D.Neudecker, M.Rising, M.Paris, G.P.A.Nobre, R.Arcilla, O.Cabellos, I.Hill, E.Dupont, A.J.Koning, D.Cano-Ott, E.Mendoza, J.Balibrea, C.Paradela, I.Duran, J.Qian, Z.Ge, T.Liu, L.Hanlin, X.Ruan, W.Haicheng, M.Sin, G.Noguere, D.Bernard, R.Jacqmin, O.Bouland, C.De Saint Jean, V.G.Pronyaev, A.V.Ignatyuk, K.Yokoyama, M.Ishikawa, T.Fukahori, N.Iwamoto, O.Iwamoto, S.Kunieda, C.R.Lubitz, M.Salvatores, G.Palmiotti, I.Kodeli, B.Kiedrowski, D.Roubtsov, I.Thompson, S.Quaglioni, H.I.Kim, Y.O.Lee, U.Fischer, S.Simakov, M.Dunn, K.Guber, J.I.Marquez Damian, F.Cantargi, I.Sirakov, N.Otuka, A.Daskalakis, B.J.McDermott, S.C.Van Der Marck, Nucl. Data Sheets. 148 (2018) pp. 189-213. doi:10.1016/j.nds.2018.02.003 |
Abstract The CIELO collaboration has studied neutron cross sections on nuclides that significantly impact criticality in nuclear technologies - 235,238U, 239Pu, 56Fe, 16O and 1H - with the aim of improving the accuracy of the data and resolving previous discrepancies in our understanding. This multi-laboratory pilot project, coordinated via the OECD/NEA Working Party on Evaluation Cooperation (WPEC) Subgroup 40 with support also from the IAEA, has motivated experimental and theoretical work and led to suites of new evaluated libraries that accurately reflect measured data and also perform well in integral simulations of criticality. This report summarizes our results on cross sections and preliminary work on covariances, and outlines plans for the next phase of this collaboration. | |
|
Rod insertion method analysis - A methodology update and comparison
to boron dilution method [Abstract] |
V. Merljak, M. Kromar, A. Trkov, Ann. Nucl. En. 113 (2018) pp. 96-104. doi:10.1016/j.anucene.2017.11.020 |
Abstract The rod insertion method for control rod worth measurement is explained and past as well as recent
developments are outlined. The original methodology is updated with a more consistent use of the flux
redistribution correction, conversion from dynamic to static reactivity and a new procedure to account
for the so-called reactivity overshoot. As an example, the procedure is applied to real measured data from
Krško NPP. Resulting integral and differential worth curves are compared with reference measurements
by the boron dilution method, where a previously unattainable match is observed. Additional research is
presented in order to assess the remaining small deviations. Besides other advantages, the rod insertion
method is demonstrated to produce results that are in excellent agreement with those of boron dilution
method and can therefore be used as replacement. | |
|
Verification of kinetic capabilities of the GNOMER neutron diffusion code [Abstract] |
V. Merljak, M. Kromar, A. Trkov, Ann. Nucl. En. 109 (2017) pp. 431-439. doi:10.1016/j.anucene.2017.04.037 |
Abstract Recently, the GNOMER neutron diffusion code was updated to support kinetic simulations. This direct
approach to reactor kinetics is further branched into two operational modes: the so-called Lambda mode
and the (normal) implicit mode. Both approaches are described in detail. Also, calculation of point kinetic
parameters is implemented and discussed.
To verify GNOMER�s new kinetic capabilities, two numerical tests are considered; namely, the point
kinetic test case and a rod insertion simulation on a model of a typical pressurised water reactor
(PWR). The reference solutions were produced by a point kinetic script and the SKETCH-N diffusion code,
respectively. Very good agreement is found for all cases considered. Unusual behaviour and discrepancies
� where observed � are explained satisfactorily. With the evidence provided in the paper, GNOMER is
deemed to be a reliable tool for (both static and) dynamic simulation. | |
|
Nuclear Data for Nuclear Sciences and Applications |
P. Dimitriou, Proc. Int. Nucl. Phys. Conf. INPC2016, Proc. Sci. (2016) PoS(INPC2016)118. |
|
The IAEA stopping power database, following the trends in stopping
power of ions in matter [Abstract] |
C.C. Montanari, P. Dimitriou, Nucl. Instrum. Meth. B 408 (2017) pp. 50-55. doi:10.1016/j.nimb.2017.03.138 |
Abstract The aim of this work is to present an overview of the state of art of the energy loss of ions in matter, based
on the new developments in the stopping power database of the International Atomic Energy Agency
(IAEA). This exhaustive collection of experimental data, graphs, programs and comparisons, is the legacy
of Helmut Paul, who made it accessible to the global scientific community, and has been extensively
employed in theoretical and experimental research during the last 25 years. The field of stopping power
in matter is evolving, with new trends in materials of interest, including oxides, nitrides, polymers, and
biological targets. Our goal is to identify areas of interest and emerging data needs to meet the requirements
of a continuously developing user community. | |
|
Cross-section measurements for the 57Fe(n,nγ )57Fe and 57Fe(n,2nγ )56Fe reactions [Abstract] |
A. Negret, M. Sin, C. Borcea, R. Capote, Ph. Dessagne, M. Kerveno, N. Nankov, A. Olacel,
A. J. M. Plompen, and C. Rouki, Phys. Rev. C 96 (2017) 024620. doi:10.1103/PhysRevC.96.024620 |
Abstract A neutron inelastic scattering experiment was performed on an enriched 57Fe sample at the Geel Electron
Linear Accelerator neutron source using the Gamma Array for Neutron Inelastic Scattering spectrometer. Several
γ -production cross sections were determined, but the first transition (14.4 keV) could not be detected owing to
the steadily increased γ background at low energies. Consequently, we use an interplay between experimental
data and carefully tuned theoretical calculations to generate the total inelastic cross section. | |
|
Nucleon scattering on actinides using a dispersive optical model with extended couplings [Abstract] |
E. Sh. Soukhovitskii, R. Capote, J. M. Quesada, S. Chiba, and D. S. Martyanov, Phys. Rev. C 94 (2016) 064605. doi:10.1103/PhysRevC.94.064605 |
Abstract The Tamura coupling model [Rev. Mod. Phys. 37, 679 (1965)] has been extended to consider the coupling of
additional low-lying rotational bands to the ground-state band. Rotational bands are built on vibrational bandheads
(even-even targets) or single-particle bandheads (odd-A targets) including both axial and nonaxial deformations.
These additional excitations are introduced as a perturbation to the underlying axially symmetric rigid-rotor
structure of the ground-state rotational band. Coupling matrix elements of the generalized optical model are
derived for extended multiband transitions in even-even and odd-A nuclei. Isospin symmetric formulation of
the optical model is employed. A coupled-channels optical-model potential (OMP) containing a dispersive
contribution is used to fit simultaneously all available optical experimental databases including neutron strength
functions for nucleon scattering on 232Th, 233,235,238U, and 239Pu nuclei. Quasielastic (p,n) scattering data on
232Th and 238U to the isobaric analog states of the target nucleus are also used to constrain the isovector part of the optical potential. Lane consistent OMP is derived for all actinides if corresponding multiband
coupling schemes are defined. For even-even (odd-A) actinides almost all low-lying collective levels below
1 MeV (0.5 MeV) of excitation energy are coupled. OMP parameters show a smooth energy dependence and
energy-independent geometry. A phenomenological optical-model potential that couples multiple bands in odd-A
actinides is published for a first time. Calculations using the derived OMP potential reproduce measured total
cross-section differences between several actinide pairs within experimental uncertainty for incident neutron
energies from 50 keV up to 150 MeV. The importance of extended coupling is studied. Multiband coupling is
stronger in even-even targets owing to the collective nature of the coupling; the impact of extended coupling
on predicted compound-nucleus formation cross section reaches 5% below 3 MeV of incident neutron energy.
Excitation of multiple bands in odd-A targets is weaker owing to the single-particle nature of the coupling.
Coupling of ground-state rotational band levels in odd-A nuclei is sufficient for a good description of the
compound-nucleus formation cross sections as long as the coupling is saturated (a minimum of seven coupled
levels are typically needed). | |
|
Excitation function shape and neutron spectrum of the 7Li( p,n)7Be reaction near threshold [Abstract] |
Guido Martin-Hernandez, Pierfrancesco Mastinu, Mario Maggiore, Lorenzo Pranovi, Gianfranco Prete, Javier Praena,
Roberto Capote-Noy, Fabiana Gramegna, Augusto Lombardi, Luca Maran, Carlo Scian, and Enrico Munaron, Phys. Rev. C 94 (2016) 034620. doi:10.1103/PhysRevC.94.034620 |
Abstract The forward-emitted low energy tail of the neutron spectrum generated by the 7Li( p,n)7Be reaction on a thick target at a proton energy of 1893.6 keV was measured by time-of-flight spectroscopy. The measurement was
performed at BELINA (Beam Line for Nuclear Astrophysics) of the Laboratori Nazionali di Legnaro. Using the
reaction kinematics and the proton on lithium stopping power the shape of the excitation function is calculated
from the measured neutron spectrum. Good agreement with two reported measurements was found. Our data,
along with the previous measurements, are well reproduced by the Breit-Wigner single-resonance formula for
s-wave particles. The differential yield of the reaction is calculated and the widely used neutron spectrum at a
proton energy of 1912 keV was reproduced. Possible causes regarding part of the 6.5% discrepancy between the
197Au(n,γ ) cross section measured at this energy by Ratynski and Kappeler [Phys. Rev. C 37, 595 (1988)] and
the one obtained using the Evaluated Nuclear Data File version B-VII.1 are given. | |
|
Statistical Hauser-Feshbach theory with width-fluctuation correction including direct reaction
channels for neutron-induced reactions at low energies [Abstract] |
T. Kawano, R. Capote, S. Hilaire and P. Chau Huu-Tai, Phys. Rev. C 94 (2016) 014612. doi:10.1103/PhysRevC.94.014612 |
Abstract A model to calculate particle-induced reaction cross sections with statistical Hauser-Feshbach theory including
direct reactions is given. The energy average of the scattering matrix from the coupled-channels optical model
is diagonalized by the transformation proposed by Engelbrecht and Weidenm¨uller [C. A. Engelbrecht and H. A.
Weidenm¨uller, Phys. Rev. C 8, 859 (1973)]. The ensemble average of S-matrix elements in the diagonalized
channel space is approximated by a model of Moldauer [P. A. Moldauer, Phys. Rev. C 12, 744 (1975)] using the
newly parametrized channel degree-of-freedom νa to better describe the Gaussian orthogonal ensemble (GOE)
reference calculations. The Moldauer approximation is confirmed by a Monte Carlo study using a randomly
generated S matrix, as well as the GOE threefold integration formula. The method proposed is applied to the
238U(n,n') cross-section calculation in the fast-energy range, showing an enhancement in the inelastic scattering
cross sections. | |
|
Extended optical model for fission [Abstract] |
M. Sin, R. Capote, M. W. Herman, and A. Trkov, Phys. Rev. C 93 (2016) 034605. doi:10.1103/PhysRevC.93.034605 |
Abstract A comprehensive formalism to calculate fission cross sections based on the extension of the optical model
for fission is presented. It can be used for description of nuclear reactions on actinides featuring multi-humped
fission barriers with partial absorption in the wells and direct transmission through discrete and continuum fission
channels. The formalism describes the gross fluctuations observed in the fission probability due to vibrational
resonances, and can be easily implemented in existing statistical reaction model codes. The extended optical
model for fission is applied for neutron induced fission cross-section calculations on 234,235,238U and 239Pu
targets. A triple-humped fission barrier is used for 234,235U(n,f ), while a double-humped fission barrier is used
for 238U(n,f) and 239Pu(n,f ) reactions as predicted by theoretical barrier calculations. The impact of partial
damping of class-II/III states, and of direct transmission through discrete and continuum fission channels, is
shown to be critical for a proper description of the measured fission cross sections for 234,235,238U(n,f ) reactions.
The 239Pu(n,f ) reaction can be calculated in the complete damping approximation. Calculated cross sections for
235,238U(n,f) and 239Pu(n,f ) reactions agree within 3% with the corresponding cross sections derived within
the Neutron Standards least-squares fit of available experimental data. The extended optical model for fission
can be used for both theoretical fission studies and nuclear data evaluation. | |
|
Scission neutrons for U, Pu, Cm, and Cf isotopes: Relative multiplicities calculated
in the sudden limit [Abstract] |
R. Capote, N. Carjan, and S. Chiba, Phys. Rev. C 93 (2016) 024609. doi:10.1103/PhysRevC.93.024609 |
Abstract The multiplicities of scission neutrons νsc are calculated for series of U, Pu, Cm, and Cf isotopes assuming
a sudden transition between two different nuclear configurations (αi
�?? αf ): one just before the neck rupture
and one immediately after the disappearance of the neck. This calculation requires only the knowledge of the
corresponding two sets of neutron eigenstates. The nuclear shapes around the scission point are described in terms
of Cassinian ovals with only two parameters: α (that positions the shape with respect to the zero-neck shape) and
α1 (that defines the mass asymmetry). Based on these shapes, a neutron mean field of the Woods-Saxon type is
constructed using two prescriptions to calculate the distance to the nuclear surface. The accent in the present work
is put on the dependence of νsc on the neutron number Nf of the fissioning nucleus and on the mass asymmetry
AL/AH of the primary fission fragments. The relative dependence of these multiplicities, averaged over the mass
yields, νsc
, are finally compared with existing experimental data on prompt fission neutrons νp
. | |
|
Modelling Neutron-induced Reactions on 232-237U from 10 keV up to 30 MeV [Abstract] |
M. Sin, R. Capote, M. W. Herman, and A.Trkov, Nucl. Data Sheets 139 (2017) pp. 138-170. |
Abstract Comprehensive calculations of cross sections for neutron-induced reactions on 232�??237U targets
are performed in the 10 keV�??30 MeV incident energy range with the code EMPIRE�??3.2 Malta.
The advanced modelling and consistent calculation scheme are aimed at improving our knowledge
of the neutron scattering and emission cross sections, and to assess the consistency of available
evaluated libraries for light uranium isotopes. The reaction model considers a dispersive optical
potential (RIPL 2408) that couples from five (even targets) to nine (odd targets) levels of the groundstate
rotational band, and a triple-humped fission barrier with absorption in the wells described
within the optical model for fission. A modified Lorentzian model (MLO) of the radiative strength
function and Enhanced Generalized Superfluid Model nuclear level densities are used in Hauser-
Feschbach calculations of the compound-nuclear decay that include width fluctuation corrections.
The starting values for the model parameters are retrieved from RIPL. Excellent agreement with
available experimental data for neutron emission and fission is achieved, giving confidence that the
quantities for which there is no experimental information are also accurately predicted. Deficiencies
in existing evaluated libraries are highlighted. | |
|
Prompt Fission Neutron Spectra of Actinides |
R. Capote, et al., Nucl Data Sheets 131 (2016) pp. 1-106. doi:10.1016/j.nds.2015.12.002 |
|
A Theoretical Study of Deuteron-induced Surrogate
Reactions [Abstract] |
B.V. Carlson, R. Capote and M. Sin J. Physics: Conference Series 863 (2017) 012039. doi:10.1088/1742-6596/863/1/012039 |
Abstract We use the zero-range post-form DWBA approximation to calculate deuteron
elastic and nonelastic breakup cross sections and estimate the breakup-fusion cross section that
could serve as a surrogate for a neutron-induced reaction cross section. We compare the angular
momentum dependence of the breakup-fusion compound nucleus formation cross section with
that of the corresponding neutron-induced cross section. | |
|
A New Formulation of the Unified Monte
Carlo Approach (UMC-B) and Cross-Section
Evaluation for the Dosimetry Reaction
55Mn(n,c)56Mn |
Roberto Capote, Donald L. Smith, Andrej Trkov, and Mehdi Meghzifene J. ASTM International 9 (2012) pp. 179-196. doi:10.1520/JAI104115 |
|
Inclusive Proton Emission Spectra from Deuteron Breakup
Reactions [Abstract] |
B. V. Carlson, R. Capote, M. Sin, Few-Body Syst. 57 (2016) pp. 307-314 doi:10.1007/s00601-016-1054-8 |
Abstract We present calculations of deuteron elastic and nonelastic breakup cross sections and angular distributions
at deuteron energies below 100 MeV obtained using the post-form DWBA approximation. The elastic
breakup cross section was extensively studied in the past. Very few calculations of nonelastic breakup have
been performed, however. We compare two forms of the elastic DWBA breakup amplitude but conclude that
neither provides a correct description of the inclusive proton emission cross section. | |
|
Inter-comparison of Hauser-Feshbach model codes toward
better actinide evaluations [Abstract] |
Roberto Capote, Stephane Hilaire, Osamu Iwamoto, Toshihiko Kawano, and Mihaela Sin, EPJ Web of Conferences 146 (2017) 12034. doi:10.1051/epjconf/201714612034 |
Abstract The Hauser-Feshbach codes, EMPIRE, TALYS, CCONE, and CoH3, which are widely utilized
in nuclear data evaluations, are compared, with a particular focus on neutron-induced reactions on major
actinides. We report the results of Hauser-Feshbach calculations using well-defined input parameters, and
discuss the differences among these codes. | |
|
Optical model with multiple band couplings using
soft rotator structure [Abstract] |
Dmitry Martyanov, Efrem Soukhovitskii, Roberto Capote, Jose Manuel Quesada, and Satoshi Chiba, EPJ Web of Conferences 146 (2017) 12031. doi:10.1051/epjconf/201714612031 |
Abstract A new dispersive coupled-channel optical model (DCCOM) is derived that describes nucleon
scattering on 238U and 232Th targets using a soft-rotator-model (SRM) description of the collective levels
of the target nucleus. SRM Hamiltonian parameters are adjusted to the observed collective levels of the target
nucleus. SRM nuclear wave functions (mixed in K quantum number) have been used to calculate coupling
matrix elements of the generalized optical model. Five rotational bands are coupled: the ground-state band,
β-, γ -, non-axial- bands, and a negative parity band. Such coupling scheme includes almost all levels below
1.2 MeV of excitation energy of targets. The �??effective�?� deformations that define inter-band couplings are
derived from SRM Hamiltonian parameters. Conservation of nuclear volume is enforced by introducing a
monopolar deformed potential leading to additional couplings between rotational bands. The present DCCOM
describes the total cross section differences between 238U and 232Th targets within experimental uncertainty
from 50 keV up to 200 MeV of neutron incident energy. SRM couplings and volume conservation allow a
precise calculation of the compound-nucleus (CN) formation cross sections, which is significantly different
from the one calculated with rigid-rotor potentials with any number of coupled levels. | |
|
Saturation of coupling of collective levels in optical model
calculations of even-even actinides [Abstract] |
Jose Manuel Quesada, Dmitry Martyanova, Efrem Soukhovitski, Roberto Capote, and Satoshi Chiba, EPJ Web of Conferences 146 (2017) 12013. doi:10.1051/epjconf/201714612013 |
Abstract Saturation of the coupling-scheme is studied in dispersive optical model calculations of nucleon
induced reactions on 238U target. Recently derived potential that is based on a soft-rotator-model (SRM)
description of the collective levels of the target nucleus with volume conservation is used. It is show that
calculated direct excitation cross sections of all considered non-GS bands levels are larger than the 4+ GS band
level excitation, and can�??t be ignored in coupled-channel calculations. SRM couplings of 21 levels constitute
a saturated coupling scheme that allows a precise calculation of the compound-nucleus (CN) formation cross
sections up to several MeV. | |
|
Description of nucleon scattering on 208Pb by a fully
Lane-consistent dispersive spherical optical model potential [Abstract] |
W.L. Sun, J. Wang1, E.Sh. Soukhovitskii, R. Capote, and J.M. Quesada, EPJ Web of Conferences 146 (2017) 12010. doi:10.1051/epjconf/201714612010 |
Abstract A fully Lane-consistent dispersive spherical optical potential is proposed to describe nucleon
scattering interaction with doubly magic nucleus 208Pb up to 200MeV. The experimental neutron total cross
sections, elastically scattered nucleon angular distributions and (p,n) data had been used to search the potential
parameters. Good agreement between experiments and the calculations with this potential is observed.
Meanwhile, the application of the determined optical potential with the same parameters to neighbouring
near magic Pb-Bi isotopes is also examined to show the predictive power of this potential. | |
|
A theoretical study of deuteron-induced surrogate reactions [Abstract] |
B.V. Carlson, R. Capote, and M. Sin, EPJ Web of Conferences 146 (2017) 12001. doi:10.1051/epjconf/201714612001 |
Abstract We use the zero-range post-form DWBA approximation to calculate deuteron elastic and
nonelastic breakup cross sections and estimate the breakup-fusion cross section that could serve as a surrogate
for a neutron-induced reaction cross section.We compare the angular momentum dependence of the breakupfusion
compound nucleus formation cross section with that of the corresponding neutron-induced cross
section. | |
|
Measurement of (n, xnγ ) reaction cross sections in W isotopes [Abstract] |
G. Henning, R. Capote, et al., EPJ WEb of Conferences 146 (2017) 11016. doi:10.1051/epjconf/201714611016 |
Abstract Evaluated nuclear data bases currently used for numerical simulation for the development of
nuclear reactors still present large uncertainties. Their improvement is necessary, in particular through better
reaction models and nuclear data. Among the reactions of interest, (n, xn) reactions are of great importance
for the operation of a reactor as they modify the neutron spectrum, the neutron population, and produce
radioactive species. Experimental data on (n, xnγ ) reaction provide strong constraints on nuclear reaction
mechanism theories. Tungsten isotopes - which are deformed like actinides but do not fission - are of interest to
test the models. 182,184,186W(n, xnγ ) cross sections are measured; results are compared with model calculations
by TALYS, EMPIRE and CoH codes. | |
|
(n,xnγ) cross sections on actinides versus reaction code
calculations [Abstract] |
M. Kerveno, R. Capote, et al., EPJ Web of Conferences 146 (2017) 11012. doi:10.1051/epjconf/201714611012 |
Abstract The experimental setup GRAPhEME (GeRmanium array for Actinides PrEcise MEasurements)
has been used at GELINA (EC-JRC, Geel, Belgium) to perform (n,xn γ ) cross sections measurements.
GRAPhEME has been especially designed to take into account the specific difficulties generated by the use
of actinides samples. This work takes place in the context of new nuclear data measurements for nuclear
reactor applications. Considering the very tight accuracy requested for new experimental data, special care
has been paid to quantify as accurately as possible all the uncertainties from the instruments and the analysis
procedure. From the precise (n,xn γ ) cross sections produced with GRAPhEME, the use of model calculations
is required to obtain (n,xn) cross sections. Beyond the measurements, extensive work on theoretical models
is necessary to achieve a better evaluation of the (n,xn) processes. In this paper, we will discuss the final step
of the 238U data analysis and present some recent results obtained on 232Th compared to TALYS modellings.
A new measurement campaign on 233U has started recently, a first assessment of the recorded data will be
presented. | |
|
IAEA coordinated research project on nuclear data
for charged-particle monitor reactions and medical
isotope production [Abstract] |
Roberto Capote, et al., EPJ Web of Conferences 146 (2017) 08007. doi:10.1051/epjconf/201714608007 |
Abstract An IAEA coordinated research project was launched in December 2012 to establish and improve
the nuclear data required to characterise charged-particle monitor reactions and extend data for medical
radionuclide production. An international team was assembled to undertake work addressing the requirements
for more accurate cross-section data over a wide range of targets and projectiles, undertaken in conjunction
with a limited number of measurements and more extensive evaluations of the decay data of specific
radionuclides. These studies are nearing completion, and are briefly described below. | |
|
Recommended nuclear data for medical
radioisotope production: diagnostic
positron emitters [Abstract] |
F.T. Tarkanyi, R. Capote, et al., J. Radioanal. Nucl. Chem. 319 (2019) 533-666. doi:10.1007/s10967-018-6380-5 |
Abstract An IAEA coordinated research project that began in 2012 and ended in 2016 was primarily dedicated to the compilation,
evaluation and recommendation of cross-section data for the production of medical radionuclides. One significant part of
this work focused on diagnostic positron emitters. These particular studies consist of 69 reactions for direct and indirect or
generator production of 44Sc(44Ti), 52mMn(52Fe), 52gMn, 55Co, 61Cu, 62Cu(62Zn), 66Ga, 68Ga(68Ge), 72As(72Se), 73Se, 76Br,
82Rb(82Sr), 82mRb, 86Y, 89Zr, 90Nb, 94mTc, 110mIn(110Sn), 118Sb(118Te), 120I, 122I(122Xe), 128Cs(128Ba), and 140Pr(140Nd) medical
radionuclides. The resulting reference cross-section data were obtained from Pad� fits to selected and corrected experimental
data, and integral thick target yields were subsequently deduced. Uncertainties in the fitted results were estimated via a
Pad� least-squares method with the addition of a 4% assessed systematic uncertainty. Experimental data were also compared
with theoretical predictions available from the TENDL-2015 and TENDL-2017 libraries. All of the numerical reference
cross-section data with their corresponding uncertainties and deduced integral thick target yields are available on-line at
the IAEA-NDS medical portal www-nds.iaea.org/medic alpor tal and also at the IAEA-NDS web page www-nds.iaea.org/
medic al/posit ron_emitt ers.html. | |
|
New fit of thermal neutron constants (TNC) for 233,235U, 239,241Pu
and 252Cf(sf): Microscopic vs. Maxwellian data [Abstract] |
Vladimir G. Pronyaev, Roberto Capote, Andrej Trkov, Gilles Noguere, and Anton Wallner, EPJ Web of Conferences 146 (2017) 02045. doi:10.1051/epjconf/201714602045 |
Abstract An IAEA project to update the Neutron Standards is near completion. Traditionally, the Thermal
Neutron Constants (TNC) evaluated data by Axton for thermal-neutron scattering, capture and fission on
four fissile nuclei and the total nu-bar of 252Cf(sf) are used as input in the combined least-square fit with
neutron cross section standards. The evaluation by Axton (1986) was based on a least-square fit of both
thermal-spectrum averaged cross sections (Maxwellian data) and microscopic cross sections at 2200 m/s.
There is a second Axton evaluation based exclusively on measured microscopic cross sections at 2200 m/s
(excluding Maxwellian data). Both evaluations disagree within quoted uncertainties for fission and capture
cross sections and total multiplicities of uranium isotopes. There are two factors, which may lead to such
difference: Westcott g-factors with estimated 0.2% uncertainties used in the Axton�??s fit, and deviation of the
thermal spectra from Maxwellian shape. To exclude or mitigate the impact of these factors, a new combined
GMA fit of standards was undertaken with Axton�??s TNC evaluation based on 2200 m/s data used as a prior.
New microscopic data at the thermal point, available since 1986, were added to the combined fit. Additionally,
an independent evaluation of TNC was undertaken using CONRAD code. Both GMA and CONRAD results
are consistent within quoted uncertainties. New evaluation shows a small increase of fission and capture
thermal cross sections, and a corresponding decrease in evaluated thermal nubar for uranium isotopes and
239Pu. | |
|
On the use of the generalized SPRT method in the equivalent
hard sphere approximation for nuclear data evaluation [Abstract] |
Gilles Noguere, Pascal Archier, Olivier Bouland, Roberto Capote, Cyrille De Saint Jean, Stefan Kopecky,
Peter Schillebeeckx, Ivan Sirakov, and Pierre Tamagno, EPJ Web of Conferences 146 (2017) 02036. doi:10.1051/epjconf/201714602036 |
Abstract A consistent description of the neutron cross sections from thermal energy up to the MeV region
is challenging. One of the first steps consists in optimizing the optical model parameters using average
resonance parameters, such as the neutron strength functions. They can be derived from a statistical analysis
of the resolved resonance parameters, or calculated with the generalized form of the SPRT method by using
scattering matrix elements provided by optical model calculations. One of the difficulties is to establish the
contributions of the direct and compound nucleus reactions. This problem was solved by using a slightly
modified average R-Matrix formula with an equivalent hard sphere radius deduced from the phase shift
originating from the potential. The performances of the proposed formalism are illustrated with results
obtained for the 238U+n nuclear systems. | |
|
Evaluation of the neutron induced reactions on 235U from
2.25 keV up to 30MeV [Abstract] |
Andrej Trkov, Roberto Capote, Marco T. Pigni, Vladimir G. Pronyaev, Mihaela Sin, and Efrem S. Soukhovitskii, EPJ Web of Conferences 146 (2017) 02029. doi:10.1051/epjconf/201714602029 |
Abstract An evaluation of fast neutron induced reactions on 235U is performed in the 2.25 keV�??30MeV
incident energy range with the code EMPIRE�??3.2 Malta, combined with selected experimental data. The
reaction model includes a dispersive optical model potential (RIPL 2408) that couples seven levels of the
ground-state rotational band and a triple-humped fission barrier with absorption in the wells described within
the optical model for fission. EGSM nuclear level densities are used in Hauser-Feshbach calculations of the
compound-nuclear decay. The starting values for the model parameters are retrieved from the RIPL-3 database.
Excellent agreement is achieved with available experimental data for neutron emission, neutron capture
and fission, which gives confidence that the quantities for which there is no experimental information are also
predicted accurately.
In the fast neutron region of the evaluated file, the fission cross section is taken from Neutron Standards,
and neutron capture includes fluctuations observed in recent experiments. Other channels are taken directly
from model calculations. New evaluation is validated against ICSBEP criticality benchmarks with fast neutron
spectra with excellent results. | |
|
A new evaluation of the neutron data standards
A. [Abstract] |
A.D. Carlson, et al., EPJ Web of Conferences 146 (2017) 02025.
doi:10.1051/epjconf/201714602025 |
Abstract Evaluations are being done for the H(n,n), 6Li(n,t), 10B(n,αγ ), 10B(n,α), C(n,n), Au(n,γ ), 235U(n,f)
and 238U(n,f) standard cross sections. Evaluations are also being done for data that are not traditional standards
including: the Au(n,γ ) cross section at energies below where it is considered a standard; reference cross
sections for prompt gamma-ray production in fast neutron-induced reactions; reference cross sections for
very high energy fission cross sections; the 235U thermal neutron fission spectrum and the 252Cf spontaneous
fission neutron spectrum and the thermal constants. | |
|
n+235U resonance parameters and neutron multiplicities
in the energy region below 100 eV [Abstract] |
Marco T. Pigni, Roberto Capote, Andrej Trkov, and Vladimir G. Pronyaev, EPJ Web of Conferences 146 (2017) 02011. doi:10.1051/epjconf/201714602011 |
Abstract In August 2016, following the recent effort within the Collaborative International Evaluated
Library Organization (CIELO) pilot project to improve the neutron cross sections of 235U, Oak Ridge National
Laboratory (ORNL) collaborated with the International Atomic Energy Agency (IAEA) to release a resonance
parameter evaluation. This evaluation restores the performance of the evaluated cross sections for the thermaland
above-thermal-solution benchmarks on the basis of newly evaluated thermal neutron constants (TNCs)
and thermal prompt fission neutron spectra (PFNS). Performed with support from the US Nuclear Criticality
Safety Program (NCSP) in an effort to provide the highest fidelity general purpose nuclear database for nuclear
criticality applications, the resonance parameter evaluation was submitted as an ENDF-compatible file to
be part of the next release of the ENDF/B-VIII.0 nuclear data library. The resonance parameter evaluation
methodology used the Reich-Moore approximation of the R-matrix formalism implemented in the code
SAMMY to fit the available time-of-flight (TOF) measured data for the thermal induced cross section of
n+235U up to 100 eV.While maintaining reasonably good agreement with the experimental data, the validation
analysis focused on restoring the benchmark performance for 235U solutions by combining changes to the
resonance parameters and to the prompt resonance ¯ν below 100 eV. | |
|
The CIELO collaboration: Progress in international evaluations
of neutron reactions on Oxygen, Iron, Uranium and Plutonium, [Abstract] |
M.B. Chadwick, R. Capote, et al., EPJ Web of Conferences 146 (2017) 02001. doi:10.1051/epjconf/201714602001 |
Abstract The CIELO collaboration has studied neutron cross sections on nuclides that significantly impact
criticality in nuclear technologies �?? 16O, 56Fe, 235,8U and 239Pu �?? with the aim of improving the accuracy
of the data and resolving previous discrepancies in our understanding. This multi-laboratory pilot project,
coordinated via the OECD/NEA Working Party on Evaluation Cooperation (WPEC) Subgroup 40 with
support also from the IAEA, has motivated experimental and theoretical work and led to suites of new
evaluated libraries that accurately reflect measured data and also perform well in integral simulations of
criticality.
| |
|
Evaluation of cross sections for neutron interactions with 238U in
the energy region between 5 keV and 150 keV [Abstract] |
I. Sirakov, R. Capote, O. Gritzay, H.I. Kim, S. Kopecky, B. Kos, C. Paradela, V.G. Pronyaev, P. Schillebeeckx and A. Trkov, Eur. Phys. J. A 53 (2017) 199. doi:10.1140/epja/i2017-12394-2 |
Abstract Cross sections for neutron interactions with 238U in the energy region from 5 keV to 150 keV
have been evaluated. Average total and capture cross sections have been derived from a least squares
analysis using experimental data reported in the literature. The resulting cross sections have been parameterised
in terms of average resonance parameters maintaining full consistency with results of optical model
calculations by using a dispersive coupled channel optical model potential. The average compound partial
cross sections have been expressed in terms of transmission coefficients by applying the Hauser-Feshbach
statistical reaction theory including width-fluctuations. A generalized single-level representation compatible
with the energy-dependent options of the ENDF-6 format has been applied using standard boundary
conditions. The results have been transferred into a full ENDF-6 compatible data file. | |
|
Neutron capture cross section measurements
for 238U in the resonance region at GELINA [Abstract] |
C. Paradela, R. Capote, et al., Eur. Phys. J. A 52 (2016) 170. doi:10.1140/epja/i2016-16170-6 |
Abstract Measurements were performed at the time-of-flight facility GELINA to determine the 238U(n,γ)
cross section in the resonance region. Experiments were carried out at a 12.5 and 60m measurement station.
The total energy detection principle in combination with the pulse height weighting technique was applied
using C6D6 liquid scintillators as prompt γ-ray detectors. The energy dependence of the neutron flux
was measured with ionisation chambers based on the 10B(n,α) reaction. The data were normalised to the
isolated and saturated 238U resonance at 6.67 eV. Special procedures were applied to reduce bias effects due
to the weighting function, normalization, dead time and background corrections, and corrections related
to the sample properties. The total uncertainty due to the weighting function, normalization, neutron
flux and sample characteristics is about 1.5%. Resonance parameters were derived from a simultaneous
resonance shape analysis of the GELINA capture data and transmission data obtained previously at a
42m and 150m station of ORELA. The parameters of resonances below 500 eV are in good agreement
with those resulting from an evaluation that was adopted in the main data libraries. Between 500 eV and
1200 eV a systematic difference in the neutron width is observed. Average capture cross section data were
derived from the experimental capture yield in the energy region between 3.5 keV and 90 keV. The results
are in good agreement with an evaluated cross section resulting from a least squares fit to experimental
data available in the literature prior to this work. The average cross section data derived in this work were
parameterised in terms of average resonance parameters and included in a least squares analysis together
with other experimental data reported in the literature. | |
|
Predicting the optical observables for nucleon scattering on
even-even actinides [Abstract] |
D.S. Martyanov, E.Sh. Soukhovitski, R. Capote, J.M. Quesada, S. Chiba, Chin. Phys. C 41 No. 9 (2017) 094105 doi:10.1088/1674-1137/41/9/094105 |
Abstract The previously derived Lane consistent dispersive coupled-channel optical model for nucleon scattering
on 232Th and 238U nuclei is extended to describe scattering on even-even actinides with Z =90{98. A soft-rotatormodel
(SRM) description of the low-lying nuclear structure is used, where the SRM Hamiltonian parameters are
adjusted to the observed collective levels of the target nucleus. SRM nuclear wave functions (mixed in K quantum
number) have been used to calculate the coupling matrix elements of the generalized optical model. The \eective"
deformations that dene inter-band couplings are derived from the SRM Hamiltonian parameters. Conservation of
nuclear volume is enforced by introducing a dynamic monopolar term to the deformed potential, leading to additional
couplings between rotational bands. The tted static deformation parameters are in very good agreement with those
derived by Wang and collaborators using the Weizsacker-Skyrme global mass model (WS4), allowing use of the latter
to predict cross sections for nuclei without experimental data. A good description of the scarce \optical"experimental
database is achieved. SRM couplings and volume conservation allow a precise calculation of the compound-nucleus
formation cross sections, which is signicantly dierent from that calculated with rigid-rotor potentials coupling the
ground-state rotational band. The derived parameters can be used to describe both neutron- and proton-induced
reactions. | |
|
Uncertainty propagation in activation cross section measurements [Abstract] |
N. Otuka, B. Lalremruata, M.U. Khandaker, A.R. Usman, L.R.M. Punte, Radiat. Phys. Chem.140 (2017) pp. 502-510. doi:10.1016/j.radphyschem.2017.01.013 |
Abstract The IAEA Nuclear Data Section (IAEA NDS) has emphasized the importance of archiving experimental nuclear data with detailed description of the uncertainties to provide reasonable evaluated (recommended) data sets with their uncertainties to end-usersof nuclear data. In order to achieve this goal, the IAEA NDS is transferring relevant knowledge to experimentalists by instructing uncertainty propagation for their specific experiments. This article discusses uncertainty propagation based on detailed description of uncertainties in neutron- and charged-particle-induced activation cross sections measured in our studies. | |
|
Inter-comparison of Hauser-Feshbach model codes toward better actinide evaluations |
R. Capote, S. Hilaire, O. Iwamoto, T. Kawano and M. Sin, Proc. ND2016, EPJ Web of Conferences 146 (2017) 12034. doi:10.1051/epjconf/201714612034 |
|
Optical model with multiple band couplings using soft rotator structure |
D. Martyanov, E. Soukhovitskii, R. Capote, J.M. Quesada and S. Chiba , Proc. ND2016, EPJ Web of Conferences 146 (2017) 12031. doi:10.1051/epjconf/201714612031 |
|
A tool for calculation of 7Li(p,n)7Be neutron source spectra below the three-body break-up reaction threshold [Abstract] |
R. Pachuau, B. Lalremruata, N. Otuka, L.R. Hlondo, L.R.M. Punte and H.H. Thanga, Proc. ND2016, EPJ Web of Conferences 146 (2017) 12016. doi:10.1051/epjconf/201714612016 |
Abstract We developed a new deterministic neutron source spectrum code EPEN - Energy of Proton Energy of Neutron - for a given lithium target thickness, sample angular coverage and proton energy from the reaction threshold to the three-body break-up threshold. The angular differential cross sections of the 7Li(p,n0)7Be and 7Li(p,n1)7Be reactions evaluated by Liskien and Paulsen were adopted above 1.95 MeV while the functional form suggested by Macklin and Gibbons was adopted for the 7Li(p,n0)7Be reaction cross section near threshold. The spectra obtained by EPEN are validated by the experimental spectra and also compared with the spectra predicted by two Monte Carlo codes, SimLiT and PINO. The results of comparison are discussed in detail. | |
|
Saturation of coupling of collective levels in optical model calculations of even-even actinides |
J.M. Quesada, D. Martyanov, E. Soukhovitski?, R. Capote and S. Chiba, Proc. ND2016, EPJ Web of Conferences 146 (2017) 12013. doi:10.1051/epjconf/201714612013 |
|
Description of nucleon scattering on 208Pb by a fully Lane-consistent dispersive spherical optical model potential |
W.L. Sun, J. Wang, E.Sh. Soukhovitskii, R. Capote and J.M. Quesada, Proc. ND2016, EPJ Web of Conferences 146 (2017) 12010. doi:10.1051/epjconf/201714612010 |
|
A theoretical study of deuteron-induced surrogate reactions |
B.V. Carlson, R. Capote and M. Sin, Proc. ND2016, EPJ Web of Conferences 146 (2017) 12001. doi:10.1051/epjconf/201714612001 |
|
Investigation of the 27Al(d,x)24Na nuclear reaction for deuteron beam monitoring purpose [Abstract] |
M.U. Khandaker, H. Haba, N. Otuka and H.A. Kassim, Proc. ND2016, EPJ Web of Conferences 146 (2017) 11029. doi:10.1051/epjconf/201714611029 |
Abstract Activation cross-sections for the 27Al(d,x)24Na nuclear reaction was measured by using a stacked-foil activation technique combined with high purity germanium (HPGe) γ-ray spectrometry over deuteron energy range of 2�??24�??MeV. Measured data were critically compared with the available literature data and also with the theoretical data extracted from the TENDL data base. Accuracy of the 27Al(d,x)24Na cross-sections were confirmed by the simultaneous measurements of the natTi(d,x)48V monitor reaction cross-sections. Present results reproduced well the IAEA recommended natTi(d,x)48V reaction cross-sections, but provide slight deviation with the IAEA recommended 27Al(d,x)24Na cross-sections. It may be concluded that the use of 27Al(d,x)24Na in deuteron beam monitoring should not be a perfect choice if one has the option to use the natTi(d,x)48V reaction. | |
|
Measurement of (n, xnγ) reaction cross sections in W isotopes |
G. Henning, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 11016. doi:10.1051/epjconf/201714611016 |
|
(n,xnγ) cross sections on actinides versus reaction code calculations |
M. Kerveno, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 11012. doi:10.1051/epjconf/201714611012 |
|
Fission yield covariances for JEFF: A Bayesian Monte Carlo method |
O. Leray, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 09023. doi:10.1051/epjconf/201714609023 |
|
Nuclear data for ion beam analysis applications |
P. Dimitriou, V. Semkova and V. Zerkin , Proc. ND2016, EPJ Web of Conferences 146 (2017) 09014. doi:10.1051/epjconf/201714609014 |
|
Nuclear data for fusion technology - the European approach |
U. Fischer, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 09003. doi:10.1051/epjconf/201714609003 |
|
IAEA coordinated research project on nuclear data for charged-particle monitor reactions and medical isotope production |
R. Capote, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 08007. doi:10.1051/epjconf/201714608007 |
|
Experiments in the EXFOR library for evaluation of thermal neutron constants [Abstract] |
N. Otuka, R. Capote, V. Semkova, T. Kawai and G. Noguere, Proc. ND2016, EPJ Web of Conferences 146 (2017) 07005. doi:10.1051/epjconf/201714607005 |
Abstract E.J. Axton�??s experimental database adopted in evaluation of thermal neutron constants by himself and also by a recent project to update the IAEA Neutron Standard was checked against the experimental literature and EXFOR library. We discovered that many data are found neither in the EXFOR library nor in the articles quoted by Axton due to various reasons. This paper summarizes the status of the experimental data cited by Axton in the experimental literature as well as in the EXFOR library. | |
|
EXFOR ? a global experimental nuclear reaction data repository: Status and new developments [Abstract] |
V. Semkova, N. Otuka, M. Mikhailiukova, B. Pritychenko and O. Cabellos, Proc. ND2016, EPJ Web of Conferences 146 (2017) 07003. doi:10.1051/epjconf/201714607003 |
Abstract Members of the International Network of Nuclear Reaction Data Centres (NRDC) have collaborated since the 1960s on the worldwide collection, compilation and dissemination of experimental nuclear reaction data. New publications are systematically complied, and all agreed data assembled and incorporated within the EXFOR database. Recent upgrades to achieve greater completeness of the contents are described, along with reviews and adjustments of the compilation rules for specific types of data. | |
|
Dissemination of data measured at the CERN n_TOF facility [Abstract] |
E. Dupont, N. Otuka, O. Cabellos et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 07002. doi:10.1051/epjconf/201714607002 |
Abstract The n_TOF neutron time-of-flight facility at CERN is used for high quality nuclear data measurements from thermal energy up to hundreds of MeV. In line with the CERN open data policy, the n_TOF Collaboration takes actions to preserve its unique data, facilitate access to them in standardised format, and allow their re-use by a wide community in the fields of nuclear physics, nuclear astrophysics and various nuclear technologies. The present contribution briefly describes the n_TOF outcomes, as well as the status of dissemination and preservation of n_TOF final data in the international EXFOR library. | |
|
Recommended Nuclear Data for the Production of Selected Therapeutic Radionuclides [Abstract] |
J.W. Engle, R. Capote, et al., Nucl. Data Sheets 155 (2019) 56-74. doi:10.1016/j.nds.2019.01.003 |
Abstract Increasing interest in the treatment of human disease by means of targeted radionuclide-based
therapies requires an accurate understanding of achievable yields and quantification of realisable
degrees of purity. Important studies within a more extensive Coordinated Research Project of
the International Atomic Energy Agency (IAEA CRP) have included in-depth assessments and
evaluations of all available measured cross-section data for ten nuclear reactions leading to the
formation of 131Cs, 131Ba, 225Ac, 225Ra, 227Th, 227Ac, 230U and 230Pa for various on-going and
proposed therapeutic applications in nuclear medicine. Equivalent studies were also undertaken of
possible reactions to produce the 178W/low-spin 178mTa generator system that has been clinically
applied in diagnosis by means of SPECT - these particular cross-section studies and recommendations
are included in this paper for completeness. All available measured data have been critically reviewed
and assessed to produce statistically consistent datasets. Selected datasets have been fitted by a
least-squares method with Pad�e approximations of variable order to evaluate the production cross
sections and corresponding uncertainties. New measurements have been made in some instances,
and reported data have been adjusted to accommodate new nuclear decay or monitor reaction data
which altered the original reported quantities adversely. Insufficient measured data are available
in many cases to permit a reliable evaluation of cross sections, and these instances are discussed.
Recommended therapeutic radionuclide production reaction data and their uncertainties are available
on the Web page of the IAEA Nuclear Data Section at www-nds.iaea.org/radionuclides/ and also at
the IAEA medical portal www-nds.iaea.org/medportal/ . | |
|
Improving activation cross section data with TALYS |
N. Dzysiuk and A. Koning, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02047. doi:10.1051/epjconf/201714602047 |
|
New fit of thermal neutron constants (TNC) for 233,235U, 239,241Pu and 252Cf(sf): Microscopic vs. Maxwellian data |
V.G. Pronyaev, R. Capote, A. Trkov, G. Noguere and A. Wallner, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02045. doi:10.1051/epjconf/201714602045 |
|
Nuclear structure and decay data evaluation in Europe |
A. Negret, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 02042. doi:10.1051/epjconf/201714602042 |
|
On the use of the generalized SPRT method in the equivalent hard sphere approximation for nuclear data evaluation |
G. Noguere, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 02036. doi:10.1051/epjconf/201714602036 |
|
Propagation of nuclear data uncertainties for fusion power measurements |
H. Sjostrand, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 02034. doi:10.1051/epjconf/201714602034 |
|
TALYS/TENDL verification and validation processes: Outcomes and recommendations |
M. Fleming, J.-C. Sublet, M.R. Gilbert, A. Koning and D. Rochman, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02033. doi:10.1051/epjconf/201714602033 |
|
Evaluation of the neutron induced reactions on 235U from 2.25 keV up to 30 MeV |
A. Trkov, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 02029. doi:10.1051/epjconf/201714602029 |
|
A new evaluation of the neutron data standards |
A.D. Carlson, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 02025. doi:10.1051/epjconf/201714602025 |
|
Covariances for the 56Fe radiation damage cross sections |
S.P. Simakov, A. Koning and A.Yu. Konobeyev, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02012. doi:10.1051/epjconf/201714602012 |
|
n+235U resonance parameters and neutron multiplicities in the energy region below 100 eV |
M.T. Pigni, R. Capote, A. Trkov and V.G. Pronyaev, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02011. doi:10.1051/epjconf/201714602011 |
|
Implementation of a new energy-angular distribution of particles emitted by deuteron induced nuclear reaction in transport simulations |
P. Sauvan, A. Koning, F. Ogando and J. Sanz, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02010. doi:10.1051/epjconf/201714602010 |
|
Characterization of the energy-dependent uncertainty and correlation in silicon neutron displacement damage metrics |
P. Griffin, D. Rochman and A. Koning, Proc. ND2016, EPJ Web of Conferences 146 (2017) 02008. doi:10.1051/epjconf/201714602008 |
|
The CIELO collaboration: Progress in international evaluations of neutron reactions on Oxygen, Iron, Uranium and Plutonium |
M.B. Chadwick, et al., Proc. ND2016, EPJ Web of Conferences 146 (2017) 02001 doi:10.1051/epjconf/201714612034 |
|
Study of deuteron-induced nuclear reactions on natural tungsten for the production of theranostic 186Re via AVF cyclotron up to 38 MeV [Abstract] |
M.U. Khandaker, K. Nagatsu, K. Minegishi, T. Wakui, M.R. Zhang, N. Otuka, Nucl. Instrum. Meth. B 403 (2017) pp. 51-68. doi:10.1016/j.nimb.2017.04.087 |
Abstract Activation cross-sections for the natW(d,x)181,182 m,182 g,183,184m,184g,184g(cum),186gRe, 187W and 182g+m+nTa nuclear reactions were measured from the respective thresholds up to 38 MeV by using a stacked-foil activation technique combined with HPGe γ-ray spectrometry. The results are compared with the available literature data and theoretical data extracted from the TENDL-2015 library, and found only a partial agreement among them. Independent cross-sections for the natW(d,x)182g+m+nTa reactions are reported here for the first time. Physical thick target yields for the investigated reaction products were deduced from the measured cross-sections and compared with the directly measured yields found in the literature. The deduced yield curves indicate that a typical irradiation of an enriched 186W target with 100 μA current from a low energy (<18 MeV) deuteron cyclotron is suitable to obtain more than a hundred GBq activity of 186gRe in no carrier added form. | |
|
Thick and thin target 7Li(p,n)7Be neutron spectra below the three-body breakup reaction threshold [Abstract] |
R. Pachuau, B. Lalremruata, N. Otuka, L.R. Hlondo, L.R.M. Punte, H.H. Thanga, Nucl. Sci. Eng. 187 (2017) pp. 70-80. doi:10.1080/00295639.2017.1291053 |
Abstract Recently, we measured the 70Zn(n,γ)71Znm activation cross sections using the 7Li(p,n)7Be neutron source for 2.0 MeV < Ep < 3.7 MeV. Since the time-of-flight and multiple foil activation techniques cannot be applied due to the continuous beam structure and weak neutron flux at the facility, we have to rely on calculated neutron energy spectra for data reduction procedure. There are existing Monte Carlo�??based codes such as Protons In Neutrons Out (PINO) and SimLiT for calculation of 7Li(p,n)7Be neutron source spectra at these energies. However, these two codes predicted different neutron spectra at these energy regions. We therefore decided to study the thick and thin target 7Li(p,n)7Be neutron spectra from the reaction threshold to the three-body breakup threshold by deterministic calculation. The predicted neutron spectra near threshold were validated by experimental neutron spectra. Our neutron spectra were compared with those predicted by PINO and SimLiT. Our neutron spectra at Ep = 2.8 and 3.5 MeV agree perfectly with those predicted by SimLiT but not with those predicted by PINO. | |
|
Measurements of neutron capture cross sections on 70Zn at 0.96 and 1.69 MeV [Abstract] |
L.R.M. Punte, B. Lalremruata, N. Otuka, S.V. Suryanarayana, Y. Iwamoto, R. Pachuau, B. Satheesh, H.H. Thanga, L.S. Danu, V.V. Desai, L.R. Hlondo, S. Kailas, S. Ganesan, B.K. Nayak, A. Saxena, Phys. Rev. C 95 (2017) p.024619. doi:10.1103/PhysRevC.95.024619 |
Abstract The cross sections of the 70Zn(n,γ)71Znm(T1/2=3.96 ±0.05-h) reaction have been measured relative to the 197Au(n,γ)198Au cross sections at 0.96 and 1.69 MeV using a 7
Li(p,n)7Be neutron source and activation technique. The cross section of this reaction has been measured for the first time in the MeV region. The new experimental cross sections have been compared with the theoretical prediction by talys-1.6 with various level-density models and γ-ray strength functions as well as the tendl-2015 library. The talys-1.6 calculation with the generalized superfluid level-density model and Kopecky-Uhl generalized Lorentzian γ-ray strength function predicted the new experimental cross sections at both incident energies. The 70Zn(n,γ)71Zn>g+m total capture cross sections have also been derived by applying the evaluated isomeric ratios in the tendl-2015 library to the measured partial capture cross sections. The spectrum averaged total capture cross sections derived in the present paper agree well with the jendl-4.0 library at 0.96 MeV, whereas it lies between the tendl-2015 and the jendl-4.0 libraries at 1.69 MeV. | |
|
The TENDL library: Hope, reality and future |
D. Rochman, et al., Proc. ND 2016, EPJ Web of Conferences 146 (2017) 02006. doi:10.1051/epjconf/201714602006 |
|
Update of the α - n Yields for Reactor Fuel Materials for the Interest of Nuclear Safeguards [Abstract] |
S.P. Simakov, Q.Y. van den Berg Nucl. Data Sheets 139 (2017) pp. 190-203.
doi:10.1016/j.nds.2017.01.005 |
Abstract The neutron yields caused by spontaneous α-decay of actinides and subsequent (α ,xn) reactions were re-evaluated for the reactor fuel materials UO2, UF6, PuO2 and PuF4. For this purpose, the most recent reference data for decay parameters, α-particle stopping powers and (α,xn) cross sections were collected, analysed and used in calculations. The input data and elaborated code were validated against available thick target neutron yields in pure and compound materials measured at accelerators or with radioactive sources. This paper provides the specific neutron yields and their uncertainties resultant from α -decay of actinides 241Am, 249Bk, 252Cf, 242,244Cm, 237Np, 238�??242Pu, 232Th and 232�??236,238U in oxide and fluoride compounds. The obtained results are an update of previous reference tables issued by the Los Alamos National Laboratory in 1991 which were used for the safeguarding of radioactive materials by passive non-destructive techniques. The comparison of the updated values with previous ones shows an agreement within one estimated uncertainty (�??10%�??10%) for oxides, and deviations of up to 50% for fluorides. | |
|
Production cross-sections of radionuclides from ?-induced reactions on natural copper up to 50 MeV [Abstract] |
A.R. Usman, M.U. Khandaker, H. Haba, N. Otuka, M. Murakami, Y. Komori, Appl. Radiat. Isot. 114 (2016) pp. 104-113. doi:10.1016/j.apradiso.2016.04.027 |
Abstract The excitation functions were measured for the natCu(α,x)66,67Ga,65Zn,57,58,60Co reactions in the energy range of 16.5 �?? 50 MeV. A conventional stacked-foil activation technique combined with HPGe γ-ray spectrometry was employed to determine cross-sections. The measured cross-sections were critically compared with relevant previous experimental data and also with the evaluated data in the TENDL-2014 library. Present results confirmed some of the previous experimental data, whereas only a partial agreement was found with the evaluated data. The measured data are useful for reducing the existing discrepancies in the literature, to improve the nuclear reaction model codes, and to enrich the experimental database towards various applications. | |
|
Neutron-induced fission cross section of237Np in the keV to MeV range at the CERN n TOF facility [Abstract] |
M. Diakaki, P. Dimitriou, R. Capote, et al. (n_TOF Collaboration) Phys. Rev. C 93 (2016) 034614. doi:10.1103/PhysRevC.93.034614 |
Abstract The neutron-induced fission cross section of 237Np was experimentally determined at the high-resolution
and high-intensity facility n TOF, at CERN, in the energy range 100 keV to 9 MeV, using the 235U(n,f) and
238U(n,f ) cross section standards below and above 2 MeV, respectively. A fast ionization chamber was used
in order to detect the fission fragments from the reactions and the targets were characterized as far as their
mass and homogeneity are concerned by means of α spectroscopy and Rutherford backscattering spectroscopy
respectively. Theoretical calculations within the Hauser-Feshbach formalism have been performed, employing
the EMPIRE code, and the model parameters were tuned in order to successfully reproduce the experimental fission
cross-sectional data and simultaneously all the competing reaction channels. | |
|
Effects of Fission Yield Data in the Calculation of Antineutrino Spectra for
235U(n,fission) at Thermal and Fast Neutron Energies [Abstract] |
A.A. Sonzogni, E.A. McCutchan, T.D. Johnson and P. Dimitriou, Phys. Rev. Lett. 116 (2016) 132502. doi:10.1103/PhysRevLett.116.132502 |
Abstract Fission yields form an integral part of the prediction of antineutrino spectra generated by nuclear
reactors, but little attention has been paid to the quality and reliability of the data used in current
calculations. Following a critical review of the thermal and fast ENDF/B-VII.1 235U fission yields,
deficiencies are identified and improved yields are obtained, based on corrections of erroneous yields,
consistency between decay and fission yield data, and updated isomeric ratios. These corrected yields are
used to calculate antineutrino spectra using the summation method. An anomalous value for the thermal
fission yield of 86Ge generates an excess of antineutrinos at 5�??7 MeV, a feature which is no longer present
when the corrected yields are used. Thermal spectra calculated with two distinct fission yield libraries
(corrected ENDF/B and JEFF) differ by up to 6% in the 0�??7 MeV energy window, allowing for a basic
estimate of the uncertainty involved in the fission yield component of summation calculations. Finally, the
fast neutron antineutrino spectrum is calculated, which at the moment can only be obtained with the
summation method and may be relevant for short baseline reactor experiments using highly enriched
uranium fuel. | |
|
Generalized Collisional Radiative Model Using Screened Hydrogenic Levels |
H.-K. Chung, S. H. Hansen, H. A. Scott, Modern Methods in Collisional-Radiative Modeling of Plasmas, pp. 51-79, Ralchenko, Yuri(Ed.), Springer (2016)
doi:10.1007/978-3-319-27514-7_3 |
|
Nanoscale femtosecond imaging of transient hot solid density plasmas with elemental and charge state sensitivity using resonant coherent diffraction |
T. Kluge, M. Bussmann, H.-K. Chung, C. Gutt, L. G. Huang, M. Zacharias, U. Schramm and T. E. Cowan, >Phys. Plasmas 23, 033103 (2016) doi:10.1063/1.4942786 |
|
Detailed model for hot-dense aluminum plasmas generated by an x-ray free electron laser |
O. Ciricosta, S. M. Vinko, H.-K. Chung, C. Jackson, R. W. Lee, T. R. Preston, D. S. Rackstraw and J. S. Wark Phys. Plasmas 23, 022707 (2016) doi:10.1063/1.4942540 |
|
The virtual atomic and molecular data centre (VAMDC) consortium |
M. L. Dubernet, B K Antony, Y A Ba, Yu L Babikov, K Bartschat, V Boudon, B J Braams, H-K Chung et al. J. Phys. B: At. Mol. Opt. Phys. 49 074003 (2016) |
|
Simulations of the time and space-resolved x-ray transmission of a free-electron-laser-heated aluminium plasma |
D S Rackstraw, S M Vinko, O Ciricosta, H-K Chung, R W Lee and J S Wark, J. Phys. B: At. Mol. Opt. Phys. 49 035603 (2016) |
|
Free-Electron X-Ray Laser Measurements of Collisional-Damped Plasmons in Isochorically Heated Warm Dense Matter
|
P. Sperling, E. J. Gamboa, H. J. Lee, H. K. Chung, E. Galtier, Y. Omarbakiyeva, H. Reinholz,
G. Röpke, U. Zastrau, J. Hastings, L. B. Fletcher, and S. H. Glenzer, Phys. Rev. Lett. 115, 115001 (2015)
doi:10.1103/PhysRevLett.115.115001 |
|
Benchmark experiment for the cross section of the 100Mo(p,2n)99mTc and 100Mo(p,pn)99Mo reactions [Abstract] |
S. Takacs, F. Ditroi, M. Aikawa, H. Haba, N. Otuka, Nucl. Instrum. Meth. B 375 (2016) pp. 60-66. doi:10.1016/j.nimb.2016.03.040 |
Abstract As nuclear medicine community has shown an increasing interest in accelerator produced 99mTc radionuclide, the possible alternative direct production routes for producing 99mTc were investigated intensively. One of these accelerator production routes is based on the 100Mo(p,2n)99mTc reaction. The cross section of this nuclear reaction was studied by several laboratories earlier but the available data-sets are not in good agreement. For large scale accelerator production of 99mTc based on the 100Mo(p,2n)99mTc reaction, a well-defined excitation function is required to optimise the production process effectively. One of our recent publications pointed out that most of the available experimental excitation functions for the 100Mo(p,2n)99mTc reaction have the same general shape while their amplitudes are different. To confirm the proper amplitude of the excitation function, results of three independent experiments were presented (Takács et al., 2015). In this work we present results of a thick target count rate measurement of the Eγ = 140.5 keV gamma-line from molybdenum irradiated by Ep = 17.9 MeV proton beam, as an integral benchmark experiment, to prove the cross section data reported for the 100Mo(p,2n)99mTc and 100Mo(p,pn)99Mo reactions in Takács et al. (2015). | |
|
Development of a Reference Database for Particle-Induced Gamma-ray Emission spectroscopy [Abstract] |
P. Dimitriou, H.-W. Becker, Bogdanovic´-Radovic´ , M. Chiari, A. Goncharov, A.P. Jesus, O. Kakuee, A.Z. Kiss, A. Lagoyannis, J. Räisänen, D. Strivay, A. Zucchiatti, Nucl. Instrum. Meth. B 371(2016) pp. 33-36.
doi:10.1016/j.nimb.2015.09.052 |
Abstract Particle-Induced Gamma-ray Emission (PIGE) is a powerful analytical technique that exploits the interactions of rapid charged particles with nuclei located near a sample surface to determine the composition and structure of the surface regions of solids by measurement of characteristic prompt γ rays. The potential for depth profiling of this technique has long been recognized, however, the implementation has been limited owing to insufficient knowledge of the physical data and lack of suitable user-friendly computer codes for the applications. Although a considerable body of published data exists in the nuclear physics literature for nuclear reaction cross sections with γ rays in the exit channel, there is no up-to-date, comprehensive compilation specifically dedicated to IBA applications. A number of PIGE cross-section data had already been uploaded to the Ion Beam Analysis Nuclear Data Library (IBANDL) (http://www-nds.iaea.org/ibandl) by members of the IBA community by 2011, however a preliminary survey of this body of unevaluated experimental data has revealed numerous discrepancies beyond the uncertainty limits reported by the authors. Using the resources and coordination provided by the IAEA, a concerted effort to improve the situation was made within the Coordinated Research Project on the Development of a Reference Database for PIGE spectroscopy, from 2011 to 2015. The aim of the CRP was to create a data library for Ion Beam Analysis that contains reliable and usable data on charged particle γ-ray emission cross sections that would be made freely available to the user community. As the CRP has reached its completion, we shall present its main achievements, including the results of nuclear cross-section evaluations and the development of a computer code that will become available to the public allowing for the implementation of a standardless PIGE technique. | |
|
Validation of IRDFF in 252Cf Standard and IRDF-2002 Reference Neutron Fields [Abstract] |
Stanislav Simakov, Roberto Capote, Lawrence Greenwood, Patrick Griffin, Albert Kahler, Vladimir Pronyaev, Andrej Trkov and Konstantin Zolotarev, EPJ Web of Conferences 106 (2016) 04011. doi:10.1051/epjconf/201610604011 |
Abstract The results of validation of the latest release of International Reactor Dosimetry and Fusion File, IRDFF-1.03, in the standard 252Cf(s.f.) and reference 235U(nth,f) neutron benchmark fields are presented. The spectrum-averaged cross sections were shown to confirm IRDFF-1.03 in the 252Cf standard spontaneous fission spectrum; that was not the case for the current recommended spectra for 235U(nth,f). IRDFF was also validated in the spectra of the research reactor facilities ISNF, Sigma-Sigma and YAYOI, which are available in the IRDF-2002 collection. The ISNF facility was re-simulated to remove unphysical oscillations in the spectrum. IRDFF-1.03 was shown to reproduce reasonably well the spectrum-averaged data measured in these fields except for the case of YAYOI. | |
|
Toward a New Evaluation of Neutron Standards [Abstract] |
A.D. Carlson, V.G. Pronyaev, R. Capote, G.M. Hale, F.-J. Hambsch, T. Kawano, S. Kunieda, W. Mannhart, R.O. Nelson, D. Neudecker, P. Schillebeeckx, S. Simakov, D.L. Smith, P. Talou, X. Tao, A. Wallner and W. Wang, EPJ Web of Conferences 106 (2016) 04002.
doi:10.1051/epjconf/201610604002 |
Abstract Measurements related to neutron cross section standards and certain prompt neutron fission spectra are being evaluated. In addition to the standard cross sections, investigations of reference data that are not as well known as the standards are being considered. Procedures and codes for performing this work are discussed. A number of libraries will use the results of this standards evaluation for new versions of their libraries. Most of these data have applications in neutron dosimetry. | |
|
Systematic study of proton capture reactions in medium-mass nuclei relevant to the p process: The case of 103Rh and 113,115In [Abstract] |
S. Harissopulos, A. Spyrou, V. Foteinou, M. Axiotis, G. Provatas, P. Demetriou, Phys. Rev. C 93 (2016) 025804. doi:10.1103/PhysRevC.93.025804 |
Abstract The cross sections of the 103Rh(p,γ ) 104Pd and the 113,115In(p,γ ) 114,116Sn reactions have been determined from γ angular distribution measurements carried out at beam energies from 2 to 3.5 MeV. An array of four highly efficient HPGe detectors all shielded with BGO crystals for Compton background suppression was used. Astrophysical S factors and reaction rates were deduced from the measured cross sections. Statistical model calculations were performed using the Hauser-Feshbach (HF) code TALYS and were compared with the new data. A good agreement between theory and experiment was found. In addition, the effect of different combinations of the nuclear input parameters entering the HF calculations on the ground-state reaction rates was investigated. It was found that these rates differ by a factor 3 at the most, being thus within the average discrepancies observed between calculated p-nuclei abundances and observations, if certain combinations of optical model potentials,
nuclear level densities, and γ -ray strength functions are used. | |
|
Updated Photonuclear Data Library and Database for Photon Strength Functions [Abstract] |
P. Dimitriou, R.B. Firestone, S. Siem, F. Becvar, M. Krticka, V.V. Varlamov, M. Wiedeking, EPJ Web of Conferences 93 (2015) 06004.
doi:10.1051/epjconf/20159306004 |
Abstract Photonuclear cross sections and gamma-ray data used to extract Photon Strength Functions are important
for a large range of applications including basic sciences. The recommendations of an IAEA Consultant�??s Meeting to
update the IAEA Photonuclear Data Library and create a Reference Database for Photon Strength Functions are
presented. | |
|
Nuclear Data Sheets for A = 227 |
B. Singh, F. Kondev, E. McCutchan, J. Tuli, et al. Nucl. Data Sheets 132 (2016) 257. |
|
Measurements of deuteron-induced reaction cross-sections on natural
nickel up to 24 MeV [Abstract] |
A.R. Usman, M.U. Khandaker, H. Haba, M. Murakami, N. Otuka, Nucl. Instrum. Meth. B 368 (2016) pp. 112-119. doi:10.1016/j.nimb.2015.10.077 |
Abstract Deuteron-induced cross-sections of the natNi(d,x)55�??58,60Co, 57Ni, 52g,54Mn and 61Cu reactions were measured from the respective threshold energies to 24 MeV by using a stacked-foil activation technique combined with HPGe γ-ray spectrometry. The results were compared with the available experimental data and also with the evaluated data in the TENDL-2014 library. Present results show a reasonable agreement with the recently reported experimental data while a partial agreement is found with the evaluated data. The results are expected to further enrich the experimental database and to understand the discrepancies among the previous measurements. The natNi(d,x)61Cu cross-sections recommended by the IAEA overestimate recent experimental ones, and their upgrade has been proposed. | |
|
Excitation functions of deuteron-induced nuclear reactions on natural platinum up to 24 MeV [Abstract] |
M.U. Khandaker, H. Haba, M. Murakami, N. Otuka, H.A. Kassim, Nucl. Instrum. Meth. B 362 (2015) pp. 151-162. doi:10.1016/j.nimb.2015.09.045 |
Abstract Excitation functions of the natPt(d,x)192,193,194,195,196m2,196,198m,198,199Au, 195m,197Pt and 190(g+m1+0.086m2),192(g+m1),194mIr nuclear reactions were measured from the respective threshold up to 24 MeV deuteron energy by using the stacked foil activation technique combined with HPGe gamma-ray spectrometry. Measured data were critically compared with the available literature data and theoretical data extracted from the TENDL-2013 library, and only partial agreement among them was found. Physical thick target yields for the investigated reaction products were also deduced and compared with the directly measured ones in the literature. The deduced yield curves indicate that a low energy cyclotron (<15 MeV) and a highly enriched 198Pt target could be used to obtain 198,199Au in no carrier added form. All cross-sections for 190(g+m1+0.086m2),194mIr and those for 193,194,196m2,196,199Au, and 195m,197Pt in the lower energy region are reported for the first time. | |
|
Investigation of femtosecond collisional ionization rates in a solid-density aluminium plasma [Abstract] |
S. M. Vinko, O. Ciricosta, T. R. Preston, D. S. Rackstraw, C.R.D. Brown, T. Burian, J. Chalupsky, B. I. Cho, H.-K. Chung, K. Engelhorn, R. W. Falcone, R. Fiokovinini, V. Hajkova, P. A. Heimann, L. Juha, H. J. Lee, R. W. Lee, M. Messerschmidt, B. Nagler, W. Schlotter et al. Nature Communications 6. (2015) pp. 6397 doi:10.1038/ncomms7397 |
Abstract The rate at which atoms and ions within a plasma are further ionized by collisions with the
free electrons is a fundamental parameter that dictates the dynamics of plasma systems at
intermediate and high densities. While collision rates are well known experimentally in a few
dilute systems, similar measurements for nonideal plasmas at densities approaching or
exceeding those of solids remain elusive. Here we describe a spectroscopic method to study
collision rates in solid-density aluminium plasmas created and diagnosed using the Linac
Coherent light Source free-electron X-ray laser, tuned to specific interaction pathways around
the absorption edges of ionic charge states. We estimate the rate of collisional ionization in
solid-density aluminium plasmas at temperatures B30 eV to be several times higher than
that predicted by standard semiempirical models. | |
|
Prompt fission neutron spectra in fast-neutron-induced fission of 238U [Abstract] |
V.V. Desai, B.K. Nayak, A. Saxena, S.V. Suryanarayana, R. Capote, Phys. Rev. C 92 014609 doi:10.1103/PhysRevC.92.014609 |
Abstract Prompt fission neutron spectrum (PFNS) measurements for the neutron-induced fission of 238U are carried out at incident neutron energies of 2.0, 2.5, and 3.0 MeV, respectively. The time-of-flight technique is employed to determine the energy of fission neutrons. The prompt fission neutron energy spectra so obtained are analysed using Watt parametrization to derive the neutron multiplicity and average prompt fission neutron energy. The present experimental PFNS data are compared with the evaluated spectra taken from the ENDF/B-VII.1 library and the predictive calculations carried out using the EMPIRE-3.2 (Malta) code with built-in Los Alamos (LA) and Kornilov PFNS models. The sensitivity of the EMPIRE-3.2 LA model�??calculated PFNS to the nuclear level density parameter of the average fission fragment and to the total kinetic energy is investigated. EMPIRE-3.2 LA model PFNS calculations that use Madland 2006�??recommended values [D. G. Madland, Nucl. Phys. A 772,
113 (2006)] of the total kinetic energy and the level density parameter a = A/(10 ± 0.5) compare very well to measured data at all incident neutron incident energies. | |
|
High-accuracy determination of the 238U/ 235U fission cross section ratio up to ? 1 GeV
at n_TOF at CERN [Abstract] |
C. Paradela, M. Calviani, D. Tarr?o, E. Leal-Cidoncha, L. S. Leong, L. Tassan-Got, C. Le Naour, I. Duran, N. Colonna, L. Audouin, M. Mastromarco, S. Lo Meo, A. Ventura, G. Aerts, S. Altstadt, H. Alvarez, F. Alvarez-Velarde, S. Andriamonje, J. Andrzejewski, G. Badurek, M. Barbagallo, P. Baumann, V. Be�cares, F. Becvar, F. Belloni, B. Berthier, E. Berthoumieux, J. Billowes, V. Boccone, D. Bosnar, M. Brugger, F. Calvino, D. Cano-Ott, R. Capote,, et al. (n_TOF Collaboration), Phys. Rev. C 91 024602 doi:10.1103/PhysRevC.91.024602 |
Abstract The 238U to 235U fission cross section ratio has been determined at n_TOF up to �??1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets has been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3�??4%. The data collected at n_TOF have been suitably combined to yield a unique fission cross section ratio as a function of neutron energy. The result confirms current evaluations up to 200 MeV. Good agreement is also observed with theoretical calculations based on the INCL++/Gemini++ combination up to the highest measured energy. The n_TOF results may help solve a long-standing discrepancy between the two most important experimental datasets available so far above 20 MeV, while extending the neutron energy range for the first time up to �??1 GeV. | |
|
TANGRA-Setup for the Investigation of Nuclear Fission induced
by 14.1 MeV neutrons [Abstract] |
I.N. Ruskov, R. Capote Noy, et al., Physics Procedia 64 (2015) pp. 163-170. doi:10.1016/j.phpro.2015.04.022 |
Abstract The new experimental setup TANGRA (Tagged Neutrons & Gamma Rays), for the investigation of neutron induced nuclear
reactions, e.g. (n,xn), (n,xngamma), (n,gamma), (n,f), on a number of important isotopes for nuclear science and engineering (235,238U, 237Np, 239Pu, 244,245,248Cm) is under construction and being tested at the Frank Laboratory of Neutron Physics (FLNP) of the Joint Institute for Nuclear Research (JINR) in Dubna. | |
|
Evaluation of the Prompt Fission Neutron Spectrum of
Thermal-neutron Induced Fission in U-235 [Abstract] |
A. Trkov, R. Capote, Physics Procedia 64 (2015) pp. 48-54. doi:10.1016/j.phpro.2015.04.007 |
Abstract A new evaluation of the prompt fission neutron spectra (PFNS) for the neutron-induced fission of the U-235 nucleus is presented.
By using differential data as �?�shape data�?� good consistency was achieved between selected sets of differential data. A fit of differential
PFNS data with the generalised least-squares method using the GANDR code allowed the estimation of the uncertainties
and correlations. All experimental data were consistently fitted in a model independent way giving a PFNS average energy of
2.000 MeV with an estimated 9 keV uncertainty. | |
|
Impact of the Normalization Condition and Model Information on
Evaluated Prompt Fission Neutron Spectra and Associated Uncertainties [Abstract] |
D. Neudecker, R. Capote, D.L. Smith, T. Burr, P. Talou, Nucl. Scie. Engineering 179 (2015) pp. 381-397. doi:10.13182/NSE14-6 |
Abstract Low evaluated uncertainties compared to experimental information and a strong model impact
were observed in some prompt fission neutron spectrum (PFNS) evaluations that include mean values and
covariances stemming from a rigid model. Here, we show by studying the 239Pu PFNS ENDF/B-VII.1
evaluation via generalized least-squares analyses that strong model correlations in combination with the
normalization condition on the estimated PFNS and its covariances result in surprisingly low evaluated
uncertainties. Furthermore, the model changes the evaluated results by w1s of combined experimental
uncertainties near the average outgoing neutron energy (*2 MeV). We show both analytically and by
means of representative numerical examples that the normalization condition on the spectrum and its
covariances naturally leads to uncertainties reduced by a fully positively correlated scaling uncertainty. | |
|
Evaluation of the 239Pu prompt fission neutron spectrum induced
by neutrons of 500 keV and associated covariances [Abstract] |
D. Neudecker, P. Talou , T. Kawanoa, D.L. Smith, R. Capote, M.E. Rising, A.C. Kahler, Nucl. Instrum. Meth. A 791 (2015) pp. 80-92. doi:10.1016/j.nima.2015.04.044 |
Abstract We present evaluations of the prompt fission neutron spectrum (PFNS) of 239Pu induced by 500 keV
neutrons, and associated covariances. In a previous evaluation by Talou et al.(2010), surprisingly low
evaluated uncertainties were obtained, partly due to simplifying assumptions in the quantification of
uncertainties from experiment and model. Therefore, special emphasis is placed here on a thorough
uncertainty quantification of experimental data and of the Los Alamos model predicted values entering
the evaluation. In addition, the Los Alamos model was extended and an evaluation technique was
employed that takes into account the qualitative differences between normalized model predicted
values and experimental shape data. These improvements lead to changes in the evaluated PFNS and
overall larger evaluated uncertainties than in the previous work. However, these evaluated uncertainties
are still smaller than those obtained in a statistical analysis using experimental information only, due to
strong model correlations. Hence, suggestions to estimate model defect uncertainties are presented,
which lead to more reasonable evaluated uncertainties. The calculated keff of selected criticality
benchmarks obtained with these new evaluations agree with each other within their uncertainties
despite the different approaches to estimate model defect uncertainties.The keff one standard deviations
overlap with some of those obtained using ENDF/B-VII.1, albeit their mean values are further away from
unity. Spectral indexes for the Jezebel critical assembly calculated with the newly evaluated PFNS agree
with the experimental data for selected(n,γ) and (n,f) reactions, and show improvements for high-
energy threshold (n,2n)reactions compared to ENDF/B-VII.1. | |
|
Random Sampling of Correlated Parameters - a Consistent Solution for Unfavourable
Conditions [Abstract] |
G. Žerovnik, A. Trkov, I.A. Kodeli, R. Capote, D.L. Smith, Nucl. Data Sheets 123 (2015) pp. 185-190. doi:10.1016/j.nds.2014.12.032 |
Abstract Two methods for random sampling according to a multivariate lognormal distribution �?? the correlated
sampling method and the method of transformation of correlation coefficients �?? are briefly
presented. The methods are mathematically exact and enable consistent sampling of correlated
inherently positive parameters with given information on the first two distribution moments. Furthermore,
a weighted sampling method to accelerate the convergence of parameters with extremely
large relative uncertainties is described. However, the method is efficient only for a limited number
of correlated parameters. | |
|
Preliminary Evaluation and Uncertainty Quantification of the Prompt Fission Neutron
Spectrum of 239Pu [Abstract] |
D. Neudecker, P. Talou, T.N. Taddeucci, R.C. Haight, T. Kawano,
H.Y. Lee, D.L. Smith, R. Capote, M.E. Rising, and M.C. White, Nucl. Data Sheets 123 (2015) pp. 146-152. doi:10.1016/j.nds.2014.12.026 |
Abstract Low evaluated uncertainties were obtained in a previous evaluation of the 239Pu prompt fission
neutron spectrum and associated covariances for incident neutrons of 0.5 MeV, which were enlarged
a-posteriori before being incorporated into ENDF/B-VII.1. These low evaluated uncertainties triggered
an in-depth study and improved estimate of experimental as well as model uncertainties. Here,
we will summarize these efforts and show that the improved estimate of experimental and model
uncertainties leads to corresponding evaluated uncertainties in good agreement with uncertainties
obtained in a statistical analysis based primarily on experimental information. | |
|
Current Issues in Nuclear Data Evaluation Methodology:
235U Prompt Fission Neutron Spectra and Multiplicity for Thermal Neutrons [Abstract] |
A. Trkov, R. Capote, V.G. Pronyaev, Nucl. Data Sheets 123 (2015) pp. 8-15. doi:10.1016/j.nds.2014.12.003 |
Abstract Issues in evaluation methodology of the prompt fission neutron spectra (PFNS) and neutron
multiplicity for the thermal-neutron-induced fission of the 235U are discussed. The inconsistency
between the experimental differential and integral data is addressed. By using differential data as
�?�shape data�?� good consistency was achieved between available sets of differential data. Integral
dosimetry data have been used to define the PFNS slope at high outgoing neutron energies, where
the quality of the differential data is poor. The inclusion into the fit of measured integral (spectrumaveraged)
cross sections had a very small impact in the region where differential PFNS data are
abundant and accurate, but removed the discrepancy with integral data at higher neutron emission
energies. All experimental data are consistently fitted giving a PFNS average energy of 2.008 MeV.
The impact on criticality prediction of the newly evaluated PFNS was tested. The highly enriched
235U solution assemblies with high leakage HEU-SOL-THERM-001 and HEU-SOL-THERM-009
benchmarks are the most sensitive to the PFNS. Criticality calculations for those solutions show
a significant increase in reactivity if the average neutron energy of the fission neutrons is reduced
from the ENDF/B-VI.5 value of 2.03 MeV. The proposed reduction of the PFNS average energy by
1.1% can be compensated by reducing the average number of neutrons per fission ν at the thermal
energy to the Gwin et al. measured value. The simple least-squares PFNS fit was confirmed by
a more sophisticated combined fit of differential PFNS data for 233,235U, 239Pu and 252Cf nuclides
with the generalised least-squares method using the GMA and GANDR codes. | |
|
Production cross-sections of long-lived radionuclides in deuteron-induced reactions on natural zinc up to 23 MeV [Abstract] |
M.U. Khandaker, H. Haba, M. Murakami, N. Otuka, Nucl. Instrum. Meth. B 346 (2015) pp. 8-16. doi:10.1016/j.nimb.2015.01.011 |
Abstract Production cross-sections of long-lived radionuclides 66,67Ga, 64,67Cu, 65,69mZn, and 58m+gCo via a deuteron irradiation on a natural zinc target were measured up to 23 MeV using a stacked-foil activation technique combined with HPGe γ-ray spectrometry. The present results showed partial agreements with the earlier experimental cross-sections and also with the theoretical data extracted from the TENDL-2013 library. Physical thick target yields of the investigated radionuclides were deduced using the measured cross-sections, and they found agreements with the directly measured ones in the literatures except for those reported by Dmitriev et al. for 65Zn. Optimal production pathways of the medically important 67Ga radionuclide using a low energy cyclotron are discussed. | |
|
Saturable Absorption of an X-Ray Free-Electron-Laser Heated Solid-Density Aluminum Plasma [Abstract] |
D. S. Rackstraw, O. Ciricosta, S. M. Vinko, B. Barbrel, T. Burian, J. Chalupsk� B. I. Cho, H.-K. Chung,
G. L. Dakovski, K. Engelhorn, V. H�jkov�, P. Heimann, M. Holmes, L. Juha, J. Krzywinski, R.W. Lee, S. Toleikis,
J. J. Turner U. Zastrau and J. S. Wark, Phys. Rev. Lett. 114, 015003 (2015) doi:10.1103/PhysRevLett.114.015003 |
Abstract High-intensity x-ray pulses from an x-ray free-electron laser are used to heat and probe a solid-density aluminum sample. The photon-energy-dependent transmission of the heating beam is studied through the use of a photodiode. Saturable absorption is observed, with the resulting transmission differing significantly from the cold case, in good agreement with atomic-kinetics simulations. | |
|
Definitions of radioisotope thick target yields [Abstract] |
N. Otuka and S. Tak�cs, Radiochim. Acta 103 (2015) pp. 1-6. doi:10.1515/ract-2013-2234 |
Abstract Definitions of thick target yields are reviewed in relation to their documentation for the experimental nuclear reaction data library (database). Researchers reporting experimental thick target yields are urged to define their yields clearly with an appropriate unit in order to compile them in the experimental data library (EXFOR) in a consistent manner, and also to properly utilise them for omparison with other experimental and evaluated yields. | |
|
Recent Work Leading Towards a New Evaluation of the Neutron Standards [Abstract] |
A.D. Carlson, V.G. Pronyaev, R. Capote, G.M. Hale, F.-J. Hambsch, T. Kawano, S. Kunieda, W. Mannhart, R.O. Nelson, D. Neudecker, P. Schillebeeckx, S. Simakov, D.L. Smith, P. Talou, X. Tao, A. Wallner, W. Wang Nucl. Data Sheets 123 (2015) pp. 27?35 doi:doi:10.1016/j.nds.2014.12.006 |
Abstract A new version of the ENDF/B library has been planned. The first step in producing this new library is evaluating the neutron standards. An evaluation is now underway with support from a Data Development Project of the IAEA. In addition to the neutron cross section standards, new evaluations are being done for prompt fission neutron spectra and a number of reference data. Efforts have been made to handle uncertainties in a proper way in these evaluations. | |
|
Opacity effects in a solid-density aluminium plasma created by
photo-excitation with an X-ray laser [Abstract] |
D. S., Rackstraw, S. M. Vinko, O. Ciricosta, B. I. Cho, K. Engelhorn, H.-K. Chung, ... & J. Wark, High Energy Density Physics, 11, pp. 59-69 (2014) doi:10.1016/j.hedp.2014.02.003 |
Abstract The intensities within the focal spots of the output of recently developed X-ray sources based on free electron- laser (FEL) technology are so great that atoms within the focal region can potentially absorb several photons during the few tens of femtosecond X-ray pulse. Furthermore, the duration of the FEL Xray pulse is comparable to the Auger decay times of inner-shell holes created by the X-rays themselves.
We report here how such a scenario can lead to opacity broadening of the fluorescence radiation emitted by the hot, dense plasma, which is created as a result of the X-radiation focussed onto a solid target, and in particular present calculations of the broadening of the Ka emission in a solid-density aluminium target, produced when the FEL photon energy is tuned below the Al K-edge, but is resonant with the Ka transition. | |
|
Measurement and analysis of the 243Am neutron capture cross section at the n_TOF facility at CERN [Abstract] |
E. Mendoza, R. Capote, et al., (n_TOF Collaboration) Phys. Rev. C 90 (2014) 034608 doi:10.1103/PhysRevC.90.034608 |
Abstract Background: The design of new nuclear reactors and transmutation devices requires to reduce the present
neutron cross section uncertainties of minor actinides.
Purpose: Improvement of the 243Am(n,γ) cross section uncertainty.
Method: The 243Am(n,γ) cross section has been measured at the n_TOF facility at CERN with a BaF2 total
absorption calorimeter, in the energy range between 0.7 eV and 2.5 keV.
Results: The 243Am(n,γ) cross section has been successfully measured in the mentioned energy range. The
resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region
our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data
available in EXFOR and in the literature have been used to perform a simple analysis above 2.5 keV.
Conclusions: The results of this measurement contribute to reduce the 243Am(n,γ) cross section uncertainty and
suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few
keV in the present evaluated data libraries. | |
|
Uncertainties of mass extrapolations in Hartree-Fock-Bogoliubov mass models [Abstract] |
S. Goriely, R. Capote, Phys. Rev. C 89 (2014) 054318 doi:10.1103/PhysRevC.89.054318 |
Abstract Some 27 Hartree-Fock-Bogoliubov (HFB) mass models have been developed by the Brussels-Montreal
collaboration. Each of these models has been obtained with different model prescriptions or corresponds to a
significantly differentminimum in the parameter space. The corresponding uncertainties in the mass extrapolation
are discussed. In addition, for each of these models, uncertainties associated with local variations of the model
parameters exist. Those are estimated for the HFB-24 mass model using a variant of the backward-forwardMonte
Carlo method to propagate the uncertainties on the masses of exotic nuclei far away from the experimentally
known regions. The resulting uncertainties are found to be significantly lower than those arising from the 27 HFB
mass models. In addition, the derived correlations between the calculated masses and between model parameters
are analyzed. | |
|
Neutron-induced fission cross section of 234U measured at the CERN n_TOF facility [Abstract] |
R. Sarmento, P. Demetriou, R. Capote, et al., (n_TOF Collaboration), Phys. Rev. C 89 (2014) 044606 doi:10.1103/PhysRevC.89.044606 |
Abstract The neutron-induced fission cross section of 234U has been measured at the CERN n_TOF facility relative to the
standard fission cross section of 235U from 20 keV to 1.4 MeV and of 238U from 1.4 to 200 MeV. A fast ionization
chamber (FIC) was used as a fission fragment detector with a detection efficiency of no less than 97%. The
high instantaneous flux and the low background characterizing the n_TOF facility resulted in wide-energy-range
data (0.02 to 200 MeV), with high energy resolution, high statistics, and systematic uncertainties bellow 3%.
Previous investigations around the energy of the fission threshold revealed structures attributed to β-vibrational
levels, which have been confirmed by the present measurements. Theoretical calculations have been performed,
employing the TALYS code with model parameters tuned to fairly reproduce the experimental data. | |
|
Evaluation of neutron-induced reactions on 238U nucleus [Abstract] |
R. Capote, M. Sin, A. Trkov, M.W. Herman,
D. Bernard, G. Nogu�re, A. Daskalakis, Y. Danon, Procs. Workshop "Nuclear Measurements, Evaluations and Applications (NEMEA-7) Collaborative International Evaluated Library Organisation (CIELO)", 5-8 November 2013, Geel, Belgium, NEA/NSC/DOC(2014)13, OECD 2014, pp. 113-118 |
Abstract Advanced modelling of neutron-induced reactions on 238U nucleus using the
EMPIRE system is aimed at improving our knowledge of the neutron scattering
leading to better nuclear data for nuclear power applications. Capture and fission
channels in n + 238U reaction are well constrained by available experimental data
and IAEA neutron standard evaluations allowing to focus on the impact of elastic
and inelastic scattering in evaluated cross-sections. The reaction model includes:
i) a new rotational-vibrational dispersive optical model that couples the low-lying
collective bands of vibrational character observed in even-even actinides; ii) the
Engelbrecht-Weidenmüller transformation allowing inclusion of compound-direct
interference effects enhanced by a dispersive treatment of the optical model
potential; iii) a multi-humped fission barrier with absorption in the secondary well
described within the optical model for fission. Impact of the advanced modelling
on inelastic scattering cross-section and corresponding uncertainties is being
assessed both by comparison with selected microscopic experimental data and
integral criticality benchmarks including measured reaction rates (e.g. FLATTOP,
JEMIMA, BIGTEN, MASURCA, PROFIL and PROFIL-2). Additionally, neutron scattering
yields on 238U measured accurately at RPI by the time-of-flight technique at 29°,
60°, 112° and 153° have been used as a further constraint on the incident energy
dependence of elastic and inelastic scattering of neutrons. Benchmark calculations
provided feedback to improve the reaction modelling. The improvement of
scattering cross-sections in existing libraries is discussed. | |
|
Neutron-induced reactions on U and Th ? A new approach via AMS [Abstract] |
A. Wallner, R. Capote, M. Christl, L.K. Fifield, M. Hotchkis, A. Krasa, J. Lachner, J. Lippold, A. Plompen, V. Semkova, M. Srncik, P. Steier, S. Tims, S. Winkler, Procs. Workshop "Nuclear Measurements, Evaluations and Applications (NEMEA-7) Collaborative International Evaluated Library Organisation (CIELO)", 5-8 November 2013, Geel, Belgium, NEA/NSC/DOC(2014)13, OECD 2014, pp. 159-167 |
Abstract Recent studies exhibit discrepancies at keV and MeV energies between major
nuclear data libraries for 238U(n,γ), 232Th(n,γ) and also for (n,xn) reactions. We have
extended our initial (n,γ) measurements on 235,238U to higher neutron energies and
to additional reaction channels. Neutron-induced reactions on 232Th and 238U were
measured by a combination of the activation technique and atom counting of the
reaction products using accelerator mass spectrometry (AMS). Natural thorium and
uranium samples were activated with quasi-monoenergetic neutrons at IRMM.
Neutron capture data were produced for neutron energies between 0.5 and 5 MeV.
Fast neutron-induced reactions were studied in the energy range from 17 to 22 MeV.
Preliminary data indicate a fair agreement with data libraries; however at the
lower band of existing data. This approach represents a complementary method
to on-line particle detection techniques and also to conventional decay counting. | |
|
Nuclear data for medical applications ? Recent developments and future requirements [Abstract] |
A.L. Nichols, R. Capote, Nucl. Data Sheets 120 (2014) pp. 239?241 doi:10.1016/j.nds.2014.07.056 |
Abstract Cancer treatment represents a major economic and medical issue because of the extensive incidence
of the disease worldwide, with a particularly large rate of increase to be found in developing
countries. Over the previous twenty years, the International Atomic Energy Agency (IAEA) has
dedicated a series of investigations towards identifying and quantifying the production routes and
decay characteristics of radioisotopes judged to be of existing and emerging importance in nuclear
medicine and radiotherapy. Both the recommendations formulated during the course of these technical
debates and the results of recently completed and on-going IAEA coordinated research projects
are focused towards the successful evolution of improvements in nuclear data for medical applications
throughout the early 21st century. | |
|
Measurement of the MACS of 159Tb(n,?) at kT = 30 keV by activation [Abstract] |
J. Praena, P.F. Mastinu, M. Pignatari, J.M. Quesada, R. Capote, Y. Morilla, Nucl. Data Sheets 120 (2014) pp. 205?207 doi:10.1016/j.nds.2014.07.047 |
Abstract The measurement of the Maxwellian-Averaged Cross-Section (MACS) of the 159Tb(n,γ) reaction
at kT = 30 keV by the activation technique is presented. An innovative method for the generation
of Maxwellian neutron spectra at kT = 30 keV is used. An experimental value of 2166±181 mb
agrees well with the MACS value derived from the ENDF/B-VII.1 evaluation, but is higher than
KADoNiS recommended value of 1580±150 mb. Astrophysical implications are studied. | |
|
EMPIRE: A reaction model code for nuclear astrophysics [Abstract] |
A. Palumbo, M. Herman, R. Capote, Nucl. Data Sheets 120 (2014) pp. 180?183 doi:10.1016/j.nds.2014.07.040 |
Abstract The correct modeling of abundances requires knowledge of nuclear cross sections for a variety of
neutron, charged particle and γ induced reactions. These involve targets far from stability and are
therefore difficult (or currently impossible) to measure. Nuclear reaction theory provides the only
way to estimate values of such cross sections. In this paper we present application of the EMPIRE
reaction code to nuclear astrophysics. Recent measurements are compared to the calculated cross
sections showing consistent agreement for n-, p- and α- induced reactions of astrophysical relevance. | |
|
Evaluation of neutron resonance cross section data at GELINA [Abstract] |
P. Schillebeeckx, B. Becker, R. Capote, F. Emiliani, K. Guber, J. Heyse, K. Kauwenberghs,
S. Kopecky, C. Lampoudis, C. Massimi, W. Mondelaers, M. Moxon, G. Noguere,
A.J.M. Plompen, V. Pronyaev, P. Siegler, I. Sirakov, A. Trkov, K. Volev, G. Zerovnik, Nucl. Data Sheets 119 (2014) pp. 94?97 doi:10.1016/j.nds.2014.08.027 |
Abstract Over the last decade, the EC�??JRC�??IRMM, in collaboration with other institutes such as INRNE
Sofia (BG), INFN Bologna (IT), ORNL (USA), CEA Cadarache (FR) and CEA Saclay (FR), has
made an intense effort to improve the quality of neutron-induced cross section data in the resonance
region. These improvements relate to both the infrastructure of the facility and the measurement
setup, and the data reduction and analysis procedures. As a result total and reaction cross section
data in the resonance region with uncertainties better than 0.5 % and 2 %, respectively, can be
produced together with evaluated data files for both the resolved and unresolved resonance region.
The methodology to produce full ENDF compatible files, including covariances, is illustrated by the
production of resolved resonance parameter files for 241Am, Cd and W and an evaluation for 197Au
in the unresolved resonance region. | |
|
Study of 234U(n,f) resonances measured at the CERN n_TOF facility [Abstract] |
E. Leal-Cidoncha, R. Capote, et al., Nucl. Data Sheets 119 (2014) pp. 42?44 doi:10.1016/j.nds.2014.08.013 |
Abstract We present the analysis of the resolved resonance region for the 234U(n,f) cross section data
measured at the CERN n_TOF facility. The resonance parameters in the energy range from 1 eV
to 1500 eV have been obtained with the SAMMY code by using as initial parameters for the fit
the resonance parameters of the JENDL-3.3 evaluation. In addition, the statistical analysis has
been accomplished, partly with the SAMDIST code, in order to study the level spacing and the
Mehta-Dyson correlation. | |
|
Evaluation of the covariance matrix of estimated resonance parameters [Abstract] |
B. Becker, R. Capote, S. Kopecky, C. Massimi, P. Schillebeeckx, I. Sirakov, K. Volev, Nucl. Data Sheets 118 (2014) pp. 381?383 doi:10.1016/j.nds.2014.04.086 |
Abstract In the resonance region nuclear resonance parameters are mostly obtained by a least square
adjustment of a model to experimental data. Derived parameters can be mutually correlated through
the adjustment procedure as well as through common experimental or model uncertainties. In this
contribution we investigate four different methods to propagate the additional covariance caused by
experimental or model uncertainties into the evaluation of the covariance matrix of the estimated
parameters: (1) including the additional covariance into the experimental covariance matrix based
on calculated or theoretical estimates of the data; (2) including the uncertainty affected parameter
in the adjustment procedure; (3) evaluation of the full covariance matrix by Monte Carlo sampling
of the common parameter; and (4) retroactively including the additional covariance by using the
marginalization procedure of Habert et al. | |
|
Exclusive multiple emission cross sections in the hybrid Monte Carlo
pre-equilibrium model and in EMPIRE-3.1 [Abstract] |
B.V. Carlson, L. Brito, D.F. Mega, R. Capote, M. Herman, M.E. Rego, Nucl. Data Sheets 118 (2014) pp. 276?279 doi:10.1016/j.nds.2014.04.057 |
Abstract We discuss the general concept of exclusive emission cross sections and spectra and the exclusive
spectra of the ENDF library. We briefly review the exclusive hybrid Monte Carlo simulation model
and show how its exclusive cross sections can be integrated into the reaction code EMPIRE-3.1. We
close by discussing several examples. | |
|
Rotational-vibrational description of nucleon scattering on actinide nuclei
using a dispersive coupled-channel optical model [Abstract] |
J.M. Quesada, R. Capote, E.Sh. Soukhovitski?, S. Chiba, Nucl. Data Sheets 118 (2014) pp. 270-272 doi:10.1016/j.nds.2014.04.055 |
Abstract Tamura�??s coupling formalism has been extended to consider low-lying rotational bands built on
vibrational (single-particle) band heads in well-deformed even-even (odd) actinides. These additional
excitations are introduced as a perturbation to the underlying rigid rotor structure that is
known to describe well the ground state rotational band of major actinides. Coupling matrix elements
needed in extended Tamura�??s formalism are derived for both even-even and odd actinides.
Employed dispersive optical model (DCCOMP) replaces the incident proton energy Ep (for proton
induced reactions) by the equivalent Coulomb subtracted energy in all potential terms including
both the imaginary and real potentials with the corresponding dispersive corrections. Therefore,
the optical potential becomes fully symmetric for protons and neutrons. This potential is used to
fit simultaneously all the available optical experimental databases (including neutron strength functions)
for nucleon scattering on 238U and 232Th (even even) nuclei. Quasi-elastic (p,n) scattering
data to the isobaric analogue states of the target nuclei are also used to constrain the isovector
part of the optical potential. Derived Lane-consistent DCCOMP is based on coupling of almost all
levels below 1 MeV of excitation energy. The ground state, octupole, beta, gamma and non-axial
rotational bands are considered for even nuclei, and rotational bands built on single-particle levels
�?? for odd nuclei. Application of derived potential to odd targets based on a new coupling scheme is
foreseen. | |
|
Fitting prompt fission neutron spectra using Kalman filter integrated with Empire code [Abstract] |
G.P.A. Nobre, M. Herman, S. Hoblit, A. Palumbo, R. Capote, A. Trkov, Nucl. Data Sheets 118 (2014) pp. 224-226 doi:10.1016/j.nds.2014.04.042 |
Abstract Prompt fission neutron spectra (PFNS) have proven to have a significant effect on criticality of
selected benchmarks, in some cases as important as cross-sections. Therefore, a precise determination
of uncertainties in PFNS is desired. Existing PFNS evaluations in nuclear data libraries relied
so far almost exclusively on the Los Alamos model. However, deviations of evaluated data from
available experiments have been noticed at both low and high neutron emission energies. New experimental
measurements of PFNS have been recently published, thus demanding new evaluations.
The present work describes the effort of integrating Kalman and EMPIRE codes in such a way to
allow for parameter fitting of PFNS models. The first results are shown for the major actinides
for two different PFNS models (Kornilov and Los Alamos). This represents the first step towards
reevaluation of both cross-section and fission spectra data considering both microscopic and integral
experimental data for major actinides. | |
|
A fully Lane-consistent dispersive optical model potential for even Fe isotopes
based on a soft-rotator model [Abstract] |
W. Sun, R. Li, E.Sh. Soukhovitski?, J.M. Quesada, R. Capote, Nucl. Data Sheets 118 (2014) pp. 191-194 doi:10.1016/j.nds.2014.04.034 |
Abstract A fully Lane-consistent dispersive coupled-channel optical model (DCCOM) potential is derived
that describes nucleon induced reactions on even iron isotopes. Low-lying structure of excited levels
in iron even-even isotopes is described by a soft-rotator model that allows for dynamical deformation
around the spherical shape. Soft-rotator Hamiltonian parameters are adjusted to reproduce
the experimental energies of the low-lying collective levels of these isotopes. The comprehensive
experimental database used in the fitting process included all scattering data for neutron and proton
scattering up to 200 MeV. Employed Lane-consistent formalism allows deriving a potential
fully symmetric for neutrons and protons. Lane consistency of the derived potential was validated
by describing the quasi-elastic (p,n) scattering with excitation of IAS states. An exact approach
for calculation of inelastic analyzing powers is derived. Calculated elastic and inelastic analyzing
powers both for neutron and proton induced reactions were shown to be in good agreement with
experimental data demonstrating the reliability of dispersive spin-orbit potential. | |
|
Fluctuations above the resonance range in evaluated data of 55Mn [Abstract] |
A. Trkov, R. Capote, L.C. Leal, D.W. Muir, E.Sh. Soukhovitski?, Nucl. Data Sheets 118 (2014) pp. 161-164 doi:10.1016/j.nds.2014.04.026 |
Abstract The evaluation procedures for 55Mn are elaborated, focusing on the issues related to the fluctuations
in the cross sections above the resolved resonance range. Smooth cross sections are defined in
the unresolved resonance range, based on the resolution-broadened total cross section measurements,
where relevant. Above this energy fluctuations in the measured total cross section are introduced
by scaling all reaction cross sections, but preserving the resolution-broadened total cross section.
Special procedures are designed to match the observed structure in the average cosine of scattering
by adjusting the ratio of the shape-elastic and compound-elastic contributions to the elastic scattering
cross sections. The evaluated data file is being assembled and subjected to rigorous testing,
verification and validation. | |
|
Zirconium evaluations for ENDF/B-VII.2 for the fast region [Abstract] |
D.A. Brown, R. Arcilla, R. Capote, S.F. Mughabghab, M.W. Herman, A. Trkov, H.I. Kim, Nucl. Data Sheets 118 (2014) pp. 144?146 doi:10.1016/j.nds.2014.04.021 |
Abstract We have performed a new combined set of evaluations for 90�??96Zr, including new resolved resonance
parameterizations from Said Mughabghab for 90,91,92,94,96Zr and fast region calculations
made with EMPIRE-3.1. Because 90Zr is a magic nucleus, stable Zr isotopes are nearly spherical.
A new soft-rotor optical model potential is used allowing calculations of the inelastic scattering on
low-lying coupled levels of vibrational nature. A soft rotor model describes dynamical deformations
of the nucleus around the spherical shape and is implemented in EMPIRE/OPTMAN code. The
same potential is used with rigid rotor couplings for odd-A nuclei. This then led to improved elastic
angular distributions, helping to resolve improper leakage in the older ENDF/B-VII.1β evaluation
in KAPL proprietary, ZPR and TRIGA benchmarks. Another consequence of 90Zr being a magic
nucleus is that the level densities in both 90Zr and 91Zr are unusually low causing the (n,el) and
(n,tot) cross sections to exhibit large fluctuations above the resolved resonance region. To accommodate
these fluctuations, we performed a simultaneous constrained generalized least-square fit to
(n,tot) for all isotopic and elemental Zr data in EXFOR, using EMPIRE�??s TOTRED scaling factor.
TOTRED rescales total cross sections so that the optical model calculations are unaltered by the
rescaling and the correct competition between channels is maintained. In this fit, all (n,tot) data
in EXFOR was used for Ein > 100 keV, provided the target isotopic makeup could be correctly
understood, including spectrum averaged data and data with broad energy resolution. As a result
of our fitting procedure, we will have full cross material and cross reaction covariance for all Zr
isotopes and reactions. | |
|
Physics of neutron interactions with 238U: New developments and challenges [Abstract] |
R. Capote, A. Trkov, M. Sin, M. Herman, A. Daskalakis, Y. Danon, Nucl. Data Sheets 118 (2014) pp. 26-31 doi:10.1016/j.nds.2014.04.003 |
Abstract The latest release of the EMPIRE-3.1 system (codename Rivoli) is being used in the advanced
modeling of neutron induced reactions on the 238U nucleus with the aim of improving our knowledge
of neutron scattering. The reaction model includes: (i) a new rotational-vibrational dispersive
optical model potential coupling the low-lying collective bands of vibrational character observed
in even-even actinides, (ii) the Engelbrecht-Weidenmüller transformation allowing for inclusion of
compound-direct interference effects enhanced by a dispersive treatment of the optical model potential,
(iii) a multi-humped fission barrier with absorption in the secondary well as described within
the optical model for fission, and (iv) a modified Lorentzian model (MLO) of the radiative strength
function. Impact of the advanced modeling on elastic and inelastic scattering cross section is being
assessed by both comparison with selected microscopic experimental data and integral criticality
benchmarks (e.g. FLATTOP, JEMIMA and BIGTEN assemblies). Benchmark calculations provide
feedback to improve the reaction modeling and reduce both model and model-parameters uncertainties.
Additionally, neutron scattering yields on 238U measured accurately at RPI by the time-of-flight
technique at 29, 60, 112 and 153 degrees have been used as a further constraint on the incident energy
dependence of elastic and inelastically scattered neutrons. Improvement of scattering cross
sections in existing libraries is discussed. | |
|
Elastic and inelastic scattering of neutrons on 238U nucleus [Abstract] |
R. Capote, A. Trkov, M. Sin, M.W. Herman, E.Sh. Soukhovitski?, EPJ Web of Conferences 69 00008 (2014) doi:10.1051/epjconf/20136900008 |
Abstract Advanced modelling of neutron induced reactions on the 238U nucleus is aimed
at improving our knowledge of neutron scattering. Capture and fission channels are well
constrained by available experimental data and neutron standard evaluation. A focus
of this contribution is on elastic and inelastic scattering cross sections. The employed
nuclear reaction model includes �?? a new rotational-vibrational dispersive optical model
potential coupling the low-lying collective bands of vibrational character observed in
even-even actinides; �?? the Engelbrecht-Weidenmüller transformation allowing for inclusion
of compound-direct interference effects; �?? and a multi-humped fission barrier with
absorption in the secondary well described within the optical model for fission. Impact
of the advanced modelling on elastic and inelastic scattering cross sections including angular
distributions and emission spectra is assessed both by comparison with selected
microscopic experimental data and integral criticality benchmarks including measured
reaction rates (e.g. JEMIMA, FLAPTOP and BIG TEN). Benchmark calculations provided
feedback to improve the reaction modelling. Improvement of existing libraries will
be discussed. | |
|
Quasi-differential neutron scattering from 238U from 0.5 to 20 MeV [Abstract] |
A.M. Daskalakis, R.M. Bahran, E.J. Blain, B.J. McDermott, S. Piela, Y. Danon, D.P. Barry, G. Leinweber, R.C. Block, M.J. Rapp, R. Capote, A. Trkov, Ann. Nucl. Energy 73 (2014) pp. 455-464
doi:10.1016/j.anucene.2014.07.023 |
Abstract The Rensselaer Polytechnic Institute Linear Accelerator was used to produce a pulsed neutron beam that was incident on a 238U scattering sample 30 m from the source. Eight liquid scintillator (EJ-301) proton recoil fast neutron detectors located at several angles surrounding the sample were positioned at a distance 0.5 m. Neutrons resulting from elastic scattering, inelastic scattering, and fission reactions were recorded as a function of time-of-flight. Pulse shape analysis including a new gamma misclassification correction was used to reduce erroneous counts from gamma events produced from fission and inelastic scattering reactions. The experimental data were simulated using an improved model of the Rensselaer
Polytechnic Institute neutron scattering system that included individual detector efficiencies and neutron flux shape. The experimental data were compared with several evaluated nuclear data libraries using a figure-of-merit. Overall, the JENDL-4.0 evaluation provided the best agreement with the 238U experimental data. Furthermore, the Rensselaer Polytechnic Institute scattering model was used to constrain uncertainties that allowed for improvements to a new 238U evaluation. | |
|
Recent Developments in the Experimental Nuclear Reaction Data Library EXFOR [Abstract] |
V. Semkova, N. Otuka, S. Simakov, V. Zerkin, EPJ Web of Conferences 66 03078 (2014) doi:10.1051/epjconf/20146603078 |
Abstract The International Network of Nuclear Reaction Data Centres (NRDC)
provides nuclear reaction data services to users through collection and compilation of
experimental nuclear reaction data in the EXFOR database. The database includes
neutron-induced, charged-particle-induced, and photonuclear data for projectile energies
up to 1 GeV. Sophisticated search options and user-friendly retrieval interface for
downloading data in different formats have been developed at IAEA Nuclear Data
Section. Additional output options such as data plotting capabilities are provided as well. The database is constantly revised and extended and at present contains about 20,000 experimental works accumulated in its 40 years of history. The paper will present several recent IAEA NDS activities related to the development of the EXFOR database and retrieval system. | |
|
Measurement of Neutron Activation Cross Sections on Mo isotopes in the Energy Range from 7 MeV to 15 MeV [Abstract] |
Valentina Semkova, Ralf Nolte, EPJ Web of Conferences 66 03077 (2014) doi:10.1051/epjconf/20146603077 |
Abstract An experimental study of the 92Mo(n,p)92Nbm, 92Mo(n,α)89Zr, 95Mo(n,p)95mNb, 95Mo(n,p)95Nb, 96Mo(n,p)96Nb, 97Mo(n,p)97Nb, 98Mo(n,p)98Nbm, 98Mo(n,α)95Zr, 100Mo(n,α) 97Zr, and 92Mo(n,2n)99Mo activation reaction cross sections were carried out in the 7-15 MeV energy range at the CV28 compact cyclotron at Physikalisch-Technische
Bundesanstalt, Braunschweig. The PTB TOF spectrometer with a D(d,n) source is well suited for this difficult energy range were significant correction for non-monoenergetic neutrons have to be applied. Gamma-ray spectrometry was applied for the measurements of the activity of the reaction products. | |
|
Quality Assurance of the Cross-sections Measured on p+Li/C Source [Abstract] |
M. Majerle, P. Bém, J. Novák, E.Šimečková, M.Štefánik, S. Simakov, and U. Fischer, Nuclear Data Sheets 119 (2014) 425-428 doi:doi:10.1016/j.nds.2014.08.120 |
Abstract Irradiation of material with quasi-monoenergetic neutrons with energies up to 35 MeV is routinely used for cross-section measurement. Neutron irradiation, gamma measurement, and cross-section extraction are three steps in obtaining the final cross-section, each of them contributing to the final uncertainty. The nature of the spectra, which consists of the monoenergetic peak and the continuum at lower energies, makes the extraction of the cross-sections a non-trivial problem and
different methods of extraction are used. In this paper, we identify the main sources of uncertainties, discuss possible improvements, and address the differences between some commonly used methods of cross-section extraction. | |
|
The Neutrons for Science Facility at SPIRAL-2 [Abstract] |
X. Ledoux, M. Aïche, M. Avrigeanu, V. Avrigeanu, L. Audouin, E. Balanzat, B. Ban-d´etat, G. Ban, G. Barreau, E. Bauge, G. Belier, P. Bem, V. Blideanu, C. Borcea, S. Bouffard, T. Caillaud, A. Chatillon, S. Czajkowski, P. Dessagne, D. Doré, M. Fallot, F. Farget, U. Fischer, L. Giot, T. Granier, S. Guillous, F. Gunsing, C. Gustavsson, B. Jacquot, K. Jansson, B. Jurado, M. Kerveno, A. Klix, O. Landoas, F.R. Lecolley, J.L. Lecouey, M. Majerl, N. Marie, T. Materna, J. Mrazek, F. Negoita, J. Novak, S. Oberstedt, A. Oberstedt, S. Panebianco, L. Perrot, A.J.M. Plompen, S. Pomp, J.M. Ramillon, D. Ridikas, B. Rossé, G. Rudolf, O. Serot, S.P. Simakov, E. Simeckova, A.G. Smith, J.C. Sublet, J. Taieb, L. Tassan-Got, D. Tarrio, A. Takibayev, I. Thfoin, I. Tsekhanovich, and C. Varignon, Nuclear Data Sheets 119 (2014) 353-356 doi:doi:10.1016/j.nds.2014.08.097 |
Abstract The Neutrons For Science (NFS) facility is a component of SPIRAL-2 laboratory under construction at Caen (France). SPIRAL-2 is dedicated to the production of high intensity Radioactive Ions Beams (RIB). It is based on a high-power linear accelerator (LINAG) to accelerate deuterons beams in order to produce neutrons by breakup reactions on a C converter. These neutrons will
induce fission in 238U for production of radioactive isotopes. Additionally to the RIB production, the proton and deuteron beams delivered by the accelerator will be used in the NFS facility. NFS is composed of a pulsed neutron beam and irradiation stations for cross-section measurements and material studies. The beams delivered by the LINAG will allow producing intense neutron beams in the 100 keV-40 MeV energy range with either a continuous or quasi-mono-energetic spectrum. At NFS available average fluxes will be up to 2 orders of magnitude higher than those of other existing time-of-flight facilities in the 1 MeV - 40 MeV range. NFS will be a very powerful tool for fundamental physics and application related research in support of the transmutation of nuclear waste, design of future fission and fusion reactors, nuclear medicine or test and development of
new detectors. The facility and its characteristics are described, and several examples of the first potential experiments are presented. | |
|
The CIELO Collaboration: Neutron Reactions on 1H, 16O, 56Fe, 235,238U, and 239Pu [Abstract] |
M.B. Chadwick, E. Dupont, E. Bauge, A. Blokhin, O. Bouland, D.A. Brown, R. Capote, A. Carlson, Y. Danon, C. De Saint Jean, M. Dunn, U. Fischer, R.A. Forrest, S.C. Frankle, T. Fukahori, Z. Ge, S.M. Grimes, G.M. Hale, M. Herman, A. Ignatyuk, M. Ishikawa, N. Iwamoto, O. Iwamoto, M. Jandel, R. Jacqmin, T. Kawano, S. Kunieda, A. Kahler, B. Kiedrowski, I. Kodeli,
A.J. Koning, L. Leal, Y.O. Lee, J.P. Lestone, C. Lubitz, M. MacInnes, D. McNabb, R. McKnight, M. Moxon, S. Mughabghab, G. Noguere, G. Palmiotti, A. Plompen, B. Pritychenko, V. Pronyaev, D. Rochman, P. Romain, D. Roubtsov, P. Schillebeeckx, M. Salvatores, S. Simakov, E.Sh. Soukhovitski?, J.C. Sublet, P. Talou, I. Thompson, A. Trkov, R. Vogt, and S. van der Marck, Nuclear Data Sheets 118 (2014)
pp. 1-25 doi:10.1016/j.nds.2014.04.002 |
Abstract CIELO (Collaborative International Evaluated Library Organization) provides a new working paradigm to facilitate evaluated nuclear reaction data advances. It brings together experts from across the international nuclear reaction data community to identify and document discrepancies among existing evaluated data libraries, measured data, and model calculation interpretations, and aims to make progress in reconciling these discrepancies to create more accurate ENDF-formatted files. The focus will initially be on a small number of the highest-priority isotopes, namely 1H, 16O, 56Fe, 235,238U, and 239Pu. This paper identifies discrepancies between various evaluations of the highest priority isotopes, and was commissioned by the OECD�??s Nuclear Energy Agency WPEC (Working Party on International Nuclear Data Evaluation Co-operation) during a meeting held in
May 2012. The evaluated data for these materials in the existing nuclear data libraries �?? ENDF/BVII.1, JEFF-3.1, JENDL-4.0, CENDL-3.1, ROSFOND, IRDFF 1.0 �?? are reviewed, discrepancies are identified, and some integral properties are given. The paper summarizes a program of nuclear science and computational work needed to create the new CIELO nuclear data evaluations. | |
|
Working Party on International Nuclear Data Evaluation Cooperation (WPEC) [Abstract] |
E. Dupont, M.B. Chadwick, Y. Danon, C. De Saint Jean, M. Dunn, U. Fischer, R.A. Forrest,
T. Fukahori, Z. Ge, H. Harada, M. Herman,0 M. Igashira,1 A. Ignatyuk,2 M. Ishikawa, O. Iwamoto,8
R. Jacqmin, A.C. Kahler, T. Kawano, A.J. Koning,3 L. Leal, Y.O. Lee,4 R. McKnight,
D. McNabb, R.W. Mills, G. Palmiotti, A. Plompen, M. Salvatores, and P. Schillebeeckx, Nuclear Data Sheets 118 (2014) 264-267 doi:10.1016/j.nds.2014.07.063 |
Abstract The OECD Nuclear Energy Agency (NEA) organizes cooperation between the major nuclear data evaluation projects in the world. The NEA Working Party on International Nuclear Data Evaluation Cooperation (WPEC) was established to promote the exchange of information on nuclear data evaluation, measurement, nuclear model calculation, validation, and related topics, and to provide a framework for cooperative activities between the participating projects. The working party assesses nuclear data improvement needs and addresses these needs by initiating joint activities in the framework of dedicated WPEC subgroups. Studies recently completed comprise a number of works related to nuclear data covariance and associated processing issues, as well as more specific studies related to the resonance parameter representation in the unresolved resonance region, the gamma production from fission product capture reactions, the 235U capture cross section, the EXFOR database, and the improvement of nuclear data for advanced reactor systems. Ongoing
activities focus on the evaluation of 239Pu in the resonance region, scattering angular distribution
in the fast energy range, and reporting/usage of experimental data for evaluation in the resolved resonance region. New activities include two subgroups on improved fission product yield evaluation methodologies and on modern nuclear database structures. Future activities under discussion include a pilot project for a Collaborative International Evaluated Library Organization (CIELO) and methods to provide feedback from nuclear and covariance data adjustment for improvement of nuclear data. In addition to the above mentioned short-term task-oriented subgroups, WPEC also
hosts a longer-term subgroup charged with reviewing and compiling the most important nuclear data requirements in a high priority request list (HPRL). | |
|
Deuteron-induced activation cross-sections on natural copper up to 24 MeV [Abstract] |
M.U. Khandaker, H. Haba, M. Murakami, N. Otuka, H.A.Kassim, J. Radioanal. Nucl. Chem. 302 (2014) pp. 759-764. doi:10.1007/s10967-014-3186-y |
Abstract Activation cross-sections of natCu(d,x)62,65Zn, 64Cu,60g+mCo,59Fe reactions were measured using a stacked foil activation technique combined with HPGe gamma-ray spectrometry up to the deuteron energy of 24 MeV. Measured data were critically compared with the available literature data and theoretical data extracted from the TENDL-2012 library, and found only partial agreements among them. Cross-sections of natCu(d,x)59Fe reactions are reported here for the first time in the energy region of 19�??23 MeV. Measured cross-sections of the long-lived 65Zn, 60gCo and 59Fe radionuclides are significant for understanding the activation behaviour of copper, an essential structural material used in accelerator and nuclear industry. | |
|
Activation cross-sections of deuteron-induced nuclear reactions on natural titanium [Abstract] |
M.U. Khandaker, H. Haba, J. Kanaya, N. Otuka, H.A. Kassim, Nuclear Data Sheets 119 (2014) pp. 252-254. doi:10.1016/j.nds.2014.08.069 |
Abstract Activation cross-sections of deuteron-induced nuclear reactions on natural titanium were measured up to 24-MeV energy using a stacked-foil activation technique in combination with HPGe γ-ray spectrometry. Measured cross-sections show an overall good agreement with the earlier measurements, but only a partial agreement with predictions by the TALYS code extracted from the TENDL-2011 library. The new cross-sections of the investigated reaction products find importance in nuclear medicine, accelerator and nuclear technology, and testing of nuclear reaction theories. | |
|
Documentation of uncertainties in experimental cross sections for EXFOR [Abstract] |
N. Otuka, D.L. Smith, Nuclear Data Sheets 120 (2014) pp. 281-284. doi:10.1016/j.nds.2014.07.067 |
Abstract Documentation of uncertainties and covariances in experimental nuclear reaction cross sections has been assessed. Following consideration of the importance of covariances for nuclear data in various nuclear applications, and presentation of a simple numerical example to demonstrate this point, the minimum basic concepts (mean, covariance, standard derivation, partial uncertainties, micro- and macro-correlation coefficients) are introduced. A deterministic approach to propagating the covariances in primary measured parameters (e.g., counts) to the derived cross sections is discussed, using a neutron-induced activation cross section measurement as an example. Finally, various approaches to documentation (publication, compilation) of experimental cross sections to facilitate their use in future evaluations are mentioned. | |
|
First Compilation and Evaluation of Beta-Delayed Neutron Emission Probabilities and Associated Half-Lives for A ? 72 Nuclei [Abstract] |
M. Birch, B. Singh, D. Abriola, I. Dillmann, T.D. Johnson, E.A. McCutchan, and A.A. Sonzogni, Nuclear Data Sheets 120 (2014) 66?69 doi:10.1016/j.nds.2014.07.008 |
Abstract A comprehensive compilation and evaluation of beta-delayed neutron ( β�?? n ) emission probabilities,
Pn, and associated half-lives for A �?� 72 nuclei has been performed for the first time. The
recommended values have been used to analyze the systematics of β�?? n emission in this region.
The ratio Pn/T1/2 is better correlated with the Q-value of the β�?? n decay mode than the previously
proposed Kratz-Herrmann Formula (KHF). The recommended values are also compared with
theoretical quasi-particle random phase approximation (QRPA) calculations | |
|
A New Approach to Estimating the Probability for ?-delayed Neutron Emission [Abstract] |
E.A. McCutchan, A.A. Sonzogni, T.D. Johnson, D. Abriola, M. Birch, and B. Singh, Nuclear Data Sheets 120 (2014) 62?65 doi:10.1016/j.nds.2014.07.007 |
Abstract The probability for neutron emission following β decay, Pn, is a crucial property for a wide range of
physics and applications including nuclear structure, r-process nucleosynthesis, the control of nuclear
reactors, and the post-processing of nuclear fuel. Despite much experimental effort, knowledge of
Pn values is still lacking in very neutron-rich nuclei, requiring predictions from either systematics or
theoretical models. Traditionally, systematic predictions were made by investigating the Pn value
as a function of the decay Q value and the neutron separation energy in the daughter nucleus. A
new approach to Pn systematics is presented which incorporates the half-life of the decay and the Q
value for β-delayed neutron emission. This prescription correlates the known data better, and thus
improves the estimation of Pn values for neutron-rich nuclei. Such an approach can be applied to
generate input values for r-process network calculations or in the modeling of advanced fuel cycles. | |
|
Towards a More Complete and Accurate Experimental Nuclear Reaction Data Library (EXFOR): International Collaboration Between Nuclear Reaction Data Centres (NRDC) [Abstract] |
N. Otuka, E. Dupont, V. Semkova, B. Pritychenko, A.I. Blokhin, M. Aikawa, S. Babykina, M. Bossant, G. Chen, S. Dunaeva, R.A. Forrest, T. Fukahori, N. Furutachi, S. Ganesan, Z. Ge, O.O. Gritzay, M. Herman, S. Hlavač, K. Katō, B. Lalremruata, Y.O. Lee, A. Makinaga, K. Matsumoto, M. Mikhaylyukova, G. Pikulina, V.G. Pronyaev, A. Saxena, O. Schwerer, S.P. Simakov, N. Soppera, R. Suzuki, S. Takacs, X. Tao, S. Taova, F. . Tarkanyi, V.V. Varlamov, J. Wang, S.C. Yang, V. Zerkin, Y. Zhuang, Nuclear Data Sheets 120 (2014) pp. 272?276. doi:10.1016/j.nds.2014.07.065 |
Abstract The International Network of Nuclear Reaction Data Centres (NRDC) coordinated by the IAEA Nuclear Data Section (NDS) successfully collaborates in the maintenance and development of the EXFOR library. As the scope of published data expands (e.g. to higher energy, to heavier projectile) to meet the needs of research and applications, it has become a challenging task to maintain both the completeness and accuracy of the EXFOR library. Evolution of the library highlighting recent developments is described. | |
|
Developments of the EXFOR Database: Possible New Formats [Abstract] |
R.A. Forrest, V. Zerkin, S. Simakov, Nuclear Data Sheets 120, June 2014 268?271 doi:10.1016/j.nds.2014.07.064 |
Abstract The EXFOR database is a collection of experimental nuclear reaction data, maintained by the IAEA on behalf of the International Network of Nuclear Reaction Data Centres (NRDC). The format for the storage of such data was first described in 1969 and while there have been many incremental changes over the years so that the format is now capable of containing a very wide range of measurement results, there is a growing realisation that a major change is required. Consequently the IAEA Nuclear Data Section (NDS) organised a Consultant's Meeting on �??Further Development of EXFOR�?? in 2012. This was an opportunity for a range of international experts to discuss ways of improving EXFOR and while this focused on new formats there was also discussion on ways of storing new data, new output formats and software tools such as editors. This paper will discuss recent and proposed changes to enable new quantities to be stored (such as coincidence measurements and covariances), the range of output formats available (e.g. C4 and X4+) which make interaction with the data more user friendly and the possible use of XML to modernise the database. | |
|
Inventory Simulations Under Neutron Irradiation: Visualization Techniques as an Aid to Materials Design [Abstract] |
M.R. Gilbert, L.W. Packer, J.-Ch. Sublet, and R.A. Forrest, Nuclear Science and Engineering 177 (2014) 291?306 doi:10.13182/NSE13-76 |
Abstract The simulation of neutron irradiation�??induced transmutation using inventory codes is an
important part of the research into materials in various nuclear environments, including fusion, fission,
medical physics, nuclear security, and astrophysics. These simulations, even in their simplest form, such as
the neutron irradiation of a single pure element, generate large time-dependent data sets of complex results.
For each nuclide in the inventory, as a function of time, the output data will include the number of atoms and
its contribution to a variety of radiological quantities including total or specific activity, gamma dose, heat
output, and ingestion and inhalation hazards. A key challenge when performing inventory calculations is
thus to represent the full complexity of the results in a visual and understandable format.
This paper discusses two different approaches to visualizing inventory data: (a) nuclide maps, which
allow the concentrations or activity contributions from all nuclides in the inventory to be displayed and also
for the variation to be traced in time under a specific irradiation scenario, and (b) importance diagrams,
which are a neutron spectrum�??independent representation of the dominant nuclides that contribute to the
activity of an irradiated material. Finally, these techniques are applied in parallel to investigate how the
activation response of molybdenum can be improved via isotopic tailoring (enrichment or depletion), which
could make it a more viable alternative armor material in the design of fusion reactors. | |
|
Investigation of (d,x) nuclear reactions on natural ytterbium up to 24 MeV [Abstract] |
M.U. Khandaker, H. Haba, N. Otuka, A.R. Usman, Nucl. Instrum. Meth. Phys. Res. B 335 (2013) pp. 8-18.
doi:10.1016/j.nimb.2014.05.020 |
Abstract Production cross-sections of the natYb(d,x)169,170,171,172,173,174m,174,176m,177gLu and 169,175,177Yb reactions have been measured from a 24-MeV deuteron energy down to their respective thresholds by using a stacked-foil activation technique combined with high resolution γ-ray spectrometry. Our new experimental data extended the experimental database toward the lower energy region for 169Yb, 171Lu, 172Lu, and 176mLu, and the higher region for 174Lu, 176mLu, and 177Yb. An overall good agreement is found with some of the earlier measurements, whereas a partial agreement is obtained with the theoretical data extracted from the TENDL-2013 library. The (d,p) channel contribution underestimated by the TENDL-2013 library is successfully reproduced in the global renormalization by Ignatyuk for the FENDL-3.0 library. The production cross-sections of 175Yb available in the literature were revised based on the latest γ-ray intensity adopted in 2004. Physical thick target yields for the investigated reaction products were also deduced and compared with the directly measured ones in the literature. The derived thick target yields for 173Lu and 174gLu are higher than the directly measured ones by Dmitriev et al. at 22 MeV. The deduced yield curves indicate that a low energy (<11 MeV) cyclotron and a highly enriched 176Yb target could be used to obtain 177gLu with negligible impurity from 177mLu. | |
|
Improvements and Extensions of the Neutron Cross Section and Fluence Standards [Abstract] |
A.D. Carlson, V.G. Pronyaev, R. Capote, F.-J. Hambsch, F. Kappeler, C. Lederer, W. Mannhart, A. Mengoni, R.O. Nelson, A.J.M. Plompen, P. Schillebeeckx, S. Simakov, P. Talou, S. Tagesen, H. Vonach, A. Vorobyev, and A. Wallner, Nuclear Data Sheets 118 (2014) 126-131 doi:/10.1016/j.nds.2014.04.017 |
Abstract Improvements have been made to the nuclear data standards largely as a result of an IAEA Data
Development Project. The work includes the traditional activities related to standards, extending
the energy ranges of some standards, and reference data that are not as well known as the standards
but can be very useful in the measurements of certain types of cross sections. Also included is an
effort to improve evaluations of 235U thermal and 252Cf spontaneous fission neutron spectra. | |
|
Validation of the International Reactor Dosimetry and Fusion File [Abstract] |
S. Simakov, L. Greenwood, R. Capote Noy, Proc. 12th Int. Conf. on Radiation Shielding (ICRS-12), 2-7 September 2012, Nara, Japan; Progress in Nuclear Science and Technology 4 (2014) pp. 591-595 |
Abstract Evaluated nuclear data files for nuclides of the thorium-uranium cycle were released as a result of a coordinated research project of the International Atomic Energy Agency. To validate the data a series of benchmark test cases were analysed, with emphasis on the most important nuclides 232Th and 233U. Remaining nuclides appearing in the benchmarks were taken from the ENDF/B-VII beta-2 library, except for a few sensitivity studies where the data were taken from other sources. The results show marked improvement in the agreement with measurements, much of it coming from the new evaluations | |
|
Databases and coordinated research projects at the IAEA on atomic processes in plasmas [Abstract] |
B.J. Braams, H.-K. Chung, AIP Conference Proceedings 1438 (2012) pp. 222-227. doi:10.1063/1.4707881 |
Abstract The Atomic and Molecular Data Unit at the IAEA works with a network of national data centres to encourage and coordinate production and dissemination of fundamental data for atomic, molecular and plasma-material interaction (A+M/PMI) processes that are relevant to the realization of fusion energy. The Unit maintains numerical and bibliographical databases and has started a Wiki-style knowledge base. The Unit also contributes to A+M database interface standards and provides a search engine that offers a common interface to multiple numerical A+M/PMI databases. Coordinated Research Projects (CRPs) bring together fusion energy researchers and atomic, molecular and surface physicists for joint work towards the development of new data and new methods. The databases and current CRPs on A+M/PMI processes are briefly described here. | |
|
First Joint IAEA-ITER Technical Meeting on Analysis of ITER Materials and Technologies. Preface [Abstract] |
R. Kamendje, B.J. Braams, Fusion Sci. Technol. 61 Issue 2 (2012) pp.III |
Abstract The first Joint IAEA-ITER Technical Meeting on Analysis of ITER Materials and Technologies was held November 23�??25, 2010, in the Principality of Monaco, in conjunction with the first Monaco ITER International Fusion Energy Days. The meeting aimed to contribute to the development of a knowledge base of properties, processes, and technologies relevant to ITER structural and plasma-facing materials and components, and of the effects of energetic particles and radiation on ITER materials. The present issue of Fusion Science and Technology features papers describing some of the material that was presented and discussed at the meeting. | |
|
Analytical potential energy surface for O + C2H2 system [Abstract] |
S. Garashchuk, V.A. Rassolov and B.J. Braams, Chem. Phys. Lett. 588 (2013) pp. 22-26. doi:10.1016/j.cplett.2013.09.060 |
Abstract Full-dimensional analytical potential energy surfaces (PESs) for the O(1P) + C2H2 and O(3P) + C2H2 reactions are presented. The PESs are constructed by fitting thousands of ab initio data points using permutationally invariant polynomials. Electronic structure data are obtained within the restricted coupled cluster theory with single and double excitations with perturbative triple corrections and correlation consistent basis set of triple-zeta with diffuse functions. Motivated by experiments, formation of DOCC and cyclic DCCO at collision energies of 2.5�??4 eV is examined using quasi-classical trajectory dynamics on the triplet surface. | |
|
Coordinated Research Projects of the IAEA (CRP). 5. Summary [Abstract] |
B.J. Braams, M. Imai and D. Kato, Journal of the Japan Society of Plasma Science and Nuclear Fusion Research 89 Issue No.9 (2013) pp. 615-621. |
Abstract A summary is provided of the twelve (12) special topic articles connected to recent CRPs or other activities of the IAEA Atomic and Molecular Data Unit. | |
|
Coordinated Research Projects of the IAEA (CRP). 1. Introduction [Abstract] |
B.J. Braams, M. Imai and D. Kato, Journal of the Japan Society of Plasma Science and Nuclear Fusion Research 89 Issue 9 (2013) pp. 579-582. |
Abstract The present special topic articles of the Journal of Plasma and Fusion Research contain contributions from (mainly) Japanese researchers in the field of fusion science or related atomic, molecular or plasma-material interaction processes reflecting the interests of one of the recent CRPs or other activities of the IAEA Atomic and Molecular Data Unit. | |
|
The upcoming international code of practice for small static photon field dosimetry [Abstract] |
H. Palmans, R. Alfonso, P. Andreo, R. Capote, M.S. Huq, J. Izewska, J. Johansson, W. Kilby, T.R. Mackie, A. Meghzifene, K. Rosser, J. Seuntjens, W. Ullrich, Med. Phys. 39 (2012) 4633. doi:10.1118/1.4740154 |
Abstract The increased use of small photon fields in stereotactic and intensity�?�modulated radiotherapy has raised the need for standardizing the dosimetry of such fields using procedures consistent with those for conventional radiotherapy. An international working group, established by the IAEA in collaboration with AAPM and IPEM, is finalising a Code of Practice for the dosimetry of small static photon fields. Procedures for reference dosimetry in nonstandard machine specific reference (msr) fields are provided following the formalism of Alfonso et al. (Med. Phys. 35: 5179; 2008). Reference dosimetry using ionization chambers in machines that cannot establish a conventional 10 cm �? 10 cm reference field is based on either a direct calibration in the msr field traceable to primary standards, a calibration in a reference field and a generic correction factor or the product of a correction factor for a virtual reference field and a correction factor for the difference between the msr and virtual fields. For the latter method, procedures are provided for determining the beam quality in non�?�reference conditions. For the measurement of field output factors in small fields, procedures for connecting large field measurements using ionization chambers to small field measurements using high�?�resolution detectors such as diodes, diamond,liquidion chambers, organic scintillators and radiochromic film are given. The Code of Practice also presents consensus data on correction factors for use in conjunction with measured, detector�?�specific output factors. Further research to determine missing data according to the proposed framework will be strongly encouraged by publication of this document. | |
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Astrophysical (?,?) reaction in inverse kinematics; Electron screening effect in the beta-decay
[Abstract] |
P. Ujic, F. de Oliveira Santos, A. Lagoyannis, T.J. Mertzimekis, S. Harissopulos, P. Demetriou, A. Spyrou et al., J. Phys.: Conf. Ser. 337 (2012) 012015.
doi:10.1088/1742-6596/337/1/012015 |
Abstract The abundance calculations of the p-nuclei produced in explosive stellar sites rely
on the Hauser-Feshbach (HF) theory with the alpha-article optical model potential (α-OMP)
one of its major ingredients. To date, most of the (α, γ) cross sections measured show that
HF calculations can be wrong by a factor of ten or more especially when phenomenological α-
OMP are employed. To investigate the relevant uncertainties entering the HF calculations and
furthermore develop global microscopic α-OMPs, systematic (α, γ) cross-section measurements
are necessary. This led us to perform a feasibility study of (α, γ) measurements in inverse
kinematics that will allow us to employ also radioactive beams in the future. Hence, the
4He(78Kr,γ)
82Sr reaction was studied using the LISE3 spectrometer to separate the 82Sr recoils
from the primary 78Kr beam. Although an excellent rejection factor > 1010 was achieved, the
position of the ions of interest was unexpectedly masked by a secondary beam of high intensity.
Given these, new setup improvements are proposed to remove the pollutant ions | |
|
Experimental and theoretical study of the (n,2n) reaction on 174,176Hf isotopes [Abstract] |
M. Serris, S. Galanopoulos, M. Kokkoris, C.T. Papadopoulos, M. Lamprou, R. Vlastou, P. Demetriou, C.A. Kalfas, A. Lagoyannis, Phys. Rev. C 86 (2012) 034602.
doi:10.1103/PhysRevC.86.034602 |
Abstract Cross sections for the 174Hf(n, 2n)173Hf and 176Hf(n, 2n)175Hf reactions have been measured at
the 5.5 MV VdG Tandem accelerator of NCSR \Demokritos" in Athens, in the neutron energy region
from 8.8 to 11.0 MeV, using the activation technique. An experimental method to account for the
contamination of the 176Hf(n, 2n) reaction by the 174Hf(n,
) reaction activated by the parasitic
neutrons of the beam is presented. Statistical model calculations have also been performed using
the nuclear-reaction codes EMPIRE-II and TALYS. The results and the eect of the nuclear input
parameters as well as pre-equilibrium emission are discussed in detail | |
|
Nuclear Data Sheets for A=211 [Abstract] |
B. Singh, D. Abriola, C. Baglin, P. Demetriou et al., Nuclear Data Sheets 114 (2013) 661-749 doi:10.1016/j.nds.2013.05.001 |
Abstract The evaluated spectroscopic data are presented for 11 known nuclides of mass 211 (Hg, Tl, Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th). The 211Pa nuclide is included here but its identification remains uncertain. For 211Hg, 211Tl, 211Ac and 211Th nuclei, only the ground�??state information is available. Their decay characteristics are mostly unknown. 211Fr is suggested to decay partially through ε decay mode, but its decay scheme remains poorly known. While high�??spin excitations, including several isomers, are well studied in 211Pb, 211Bi, 211Po, 211At, 211Rn and 211Fr, the particle�??transfer data are available for only 211Po and 211Bi.
This evaluation was carried out as part of joint IAEA�??ICTP workshop for Nuclear Structure and Decay Data, organized and hosted by the IAEA, Vienna and ICTP, Trieste, August 6�??17, 2012. This work supersedes previous A=211 evaluation (2004Br45) published by E. Browne which covered literature before January 2003. | |
|
Investigation of ?-induced reactions on the p nucleus 168Yb [Abstract] |
L. Netterdon, P. Demetriou, J. Endres, U. Giesen, G.G. Kiss, A. Sauerwein, T. Sz�cs, K.O. Zell, A. Zilges, Nucl. Phys. A 916 (2013) 149-167 doi:10.1016/j.nuclphysa.2013.08.002 |
Abstract Cross sections for the 168Yb(α,γ)172Hf and 168Yb(α,n)171Hf reactions were measured by means of the activation method using α particles with energies between 12.9 MeV and 15.1 MeV. The spectroscopy of the γ rays emitted by there action products was performed using three different HPGe detector types, namely clover-type high-purity germanium detectors, a low-energy photon spectrometer detector, and a coaxial high-purity germanium detector. The results were compared to Hauser�??Feshbach statistical model calculations. Within certain assumptions, astrophysical conclusions could be drawn concerning the production of the p nucleus 168Yb. The data in this work can serve as a contribution to the current very fragmentary experimental database for charged-particle induced reactions. In addition, the absolute intensity for nine γ-ray transitions following the electron capture decay of 171Hf could be derived. | |
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Cross section measurements of proton capture reactions relevant to the p process: The case of 89Y(p,?)90Zr and 121,123Sb(p,?)122,124Te [Abstract] |
S. Harissopulos, A. Spyrou, A. Lagoyannis, M. Axiotis, P. Demetriou, J.W. Hammer, R. Kunz, H.-W. Becker, Phys. Rev. C 87 (2013) 025806 doi:10.1103/PhysRevC.87.025806 |
Abstract The cross sections of the 89Y(p,γ)90Zr and the 121,123Sb(p,γ)122,124Te reactions were determined from γ-angular distribution measurements at beam energies from 1.6 to 3.4 MeV. In addition, angle-integrated cross sections were also measured at Ep=2, 3, 4, and 4.8 MeV for the 89Y(p,γ)90Zr reaction using the 4�? γ-summing method. Astrophysical S factors and reaction rates were deduced from the measured cross sections. Statistical model calculations were performed using the nuclear-reaction code Talys. The results from the comparison between theory and experiment are discussed in detail. | |
|
Nuclear Data Sheets for A = 215 [Abstract] |
B. Singh, G. Mukherjee, D. Abriola, S. Basu, P. Demetriou et al., Nuclear Data Sheets 114 (2013) 2023-2078 doi:10.1016/j.nds.2013.11.003 |
Abstract The evaluated spectroscopic data are presented for 12 known nuclides of mass 215 (Hg, Tl, Pb, Bi, Po,
At, Rn, Fr, Ra, Ac, Th, Pa). For 215Hg, 215Tl, 215Pb, and 215Pa nuclei, no excited states are known. The decay
characteristics of 215Hg and 215Tl are unknown. The decay scheme of 215Pb is considered as incomplete. Ordering
of γ cascades in the decay of 36.9�??s isomer of 215Bi and for high�??spin states above 2251 keV in 215Fr are not
established. High�??spin excitations, including several isomeric states, are well known in 215Bi, 215Po, 215Rn,
215Fr, 215Ra, and 215Ac. No particle�??transfer reaction data are available for any of the A=215 nuclei.
The rms charge radii for 215Pb, 215Bi, 215Po, 215Rn, 215Fr and 215Ra have been evaluated by Daniel Abriola, from
extrapolation or interpolation of available evaluated data in 2013An02 for radii of respective Z chains using
formula 9 in 2004An14.
This evaluation was carried out as part of ENSDD�??workshop at VECC, Kolkata for Nuclear Structure and Decay Data,
organized and hosted by VECC and Board of Research in Nuclear Sciences (BRNS) in Kolkata, India, November
26�??29, 2012. This work supersedes the previous A=215 evaluation (2001Br31) published by E. Browne which
covered literature prior to May 2001. | |
|
Coordinated activities on evaluation of collisional data for fusion applications [Abstract] |
H.-K. Chung and B.J. Braams, AIP Conf. Proc. 1545 (2013) 260 doi:10.1063/1.4815862 |
Abstract It is the role of the Atomic and Molecular Data Unit of the International Atomic Energy Agency to review progress in the production, compilation and evaluation of atomic, molecular and plasma-surface interaction (AM/PSI) data for the fusion program and to support the development of internationally recommended libraries of AM/PSI data for fusion. In response to increasing requests from the fusion community the Unit has increased its effort to promote the assessment of data quality by organizing a series of meetings on the relevant issues: 1) Error propagation and sensitivity analysis, 2) Current status of evaluated databases, 3) Uncertainty estimates of theoretical data, 4) Experimental data evaluation, 5) Data evaluation methods and semi-empirical fits and 6) Establishment of an evaluators�?? network. The discussions and conclusions are summarized here. | |
|
Comparison and analysis of collisional-radiative models at the NLTE-7 workshop
[Abstract] |
H.-K. Chung, C. Bowen, C.J. Fontes, S.B. Hansen, Yu. Ralchenko, High Energy Dens. Phys. 9, 645 (2013) doi:10.1016/j.hedp.2013.06.001 |
Abstract We present the main results of the 7th Non-Local Thermodynamic Equilibrium Code Comparison Workshop held in December 2011 in Vienna, Austria. More than twenty researchers from nine countries, who actively work on development of collisional-radiative codes for plasma kinetics modeling, attended the meeting and submitted their results for a number of comparison cases. The cases included free-electron-laser-inspired time-dependent relaxation of photoexcited Ne-like Ar, ionization balance and spectra for highly charged tungsten, spectroscopic diagnostics of krypton L-shell spectra, and an investigation of Ne model convergence with principal quantum number. | |
|
Observations of the Effect of Ionization-Potential Depression in Hot Dense Plasma [Abstract] |
D.J. Hoarty, P. Allan, S.F. James, C.R.D. Brown, L.M.R. Hobbs, M.P. Hill, J.W.O. Harris, J. Morton, M.G. Brookes, R. Shepherd, J. Dunn, H. Chen, E. Von Marley, P. Beiersdorfer, H.K. Chung, R.W. Lee, G. Brown, and J. Emig, Phys. Rev. Lett. 110, 265003 (2013) doi:10.1103/PhysRevLett.110.265003 |
Abstract The newly commissioned Orion laser system has been used to study dense plasmas created by a
combination of short pulse laser heating and compression by laser driven shocks. Thus the plasma density
was systematically varied between 1 and 10 g=cc by using aluminum samples buried in plastic foils or
diamond sheets. The aluminum was heated to electron temperatures between 500 and 700 eVallowing the
plasma conditions to be diagnosed by K-shell emission spectroscopy. The K-shell spectra show the effect
of the ionization potential depression as a function of density. The data are compared to simulated spectra
which account for the change in the ionization potential by the commonly used Stewart and Pyatt
prescription and an alternative due to Ecker and Kro¨ll suggested by recent x-ray free-electron laser
experiments. The experimental data are in closer agreement with simulations using the model of Stewart
and Pyatt. | |
|
Results of total cross section measurements for 197Au in the neutron energy region from 4 to 108 keV at GELINA [Abstract] |
I. Sirakov, B. Becker, R. Capote, E. Dupont, S. Kopecky, C. Massimi and P. Schillebeeckx, Eur. Phys. J. A 49 (2013) 144 doi:10.1140/epja/i2013-13144-2 |
Abstract Transmission measurements have been performed to determine the total cross section for
neutron-induced reactions with 197Au in the energy region from 4 keV to 108 keV. The experiments were
carried out at a 50m measurement station of the time-of-flight facility GELINA using a 6Li glass scintillator.
The average total cross section as a function of neutron energy was derived after correcting the observed
average transmission for cross section fluctuations due to resonance structures. The results have been compared
with literature data and with the total cross section resulting from a dispersive coupled-channel
optical model potential. The neutron strength function for s-wave neutrons and an orbital-independent
scattering radius, together with their covariance matrix, have been derived in the neutron energy region between
4 keV and 108 keV through a parameterization of the total cross section based on a nuclear reaction
theory. | |
|
A dispersive optical model potential for nucleon induced reactions on 238U and 232Th nuclei with full coupling
[Abstract] |
J.M. Quesada, E.S. Soukhovitski, R. Capote and S. Chiba, EPJ Web of Conferences 42 (2013) 02005 doi:10.1051/epjconf/20134202005 |
Abstract A dispersive coupled-channel optical model potential (DCCOMP) that couples the ground-state rotational and low-lying vibrational bands of 238U and 232Th nuclei is studied. The derived DCCOMP couples almost all excited levels below 1 MeV of excitation energy of the corresponding even-even actinides. The ground state, octupole, beta, gamma, and non-axial bands are coupled. The first two isobar analogue states (IAS) populated in the quasi-elastic (p,n) reaction are also coupled in the proton induced calculation, making the potential approximately Lane consistent. The coupled-channel potential is based on a soft-rotor description of the target nucleus structure, where dynamic vibrations are considered as perturbations of the rigid rotor underlying structure. Matrix elements required to use the proposed structure model in Tamura coupled-channel scheme are derived. Calculated ratio R(U238/Th232) of the total cross-section difference to the averaged �?T for 238U and 232Th nuclei is shown to be in excellent agreement with measured data. | |
|
Dispersive coupled-channels optical-model potential with soft-rotator couplings for Cr, Fe, and Ni isotopes [Abstract] |
Li Rui, Sun Weili, E. Sh. Soukhovitski, J.M. Quesada, R. Capote, Phys. Rev. C 87 (2013) 054611 doi:10.1103/PhysRevC.87.054611 |
Abstract An approximate Lane-consistent dispersive coupled-channels optical potential is derived that describes
nucleon-induced reactions on even iron isotopes. Realistic saturated couplings for 54,56,58Fe nuclei are built
using nuclear wave functions of the soft-rotator model with the Hamiltonian parameters adjusted to reproduce the
energy of the low-lying collective levels of these isotopes.E2- andE3-transition probabilities between low-lying
collective levels are well reproduced. The comprehensive experimental database used in the fitting process
includes all scattering data for neutron and proton scattering up to 200 MeV on iron nuclei. The derived potential
is shown to be applicable to Ni and Cr isotopes, assuming the applicability of the soft-rotator model to these
nuclei and to the odd 57Fe nucleus within the rigid-rotor model. The approximate Lane consistency of the derived
potential is validated by describing the quasielastic (p, n) scattering with excitation of isobaric analog states.
Elastic and inelastic analyzing powers for both neutron- and proton-induced reactions are shown to be in good
agreement with experimental data, demonstrating the reliability of the derived dispersive spin-orbit potential | |
|
Measurement and modeling of the cross sections for the reaction 230Th(3He,3n)230U [Abstract] |
A. Morgenstern, K. Abbas, F. Simonelli, R. Capote, M. Sin, B. Zielinska, F. Bruchertseifer, C. Apostolidis, Phys. Rev. C 87 (2013) 064602 doi:10.1103/PhysRevC.87.064602 |
Abstract 230U and its daughter nuclide 226Th are promising therapeutic nuclides for application in targeted α therapy of cancer. We investigated the feasibility of producing 230U/226Th via irradiation of 230Th with 3He particles according to the reaction 230Th(3He,3n)230U. The experimental excitation function for this reaction is reported here. Cross sections were measured by using thin targets of 230Th prepared by electrodeposition, and 230U yields were analyzed by using α spectrometry. Beam intensities were obtained via monitor reactions on aluminum foils by using high-resolution γ spectrometry and International Atomic Energy Agency recommended cross sections. Incident particle energies were calculated by using the SRIM-2003 code. The experimental cross sections for the reaction 230Th(3He,3n)230U are in good agreement with model calculations by the EMPIRE-3 code once breakup and transfer reactions are properly considered in the incident channel. The obtained cross sections are too low to allow for the production of 230U/226Th in clinically relevant levels. | |
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Impact of model defect and experimental uncertainties on evaluated output [Abstract] |
D. Neudecker, R. Capote, H. Leeb, Nucl. Instrum. Meth. A 723 (2013) pp. 163-172 doi:10.1016/j.nima.2013.05.005 |
Abstract One of the current major problems in nuclear data evaluation is the unreasonably small evaluated uncertainties often obtained. These small uncertainties are partly attributed to missing correlations of experimental uncertainties as well as to deficiencies of the model employed for the prior information. In this article, both uncertainty sources are included in an evaluation of 55Mn cross-sections for incident neutrons. Their impact on the evaluated output is studied using a prior obtained by the Full Bayesian Evaluation Technique and a prior obtained by the nuclear model program EMPIRE. It is shown analytically and by means of an evaluation that unreasonably small evaluated uncertainties can be obtained not only if correlated systematic uncertainties of the experiment are neglected but also if prior uncertainties are smaller or about the same magnitude as the experimental ones. Furthermore, it is shown that including model defect uncertainties in the evaluation of 55Mn leads to larger evaluated uncertainties for channels where the model is deficient. It is concluded that including correlated experimental uncertainties is equally important as model defect uncertainties, if the model calculations deviate significantly from the measurements. | |
|
Measurement of the MACS of 181Ta(n,?) at kT=30 keV as a test of a method for Maxwellian neutron spectra generation [Abstract] |
J. Praena, P.F. Mastinu, M. Pignatari, J.M. Quesada, J. Garcia-Lopez, M. Lozano, N. Dzysiuk, R. Capote, G. Martin-Hernandez, Nucl. Instrum. Meth. A 727 (2013) pp. 1-6 doi:10.1016/j.nima.2013.05.151 |
Abstract Measurement of the Maxwellian-Averaged Cross-Section (MACS) of the reaction at kT=30 keV by the activation technique using an innovative method for the generation of Maxwellian neutron spectra is presented. The method is based on the shaping of the proton beam to produce a desired neutron spectrum using the 7Li(p,n) reaction as a neutron source. The characterization of neutron spectra has been performed by combining measured proton distributions, an analytical description of the differential neutron yield in angle and energy of the 7Li(p,n) reaction, and with Monte Carlo simulations of the neutron transport. A measured value equal to 815±73 mbarn is reported for the MACS of the reaction at kT=30 keV. The MACS of the reaction provided by KADoNiS has been used as a reference. | |
|
Activation cross-sections of deuteron-induced nuclear reactions on natural iron up to 24 MeV
[Abstract] |
M.U. Khandaker, H. Haba, J. Kanaya, N. Otuka, Nucl. Instrum. Meth. B 316 (2013) pp. 33-41. doi:10.1016/j.nimb.2013.08.032 |
Abstract Activation cross-sections of the natFe(d,x)55,56,57,58g+mCo, 52g,54,56Mn, 51Cr, 59Fe reactions were measured from their respective thresholds to 24 MeV via a stacked foil activation technique combined with HPGe γ-ray spectrometry. An overall good agreement is found with some of the earlier measurements, whereas partial agreements are obtained with the theoretical data extracted from the TENDL-2011 library. The
present measurement reports four cross-sections of 58g+mCo, 56Mn and 59Fe radionuclides in the energy range of 20�??24 MeV for the first time. Physical thick target yields deduced from the measured cross-sections are compared with the directly measured yields available in the literature. The measured 58Fe(d,p)59Fe cross section is underestimated by the original TENDL-2011 library while overestimated by the TENDL-2011 library renormalized by Ignatyuk for the FENDL-3 library. | |
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Status of the McDeLicious Approach for the D-Li Neutron Source Term Modeling in IFMIF Neutronics Calculations [Abstract] |
S.P. Simakov, U. Fischer, K. Kondo, P. Pereslavtsev, Fusion Science & Technology 62 (2012) pp. 233.
|
Abstract McDeLicious is an extension to the MCNP Monte Carlo code with the ability to simulate the generation of source neutrons based on D-Li interaction processes.
This paper presents an overview of the McDeLicious approach for the D-Li neutron source term modeling including latest code extensions, improvements, validation
efforts, and applications to IFMIF neutronics analyses. The current McDeLicious capabilities include the generation of source neutrons and photons based on evaluated
d+6,7Li cross-section data and the sampling of the impinging deuteron beam intensity distribution using fitting functions or probability tables. The McDeLicious
software has been updated to comply with the standard of the state-of-the-art version 5 of the MCNP code. A message passing interface program version enables one to
run McDeLicious in parallel mode on large computer clusters. McDeLicious is in routine use for IFMIF neutronics calculations employing different nuclear data including
a test version of the recent FENDL-3 nuclear data.
| |
|
Spectroscopic studies of hard x-ray free-electron laser-heated foils at 1016 Wcm-2 [Abstract] |
J. Dunn, R. Shepherd, A. Graf, A. Steel, J. Park, S.J. Moon, R.W. Lee, P. Audebert, A. Levy, M. Gauthier, J. Fuchs, D.M. Fritz, M. Cammarata, D. Milathianaki, H.J. Lee, B. Nagler, C. Fourment, F. Deneuville, G. Williams, M. Fajardo, J. Gaudin, S. Vinko, O. Ciricosta, J. Wark, H.K. Chung, Proc. SPIE 8140, X-Ray Lasers and Coherent X-Ray Sources: Development and Applications IX, 81400O (October 05, 2011) doi:10.1117/12.895264 |
Abstract We report a recent experiment where the first hard x-ray beam line, X-ray Pump Probe (XPP) instrument using the SLAC National Accelerator Laboratory's Linac Coherent Light Source (LCLS) free electron laser, was used to heat thin foils to high energy densities ~ 107 J/cm3. An intense 9 keV, 60 fs (FWHM) duration beam with energy of 2 - 4 mJ at the XPP beam line was focused using beryllium lenses to an irradiance approaching 1016 Wcm-2. Targets of 0.5 - 3.5 μm thick foils of Ag and Cu were studied using a suite of diagnostics including Fourier Domain Interferometry, energy calorimetry and grating and crystal spectrometers. The experimental details and spectroscopic results from the campaign will be described. Preliminary results indicate that the target is heated relatively uniformly to a temperature lower than 20 eV. | |
|
IAEA coordinated activities on evaluation of atomic, molecular and plasma-surface interaction data for fusion applications [Abstract] |
H.-K. Chung and B. J. Braams, Fusion Sci. Tech. 63 413 (2013) |
Abstract The Atomic and Molecular Data Unit of the International Atomic Energy Agency collaborates with an international network of data centres and fusion laboratories to support the production, compilation and evaluation of atomic, molecular and plasma-surface interaction (AM/PSI) data relevant to fusion energy research. In recent years, there have been increasing requests from the fusion community for the development of internationally recommended libraries of AM/PSI data for fusion and the Unit has increased its effort to promote the assessment of data quality by organizing a series of meetings on the relevant issues. Meeting participants from the AM/PSI data community developed plans for increased collaboration on the evaluation and recommendation of AM/PSI data. The discussions, conclusions and future plans are summarized here. | |
|
Method of time resolved refractive index measurements of x-ray laser heated solids [Abstract] |
G.O. Williams, H.-K. Chung, S.M. Vinko, S. Kunzel, A.B. Sardinha, Ph. Zeitoun and M. Fajardo, Phys. of Plasmas 20, 042701 (2013) doi:10.1063/1.4794964 |
Abstract With the advent of new x-ray light-sources worldwide, the creation of dense, uniformly heated plasma states arising from intense x-ray irradiation of solids has been made possible. In the early stages of x-ray solid heating, before significant hydrodynamic motion occurs, the matter exists in a highly non-equilibrium state. A method based on wavefront sensing is proposed to probe some of the fundamental properties of these states. The deflection and absorption of a high harmonic probe
beam propagated through the plasma can be measured with a wavefront sensor, and allow for the determination of the complex refractive index (RI) of the plasma, giving a 2D map of the optical properties as function of time in a pump-probe arrangement. A solid heating model has been used to estimate the expected temperatures of x-ray heated thin foils, and these temperatures are used in three separate models to estimate the changes in the refractive index. The calculations show the changes induced on an extreme ultra-violet (XUV) probe beam by a solid density thin foil plasma are significant, in terms of deflection angle and absorption, to be measured by already existing XUV Hartmann wavefront sensors. The method is applicable to a wide range of photon energies in the XUV (10 s to several 100 s of eV) and plasma parameters, and can add much needed experimental data to the fundamental properties of such dense plasma states. | |
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Combination of resonance integral and Maxwellian 30 keV data ? A sensitive test of the resonance region [Abstract] |
J. Kopecky, R.A. Forrest, Fusion Engineering and Design 88 (2013) pp. 177-187. doi:10.1016/j.fusengdes.2013.01.095 |
Abstract This paper presents the approach of a combined use of resonance integrals and average Maxwellian cross
sections (MACS) at kT = 30 keV to test and validate the resolved resonance range or its reconstructed cross
section curve. Based on these two integral measurements a sensitive and energy dependent test can be
provided. These two integral quantities cover with their neutron spectra the energy region between
En = 0.5 eV up to several hundred keV, respectively, with different weighting. Our principal motivation is
to produce a validation tool, sensitive to the lower and upper parts of the resonance region through the
difference in the applied 1/E and kT = 30 keV Maxwell�??Boltzmann spectra of the resonance integral and
MACS data. | |
|
The 93Zr(n,γ) reaction up to 8 keV neutron energy [Abstract] |
G. Tagliente, R. Capote, et al., (n_TOF Collaboration), Physical Review C 87 (2013) 014622 doi:10.1103/PhysRevC.87.014622 |
Abstract The (n, γ ) reaction of the radioactive isotope 93Zr has been measured at the n_TOF high-resolution time-offlight
facility at CERN. Resonance parameters have been extracted in the neutron energy range up to 8 keV, yielding capture widths smaller (14%) than reported in an earlier experiment. These results are important for detailed nucleosynthesis calculations and for refined studies of waste transmutation concepts. | |
|
Experimental Uncertainty and Covariance Information in EXFOR Library [Abstract] |
N. Otuka, R. Capote, S. Kopecky, A.J.M. Plompen, V.G. Pronyaev, P. Schillebeeckx and D.L. Smith, EPJ Web of Conferences 27 (2012) 00007. doi:10.1051/epjconf/20122700007 |
Abstract Compilation of experimental uncertainty and covariance information in the EXFOR Library is discussed. Following the presentation of a brief history of information provided in the EXFOR Library, the current EXFOR Formats and their limitations are reviewed. Proposed extensions for neutron-induced reaction cross sections in the fast neutron region and resonance region are also presented. | |
|
Thermal Neutron Capture onto the Stable Tungsten Isotopes [Abstract] |
A.M. Hurst, R.B. Firestone, B.W. Sleaford, N.C. Summers, Zs. Revay, L. Szentmikl�si, T. Belgya, M.S. Basunia, R. Capote, et al.,
EPJ Web of Conferences 21 (2012) 10005 doi:10.1051/epjconf/20122110005 |
Abstract Thermal neutron-capture measurements of the stable tungsten isotopes have been carried out using the guided thermal-neutron beam at the Budapest Reactor. Prompt singles spectra were collected and analyzed using the HYPERMET
γ-ray analysis software package for the compound tungsten systems 183W, 184W, and 187W, prepared from isotopically-enriched samples of 182W, 183W, and 186W, respectively. These new data provide both confirmation and new insights into the decay schemes and structure of the tungsten isotopes reported in the Evaluated Gamma-ray Activation File based upon previous elemental analysis. The experimental data have also been compared to Monte Carlo simulations of γ-ray emission following the thermal neutron-capture process using the statistical-decay code DICEBOX. Together, the experimental cross sections and modeled feeding contribution from the quasi continuum, have been used to determine the total radiative thermal neutron-capture cross sections for the tungsten isotopes and provide improved decay-scheme information for the structural- and neutron-data libraries. | |
|
An implementation to read and write IAEA phase-space files in GEANT4-based simulations [Abstract] |
M.A. Cort�s-Giraldo, J.M. Quesada, M.I. Gallardo, R. Capote, International Journal of Radiation Biology 88 (1-2) (2012) pp. 200-208 doi:10.3109/09553002.2011.627977 |
Abstract Purpose: To develop a stand-alone code to make any
application coded with the GEANT4 (GEometry ANd Tracking,
version 4) toolkit capable of reading and writing phase-space
(phsp) files in the format created by the IAEA (International
Atomic Energy Agency), so that the exchange of phsp files
between other validated Monte Carlo (MC) codes and GEANT4
is possible. Methods: We present a stand-alone code, written
in C++ object-oriented language, developed in a way that
ensures the compatibility with future versions of the IAEA phsp
format. The aim of the reader part is to get the information
from a given IAEA phsp file and create the primary particles
in a GEANT4 user application. On the other hand, the writer
part of the code is the responsible for writing the IAEA phsp
files during a run of the GEANT4 application. Results: A testing
simulation was written with GEANT4 to verify the performance
of this code, with satisfactory results. An example of use in
a GEANT4 application which simulates the treatment head
of a radiotherapy linear electron accelerator (linac) is also
shown, comparing dose calculations with experimental data.
Conclusions: This stand-alone package, which can be used in
any GEANT4 application, allows the exchange of validated phsp
files between different MC codes and the use of phsp data from
many different accelerators and fields in dosimetry studies.
Furthermore, it also offers additional utilities of interest in
medical applications. | |
|
Neutron-induced fission cross section of 245Cm: New results from data taken at the time-of-flight facility n_TOF [Abstract] |
M. Calviani, R. Capote, et al., (n_TOF collaboration), Physical Review C 85 (2012) 034616 doi:10.1103/PhysRevC.85.034616 |
Abstract The neutron-induced fission cross section of 245Cm was measured at n TOF in a wide energy range and with
high resolution. The energy dependence, measured in a single measurement from 30 meV to 1 MeV neutron
energy, has been determined with 5% accuracy relative to the 235U(n,f) cross section. In order to reduce the
uncertainty on the absolute value, the data have been normalized at thermal energy to recent measurements
performed at ILL and BR1. In the energy range of overlap, the results are in fair agreement with some previous
measurements and confirm, on average, the evaluated cross section in the ENDF/B-VII.0 database, although
sizable differences are observed for some important resonances below 20 eV. A similar behavior is observed
relative to JENDL/AC-2008, a reactor-oriented database for actinides. The new results contribute to the overall
improvement of the databases needed for the design of advanced reactor systems and may lead to refinements of
fission models for the actinides. | |
|
Measurement and resonance analysis of the 237Np neutron capture cross section [Abstract] |
C. Guerrero, R. Capote, et al., (n_TOF collaboration), Physical Review C 85 (4) (2012) 044616 doi:10.1103/PhysRevC.85.044616 |
Abstract The neutron capture cross section of 237Np was measured between 0.7 and 500 eV at the CERN n_TOF facility
using the 4�? BaF2 Total Absorption Calorimeter. The experimental capture yield was extracted minimizing all the
systematic uncertainties and was analyzed together with the most reliable transmission data available using the
SAMMY code. The result is a complete set of individual as well as average resonance parameters [D0 = 0.56(2) eV,
γ = 40.9(18) meV, 104S0 = 0.98(6), R = 9.8(6) fm]. The capture cross section obtained in this work is in
overall agreement with the evaluations and the data of Weston and Todd [Nucl. Sci. Eng. 79, 184 (1981)], thus
showing sizable differences with respect to previous data from Scherbakov et al. [J. Nucl. Sci. Technol. 42, 135
(2005)] and large discrepancies with data Kobayashi et al. [J. Nucl. Sci. Technol. 39, 111 (2002)]. The results
indicate that a new evaluation combining the present capture data with reliable transmission data would allow
reaching an accuracy better than 4%, in line with the uncertainty requirements of the nuclear data community for
the design and operation of current and future nuclear devices | |
|
Resonance neutron-capture cross sections of stable magnesium isotopes and their astrophysical implications [Abstract] |
C. Massimi, R. Capote, et al., (n_TOF collaboration), Physical Review C 85 (4) (2012) 044615 doi:10.1103/PhysRevC.85.044615 |
Abstract We have measured the neutron capture cross sections of the stable magnesium isotopes 24,25,26Mg in the
energy range of interest to the s process using the neutron time-of-flight facility n_TOF at CERN. Capture
events from a natural metal sample and from samples enriched in 25Mg and 26Mg were recorded using the total energy method based on C6 2H6 detectors. Neutron resonance parameters were extracted by a simultaneous
resonance shape analysis of the present capture data and existing transmission data on a natural isotopic sample.
Maxwellian-averaged capture cross sections for the three isotopes were calculated up to thermal energies of
100 keV and their impact on s-process analyses was investigated. At 30 keV the new values of the stellar cross
section for 24Mg, 25Mg, and 26Mg are 3.8±0.2 mb, 4.1±0.6 mb, and 0.14±0.01 mb, respectively. | |
|
Measurement of resolved resonances of 232Th(n,γ) at the n-TOF facility at CERN [Abstract] |
F. Gunsing, R. Capote, et al., (n_TOF collaboration), Physical Review C 85 (6) (2012) 064601. doi:10.1103/PhysRevC.85.064601 |
Abstract The yield of the neutron capture reaction 232Th(n, γ ) has been measured at the neutron time-of-flight facility
n_TOF at CERN in the energy range from 1 eV to 1 MeV. The reduction of the acquired data to the capture
yield for resolved resonances from 1 eV to 4 keV is described and compared to a recent evaluated data set. The
resonance parameters were used to assign an orbital momentum to each resonance. A missing level estimator
was used to extract the s-wave level spacing of D0 = 17.2 ± 0.9 eV. | |
|
Status of the LEgnaro NeutrOn Source facility (LENOS) [Abstract] |
Pierfrancesco Mastinu, J. Praena, G. Mart�n-Hern�ndez, N. Dzysiuk, G. Prete, R. Capote, M. Pignatari, A. Ventura,
Physics Procedia 26 (2012) 261 ? 273 doi:10.1016/j.phpro.2012.03.034 |
Abstract LENOS is a new facility under development at Laboratori Nazionali di Legnaro (LNL). It is based on a new
technic for neutron beam shaping in accelerator based neutron sources. The main advantage of this method is to be
able to shape the primary charged-particle beam to a defined energy distribution that, impinging on a neutron
producing target, generates the desired neutron spectra at the sample position. Together with the proton energy
distribution, other degrees of freedom are used to obtain the desired neutron energy spectra, e.g. the angular
distribution of produced neutrons, the nuclear reactions used for the neutron spectra production, and the
convolution of neutron spectra coming from different target materials. The main advantage of this new approach is
the good control over the energy and spatial distribution of the produced neutron spectrum avoiding most of the
problems due to neutron moderation, since it is easier to work with charged particles than with neutrons. The goal
of the LENOS facility is to obtain a Maxwell-Boltzmann neutron energy spectrum with tunable temperature and a
high neutron flux at sample position by using the 7Li(p,n) reaction. To maximize the neutron flux a very narrow
primary proton beam has to be used, so the target has to remove a very high specific power. Currently available
lithium targets are inadequate to sustain the high specific power that needs to be dissipated in the LENOS facility.
A dedicated target based on micro-channel geometry and liquid metal cooling has been developed and tested. This
contribution describes the status of the LENOS facility. | |
|
Temperature-tuned Maxwell-Boltzmann neutron spectra for kT ranging from 30 up to 50keV for nuclear astrophysics studies [Abstract] |
G. Mart�n-Hern�ndez, P.F. Mastinu, J. Praena, N. Dzysiuk, R. Capote, M. Pignatari, Applied Radiation and Isotopes 70 (8) (2012), pp. 1583-1589 doi:10.1016/j.apradiso.2012.05.004 |
Abstract The need of neutron capture cross section measurements for astrophysics motivates present work,
where calculations to generate stellar neutron spectra at different temperatures are performed. The
accelerator-based 7Li(p,n)7Be reaction is used. Shaping the proton beam energy and the sample
covering a specific solid angle, neutron activation fo rmeasuring stellar-averaged capture cross section
can be done. High-quality Maxwell�??Boltzmann neutron spectra are predicted. Assuming a general
behavior of the neutron capture cross section a weighted fit of the spectrum to Maxwell�??Boltzmann
distributions is successfully introduced. | |
|
Neutron-induced fission cross section measurement of 233U, 241Am and 243Am in the energy range 0.5MeV < En < 20MeV at n-TOF at CERN [Abstract] |
F. Belloni, R. Capote, et al., (n_TOF collaboration), Physica Scripta, (2012) 014005 doi:10.1088/0031-8949/2012/T150/014005 |
Abstract Neutron-induced fission cross section measurements of 233U, 243Am and 241Am relative to 235U have been carried out at the neutron time-of-flight facility n_TOF at CERN. A fast ionization chamber has been employed. All samples were located in the same detector; therefore the studied elements and the reference 235U target are subject to the same neutron beam. | |
|
Estimation of neutron-equivalent dose in organs of patients undergoing radiotherapy by the use of a novel online digital detector [Abstract] |
F. S�nchez-Doblado, C ,Domingo, F. G�mez, B. S�nchez-Nieto, J.L. Mu�iz, M.J. Garc�a-Fust�, M.R. Exp�sito, R. Barquero, F. Fern�ndez, F., Physics in Medicine and Biology 57 (19) (2012) pp. 6167 doi:10.1088/0031-9155/57/19/6167 |
Abstract Neutron peripheral contamination in patients undergoing high-energy photon
radiotherapy is considered as a risk factor for secondary cancer induction.
Organ-specific neutron-equivalent dose estimation is therefore essential for a
reasonable assessment of these associated risks. This work aimed to develop a
method to estimate neutron-equivalent doses in multiple organs of radiotherapy
patients. The method involved the convolution, at 16 reference points in an
anthropomorphic phantom, of the normalized Monte Carlo neutron fluence
energy spectra with the kerma and energy-dependent radiationweighting factor.
This was then scaled with the total neutron fluence measured with passive detectors, at the same reference points, in order to obtain the equivalent doses
in organs. The latter were correlated with the readings of a neutron digital
detector located inside the treatment room during phantom irradiation. This
digital detector, designed and developed by our group, integrates the thermal
neutron fluence. The correlation model, applied to the digital detector readings
during patient irradiation, enables the online estimation of neutron-equivalent
doses in organs. The model takes into account the specific irradiation site, the
field parameters (energy, field size, angle incidence, etc) and the installation
(linac and bunker geometry). This method, which is suitable for routine clinical
use, will help to systematically generate the dosimetric data essential for the
improvement of current risk-estimation models. | |
|
Updating and extending the IRDF-2002 dosimetry library [Abstract] |
R. Capote, K.I. Zolotarev, V.G. Pronyaev, A. Trkov, ASTM Special Technical Publication 1550 STP (2012) pp.197-202 doi:10.1520/STP155020120015 |
Abstract The International Reactor Dosimetry File (IRDF)-2002 released in 2004 by the IAEA (see http://www-nds.iaea.org/irdf2002/) contains cross-section data and corresponding uncertainties for 66 dosimetry reactions. New cross-section evaluations have become available recently that re-define some of these dosimetry reactions including: (1) high-fidelity evaluation work undertaken by one of the authors (KIZ); (2) evaluations from the US ENDF/B-VII.0 and candidate evaluations from the US ENDF/B-VII.1 libraries that cover reactions within the International Evaluation of Neutron Cross-Section Standards; (3) European JEFF3.1 library; and (4) Japanese JENDL-4.0 library. Additional high-threshold reactions not included in IRDF-2002 (e.g.,59Co(n,3n) and 209Bi(n,3n)) have been also evaluated to characterize higher-energy neutron fields. Overall, 37 new evaluations of dosimetry reactions have been assessed and intercomparisons made with integral measurements in reference neutron fields to determine whether they should be adopted to update and improve IRDF-2002. Benchmark calculations performed for newly evaluated reactions using the ENDF/B-VII.0 235U thermal fission and 252Cf spontaneous fission neutron spectra show that calculated integral cross sections exhibit improved agreement with evaluated experimental data when compared with the equivalent data from the IRDF-2002 library. Data inconsistencies or deficiencies of new evaluations have been identified for 63Cu(n,2n), 60Ni(n,p)60m+gCo, 55Mn(n,γ), and 232Th(n,f) reactions. Compared with IRDF-2002, the upper neutron energy boundary was formally increased from the actual maximum energy of typically 20 MeV up to 60 MeV by using the TENDL-2010 cross sections and covariance matrices. This extension would allow the updated IRDF library to be also used in fusion dosimetry applications. Uncertainties in the cross sections for all new evaluations are given in the form of relative covariance matrices. Newly evaluated excitation functions should be considered as suitable candidates in the preparation of an improved version of the IRDF that was planned to be released for testing in December 2011. | |
|
New work on updating and extending the nuclear data standards [Abstract] |
A.D. Carlson, V.G. Pronyaev, R. Capote, F.-J. Hambsch, F. K�ppeler, C. Lederer, W. Mannhart, A. Mengoni, A. Wallner, ASTM Special Technical Publication 1550 STP (2012) pp. 141-160. doi:10.1520/STP155020120012 |
Abstract An International Atomic Energy Agency (IAEA) Data Development Project was initiated to provide a mechanism for allowing new experimental data and improvements in evaluation procedures to be incorporated into new evaluations of the standards. The work on this project is ongoing. In the past very long periods sometimes occurred between evaluations of the standards. Through the use of this Project, such long periods should not occur. Work on the cross section standards through this Project has included an update of the experimental data to be used in the cross section standards evaluations, a study of the uncertainties obtained in the international standards evaluation, and improvements in the smoothing procedure for capture cross sections. It was decided that this Project should have a broader range of activities than just the cross section standards and thus encompass standards related activities. The following are being investigated: improvements in the gold cross section at energies below where it is considered a standard and work on certain cross sections that are not as well known as the cross section standards but could be very useful as reference cross sections relative to which certain types of cross section measurements can be made. This work includes prompt gamma-ray production in fast neutron-induced reactions, and work on the 252Cf spontaneous fission neutron spectrum and the 235U thermal neutron fission spectrum. Most of the data investigated through this Project are used in dosimetry applications.
| |
|
A New Formulation of the Unified Monte Carlo Approach (UMC-B) and Cross-Section Evaluation for the Dosimetry Reaction 55Mn(n,?)56Mn
[Abstract] |
R. Capote, D.L. Smith, A. Trkov, M. Meghzifene, 2012 ASTM Special Technical Publication 1550 STP (2012) pp. 179-196. doi:10.1520/STP155020120014 |
Abstract Two relatively new approaches to neutron cross section data evaluation are described. They are known collectively as Unified Monte Carlo (versions UMC-G and UMC-B). Comparisons are made between these two methods, as well as with the well-known generalized least-squares (GLSQ) technique, through the use of simple, hypothetical (toy) examples. These new Monte Carlo methods are based on stochastic sampling of probability functions that are constructed with the use of theoretical and experimental data by applying the principle of maximum entropy. No further assumptions are involved in either UMC-G or UMC-B. However, the GLSQ procedure requires the linearization of non-linear terms, such as those that occur when cross section ratio data are included in an evaluation. It is shown that these two stochastic techniques yield results that agree well with each other, and with the GLSQ method, when linear data are involved, or when the perturbations due to data discrepancies and nonlinearity effects are small. Otherwise, there can be noticeable differences. The present investigation also demonstrates, as observed in earlier work, that the least-squares approach breaks down when these conditions are not satisfied. This paper also presents an actual evaluation of the 55Mn(n,γ)56Mn neutron dosimetry reaction cross section in the energy range from 100 keV to 20 MeV, which was performed using both GLSQ and UMC-G approaches. | |
|
Validating the ENDF-B/VII 235U(nth,f) Prompt Fission Neutron Spectrum Using Updated Dosimetry Cross Sections (IRDFF) [Abstract] |
R. Capote, K.I. Zolotarev, V.G. Pronyaev, A. Trkov, International Conference on the Physics of Reactors 2012, PHYSOR 2012: Advances in Reactor Physics 3 (2012) pp. 2690. |
Abstract The International Reactor Dosimetry File IRDF-2002 released in 2004 by the IAEA contains
cross-section data and corresponding uncertainties for 66 dosimetry reactions. New cross-section
evaluations have become available recently that re-define some of these dosimetry reactions for
reactor applications including: 1) high fidelity evaluation work undertaken by one of the authors
(KIZ); 2) evaluations from the ENDF/B-VII libraries that cover reactions within the International
Evaluation of Neutron Cross-Section Standards; and 3) evaluations from JENDL-3.1 and JENDL-
4 libraries. Overall, 37 new evaluations of dosimetry reactions have been assessed to determine
whether they should be adopted to update and improve IRDF-2002. A new dosimetry library
(International Reactor Dosimetry File for Fission and Fusion - IRDFF) was assembled based on
new evaluations combined with selected IRDF-2002 evaluations. A grand-total of 74 dosimetry
reactions are included into the IRDFF dosimetry library available at www-nds.iaea.org/IRDFF1
.
The assembled library was used to validate the 235U(nth,f) ENDF-B/VII.0 prompt fission neutron
spectrum. An excellent average C/E value of 1.002 +/- 0.02 is achieved for reactions with mean
neutron energy of the integrated response (E50%) lower than 11 MeV. C/E data for reactions with
E50%-response higher than 11 MeV decreases up to 0.8. We conclude that the ENDF-B/VII.0
235U(nth,f) prompt fission neutron spectrum from 1-11 MeV is validated within quoted
uncertainties by available integral measurements in 235U(nth,f) neutron field. Further investigations
for high-threshold reactions are needed and new measurements of spectrum average cross sections
for those reactions in the 235U(nth,f) neutron field are recommended | |
|
48Ti(n,n'gamma) gamma production cross section as a candidate for a reference cross section [Abstract] |
S.P. Simakov, V.G. Pronyaev, R. Capote, R.O. Nelson, Proc. of 13th Int. Conf. on Nuclear Reaction Mechanisms, Varenna, 11-15 June 2012, CERN-Proceedings-2012-002 (2012) pp. 321-330. |
Abstract The yield of 984 keV gamma-rays from 48Ti(n,n') reaction has been evaluated from threshold up to 20 MeV. For this purpose all currently available measured discrete gamma production and neutron inelastic cross sections were thoroughly analysed and renormalised to the updated standards when possible. The TALYS and EMPIRE nuclear reaction codes were used to get an optimal description of these cross sections for natural Titanium and its main isotope 48Ti. The final evaluation of the 984 keV gamma-ray yield from 48Ti(n,n') reaction and covariance matrix was performed on the basis of collected experimental data and optimized model calculations employing the least squares code GMA. | |
|
The effects of ionization potential depression on the spectra emitted by hot dense aluminium plasmas [Abstract] |
T.R. Preston, S.M. Vinko, O. Ciricosta, H.-K. Chung, R.W. Lee and J.S. Wark, High Energy Dens. Phys. 9, 258 (2012) doi:10.1016/j.hedp.2012.12.014 |
Abstract Recent experiments at the Linac Coherent Light Source (LCLS) X-ray Free-Electron-Laser (FEL) have demonstrated that the standard model used for simulating ionization potential depression (IPD) in a plasma (the Stewart�??Pyatt (SP) model, J.C. Stewart and K.D. Pyatt Jr., Astrophysical Journal 144 (1966) 1203) considerably underestimates the degree of IPD in a solid density aluminium plasma at temperatures up to 200 eV. In contrast, good agreement with the experimental data was found by use of a modified Ecker�??Kröll (mEK) model (G. Ecker and W. Kröll, Physics of Fluids 6 (1963) 62�??69). We present here detailed simulations, using the FLYCHK code, of the predicted spectra from hot dense, hydrogenic and helium-like aluminium plasmas ranging in densities from 0.1 to 4 times solid density, and at temperatures up to 1000 eV. Importantly, we find that the greater IPDs predicted by the mEK model result in the loss of the n = 3 states for the hydrogenic ions for all densities above �??0.8 times solid density, and for the helium-like ions above �??0.65 solid density. Therefore, we posit that if the mEK model holds at these higher temperatures, the temperature of solid density highly-charged aluminium plasmas cannot be determined by using spectral features associated with the n = 3 principal quantum number, and propose a re-evaluation of previous experimental data where high densities have been inferred from the spectra, and the SP model has been used. | |
|
Resonant Ka Spectroscopy of Solid-Density Aluminum Plasmas [Abstract] |
B.I. Cho, K. Engelhorn, S.M. Vinko, H.-K. Chung et al. Phys. Rev. Lett 109 245003 (2012) doi:10.1103/PhysRevLett.109.245003 |
Abstract The x-ray intensities made available by x-ray free electron lasers (FEL) open up new x-ray matter interaction channels not accessible with previous sources. We report here on the resonant generation of Kα emission, that is to say the production of copious Kα radiation by tuning the x-ray FEL pulse to photon energies below that of the K edge of a solid aluminum sample. The sequential absorption of multiple photons in the same atom during the 80 fs pulse, with photons creating L-shell holes and then one resonantly exciting a K-shell electron into one of these holes, opens up a channel for the Kα production, as well as the absorption of further photons. We demonstrate rich spectra of such channels, and investigate the emission produced by tuning the FEL energy to the K-L transitions of those highly charged ions that have transition energies below the K edge of the cold material. The spectra are sensitive to x-ray intensity dependent opacity effects, with ions containing L-shell holes readily reabsorbing the Kα radiation. | |
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Excitation functions of (d,x) nuclear reactions on natural titanium up to 24 MeV [Abstract] |
M.U. Khandaker, H. Haba, J. Kanaya, N. Otuka, Nucl. Instrum. Meth. Phys. Res. B 296 (2013) pp. 14-21.
doi:10.1016/j.nimb.2012.12.003 |
Abstract Excitation functions of the natTi(d,x)48V and natTi(d,x)43,44m,44g,46,47,48Sc nuclear reactions were measured up to a 24-MeV deuteron energy by using a stacked-foil activation technique combined with γ-ray spectrometry with a high-purity germanium detector at the AVF cyclotron of the RIKEN RI Beam Factory, Wako, Japan. An overall good agreement is found between the measured cross-sections and the literature ones, whereas partial agreements are obtained for the theoretical calculations based on the TALYS code. Physical thick target yields, i.e., induced radioactivities per unit fluence of the 24-MeV deuteron were also deduced, and they were compared with the directly measured ones in the literature. The present results will have an important role in enrichment of the literature database of the deuteron-induced reactions on natural titanium leading to various applications. | |
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High-sensitivity isobar-free AMS measurements and reference materials for 55Fe, 68Ge and 202gPb [Abstract] |
A. Wallner, M. Bichler, K. Buczak, D. Fink, O. Forstner, R. Golser, M.A.C. Hotchkis, A. Klix, A. Krasa, W. Kutschera, C. Lederer, A. Plompen, A. Priller, D. Schumann, V. Semkova, P. Steier, J. Nucl. Instr. Meth. Phys. Res. B294 (2013) pp. 374-381. doi:10.1016/j.nimb.2012.03.029 |
Abstract Isobaric interference represents one of the major limitations in mass spectrometry. For a few cases in
AMS with tandem accelerators, isobaric interference is completely excluded like the well-known major
isotopes 14C, 26Al, 129I. Additional isotopes are 55Fe, 68Ge, and 202Pb, with 68Ge and 202Pb never been used in AMS so far. Their respective stable isobars 55Mn, 68Zn and 202Hg do not form stable negative ions. The exceptional sensitivity of AMS for 55Fe, 68Ge and 202gPb offers important insights into such different fields like nuclear astrophysics, fundamental nuclear physics and technological applications. VERA, a dedicated AMS facility is well suited for developing procedures for new and non-standard isotopes. AMS measurements at the VERA facility established low backgrounds for these radionuclides in natural samples. Limits for isotope ratios of <10-15, <10-16
and <2x10-14 were measured for 55Fe/56Fe, 68Ge/70Ge and 202Pb/Pb, respectively. In order to generate
accurate isotope ratios of sample materials, AMS relies on the parallel measurement of reference materials
with well-known ratios. A new and highly accurate reference material for 55Fe measurements with
an uncertainty of ±1.6% was produced from a certified reference solution. In case of 68Ge dedicated neutron
activations produced a sufficiently large number of 68Ge atoms that allowed quantifying them
through the activity of its decay product 68Ga. Finally, for 202Pb, the short-lived isobar 202Tl was produced
via neutron activation and served as a proxy for 202Pb AMS measurements. | |
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Nuclear data from AMS & nuclear data for AMS - some examples [Abstract] |
A. Wallner, M. Bichler, T. Belgya, K. Buczak, I. Dillmann, O. Forstner, R. Golser, F. K�ppeler, A. Klix, G.
Korschinek, A. Krasa, W. Kutschera, C. Lederer, A. Mengoni, M. Paul, A. Plompen, A. Priller1, V. Semkova,
P. Steier, EPJ Web of Conferences 35, 01003 (2012) doi:10.1051/epjconf/20123501003 |
Abstract We summarize some recent cross-section measurements using accelerator mass spectrometry
(AMS). AMS represents an ultra-sensitive technique for measuring a limited, but steadily increasing number of
longer-lived radionuclides. This method implies a two-step procedure with sample activation and subsequent
AMS measurement. Applications include nuclear astrophysics, nuclear technology (nuclear fusion, nuclear
fission and advanced reactor concepts and radiation dose estimations). A series of additional applications
involves cosmogenic radionuclides in environmental, geological and extraterrestrial studies. There is a lack of
information for a list of nuclides, as pointed out by nuclear data requests. An overview of some recent
measurements is given and the method is illustrated for some specific neutron-induced reactions. | |
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Experimental nuclear reaction data uncertainties: Basic concepts and documentation [Abstract] |
D.L. Smith, N. Otuka, Nucl. Data Sheets 113 (2012) pp. 3006-3053.
doi:10.1016/j.nds.2012.11.004 |
Abstract This paper has been written to provide experimental nuclear data researchers and data compilers with practical
guidance on dealing with experimental nuclear reaction data uncertainties. It outlines some of the properties
of random variables as well as principles of data uncertainty estimation, and illustrates them by means of simple
examples which are relevant to the field of nuclear data. Emphasis is placed on the importance of generating
mathematical models (or algorithms) that can adequately represent individual experiments for the purpose of estimating
uncertainties in their results. Several types of uncertainties typically encountered in nuclear data experiments
are discussed. The requirements and procedures for reporting information on measurement uncertainties for neutron reaction data, so that they will be useful in practical applications, are addressed. Consideration is given to the challenges and opportunities offered by reports, conference proceedings, journal articles, and computer libraries as vehicles for reporting and documenting numerical experimental data. Finally, contemporary formats used to compile reported experimental covariance data in the widely used library EXFOR are discussed, and several samples of EXFOR files are presented to demonstrate their use.
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Determination of resonance parameters and their covariances from neutron induced reaction cross section data [Abstract] |
P. Schillebeeckx, B. Becker, Y. Danon, K. Guber, H. Harada, J. Heyse, A.R. Junghans, S. Kopecky, C. Massimi, M.C. Moxon, N. Otuka, I. Sirakov, K. Volev, Nucl. Data Sheets 113 (2012) pp. 3054-3100.
doi:10.1016/j.nds.2012.11.005 |
Abstract Cross section data in the resolved and unresolved resonance region are represented by nuclear
reaction formalisms using parameters which are determined by fitting them to experimental data.
Therefore, the quality of evaluated cross sections in the resonance region strongly depends on the
experimental data used in the adjustment process and an assessment of the experimental covariance
data is of primary importance in determining the accuracy of evaluated cross section data. In this
contribution, uncertainty components of experimental observables resulting from total and reaction
cross section experiments are quantified by identifying the metrological parameters involved in
the measurement, data reduction and analysis process. In addition, different methods that can be applied to propagate the covariance of the experimental observables (i.e. transmission and reaction yields) to the covariance of the resonance parameters are discussed and compared. The methods being discussed are: conventional uncertainty propagation, Monte Carlo sampling and
marginalization. It is demonstrated that the final covariance matrix of the resonance parameters not only strongly depends on the type of experimental observables used in the adjustment process, the experimental conditions and the characteristics of the resonance structure, but also on the method that is used to propagate the covariances. Finally, a special data reduction concept and format is presented, which offers the possibility to store the full covariance information of experimental data in the EXFOR library and provides the information required to perform a full covariance evaluation. | |
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Data reduction and uncertainty propagation of time-of-flight spectra with AGS [Abstract] |
B. Becker, C. Bastian, F. Emiliani, F. Gunsing, J. Heyse, K. Kauwenberghs, S. Kopecky, C. Lampoudis, C. Massimi, N. Otuka, P. Schillebeeckx, I. Sirakov, J. Instrum. 7 (2012) P11002.
doi:10.1088/1748-0221/7/11/P11002 |
Abstract Results of neutron time-of-flight measurements are commonly used to parameterize neutron induced reaction cross sections in the resonance region based on the R-matrix reaction theory. Reaction yields or transmission as well as their covariance information are derived starting from measured counting spectra. They are then used in a least squares adjustment for obtaining model parameters.
In this paper, a compact formalism is presented to propagate both the correlated and uncorrelated uncertainty components. Full information on the origin of each correlated component of the covariance matrix is maintained. This is particularly important in order to avoid a bias on the model parameters through a phenomenon known as Peelle�??s Pertinent Puzzle (PPP). This compact formalism was implemented into the data reduction code AGS (Analysis of Geel Spectra).
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Direct Measurements of the Ionization Potential Depression in a Dense Plasma [Abstract] |
O. Ciricosta, S.M. Vinko, H.-K. Chung et al. Phys. Rev. Lett 109 (2012) pp.065002 doi:10.1103/PhysRevLett.109.065002 |
Abstract We have used the Linac Coherent Light Source to generate solid-density aluminum plasmas at temperatures of up to 180 eV. By varying the photon energy of the x rays that both create and probe the plasma, and observing the K- fluorescence, we can directly measure the position of the K edge of the highly charged ions within the system. The results are found to disagree with the predictions of the extensively used Stewart-Pyatt model, but are consistent with the earlier model of Ecker and Kroll, which
predicts significantly greater depression of the ionization potential. | |
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Creation and diagnosis of a solid-density plasma with an X-ray free-electron laser [Abstract] |
S.M. Vinko, O. Ciricosta, B.I. Cho, K. Engelhorn, H.-K. Chung, C.R.D. Brown, T. Burian, J. Chalupsk�, R.W. Falcone, C. Graves, V. H�jkov�, A. Higginbotham, L. Juha, J. Krzywinski, H.J. Lee, M. Messerschmidt, C.D. Murphy, Y. Ping, A. Scherz, W. Schlotter, S. Toleikis, J.J. Turner, L. Vysin, T. Wang, B. Wu et al. Nature 482 (2012) pp.59-62 doi:10.1038/nature10746 |
Abstract Matter with a high energy density (>105�??joules per cm3) is prevalent throughout the Universe, being present in all types of stars and towards the centre of the giant planets; it is also relevant for inertial confinement fusion. Its thermodynamic and transport properties are challenging to measure, requiring the creation of sufficiently long-lived samples at homogeneous temperatures and densities. With the advent of the Linac Coherent Light Source (LCLS) X-ray laser, high-intensity radiation (>1017�??watts per cm2, previously the domain of optical lasers) can be produced at X-ray wavelengths. The interaction of single atoms with such intense X-rays has recently been investigated8. An understanding of the contrasting case of intense X-ray interaction with dense systems is important from a fundamental viewpoint and for applications. Here we report the experimental creation of a solid-density plasma at temperatures in excess of 106 kelvin on inertial-confinement timescales using an X-ray free-electron laser. We discuss the pertinent physics of the intense X-ray�??matter interactions, and illustrate the importance of electron�??ion collisions. Detailed simulations of the interaction process conducted with a radiative-collisional code show good qualitative agreement with the experimental results. We obtain insights into the evolution of the charge state distribution of the system, the electron density and temperature, and the timescales of collisional processes. Our results should inform future high-intensity X-ray experiments involving dense samples, such as X-ray diffractive imaging of biological systems, material science investigations, and the study of matter in extreme conditions. | |
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Benchmark of Spallation Models [Abstract] |
J.-C.David, D.Filges, F.Gallmeier, M.Khandaker, A,Konobeyev, S. Leray, G.Mank, A.Mengoni, R.Michel, N.Otuka, Y.Yariv,
Prog.Nucl.Sci.Technol. 2 (2011) pp. 942-947.
doi:10.15669/pnst.2.942 |
Abstract Spallation reactions play an important role in many branches of physics. If the nuclear reaction induced by low
energy neutrons as in nuclear power plants or research reactors can be based on cross section database, it is not the
case for spallation reactions due to the energy range, from 100 MeV up to ~3 GeV, and to the candidate targets (all
nuclei). Then these reactions have to be modeled. Developments of codes are linked to new experiment and this explains
why fifteen years ago a first benchmark has been launched, restricted to particle production, followed by a
second one on residues. Since then new data have been measured and computer tools are improved day after day, so a
new benchmark has been organized, under the auspices of the IAEA, taken into account all types of results, particle
and residue production, with a possibility to update the data (experimental and code calculation) via a web site. Results
of the benchmark concerning both the analysis of the prediction capabilities of the seventeen model-participants
and the first conclusions on the physics of spallation models are presented.
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Systematic study of (n,p) reaction cross sections from the reaction threshold to 20 MeV [Abstract] |
B. Lalremruata, N. Otuka, G.J. Tambave, V.K. Mulik, B.J. Patil, S.D. Dhole, A. Saxena, S. Ganesan, V.N. Bhoraskar, Phys. Rev. C 85 (2011) 024624. doi:10.1103/PhysRevC.85.024624 |
Abstract The cross sections of natCr(n,x)52V, 52Cr(n,p)52V, natCr(n,x)53V, 53Cr(n,p)53V, natZn(n,x)66Cu, 66Zn(n,p)66Cu, natZn(n,x)68Cum, 68Zn(n,p)68Cum, natMo(n,x)97Nbg, 97Mo(n,p)97Nbg, natMo(n,x)97Nbm, 97Mo(n,p)97Nbm, natSn(n,x)116Inm1+m2, 116Sn(n,p)116Inm1+m2, natSn(n,x)117Ing, 117Sn(n,p)117Ing, natSn(n,x)118Inm1+m2,118Sn(n,p)118Inm1+m2, natSn(n,x)120
Inx , 120Sn(n,p)120Inx , natBa(n,x)138Cs, and 138Ba(n,p)138Cs reactions have been measured at 14.8 MeV neutron energy. In the present work, the contributions of (n,np), (n,pn), and (n,d) reactions from heavier isotopes are subtracted. The cross sections were also estimated with the TALYS-1.2 nuclear model code using different level density models, at neutron energies varying from the reaction threshold to 20 MeV. The variations in the (n,p) cross sections with the neutron number in the isotopes of an element are
also discussed in brief. | |
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Experimental Nuclear Reaction Data Library (EXFOR) ? Compilation and Dissemination of Nuclear Reaction Data Provided by Nuclear Reaction Data Centres Network [Abstract] |
V. Semkova, N. Otuka, S.P. Simakov, V. Zerkin, Presented at 8th Int. Conf. ?Nuclear and Radiation Physics?, 20-23 September 2011, Almaty, Kazakhstan pp. 191-194 ISBN 9965-675-78-3. |
Abstract The International Network of Nuclear Reaction Data Centres (NRDC) constitutes a worldwide cooperation of nuclear data centres under the auspices of the International Atomic Energy Agency. The main activity of the NRDC Network is collection and compilation of experimental nuclear reaction data and the related bibliographic information in the EXFOR and CINDA databases as well as dissemination of nuclear reaction data and associated documentation to users. The present status of the EXFOR database will be presented together with the latest development for data access and retreaval. | |
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Experimental Nuclear Reaction Data Collection EXFOR [Abstract] |
V. Semkova, N. Otuka, S.P. Simakov, V. Zerkin, 2nd International Conference on Advancements in Nuclear Instrumentation, Measurement Methods and their Applications (ANIMMA 2011), June 6-9, 2011, Ghent, Belgium, IEEE Conference Proceedings CFP1124I-CDR. doi:10.1109/ANIMMA.2011.6172861 |
Abstract The International Network of Nuclear Reaction Data Centres (NRDC) constitutes a worldwide cooperation of 14 nuclear data centres. The main activity of the NRDC Network is collection and compilation of experimental nuclear reaction cross section data and the related bibliographic information in the EXFOR and CINDA databases as well as dissemination of nuclear reaction data and associated documentation to users. The database contains information and numerical data from more than about 19000 experiments consisting of more than 140000 datasets. EXFOR is kept up to date by constantly adding newly published experimental information. Tools developed for data dissemination utilise modern database technologies with fast online capabilities over the Internet. Users are provided with sophisticated search options, a user-friendly retrieval interface
for downloading data in different formats, and additional output options such as improved data plotting capabilities. The present
status of the EXFOR database will be presented together with the latest development for data access and retrieval. | |
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Proton elastic scattering differential cross-sections for 12C [Abstract] |
D. Abriola, A.F. Gurbich, M. Kokkoris, A. Lagoyannis, V. Paneta, J. Nucl. Instrum. Methods in Phys. Res. B269 (2011) pp. 2011-2016. doi:10.1016/j.nimb.2011.06.002 |
Abstract Carbon depth profiling presents a strong analytical challenge for all the major ion beam analysis (IBA) techniques, with elastic backscattering spectroscopy (EBS) being widely implemented. In the past, the 12C(p,p)12C reaction has been successfully evaluated for proton beam energies up to 4.5 MeV. Currently, an attempt is being made to extend this evaluation to higher energies, namely up to Ep,lab = 7 MeV. There is a certain lack of available and/or coherent datasets in literature for these relatively high proton beam energies at backward angles, suitable for IBA. Moreover, the few existing datasets are in certain cases discrepant. Thus, in the present work, the differential cross-section of proton elastic scattering on carbon were measured between 140°and 170°, in steps of 10°, for the proton beam energy range between 2.7 and 7 MeV. The experimental results obtained, along with data from literature, were evaluated applying nuclear physics models. The evaluated results were benchmarked using a thick, mirror polished glassy carbon target at different beam energies and detector angles. | |
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Compilation, evaluation, and dissemination of covariances in microscopic nuclear reaction data [Abstract] |
N. Otuka, R. Capote, V. Zerkin, Transact. American Nucl. Soc. 104 (2011) pp. 774-775. |
Abstract Accurate uncertainty and covariance in microscopic
nuclear reaction data (e.g., resonance parameters, cross
sections) are needed for safe and economic design of new
reactors. Evaluators of nuclear data libraries are trying to
collect, evaluate, and distribute uncertainty and
covariance information to satisfy those needs. To support
these tasks, the IAEA Nuclear Data Section (NDS) is
actively developing the experimental data library,
appropriate evaluation methods and dissemination tools
that will be reviewed in this paper. | |
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Assessment of Actinide Decay Data Evaluations: Findings of an IAEA Coordinated Research Project [Abstract] |
M.A. Kellett, presented at 18th Int. Conf. on Radionuclide Metrology and its Applications (ICRM 2011), 19-23 September 2011, Tsukuba, Japan; Appl. Radiat. Isot. 70, Issue 9 (September 2012), pp.1919-1923. doi:10.1016/j.apradiso.2012.02.036 |
Abstract Organised under the auspices of the International Atomic Energy Agency, comprehensive decay scheme evaluations for over eighty actinides and their decay products have been completed on the basis of detailed assessments of the available experimental data. However, despite the application of sound evaluation procedures, such work cannot replace the need to perform and access good quality measurements for adoption. This evaluation programme provided a means of quantifying the quality of the underlying data to ensure that well-focused recommendations could be made for future experimental decay-data studies. | |
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ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data [Abstract] |
M.B. Chadwick, R. Capote, et. al., Nucl. Data Sheets 112 (2011) 2887-2996. doi:10.1016/j.nds.2011.11.002 |
Abstract The ENDF/B-VII.1 library is our latest recommended evaluated nuclear data file for use in nuclear science and technology applications, and incorporates advances made in the five years since the release of ENDF/B-VII.0. These advances focus on neutron cross sections, covariances, fission product yields and decay data, and represent work by the US Cross Section Evaluation Working Group (CSEWG) in nuclear data evaluation that utilizes developments in nuclear theory, modeling, simulation, and experiment.
The principal advances in the new library are: (1) An increase in the breadth of neutron reaction cross section coverage, extending from 393 nuclides to 423 nuclides; (2) Covariance uncertainty data for 190 of the most important nuclides, as documented in companion papers in this edition; (3) R-matrix analyses of neutron reactions on light nuclei, including isotopes of He, Li, and Be; (4) Resonance parameter analyses at lower energies and statistical high energy reactions for isotopes of Cl, K, Ti, V, Mn, Cr, Ni, Zr and W; (5) Modifications to thermal neutron reactions on fission products (isotopes of Mo, Tc, Rh, Ag, Cs, Nd, Sm, Eu) and neutron absorber materials (Cd, Gd); (6) Improved minor actinide evaluations for isotopes of U, Np, Pu, and Am (we are not making changes to the major actinides 235,238U and 239Pu at this point, except for delayed neutron data and covariances, and instead we intend to update them after a further period of research in experiment and theory), and our adoption of JENDL-4.0 evaluations for isotopes of Cm, Bk, Cf, Es, Fm, and some other minor actinides; (7) Fission energy release evaluations; (8) Fission product yield advances for fission-spectrum neutrons and 14 MeV neutrons incident on 239Pu; and (9) A new decay data sublibrary.
Integral validation testing of the ENDF/B-VII.1 library is provided for a variety of quantities: For nuclear criticality, the VII.1 library maintains the generally-good performance seen for VII.0 for a wide range of MCNP simulations of criticality benchmarks, with improved performance coming from new structural material evaluations, especially for Ti, Mn, Cr, Zr and W. For Be we see some improvements although the fast assembly data appear to be mutually inconsistent. Actinide cross section updates are also assessed through comparisons of fission and capture reaction rate measurements in critical assemblies and fast reactors, and improvements are evident. Maxwellian-averaged capture cross sections at 30 keV are also provided for astrophysics applications.
We describe the cross section evaluations that have been updated for ENDF/B-VII.1 and the measured data and calculations that motivated the changes, and therefore this paper augments the ENDF/B-VII.0 publication [M. B. Chadwick, P. Obložinský, M. Herman, N. M. Greene, R. D. McKnight, D. L. Smith, P. G. Young, R. E. MacFarlane, G. M. Hale, S. C. Frankle, A. C. Kahler, T. Kawano, R. C. Little, D. G. Madland, P. Moller, R. D. Mosteller, P. R. Page, P. Talou, H. Trellue, M. C. White, W. B. Wilson, R. Arcilla, C. L. Dunford, S. F. Mughabghab, B. Pritychenko, D. Rochman, A. A. Sonzogni, C. R. Lubitz, T. H. Trumbull, J. P. Weinman, D. A. Br, D. E. Cullen, D. P. Heinrichs, D. P. McNabb, H. Derrien, M. E. Dunn, N. M. Larson, L. C. Leal, A. D. Carlson, R. C. Block, J. B. Briggs, E. T. Cheng, H. C. Huria, M. L. Zerkle, K. S. Kozier, A. Courcelle, V. Pronyaev, and S. C. van der Marck, �??ENDF/B-VII.0: Next Generation Evaluated Nuclear Data Library for Nuclear Science and Technology,�?� Nuclear Data Sheets 107, 2931 (2006)].
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The Nuclear Science References (NSR) database and Web Retrieval System [Abstract] |
B. Pritychenko, E. B?t�k, M.A. Kellett, B. Singh, J. Totans, J. Nucl. Instrum. Methods in Phys. Res., A640 (2011) pp. 213-218. doi:10.1016/j.nima.2011.03.018 |
Abstract The Nuclear Science References (NSR) database together with its associated Web interface is the world�??s
only comprehensive source of easily accessible low- and intermediate-energy nuclear physics bibliographic
information for more than 200,000 articles since the beginning of nuclear science. The weekly
updated NSR database provides essential support for nuclear data evaluation, compilation and research
activities. The principles of the database and Web application development and maintenance are
described. Examples of nuclear structure, reaction and decay applications are specifically included.
The complete NSR database is freely available at the websites of the National Nuclear Data Center
http://www.nndc.bnl.gov/nsr and the International Atomic Energy Agency http://www-nds.iaea.org/nsr. | |
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Covariances of Evaluated Nuclear Cross Section Data for 232Th, 180,182,183,184,186W and 55Mn [Abstract] |
A. Trkov, R. Capote, E.Sh. Soukhovitskii, L.C. Leal, M. Sin, I. Kodeli, D.W. Muir, Nuclear Data Sheets 112 (2011) 3098-3119. doi:10.1016/j.nds.2011.11.007 |
Abstract The EMPIRE code system is a versatile package for nuclear model calculations that is often used
for nuclear data evaluation. Its capabilities include random sampling of model parameters, which
can be utilised to generate a full covariance matrix of all scattering cross sections, including crossreaction
correlations. The EMPIRE system was used to prepare the prior covariance matrices of
reaction cross sections of 232Th, 180,182,183,184,186W and 55Mn nuclei for incident neutron energies up
to 60 MeV. The obtained modelling prior was fed to the GANDR system, which is a package for a
global assessment of nuclear data, based on the Generalised Least-Squares method. By introducing
experimental data from the EXFOR database into GANDR, the constrained covariance matrices
and cross section adjustment functions were obtained. Applying the correction functions on the cross
sections and formatting the covariance matrices, the final evaluations in ENDF-6 format including
covariances were derived. In the resonance energy range, separate analyses were performed to
determine the resonance parameters with their respective covariances. The data files thus obtained
were then subjected to detailed testing and validation. Described evaluations with covariances of
232Th, 180,182,183,184,186W and 55Mn nuclei are included into the ENDF/B-VII.1 library release. | |
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Nuclear Data Activities at the IAEA Nuclear Data Section [Abstract] |
S.P. Simakov, Procs. 20th Int. Conf. Nuclear Energy for New Europe 2011, 305.1-305.8. |
Abstract The Nuclear Data Section of IAEA assembles, develops and disseminates nuclear data
for basic science and practical applications. This paper gives an overview of the NDS
activities aimed at the development and maintenance of general purpose databases, such as
collection of experimental and evaluated reaction cross sections data, as well as those for the
specific energy and material applications, namely for ion material beam analyses, neutron
dosimetry, fission and fusion neutronics. The latest upgrades, developments and existing
weaknesses are highlighted. | |
|
Measurement of the 236U(n,f) cross section from 170 meV to 2 MeV at the CERN n_TOF facility [Abstract] |
R. Sarmento, R. Capote, et al., (the n_TOF Collaboration) Phys. Rev. C84 (2011) 044618.
doi:10.1103/PhysRevC.84.044618 |
Abstract The neutron-induced fission cross section of 236U was measured at the neutron Time-of-Flight (n_TOF) facility
at CERN relative to the standard 235U(n,f) cross section for neutron energies ranging from above thermal to
several MeV. The measurement, covering the full range simultaneously, was performed with a fast ionization
chamber, taking advantage of the high resolution of the n_TOF spectrometer. The n_TOF results confirm that
the first resonance at 5.45 eV is largely overestimated in some nuclear data libraries. The resonance triplet
around 1.2 keV was measured with high resolution and resonance parameters were determined with good
accuracy. Resonances at high energy have also been observed and characterized and different values for the
cross section are provided for the region between 10 keV and the fission threshold. The present work indicates
various shortcomings of the current nuclear data libraries in the subthreshold region and provides the basis for an
accurate re-evaluation of the 236U(n,f) cross section, which is of great relevance for the development of emerging
or innovative nuclear reactor technologies. | |
|
96Zr(n,?) measurement at the n_TOF facility at CERN [Abstract] |
G. Tagliente, R. Capote, et al., (the n_TOF Collaboration) Phys. Rev. C84 (2011) 055802. doi:10.1103/PhysRevC.84.055802 |
Abstract The (n,γ) cross section of 96Zr has been investigated at the CERN n_TOF spallation neutron source. High resolution
time-of-flight measurements using an enriched ZrO2 sample allowed us to analyze 15 resonances
below 40 keV with improved accuracy. On average, the capture widths were found to be 25% smaller than
reported in earlier experiments. If complemented with the contribution by direct radiative capture, the derived
Maxwellian averaged cross sections are consistent with activation data at kT = 25 keV. The present results
confirm the astrophysical implications for the s-process branching at sup>95Zr. | |
|
Comparative study of the dust particle population sampled during four consecutive campaigns in full-tungsten ASDEX Upgrade [Abstract] |
N. Endstrasser, V. Rohde, M. Balden, P. Humrickhouse, U. von Toussaint, B.J Braams, H. K. Chung, R. Neu and the ASDEX Upgrade team, Phys. Scr. T145 (2011) 014021. doi:10.1088/0031-8949/2011/T145/014021 |
Abstract Scanning electron microscopy images and energy-dispersive x-ray spectra were recorded for a total of about 4�?104 dust particles collected on the same position within the vacuum vessel via silicon wafers during four consecutive full-tungsten first wall campaigns of ASDEX Upgrade between 2007 and 2009. By careful analysis of the elemental composition and shape of the sampled particles, seven statistically relevant classes of dust were identified. The particle flux and area coverage of each class were normalized to the total plasma duration of each sampling period, revealing a high sensitivity of the dust composition to device conditioning. According to the present results, particles produced by arcing on divertor tiles with delaminated coatings were transported to the main chamber first wall. | |
|
Coordinated Research Projects of the IAEA Atomic and Molecular Data Unit [Abstract] |
B.J. Braams, H.-K. Chung, 7th Int. Conf. on Atomic and Molecular data and their applications - ICAMDATA-2010, Vilnius, Lithuania, 21-24 September 2010, AIP Conf. Proc. 1344 (2011) pp. 171-178. doi:10.1063/1.3585816 |
Abstract The IAEA Atomic and Molecular Data Unit is dedicated to the provision of databases for atomic, molecular and plasma-material interaction (AM-PMI) data that are relevant for nuclear fusion research. IAEA Coordinated Research Projects (CRPs) are the principal mechanism by which the Unit encourages data evaluation and the production of new data. Ongoing and planned CRPs on AM-PMI data are briefly described here. | |
|
The Dynamics of Allyl Radical Dissociation [Abstract] |
Chao Chen, B. Braams, D.Y. Lee, J.M. Bowman, P.L. Houston, D. Stranges, J. Phys. Chem. A115 (2011) pp. 6797?6804. doi:10.1021/jp109344g |
Abstract Dissociation of the allyl radical, CH2CHCH2, and its deuterated isotopolog, CH2CDCH2, have been investigated using trajectory calculations on an ab initio ground-state potential energy surface calculated for 97�??418 geometries at the coupled cluster single and double and perturbative treatment of triple excitations, with the augmented correlation consistent triple-ζ basis set level (CCSD(T)/AVTZ). At an excitation energy of 115 kcal/mol, corresponding to optical excitation at 248 nm, the primary channel is hydrogen loss with a quantum yield of 0.94 to give either allene or propyne in a ratio of 6.4:1. The total dissociation rate for CH2CHCH2 is 6.3 �? 1010 s�??1, corresponding to a 1/e time of 16 ps. Methyl and C2H2 are produced with a quantum yield of 0.06 by three different mechanisms: a 1,3 hydrogen shift followed by C�??C cleavage to give methyl and acetylene, a double 1,2 shift followed by C�??C cleavage to give methyl and acetylene, or a single 1,2 hydrogen shift followed by C�??C cleavage to give methyl and vinylidene. In this last channel, the vinylidene eventually isomerizes to give internally excited acetylene, and the kinetic energy distribution is peaked at much lower energy (6.4 kcal/mol) than that for the other two channels (18 kcal/mol). The trajectory results also predict the v�??J correlation, the anisotropy of dissociation, and distributions for the angular momentum of the fragments. The v�??J correlation for the CH3 + HCCH channel is strongest for high rotational levels of acetylene, where v is perpendicular to J. Methyl elimination is anisotropic, with β = 0.66, whereas hydrogen elimination is nearly isotropic. In the hydrogen elimination channel, allene is rotationally excited with a total angular momentum distribution peaked near J = 17. In the methyl elimination channel, the peak of the methyl rotational distribution is at J �?? 12, whereas the peak of the acetylene rotational distribution is at J �?? 28. | |
|
Flexible, ab initio potential, and dipole moment surfaces for water. I. Tests and applications for clusters up to the 22-mer [Abstract] |
Yimin Wang, Xinchuan Huang, B.C. Shepler, B.J. Braams and J.M. Bowman, J. Chem. Phys. 134 (2011) 094509. doi:10.1063/1.3554905 |
Abstract We report full-dimensional, ab initio potential energy and dipole moment surfaces, denoted PES and DMS, respectively, for arbitrary numbers of water monomers. The PES is a sum of 1-, 2-, and 3-body potentials which can also be augmented by semiempirical long-range higher-body interactions. The 1-body potential is a spectroscopically accurate monomer potential, and the 2- and 3-body potentials are permutationally invariant fits to tens of thousands of CCSD(T)/aug-cc-pVTZ and MP2/aug-cc-pVTZ electronic energies, respectively. The DMS is a sum of 1- and 2-body DMS, which are covariant fits to tens of thousands MP2/aug-cc-pVTZ dipole moment data. We present the details of these new 2- and 3-body potentials and then extensive applications and tests of this PES are made to the structures, classical binding energies, and harmonic frequencies of water clusters up to the 22-mer. In addition, we report the dipole moment for these clusters at various minima and compare the results against available and new ab initio calculations. | |
|
Nuclear Analytical Applications within the IAEA Nuclear Data Section [Abstract] |
M.A. Kellett, Procs. 11th Int. Conf. "Applications of Nuclear Techniques", Crete, (Greece), 12?18 June 2011, AIP Conf. Procs. 1412 (2011) pp. 430-437. doi:10.1063/1.3665345 |
Abstract The Nuclear Data Section, International Atomic Energy Agency, supports Member States development of nuclear techniques through a number of targeted actions and projects. The Section fulfills this role by organizing Coordinated Research Projects, or through less formal Data Development Projects and/or Technical Meetings. Training workshops are also regularly organized in conjunction with the International Centre for Theoretical Physics (ICTP), Trieste, Italy. A number of projects relating to materials analysis techniques have been recently undertaken, e.g. neutron activation analysis, ion beam analysis, and proton induced X- or γ-ray emission. In particular, details of the Coordinated Research Project focusing on the nuclear data requirements for the k0 method of neutron activation analysis are given. The paper illustrates how the IAEA strives to bring together relevant partners and provides a unique and structured basis for international collaboration. | |
|
Investigations of 89Y(p,x)86,88,89gZr, 86m+g,87g,87m,88gY, 85gSr, and 84gRb nuclear processes up to 42 MeV [Abstract] |
M.U. Khandaker, K. Kim, M.-W. Lee, K-S. Kim, G. Kim, N. Otuka, Nucl. Instr. Meth. Phys. Res. B 271 (2012) pp. 72-81. doi:10.1016/j.nimb.2011.11.009 |
Abstract Production cross-sections of the 89Y(p,x)86,88,89gZr, 86m+g,87g,87m,88gY, 85gSr, and 84gRb nuclear processes
were investigated up to 42-MeV proton energy by using a stacked-foil activation technique at the MC-
50 cyclotron of the Korea Institute of Radiological and Medical Sciences. Cumulative cross-sections of
the 88gY radionuclide have been reported here for the first time from proton activation on natural yttrium
target. The present data were compared with the available experimental data as well as theoretical calculations
based on the TALYS and the ALICE-IPPE codes, and found in general good agreement among
them. Due to the mono-isotopic characteristics of the natural yttrium, the investigated 89Y(p,x)86,88,89gZr,
86m+g,87g,87m,88gY, 85gSr, and 84gRb processes are suitable for testing of nuclear reaction theories and/or
mechanism. A quantitative analysis has also done to understand more accurately the predictive power
of the model codes by performing calculations of deviation factors between the measured data and
respective model calculations. The thick target integral yields, i.e., induced radioactivity per unit fluence
of 42-MeV protons were also deduced from the measured cross-sections of the investigated radionuclides.
Optimal production pathway for the 89Zr-PET radionuclide using a cyclotron is discussed elaborately.
The measured cross-sections of 87gY, 88gY, 88Zr, and 89gZr radionuclides find importance due to
their suitable decay characteristics leading to medical and thin layer activation applications. In addition,
the present experimental results will play an important role in enrichment of the literature data base for
proton-induced reactions on natural yttrium leading to various applications. | |
|
Development of a genetic algorithm for the search of optical model parameters [Abstract] |
D. Abriola, Nucl. Instr. Meth. Phys. Res. B269 (2011) pp. 2984-2989. doi:10.1016/j.nimb.2011.04.054 |
Abstract The analysis of elastic scattering cross sections in terms of the Optical Model is subject to a series of well
known ambiguities. Diverse assumptions about the initial values or shape of the potentials frequently
produce different parameters, leading to different physical interpretations of the observed data. It would
be important to have a starting set of �??�??user independent�??�?? optical potentials that fit the experimental data
to allow the evaluator to consider a large array of possibilities before committing to a particular optical
potential. This work presents a Genetic Algorithm (GA) code that simulates natural selection and evolution,
allowing a �??�??blind search�??�?? of the multiparametric �?2 surface. In this GA, the genes subject to evolution
are the parameters of the optical potential. The GA variables, operators and procedures are described,
and the GA is applied to two cases in which the elastic scattering cross section is adjusted: one for the
7Li + 27Al system at energies close to the Coulomb barrier where the interaction occurs near the nuclear
surface, and another for the 16O + 16O system where the two nuclei deeply interpenetrate each other. Further
developments are described. | |
|
Development of a reference database for Ion Beam Analysis and future perspectives [Abstract] |
D. Abriola, N.P. Barradas, I. Bogdanovi?-Radovi?, M. Chiari, A.F. Gurbich, C. Jeynes, M. Kokkoris, M. Mayer, A.R. Ramos, L. Shi, I. Vickridge, Nucl. Instr. Meth. Phys. Res. B269 (2011) pp. 2972-2978. doi:10.1016/j.nimb.2011.04.056 |
Abstract Ion Beam Analysis (IBA) is a set of material characterization techniques using energetic ion beams. IBA
provides information about composition and the depth profile of elements in the near-surface layers of
a sample, from the energy spectra of backscattered primary particles, recoils, nuclear reaction products
or emitted c-radiation. All IBA methods presuppose knowledge of the differential cross-section data however,
only for strict Rutherford scattering is the cross-section known exactly. In order to address the data
needs of the IBA community, the IAEA initiated the Coordinated Research Project (CRP) �??�??Development of
a Reference Database for Ion Beam Analysis�??�?? in 2005 which will conclude in 2010. The project focuses on
the measurement, assessment, evaluation and benchmarking of elastic scattering and reaction cross sections.
Data measured in this work have been incorporated in the IBANDL database (http://wwwnds.
iaea.org/ibandl/), whereas the evaluated cross-sections (calculated from the fit to the data of a
nuclear model) are made available to the community through the on-line calculator SigmaCalc (http://
www-nds.iaea.org/sigmacalc/).
A summary of the results of the CRP activity is presented, and ways to further develop nuclear data for
IBA are indicated. In particular, a newly proposed CRP devoted to particle induced gamma-ray emission is
described. | |
|
Time-resolved plasma temperature measurements in a laser-triggered hydrogen-filled capillary discharge waveguide [Abstract] |
C.J. Woolley, K. O?Keeffe, H.-K Chung, S.M. Hooker, Plasma Sources Sci. Technol. 20 (2011) 055014. doi:10.1088/0963-0252/20/5/055014 |
Abstract Temporally resolved, spatially integrated measurements of the temperature of the plasma channel formed by a hydrogen-filled discharge capillary waveguide are presented. Plasma temperatures of 4�??7 eV are measured for peak discharge currents between 80 and 150 A. It is demonstrated that laser-triggering the capillary discharge enables capillary discharges with a peak current as low as 23 A to be driven, reducing the plasma temperature to approximately 3 eV. This plasma temperature meets the requirements of a recently proposed soft x-ray recombination laser.
| |
|
Simulations of neon irradiated by intense X-ray laser radiation [Abstract] |
O. Ciricosta, H.-K. Chung, R.W. Lee, J.S. Wark, High Energy Density Physics 7 (2011) pp.111 116. doi:10.1016/j.hedp.2011.02.003 |
Abstract We present simulations of the charge states produced by the interaction of intense X-ray laser radiation
with a neon gas. We model the results of a recent experiment (Young et al., Nature 466, 56 (2010)), where
mJ pulses of X-rays, with photon energies ranging from 800 to 2000 eV and pulse lengths ranging from
70 to 340 fs were incident on neon atoms at intensities of up to 1018 W cm2. Simulations using an
adapted version of the SCFLY collisional-radiative code, which included the effect of electron collisions
and a simple self-consistent temperature model, result in charge state distributions that are in good
agreement with the experimental data. We calculate the electron temperature of the system during the
evolution of the plasma, and comment upon the role that collisions may play in determining the charge
state distributions as a function of the neon ion number density. | |
|
Low and medium energy deuteron-induced reactions on 63,65Cu nuclei [Abstract] |
E. Simeckova, P. Bem, M. Honusek, M. Stefanik, U. Fischer, S.P. Simakov, R.A. Forrest, A.J. Koning, J.-C. Sublet, M. Avrigeanu, F.L. Roman V. Avrigeanu, Phys. Rev. C84 (2011) 014605. doi:10.1103/PhysRevC.84.014605 |
Abstract The activation cross sections of (d,p), (d,2n), (d,3n), and (d,2p) reactions on 63,65Cu were measured in the
energy range from 4 to 20 MeV using the stacked-foil technique. Then, following the available elastic-scattering
data analysis that provided the optical potential for reaction cross-section calculations, an increased effort
was devoted to the breakup mechanism, direct reaction stripping, and pre-equilibrium and compound-nucleus
cross-section calculations, corrected for the breakup and stripping decrease of the total reaction cross section. The
overall agreement between the measured and calculated deuteron activation cross sections proves the correctness
of the nuclear mechanism account, next to the simultaneous analysis of the elastic-scattering and reaction data. | |
|
Shutdown dose rate analyses for the IFMIF HFTM [Abstract] |
A. Serikov, F. Arbeiter, U. Fischer, V. Heinzel, A. Klix, S.P. Simakov, Fusion Eng. Des. 86 (2011) pp. 2639?2642. doi:10.1016/j.fusengdes.2010.11.030 |
Abstract This work contributes to neutronic support activity for the high flux test module (HFTM) designing in the
framework of the IFMIF/EVEDA project. The engineering design of the IFMIF maintenance and remote
handling systems is significantly affected by the radiation doses originating from radioactive materials
generated during operation in the IFMIF HFTM. Two aspects of shutdown doses have been analyses for
the HFTM radioactive materials removed from the IFMIF target and test cell (TTC) and then placed into the
hot cell. First aspect is machine reliability expressed through absorbed gamma dose rate in the envisaged
radiation-sensitive silicon-based electronics located closely to the radioactive HFTM materials. Second
one is radiation protection and safety of a human being presented quantitatively as human biological
dose equivalent rate around the HFTM materials. Shutdown dose rate assessments were performed for
different materials subjected to the radiation by decay photons emitted from the HFTM. Three different
decay radiation sources were considered in the analyses: a simple Eurofer specimen, a single HFTM rig
packed with specimens and an assembly consisting of 12 rigs. The shutdown dose rate has been assessed
taking into account transport of decay gammas by means of subsequent use of three computer codes:
McDeLicious, FISPACT-2007, and MCNP5. | |
|
State-of-the-art of computational tools and data for IFMIF neutronics and activation analyses [Abstract] |
U. Fischer, A. Klix, J. Li, P. Pereslavstev, S.P. Simakov, R.A. Forrest, F. Wasastjerna, J. Nucl. Mats. 417 (2011) pp.1311?1315. doi:10.1016/j.jnucmat.2010.12.266 |
Abstract An overview is presented of the state-of-the-art of computational tools, data and models developed for
neutronics and activation analyses of the IFMIF neutron source. Significant progress has been achieved
in making available computational tools for simulating the d-Li neutron (and photon) source term with
the McDeLicious Monte Carlo code and associated d+6,7Li cross-section data, in generating neutronics
Monte Carlo geometry models by the McCad conversion software, and in providing the interface programme
MCDO to enable coupled 3D Monte Carlo and discrete ordinates shielding calculations. In the
field of nuclear data for IFMIF, a major milestone has been achieved with the launching of the FENDL-
3 research project co-ordinated by the IAEA. Another major achievement is the production of the European
Activation File, version EAF-2007, which has the neutron energy range extended to the needs of
IFMIF and also provides calculated data libraries for deuteron and proton induced activation reactions. | |
|
Impact of activation cross-section uncertainties on the tritium production in the HFTM specimen cells [Abstract] |
O. Cabellos, A. Klix, U. Fischer, N. Garcia-Herranz, J. Sanz, S. Simakov, J. Nucl. Mats. 417 (2011) pp. 1307?1310. doi:10.1016/j.jnucmat.2010.12.269 |
Abstract The prediction of the tritium production is required for handling procedures of samples, safety & maintenance
and licensing of the International Fusion Materials Irradiation Facility (IFMIF). A comparison of
the evaluated tritium production cross-sections with available experimental data from the EXFOR data
base has shown insufficient validation. And significant discrepancies in evaluated cross-section libraries,
including lack of tritium production reactions for some important elements, were found.
Here, we have addressed an uncertainty analysis to draw conclusions on the reliability of the tritium
prediction under the potential impact of activation cross-section uncertainties. We conclude that there
is not sufficient experimental validation of the evaluated tritium production cross-sections, especially
for iron and sodium. Therefore a dedicated experimental validation program for those elements should
be desirable. | |
|
Displacement damage induced in iron by gammas and neutrons under irradiation in the IFMIF test cell [Abstract] |
S.P. Simakov and U. Fischer, J. Nucl. Mat., 417 (2011) pp. 1321?1324. doi:10.1016/j.jnucmat.2010.12.175 |
Abstract This work presents a complete comparative analysis of the radiation damage induced in iron-based
materials in IFMIF by photons and neutrons. The gamma induced damage takes into account, for the first
time, both photonuclear and photoatomic reaction mechanisms. The relevant cross sections were taken
from available data evaluations. The gamma and neutron radiation fields were calculated by the
McDeLicious Monte Carlo code using a 3-D geometry model. Finally the gamma and neutron induced
damages in the iron have been assessed inside the IFMIF test cell and the surrounding concrete walls.
It was found that the photoatomic mechanism dominates the photonuclear with at least one hundred
times higher damage rates. The ratio of the gamma and the neutron induced displacement damage
was found to be 10-3 inside the concrete wall and 10-5 in the components close to d-Li source. This
fraction may increase a few times due to the uncertainty of the evaluated γ-dpa cross sections and the
different surviving probabilities for defects produced by gammas and neutrons, nevertheless unlikely
exceed 1%. | |
|
Modelling d-Be and d-C neutron sources for SPIRAL-2 [Abstract] |
M. Majerle and S.P. Simakov, Procs. Workshop on Nuclear Measurements, Evaluations and Applications - NEMEA-6, 25-28 October 2010, Krakow, Poland, NEA/NSC/DOC(2011)4, (2011) pp. 131-136. |
Abstract SPIRAL-2 facility, which is currently under construction, will produce intense white neutron spectra using deuteron beams (30-40 MeV) bombarding thick Be and C targets. The experimental data describing neutron production and induced radioactivity in these types were studies and data were fitted to phenomenological models to be used in future calculations concerning SPIRAL-2 and similar facilities. | |
|
High energy density matter generation using a focused soft-X-ray laser for volumetric heating of thin foils [Abstract] |
B. Rus, T. Mocek, M. Kozlov�, J. Polan, P. Homer, M. Fajardo, M.E. Foord,*, H. Chung, S.J. Moon, R.W. Lee, J. High Energy Density Physics 7 (2011) pp. 11-16. doi:10.1016/j.hedp.2010.05.001 |
Abstract We report on time-resolved transmission measurements of a 21.2 nm X-ray laser through thin Al and
polyimide foils in the intensity range 1010-1012 Wcm-2. Absolute time-integrated and relative timedependent
transmission measurements indicate significant differences with cold opacity data, due to the
heating, leading to partially ionized states with temperatures of 0.5-20 eV. The transmission data are
compared with simulations that qualitatively reproduce the time-dependent transmission measurements
and demonstrate the importance of including detailed atomic absorption processes in the warm
dense matter regime. | |
|
ADS-related activities at IAEA: From accelerators, neutron sources to fuel cycle and databases [Abstract] |
F. Mulhauser, P. Adelfang, R.M. Capote Noy, V. Inozemtsev, G. Mank, D. Ridikas, A. Stanculescu, A. Zeman, Procs. Workshop on Technology and Components of Accelerator driven Systems, Karlsruhe, Germany, March 2010, Nuclear Science 2011, OECD-NEA, ISBN 978-92-64 11727-3, pp. 307-319. |
Abstract The ADS-related activities at the IAEA address nuclear science and nuclear energy topics, and
are implemented as a joint effort between the Departments of Nuclear Sciences and Applications
and Nuclear Energy. The IAEA is pursuing efforts on utilising accelerators and research reactors
to support the basic and applied research, provide intense neutron sources, characterise and
qualify materials of nuclear interest and concomitantly, train and qualify a highly educated
nuclear workforce. At the back end of the nuclear fuel cycle, environmental concerns linked with
the long half-life radioisotopes generated from nuclear fission have led to increased R&D efforts
to develop a technology aimed at reducing the amount of radioactive waste through
transmutation in either fast fission reactors or ADS. In the framework of the project on
Technology Advances in Fast Reactors and Accelerator-driven Systems, the IAEA has
implemented a number of initiatives on utilisation of plutonium and transmutation of long-lived
radioactive waste, accelerator-driven systems, thorium fuel options, innovative nuclear reactors
and fuel cycles, non-conventional nuclear energy systems, and fusion/fission hybrids. This paper
gives an overview of IAEA�??s accelerator-related activities in nuclear science for materials
development, and partitioning and transmutation of nuclear waste. | |
|
JENDL-4.0: A new library for nuclear science and engineering [Abstract] |
K. Shibata, O. Iwamoto, T. Nakagawa, N. Iwamoto, A. Ichihara, S. Kunieda, S. Chiba, K. Furutaka, N. Otuka, T. Ohsawa, T. Murata, H. Matsunobu, A.Zukeran, So Kamada, J.I Katakura, J. Nucl. Sci. Technol. 48 (2011) pp. 1-30. doi:10.3327/jnst.48.1 |
Abstract The fourth version of the Japanese Evaluated Nuclear Data Library has been produced in cooperation with the Japanese Nuclear Data Committee. In the new library, much emphasis is placed on the improvements of fission product and minor actinoid data. Two nuclear model codes were developed in order to evaluate the cross sections of fission products and minor actinoids. Coupled-channel optical model parameters, which can be applied to wide mass and energy regions, were obtained for nuclear model calculations. Thermal cross sections of actinoids were carefully examined by considering experimental data or by the systematics of neighboring nuclei. Most of the fission cross sections were derived from experimental data. A simultaneous evaluation was performed for the fission cross sections of important uranium and plutonium isotopes above 10 keV. New evaluations were performed for the thirty fission product nuclides that had not been contained in the previous library JENDL-3.3. The data for light elements and structural materials were partly reevaluated. Moreover, covariances were estimated mainly
for actinoids. The new library was released as JENDL-4.0, and the data can be retrieved from the Web site of the JAEA Nuclear Data Center. | |
|
Neutron capture on 94Zr: Resonance parameters and Maxwellian-averaged cross sections [Abstract] |
G. Tagliente, R. Capote, et. al., (the n_TOF collaboration), Phys. Rev. C84 (2011) 015801. doi:10.1103/PhysRevC.84.015801 |
Abstract The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The
s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus
90Zr and through 91,92,93,94Zr, but only part of the flow extends to 96Zr because of the branching point at 95Zr.
Apart from their effect on the s-process flow, the comparably small isotopic (n,γ) cross sections make Zr also an interesting structural material for nuclear reactors. The 94Zr (n,γ) cross section has been measured with high
resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV
neutron energy. | |
|
Neutron-induced fission cross section of natPb and 209Bi from threshold to 1 GeV: An improved parametrization [Abstract] |
D. Tarrio, R. Capote, et. al., (the n_TOF collaboration), Phys. Rev. C83 (2011) 044620. doi:10.1103/PhysRevC.83.044620 |
Abstract Neutron-induced fission cross sections for natPb and 209Bi were measured with a white-spectrum neutron
source at the CERN Neutron Time-of-Flight (n TOF) facility. The experiment, using neutrons from threshold up to
1 GeV, provides the first results for these nuclei above 200 MeV. The cross sections were measured relative to 235U
and 238U in a dedicated fission chamber with parallel plate avalanche counter detectors. Results are compared with
previous experimental data. Upgraded parametrizations of the cross sections are presented, from threshold energy
up to 1 GeV. The proposed new sets of fitting parameters improve former results along the whole energy range. | |
|
197Au(n,?) cross section in the unresolved resonance region [Abstract] |
C. Lederer, R. Capote, et. al., (the n_TOF collaboration), Phys. Rev. C83 (2011) 034608. doi:10.1103/PhysRevC.83.034608 |
Abstract The cross section of the reaction 197Au(n,γ ) was measured with the time-of-flight technique at the n_TOF
(neutron time-of-flight) facility in the unresolved resonance region between 5 and 400 keV using a pair of C6D6
(where D denotes 2H) liquid scintillators for the detection of prompt capture γ rays. The results with a total
uncertainty of 3.9%�??6.7% for a resolution of 20 bins per energy decade show fair agreement with the Evaluated
Nuclear Data File Version B-VII.0 (ENDF/B-VII.0), which contains the standard evaluation. The Maxwellian averaged
cross section (MACS) at 30 keV is in excellent agreement with the one according to the ENDF/B-VII.0
evaluation and 4.7% higher than the MACS measured independently by activation technique. Structures in the
cross section, which had also been reported earlier, have been interpreted as being due to clusters of resonances. | |
|
Towards an improved evaluation of neutron-induced fission cross sections on actinides [Abstract] |
S. Goriely, S. Hilaire, A.J. Koning, R. Capote, Phys. Rev. C83 (2011) 034601. doi:10.1103/PhysRevC.83.034601 |
Abstract Mean-field calculations can now provide all the nuclear ingredients required to describe the fission path
from the equilibrium deformation up to the nuclear scission point. The information obtained from microscopic
mean-field models has been included in the TALYS reaction code to improve the predictions of neutron-induced
fission cross sections. The nuclear inputs concern not only the details of the energy surface along the fission
path, but also the coherent estimate of the nuclear level density derived within the combinatorial approach
on the basis of the same single-particle properties, in particular at the fission saddle points. The predictive
power of such a microscopic approach is tested on the experimental data available for the uranium isotopic
chain. It is also shown that the various inputs can be tuned to reproduce, at best, experimental data in one
unique coherent framework, so that in a close future it should become possible to make, on the basis of such
models, accurate fission-cross-section calculations and the corresponding estimates for nuclei, energy ranges,
or reaction channels for which no data exist. Such model uncertainties are usually not taken into account in
data evaluations. | |
|
Nuclear data evaluation of 55Mn by the EMPIRE code with emphasis on the capture cross-section [Abstract] |
A. Miloccoa, A. Trkov, R. Capote, Nucl. Eng. Design 241 (2011) pp. 1071-1077. doi:10.1016/j.nucengdes.2010.05.045 |
Abstract Manganese is one of the constituents of alloys for structural components of fission and fusion devices
and a well-known neutron dosimeter; however, existing ENDF-B/VII.0 55Mn evaluation was produced by
Shibata (1989). This work is an attempt to re-evaluate neutron-induced cross-sections of 55Mn using the
latest release of the EMPIRE code. Sensitivity studies on the physical and fitting parameters are presented,
with special emphasis on the capture and neutron inelastic cross-sections. A calculated nuclear data
file in ENDF-6 format of the neutron interaction cross-sections is produced. It extends up to 150 MeV,
which is of interest for fusion and accelerator driven system applications. This evaluation is compared
with the ENDF/B-VII.0 evaluation and with a selection of experimental microscopic cross-sections. The
evaluation is tested using integral data: the OKTAVIAN integral experiment on a manganese shell and
an FNG experiment with manganese activation foils. Benchmark results provide needed feedback for the
refinement of the physics parameters. | |
|
Giant dipole resonance parameters with uncertainties from photonuclear cross sections [Abstract] |
V.A. Plujko, R. Capote, O.M. Gorbachenko, Atomic Data and Nuclear Data Tables 97 (2011) pp. 567-585. doi:10.1016/j.adt.2011.04.001 |
Abstract Updated values and corresponding uncertainties of isovector giant dipole resonance (IVGDR or GDR) model parameters are presented that are obtained by the least-squares fitting of theoretical photoabsorption cross sections to experimental data. The theoretical photoabsorption cross section is taken as a sum of the components corresponding to excitation of the GDR and quasideuteron contribution to the experimental photoabsorption cross section. The present compilation covers experimental data as of January 2010. | |
|
Neutron-induced fission cross-section of 233U in the energy range 0.5 < En < 20MeV [Abstract] |
F. Belloni, R. Capote, (the n_TOF Collaboration), Eur. Physical. J. A (2011) p. 47:2. doi:10.1140/epja/i2011-11002-y |
Abstract The neutron-induced fission cross-section of 233U has been measured at the CERN n TOF
facility relative to the standard fission cross-section of 235U between 0.5 and 20MeV. The experiment was
performed with a fast ionization chamber for the detection of the fission fragments and to discriminate
against α-particles from the natural radioactivity of the samples. The high instantaneous flux and the
low background of the n_TOF facility result in data with uncertainties of �?? 3%, which were found in
good agreement with previous experiments. The high quality of the present results allows to improve the
evaluation of the 233U(n,f) cross-section and, consequently, the design of energy systems based on the
Th/U cycle. | |
|
Influence of resonance parameters? correlations on the resonance integral uncertainty; 55Mn case [Abstract] |
G. Žerovnik, A. Trkov, R. Capote, D. Rochman, Nucl. Instr. Meth. Phys. Res. A632 (2011) pp. 137-141. doi:10.1016/j.nima.2010.12.210 |
Abstract For nuclides with a large number of resonances the covariance matrix of resonance parameters can
become very large and expensive to process in terms of the computation time. By converting covariance
matrix of resonance parameters into covariance matrices of background cross-section in a more or less
coarse group structure a considerable amount of computer time and memory can be saved. The
question is how important is the information that is discarded in the process. First, the uncertainty of
the 55Mn resonance integral was estimated in narrow resonance approximation for different levels of
self-shielding using Bondarenko method by random sampling of resonance parameters according to
their covariance matrices from two different 55Mn evaluations: one from Nuclear Research and
Consultancy Group NRG (with large uncertainties but no correlations between resonances), the other
from Oak Ridge National Laboratory (with smaller uncertainties but full covariance matrix). We have
found out that if all (or at least significant part of the) resonance parameters are correlated, the
resonance integral uncertainty greatly depends on the level of self-shielding. Second, it was shown that
the commonly used 640-group SAND-II representation cannot describe the increase of the resonance
integral uncertainty. A much finer energy mesh for the background covariance matrix would have to be
used to take the resonance structure into account explicitly, but then the objective of a more compact
data representation is lost. | |
|
Assessment of the unresolved resonance treatment for cross-section and covariance representation [Abstract] |
L. Leal, G. Nogu�re, C. de Saint John, I. Sirakov, R. Capote, J.-C. Sublet, P. Ribon, M. Coste Delclaux, C. Jouanne, O. Iwamoto, G. Chiba, K. Shibata, R.E. MacFarlane, A.C. Kahler Jr., C.R. Libutz, D. Cullen, M. Herman, (Members of Subgroup 32 ? International Evaluation Cooperation, NEA/OECD), NEA/NSC/WPEC/DOC(2011)430, OECD/NEA 2011. |
Abstract The report was issued by WPEC Subgroup 32, which investigates the methodologies used in the unresolved resonance region (URR) for cross-section and covariance representation. The objectives of the subgroup were to:
- investigate the use of the Single-level Breit-Wigner formalism in the URR for fissile and fertile isotopes;
- investigate URR parameter representation based on the LSSF = 0 or LSSF - 1 option;
- report on teh URR resonance parameter interpolation issue;
- report on the URR covariance representation. | |
|
Covariance data in the fast neutron region [Abstract] |
E. Bauge, R. Capote, U. Fisher, A.Yu. Konobeyev, P.E. Pereslavtsev, M. Herman, P. Oblo?insk�, M.T. Pigni, T. Kawano, P. Talou, I. Kodeli, A. Trkov, A. Koning, D. Rochman, H. Leeb, D. Neudecker, D.L. Smith (Members of Subgroup 24 ? International Evaluation Cooperation, NEA/OECD), NEA/NSC/WPEC/DOC(2010)427, OECD/NEA 2011. |
Abstract The report has been issued by WPEC Subgroup 24, whose
mission was to review methodologies and develop tools for producing
data uncertainties (covariance data) in the fast neutron energy region.
These involve both least-squares procedures and, more recently, stochastic
(Monte Carlo) techniques. Since all modern approaches depend on extensive
usage of nuclear reaction modelling, consideration is given to recent
attempts to determine the extent to which nuclear modelling deficiencies
contribute to the uncertainty of contemporary nuclear data evaluation. | |
|
Measurements and evaluation of differential cross-sections for ion beam analysis [Abstract] |
A.F. Gurbich, D. Abriola, N.P. Barradas, A.R. Ramos, I. Bogdanovic-Radovic, M. Chiari, C. Jeynes, M. Kokkoris, M. Mayer, L. Shi, I. Vickridge. Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 2010-2013. doi:10.3938/jkps.59.2010 |
Abstract Ion beam analysis (IBA) methods always rely on available differential cross-section data to obtain
quantitative results about composition and structure of the near-surface layer of a sample. In order
to meet the nuclear data needs of the IBA community, the Coordinated Research Project (CRP)
"Development of a Reference Database for Ion Beam Analysis" was initiated by the IAEA in 2005
and will be concluded in 2010. A summary of the results of this IAEA Coordinated Research Project
activity is presented, problems still existing in the eld are discussed, and ways to further develop
nuclear data for IBA are indicated. | |
|
Fission cross-section measurements of 233U, 245Cm and 241,243Am at CERN n_TOF facility [Abstract] |
M. Calviani, R. Capote, et al., (the n_TOF collaboration), Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1912-1915. doi:10.3938/jkps.59.1912 |
Abstract Neutron-induced fission cross-sections of minor actinides have been measured using the n_TOF
white neutron source at CERN, Geneva, as part of a large experimental program aiming at collecting
new data relevant for nuclear astrophysics and for the design of advanced reactor systems. The
measurements at n_TOF take advantage of the innovative features of the n_TOF facility, namely the
wide energy range, high instantaneous neutron flux and good energy resolution. Final results on the
fission cross-section of 233U, 245Cm and 243Am from thermal to 20 MeV are here reported, together
with preliminary results for 241Am. The measurement have been performed with a dedicated Fast
Ionization Chamber (FIC), a fission fragment detector with a very high efficiency, relative to the
very well known cross-section of 235U, measured simultaneously with the same detector. | |
|
237Np(n,f) cross section: New data and present status [Abstract] |
C. Paradela, R. Capote, et al., (the n_TOF collaboration), Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1908-1911. doi:10.3938/jkps.59.1908 |
Abstract In this document, we present the final result obtained at the n_TOF experiment for the neutron-
induced fission cross section of the 237Np, from the fission threshold up to 1 GeV. The method
applied to get this result is briefly discussed. n_TOF data are compared to the last experimental
measurements using other TOF facilities or the surrogate method, reported experiments performed
with monoenergetic sources and the FISCAL systematic, including a discussion about the existing
discrepancies. | |
|
High-energy neutron-induced fission cross sections of natural lead and bismuth-209 [Abstract] |
D. Tarr�o, R. Capote, et al., (the n_TOF collaboration), Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1904-1907. doi:10.3938/jkps.59.1904 |
Abstract The CERN Neutron Time-Of-Flight (n_TOF) facility is well suited to measure small neutron-
induced ssion cross sections, as those of subactinides. The cross section ratios of natPb and
209Bi relative to 235U and 238U were measured using PPAC detectors. The fragment coincidence
method allows to unambiguously identify the ssion events. The present experiment provides the
first results for neutron-induced fission up to 1 GeV for natPb and 209Bi. A good agreement with
previous experimental data below 200 MeV is shown. The comparison with proton-induced ssion
indicates that the limiting regime where neutron-induced and proton-induced ssion reach equal
cross section is close to 1 GeV. | |
|
Neutron capture measurements on minor actinides at the n_TOF facility at CERN: Past, present and future [Abstract] |
D. Cano-Ott. R Capote, et al., (the n_TOF collaboration), Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1809-1818. doi:10.3938/jkps.59.1809 |
Abstract The successful development of advanced nuclear systems for sustainable energy production and
nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity stud-
ies and reports [1-3] have identied the need for substantially improving the accuracy of neutron
cross-section data for minor actinides. The n TOF collaboration has initiated an ambitious exper-
imental program for the measurement of neutron capture cross sections of minor actinides. Two
experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC)
[4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set
of two low neutron sensitivity C6D6 detectors for the less radioactive materials. | |
|
The measurement of neutron activation cross section of 59Co below 36 MeV [Abstract] |
E. ?ime?kov�, P. B�m, V. Burjan, U. Fischer, R.A. Forrest, M. G�tz, M. Honusek, V. Kroha, J. Nov�k, S.P. Simakov, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1801-1804. doi:10.3938/jkps.59.1801 |
Abstract An accurate knowledge of the cross section for neutron-induced reactions on 59Co is of importance due to use of cobalt as a structural material in fission and fusion reactors, its applicability in neutron dosimetry and for testing theoretical models as well. The thin Co foils (0.25 mm thickness, 99.9% purity, Goodfellow product) were irradiated in the quasi-momoenergetic p-Li neutron field. For the production of the neutron fields, the proton beam from the NPI energy-variable cyclotron U120M at proton energies 19.8, 25.1, 27.6, 30.1, 32.7, 35.0 and 37.4 MeV and thin 7Li target with carbon stopper were used. The reaction 7Li(p,n) produces the high-energy quasi-monoenergetic neutrons with tail to lower energies. The flux density and neutron spectra were evaluated by MCNPX code using 7Li(p,n) cross section measurement of other authors and including correction to the NPI target layout. The time profile of the neutron source strength during the irradiation was monitored by the proton beam current on the neutron-source target, recorded by a calibrated current-to-frequency converter on a PC. Au foils were used as additional monitors. The foil activity determination was performed by the nuclear spectrometry method employing two calibrated HPGe detectors of 23 and 50% efficiency and of FWHM (Full Width Half Maximum) 1.8 keV at 1.3 MeV for gamma-ray measurement. The reaction rates for 59Co(n,p)59Fe, 59Co(n,α)56Mn, 59Co(n,2nα)54Mn, 59Co(n,3n)57Co, 59Co(n2n)58mCo and 59Co(n,2n)58gCo were obtained. Integral activation cross sections were estimated. The preliminary results are discussed. | |
|
Neutron-induced activation cross sections on hafnium isotopes from the threshold to 20 MeV [Abstract] |
V. Semkova, R. Jaime Tornin, N. Janeva, N. Koyumdjieva, A. Moens, A.J. Plompen, K. Volev, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1737-1740. doi:10.3938/jkps.59.1737 |
Abstract Results of new cross section measurements are presented for the following neutron-induced reactions : 178Hf(n,α)175Yb, 180Hf(n,α)177Yb, 177Hf(n,p)177Lug, 178Hf(n,x)177Lug, 180Hf(n,p)180Lu, 180Hf(n,n'γ)180Hfm, 174Hf(n,2n)173Hf, 176Hf(n,2n)175Hf, and 177Hf(n,3n)175Hf obtained with the activation technique. The irradiations were carried out at the 7-MV Van de Graaff accelerator at IRMM, Geel. Quasi monoenergetic neutrons with energies between 14.8 and 20.5 MeV were produced via the 3H(d,n)4He reaction at Ed = 1, 1.4, 2, 3, and 4 MeV. The 3H(p,n)3He reaction was employed for the production of neutrons in the 2 - 3 MeV energy range. Both natural and enriched samples were used to facilitate correction for interference between reactions leading to the same product. The radioactivity of the samples was determined by standard γ-ray spectrometry using HPGe detector. The current measurements are compared with the data from other authors and Evaluated Nuclear Data Files. Cross sections for three of the studied reactions are reported for the first time. | |
|
Renewed database of GDR parameters for atomic nuclei [Abstract] |
by V.A. Plujko, O.M. Gorbachenko, V.M. Bondar, R. Capote, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1514-1517. doi:10.3938/jkps.59.1514 |
Abstract Updated values of giant dipole resonance parameters with uncertainties are presented which were obtained by a chi-square t of the theoretical photoabsorption cross sections to the experimental data. Renewed systematics for giant dipole resonance parameters are given. Different Lorentzian-type models of dipole strength functions are tested by comparison of the calculations
with experimental data. It is demonstrated that closed-form approaches with asymmetric shape of the gamma strength provide the most reliable simple method for estimation of the γ-decay. | |
|
Study of photon strength function of actinides: The case of 235U, 238Np and 241Pu [Abstract] |
C. Guerrero, R. Capote, et al., (the n_TOF collaboration), Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1510-1513. doi:10.3938/jkps.59.1510 |
Abstract The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular 235U, 238Np and 241Pu. Our study includes the search for resonance structures in the PSF below Sn and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature. | |
|
New IAEA actinide decay data library [Abstract] |
M.A. Kellett, M.-M. B�, V. Chechev, X. Huang, F.G. Kondev, A. Luca, G. Mukherjee, A.L. Nichols, A. Pearce, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1455-1460. doi:10.3938/jkps.59.1455 |
Abstract A recently completed IAEA Coordinated Research Project (CRP) entitled "Updated Decay Data Library for Actinides" has resulted in new and comprehensive evaluations of the decay scheme data for over forty nuclear-power related actinides, along with a further forty radionuclides that arise from their natural decay. A number of data inadequacies remain despite a series of well-defined measurements being undertaken under the auspices of this CRP, which were subsequently incorporated into the relevant evaluations. A list is given of these outstanding measurement requirements as identified from observed shortcomings in the available data. The final data library is available in two standard formats: ENSDF for use in nuclear structure studies, and ENDF for nuclear plant applications including design and operation. Evaluations were undertaken by following the precise methodology of the Decay Data Evaluation Project (DDEP) to ensure that a uniform approach was applied by all participants. The library and associated documentation are available from a dedicated IAEA webpage (http://www-nds.iaea.org/act ddl/). | |
|
Production of long-lived radionuclides 10Be, 14C, 53Mn, 55Fe, 59Ni and 202gPb in a fusion environment [Abstract] |
A. Wallner, K. Buczak, C. Lederer, H. Vonach, T. Faestermann, G. Korschinek, M. Poutivtsev, G. Rugel, A. Klix, K. Seidel, A. Plompen, V. Semkova, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1378 1381. doi:10.3938/jkps.59.1378 |
Abstract In a fusion reactor and also in future advanced reactor types, long-lived activation products may lead to significant long-term waste disposals and radiation damage. Many of these production cross sections are not well-known, making it difficult to calculate concentration limits. Some prominent long-lived activation products comprise 10Be, 14C, and 26Al; in the medium-mass range the radionuclides 53Mn, 55,60Fe, 59,63Ni; and for heavier isotopes 202mPb, 210mBi. Since a few years the
technique of accelerator mass spectrometry (AMS) has been applied at the Vienna Environmental Research Accelerator (VERA) facility for the detection of long-lived radionuclides for such studies. In this respect, samples were irradiated with quasi-monoenergetic neutrons at TU Dresden's 14-MeV neutron generator and the van de Graaff accelerator at IRMM. After the activations the samples were prepared for isotope ratio measurements via AMS. Production of long-lived 53Mn and 59Ni was measured via AMS utilizing the 14-MV tandem of the Maier-Leibnitz- laboratory, TU Munich. Radionuclides 10Be, 14C, 26Al, 55Fe, 210mBi, and 202gPb are measured at the VERA facility. | |
|
Neutron activation experiments on niobium in NPI p-7Li quasi-monoenergetic neutron field [Abstract] |
M. Honusek, P. B�m, V. Burjan, U. Fischer, M. G�tz, V. Kroha, J. Nov�k, S.P. Simakov, E. ?ime?kov�, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1374 1377. doi:10.3938/jkps.59.1374 |
Abstract The work aims to make the study of neutron activation cross section data up to 35 MeV neutron energy using the reaction 7Li(p,n). This reaction produces the high energy quasi-monoenergetic neutrons with the tail to lower energies. The cross-section data for niobium for neutron energies higher than 23 MeV do not exist. These data are needed to develop the dosimetry foil method for neutron spectrometry inside the test cell of IFMIF (International Fusion Material Irradiation Facility) and for the test of nuclear models as well. The reactions (n,2n), (n,3n), (n,4n), (n,3He), (n,α), and (n,α2n) are studied. The corresponding experimental cross sections are calculated. | |
|
The European effort on the evaluation and validation of nuclear data for fusion technology applications [Abstract] |
U. Fischer, P. Batistoni, E. Dupont, R.A. Forrest, H. Henriksson, J. Izquierdo,J.-C. Sublet Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1369-1373. doi:10.3938/jkps.59.1369 |
Abstract An overview is presented of the European Fusion File (EFF) and the European Activation File (EAF) efforts which aim at developing qualified nuclear data bases and validated computational tools for nuclear calculations of fusion systems tailored to the specific needs of the European fusion programme. The related tasks are conducted in the frame of the Fusion for Energy (F4E) work programme and are devoted to the evaluation, processing, testing and benchmarking of required nuclear cross section and uncertainty data, the development of computational tools for sensitivity/uncertainty calculations, and to conduct integral benchmark experiments exploiting also new measurement techniques. The data evaluations are integrated into the Joint Evaluated Fission and Fusion File (JEFF) after having passed a series of qualification tests including their validation
through computational analyses of integral benchmark experiments. | |
|
235U(n,f), 233U(n,f) and 239Pu(n,f) prompt fission neutron spectra [Abstract] |
V.M. Maslov, N.A. Tetereva, V.G. Pronyaev, A.B. Kagalenko, K.I. Zolotarev, R. Capote, T. Granier, B. Morillon, F.-J.Hambsch, J.-C. Sublet, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1337-1342. doi:10.3938/jkps.59.1337 |
Abstract New prompt fission neutron spectra (PFNS) matrices for the n+235U, n+233U, and n+239Pu systems are prepared. Present and previous PFNS shapes are drastically different from each other, the former being consistent with measured data base. A combined generalized least-squares fit of nth+235U, nth+233U, nth+239Pu, and 252Cf(sf) measured data base is accomplished. The solution of the longstanding problem of inconsistency of 235U integral data testing and differential prompt fission neutron spectra data (PFNS) is proposed. Similar problems for the n+233U and n+239Pu are envisaged, revealing arbitrary tweaking of relevant neutron cross sections. Fast 235U integral critical assemblies like Godiva or Flattop benchmarks are reproduced with the same accuracy as with the PFNS of the major data libraries. That reveals a rather delicate compensation effect, tracking the success of the distorted PFNS of the major data libraries to the excessive number of neutrons at energies of 1-3 MeV. Thermal assembly benchmarking reveals positive biases in keff which might be attributed to the influence of a soft energy tail of the present PFNS. For some of Valduc's LCT benchmarks biases in keff are less than 20 pcm. Fast 239Pu integral critical experiments like Jezebel reveal the influence of overestimated inelastic scattering for 239Pu, arbitrarily introduced previously to diminish the influence on the keff of the distortion of the PFNS. | |
|
Exploratory data analysis of the EXFOR database [Abstract] |
E. Dupont, A.J. Koning, N. Otuka, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1333-1337. doi:10.3938/jkps.59.1333 |
Abstract The EXFOR database is a large collection of experimental nuclear reaction data for incident neutrons, charged particles and photons. The EXchange FORmat was designed to be very flexible in order to be able to store the data as published. However, this flexibility is a drawback for systematic comparison of EXFOR data with evaluated data or nuclear reaction code results. The
WPEC Subgroup 30 on "Improvement of Accessibility and Quality of the EXFOR Database" was founded with the aims to establish EXFOR as a more easily accessible and reliable database. In this framework, a directory-structured database was created in simple tabular format. The content of this database was verified with various statistical tests and compared with default results from the TALYS code. This work allowed various problems to be identified, either in the EXFOR translating
codes or in the EXFOR database, and sometimes in the original publications. | |
|
Information management tools for Evaluated Nuclear Structure Data File (ENSDF) interrogation and dissemination [Abstract] |
M. Verpelli, D. Abriola, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1322-1324. doi:10.3938/jkps.59.1322 |
Abstract The evolution of Information Technology has made it possible to provide the Nuclear Data community with various flexible tools customized to respond to individual data queries, to provide visualization, and facilitate dissemination. In another effort to further these developments, the IAEA's Nuclear Data Section has developed a set of applications based on a relational database designed for nuclear structure and decay data. The tools presented in this work mainly use the nuclear structure and decay data obtained from ENSDF and the Nuclear Wallet cards. The present set of applications comprises an interactive Chart of Nuclides (LiveChart) not only presenting the Chart graphically, but also allowing the visualization of data patterns while changing filtering criteria, a web-based query application and a desktop version of the relational database giving support to
expert users to customize their data-processing applications. Some examples of the three software tools are presented. | |
|
Database for time-of-flight spectra including covariances [Abstract] |
N. Otuka, A. Borella, S. Kopecky, C. Lampoudis, P. Schillebeeckx, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1314-1317. doi:10.3938/jkps.59.1314 |
Abstract A data format for time-of-flight spectra (transmission, reaction and self-indication yields) and their covariance matrices based on the AGS (Analysis of Geel Spectra) format is discussed in collaboration between EC-JRC IRMM and IAEA-NDS for the EXFOR library. Experimentalists are encouraged to consider the uncertainty propagation following the AGS principle and submission
of their data to the International Networks Nuclear Reaction Data Centres (NRDC) for EXFOR compilation using a proposed template. | |
|
Nuclear data activities in the International Atomic Energy Agency-Nuclear Data Section (IAEA-NDS) [Abstract] |
R.A. Forrest, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1303-1308. doi:10.3938/jkps.59.1303 |
Abstract As part of its function the IAEA-NDS coordinates and supports nuclear data activities in the fields of neutron and charged-particle reactions and nuclear structure and decay data, and disseminates the resulting reports and databases. The NDS coordinates two international nuclear networks (and one atomic and molecular) - the International Network of Nuclear Reaction Data Centres (NRDC) and the International Network of Nuclear Structure and Decay Data Evaluators (NSDD). The NDS
staff are also involved in several compilations and evaluations of nuclear data. Main activities include compilation for NSR and EXFOR, evaluation for ENSDF and DDEP and evaluation of neutron and charged-particle reaction cross sections and covariances. Most of the NDS support for nuclear data activities is in the form of Coordinated Research Projects and Data Development
Projects; a summary of past, present and future activities is presented. | |
|
The role of the nuclear reaction data centres in experimental nuclear data knowledge sharing [Abstract] |
N. Otuka, S. Dunaeva, E. Dupont, O. Schwerer, A. Blokhin, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1292-1297. doi:10.3938/jkps.59.1292 |
Abstract The International Network of Nuclear Reaction Data Centres (NRDC) consists of 14 data centres from 10 countries and 2 international organisations, and is collaborating for compilation, exchange and dissemination of various types of nuclear reaction data information. The nuclear data centres common data collection, the EXFOR library today contains experimental information and numerical data from more than 18,000 experiments consisting of more than 134,000 data sets mainly of nuclear
reaction data for incident neutrons, charged-particles and photons with incident energy lower than 1 GeV. A brief history and the current status of NRDC collaboration are presented for EXFOR as well as CINDA and ENDF. | |
|
Unified Monte Carlo and mixed probability functions [Abstract] |
R. Capote, D.L. Smith, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010,J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1284-1287. doi:10.3938/jkps.59.1284 |
Abstract The possibility of using the recently suggested Unified Monte Carlo (UMC) technique for the evaluation of nuclear reaction data other than those that are normally distributed is discussed in this paper. The alternative probability distributions examined here are: 1) lognormal distribution; 2) uniform interval distribution; and 3) exponential distribution. These distributions, together with
the normal distribution, are capable of addressing most situations that are likely to be encountered in evaluating nuclear reaction data. The mathematical formalism is described and numerical examples are provided showing instances when the UMC method can lead to results which are quite different from those obtained using the Generalized Least Squares (GLS) method. We conclude that: 1) the GLS method gives reasonable results comparable to UMC for probability functions closely resembling symmetric normal distributions with small to modest uncertainties, but the UMC results are more reliable for broad or strongly asymmetric distributions; 2) the lognormal distribution can be used to good advantage in certain situations involving large uncertainties; 3) use of the uniform and exponential distributions by evaluators should be discouraged. | |
|
Covariance evaluation for actinide nuclear data in JENDL-4 [Abstract] |
O. Iwamoto, T. Nakagawa, S. Chiba, N. Otuka, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1224-1229. doi:10.3938/jkps.59.1224 |
Abstract Covariances of actinide nuclear data stored in JENDL-4.0 have been evaluated based on available experimental data and reaction model calculation. The covariance matrix was basically deduced applying the consistent method with the nuclear data evaluation. For the fast neutron fission cross sections of 6 major actinides of 233,235,238U and 239,240,241Pu were evaluated simultaneously with experimental data of both cross sections and their ratios using the least-squares code SOK, resulting
in giving the covariance matrices that has correlations between the data of different nuclei. For the minor actinide, the least-squares fitting code GMA was used for fission cross section evaluation. The covariances were obtained from the same calculation. For other reaction cross sections, covariances were evaluated using KALMAN code with the sensitivities calculated by CCONE code. Covariances for other data such as resonance parameters and average numbers of fission neutrons were also
evaluated. The evaluated covariance data have been complied to the ENDF-6 format files. The JENDL-4.0 library contains covariance data of (1) average number of neutrons per fission (MF = 31), (2) resonance parameters (MF = 32), (3) cross sections (MF = 33), (4) angular distributions of elastic scattering (MF = 34), and (5) prompt fission spectra (MF = 35) for all 79 actinides. | |
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On the effects of correlations in evaluated nuclear data on the uncertainties in integral parameters [Abstract] |
A. Trkov, I. Kodeli, G. Žerovnik, R. Capote, D.W. Muir, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1213-1217. doi:10.3938/jkps.59.1213 |
Abstract Taking the FNG-W benchmark with a D-T source in front of a large tungsten block as an example, the impact of the reaction cross-section covariance data on the predicted activities of monitor foils inside the block and the associated uncertainties were studied. Cross-material covariances between the isotopic cross sections of tungsten were obtained by including experimental measurements of the elemental total cross sections above the resonance range. Cross-material covariances of the elastic
and the radiative capture reactions were considered. Since the original cross sections were evaluated accurately from the reasonably abundant isotopic data, the impact of introducing elemental data on the isotopic cross sections and their uncertainties were small. Correlations were observed mainly in the elastic channel, which has a relatively low sensitivity to the calculated monitor activities of the benchmark. Consequently, the impact on the predicted monitor sample activities was also
small in terms of the absolute value and the uncertainty. The main achievement of the work was the demonstrated data consistency and the development of tools for including elemental data in isotopic cross section evaluation and the evaluation of cross-material covariances. | |
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Recent progress in neutron-, proton- and deuteron-induced reaction nuclear data for EAF-2010 and the European activation system [Abstract] |
L.W. Packer, J.-C. Sublet, J. Kopecky, R.A. Forrest, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1100-1103. doi:10.3938/jkps.59.1100 |
Abstract The European Activation System (EASY) has been continuously developed and improved for more than 20 years. Its primary purpose is to carry out neutron- proton- and deuteron-induced activation calculations in support of nuclear technology, particularly for nuclear material selection, design and optimization. It comprises the EAF nuclear data libraries and the FISPACT inventory code. For fusion applications, materials used for the construction of ITER, particularly plasma facing components, will be submitted to intense neutron irradiation. These materials may be evaluated using EASY for their nuclide inventory, He gas production and decay heat production over time, for example. EASY includes data to 60 MeV, making it also relevant for IFMIF analysis, and now covers 66,256 reactions. Such large libraries require an extensive validation process, which includes the statistical analysis of cross sections (SACS) and comparisons with differential and integral data. The suite of these methods has now been extended to evaluate the next library release, EAF-2010. Furthermore, significant attention has been focused on improving the uncertainty file, a unique feature of EAF libraries. In this work we discuss recent data improvements to be included
in EAF-2010 and extensions to the treatment of uncertainties both in EAF and within EASY. | |
|
Status of the JEFF nuclear data library [Abstract] |
A.J. Koning, E. Bauge, C.J. Dean, E. Dupont, U. Fischer, R.A. Forrest, R. Jacqmin, H. Leeb, M.A. Kellett, R.W. Mills, C. Nordborg, M. Pescarini, Y. Rugama, P. Rullhusen, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1057-1062. doi:10.3938/jkps.59.1057 |
Abstract The status of the Joint Evaluated Fission and Fusion file (JEFF) is described. Recently, the JEFF-3.1.1 nuclear data library was released and shortly after adopted by the French nuclear power industry for inclusion in their production and analysis codes. Recent updates include actinide evaluations, materials evaluations that have emerged from various European nuclear data projects, the activation library, the decay data and fission yield sub-libraries, and fusion-related data files from the European F4E project. The revisions were motivated by the availability of new measurements, modelling capabilities and trends from integral experiments. Validations have been performed, mainly for criticality, reactivity temperature coefficients, fuel inventory, decay heat and shielding of thermal and fast systems. The next release of the library, JEFF-3.2, will be discussed. This will contain among others a significant increase of covariance data evaluations, modern evaluations for various structural materials, a larger emphasis on minor actinides and addition of high-quality gamma production data for many fission products. | |
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JENDL-4.0: A new library for innovative nuclear energy systems [Abstract] |
K. Shibata, O. Iwamoto, T. Nakagawa, N. Iwamoto, A. Ichihara, S.Kunieda, S. Chiba, J. Katakura, N. Otuka, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1046-1051. doi:10.3938/jkps.59.1046 |
Abstract The fourth version of Japanese Evaluated Nuclear Data Library (JENDL-4.0) has been produced in cooperation with the Japanese Nuclear Data Committee. In the new library, much emphasis is placed on the improvements of fission product and minor actinide data. Achieving this, nuclear model codes were developed. Coupled-channel optical model parameters, which can be applied to
a wide mass range, were obtained for evaluations. Thermal cross sections of many actinides were revised on the basis of experimental data or systematics. Simultaneous evaluation was performed for the fission cross sections of important uranium and plutonium isotopes above 10 keV. The new library JENDL-4.0 is made available on the Web site of the JAEA Nuclear Data Center. | |
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Self-consistent analyses of nuclear level structures, and nucleon interaction data of even-even Sn isotopes [Abstract] |
J.-Y. Lee, E. Sh. Soukhovitski, Y. Kim, R. Capote, S. Chiba, J.M. Quesada, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1019 1022. doi:10.3938/jkps.59.1019 |
Abstract We have analyzed, within a unified approach, nuclear level structure, and nucleon interaction data of the even-even Sn isotopes - 116Sn, 118Sn, and 120Sn - using the soft-rotator nuclear model and an appropriate coupled-channels optical model with a dispersive Lane-consistent optical potential. Determined best-fit optical model potential is capable of simultaneously describing all the experimental nucleon interaction data available up to 200 MeV - total neutron cross sections, proton
reaction cross sections, nucleon elastic and inelastic scattering cross sections, and direct (p,n) charge exchange reaction cross sections. | |
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Fission cross section calculations of actinides with EMPIRE code [Abstract] |
M. Sin, P. Oblo?insk�, M. Herman, R. Capote, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1015-1018. doi:10.3938/jkps.59.1015 |
Abstract Theoretical calculations of neutron induced reactions on 233,234,236U, 237Np, 238-242Pu, 241,243Am, 242-246Cm carried out in the energy range 1 keV - 20 MeV with EMPIRE code are presented, with emphasis on the fission channel. Beside a consistent, accurate set of calculations, the paper contains arguments supporting the choice of the reaction models and input parameters. A special attention is paid to the fission model parameters and their uncertainties. | |
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Towards improved evaluation of neutron-induced fission cross section [Abstract] |
S. Goriely, S. Hilaire, A.J. Koning, R. Capote, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 979-982. doi:10.3938/jkps.59.979 |
Abstract Mean-field calculations can nowadays provide all the nuclear ingredients required to describe the fission path from the equilibrium deformation up to the nuclear scission point. The information obtained from microscopic mean-field models has been included in reaction codes to improve the predictions of neutron-induced fission cross section. The nuclear inputs concern not only the details of the energy surface along the fission path, but also the coherent estimate of the nuclear level density
derived within the combinatorial approach on the basis of the same single-particle properties, in particular at the fission saddle points. The predictive power of such a microscopic approach is tested. It is also shown that the various inputs can be tuned to reproduce at best experimental data in one unique coherent framework, so that it is now possible to make reliable and accurate
fission cross-section calculations on the basis of microscopic models, but also to use such approaches to estimate the corresponding modeling uncertainties for nuclei, energy ranges or reaction channels for which no data exist. | |
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Results from the IAEA benchmark of spallation models [Abstract] |
S. Leray, J.C. David, M. Khandaker, G. Mank, A. Mengoni, N. Otsuka, D. Filges, F. Gallmeier, A. Konobeyev, R. Michel, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 791-796. doi:10.3938/jkps.59.791 |
Abstract Spallation reactions play an important role in a wide domain of applications. In the simulation codes used in this field, the nuclear interaction cross-sections and characteristics are computed by spallation models. The International Atomic Energy Agency (IAEA) has recently organised a benchmark of the spallation models used or that could be used in the future into high-energy transport codes. The objectives were, first, to assess the prediction capabilities of the different spallation models for the different mass and energy regions and the different exit channels and, second, to understand the reason for the success or deficiency of the models. Results of the benchmark concerning both the analysis of the prediction capabilities of the models and the first conclusions on the physics of spallation models are presented. | |
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The role of nuclear data for fusion technology studies [Abstract] |
R.A. Forrest, Procs. Int. Conf. Nuclear Energy for New Europe 2010, 6-9 September 2010, Portoro?, Slovenia, pp. 001.1-001.8, Nucl. Eng. Des. 241 (2011) pp. 4326-4330. doi:10.1016/j.nucengdes.2011.08.033 |
Abstract Nuclear data are of fundamental importance in studies of nuclear technology. In these studies, experiments
to measure cross sections and decay properties and simulations of the design of fission power
plants, fusion devices and accelerators are included. The large amount of data required is stored in computer
readable formats in data libraries and the most common of these are the general purpose files
used for neutronics or transport calculations. These files also contain the standards against which most
measurements are made. The other class of libraries are the special purpose ones containing decay data,
fission yields and cross section data for dosimetry and activation.
This paper gives examples of what data are available and describes their use for various fusion applications.
The focus will be on neutron-induced activation data with examples of how the reactions of
particular importance can be identified. All data should be accompanied by estimates of the uncertainty.
This is best achieved by including covariance data; however, this is extremely challenging and only a
subset of the available data has such uncertainty data. The general principles of how covariance matrices
are used are outlined. | |
|
Experimental data for nuclear resonance fluorescence [Abstract] |
S.P. Simakov, N. Otsuka, V. Semkova, V. Zerkin, S. Hlavac, Procs. 52nd Annual Meeting of the Institute of Nuclear Materials Management (INMM), 17-21 July 2011, Palm Desert, U.S.A. |
Abstract The paper reports on compilation of all published NRF data for actinides in the EXFOR
database. The Entries contain detailed information on experimental set-up and measured
quantities. The survey of compiled data has indicated the relatively large uncertainties and
discrepancies between different experiments even for the most intensive transitions. | |
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Analysis of the dosimetry cross sections measurements up to 35 MeV with
a 7Li(p,xn) quasi-monoenergetic neutron source [Abstract] |
S.P. Simakov, P. B�m, V. Burjan, U. Fischer, R.A. Forrest, M. G�tz, M. Honusek, V. Kroha, J. Novak, E. ?ime?kov�, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1856-1859. doi:10.3938/jkps.59.1856 |
Abstract To improve the status of the dosimetry reaction data above 20 MeV, the activation cross sections on Bi, Au, Co and Nb have been measured at the NPI/�?ež cyclotron facility with a quasi-monoenergetic p-7Li neutron source. The present work comprises the computational analysis of this experiment. It includes the Monte-Carlo simulation of the experimental set-up with the MCNPX
code and relevant cross section data for proton and neutron induced reactions to predict the energy differential neutron flux in the irradiated foils. This approach has been validated against p-Li neutron spectra measured by different techniques. By making use of the modified unfolding code SAND-II, the dosimetry cross sections have been derived from the detected γ-ray activities. This has brought the new experimental results in the neutron energy domain between 18 and 35 MeV with estimated uncertainty at the level of 10%. They were used for validation of the activation (EAF, IEAF, IRDF) and the general purpose (ENDF) cross section files. | |
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On low and medium energy deuteron-induced reactions on 63,65Cu [Abstract] |
E. ?imeckov�, P. P. B�m, M. Honusek, L. Z�vorka, U. Fischer, S.P. Simakov, R.A. Forrest, M. Avrigeanu, V. Avrigeanu, F.L. Roman, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1928-1931. doi:10.3938/jkps.59.1928 |
Abstract The activation cross sections of (d,p), (d,2n), (d,3n), and (d,2p) reactions on 63,65Cu were
measured in the energy range from 4 to 20 MeV using the stacked-foils technique. Errors of present
experimental cross section data are composed of the scale factor (~5%, due to energy and beam
current uncertainty) and datum uncertainty of the foil thickness ~2%) and a mean statistical
error in the determination of specific activities ~3%). Following a previous extended analysis of
elastic-scattering, breakup and direct-reaction of deuterons on light nuclei, for energies from 3 to
60 MeV, the pre-equilibrium and statistical emissions are considered in the same energy range.
Finally, all available deuteron-induced reaction cross sections for 63,65Cu have been involved within
a simultaneous analysis of the deuteron elastic-scattering and reaction data. | |
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Spectral flux of the p-7Li(C) q-m neutron source measured by proton recoil telescope [Abstract] |
J. Nov�k, P. B�m, U. Fischer, M. G�tz, M. Honusek, S.P. Simakov, E. ?imeckov�, M. ?tefa�nik, Proc. Int. Conf. on Nuclear Data for Science and Technology 2010, J. Korean Physical Soc. 59 Vol. 2 (2011) pp. 1577-1580. doi:10.3938/jkps.59.1577 |
Abstract The cyclotron-based fast neutron source at NPI produces mono-energetic neutron fields up to
35 MeV neutron energy using the p+7Li(carbon backing) reactions. To be applied for activation
cross-section measurements, not only the intensity of neutron peak, but also the contribution of
low-energy continuum in the spectra must be well determined. Simulations of the spectral flux
from present source at a position of irradiated samples were performed using CYRIC TOF-data
validated in the present work against LA150h by calculations with the transport Monte Carlo code
MCNPX.
Simulated spectra were tested by absolute measurements using a proton-recoil telescope technique.
The recoil-proton spectrometer consisted of a shielded scattering chamber with polyethylene
and carbon radiators and the �??E1-�??E2-E telescope of silicon-surface detectors located to the neutron
beam axis at 45o in the laboratory system. Si-detectors were handled by usual data acquisition
system. Dead-time - and pulse-overlap losses of events were determined from the count rate of pulse
generator registered during duty cycle of accelerator operation. The proton beam charge and data
were taken in the list mode for later replay and analysis.
The calculations for 7Li(p,n) and 12C(p,n) reactions reasonably reproduce CYRIC TOF neutron
source spectra. The influence of neutron source set-up (proton beam dimensions, 7Li-foil, carbon
stopper, cooling medium, target support/chamber and the geometry-arrangement of irradiated
sample) on the spectral flux is discussed in details. | |
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Nuclear science and data needs for advanced nuclear systems [Abstract] |
R.A. Forrest, Energy Procedia 7 (2011) pp. 540-552. doi:10.1016/j.egypro.2011.06.075 |
Abstract Nuclear data are of fundamental importance in studies of nuclear technology such as the design of fission power plants, fusion devices and accelerators. The large amounts of data required are stored in computer readable formats in data libraries and include the general purpose files used for neutronics calculations. The other class of libraries are special purpose ones containing decay data and cross sections for dosimetry and activation. This paper gives examples of available data and discusses some needs for various applications. The focus is on neutron-induced activation with examples of how the reactions of particular importance can be identified. All data should be accompanied by estimates of uncertainty. The climate of budget cuts worldwide means that the greatest nuclear data need is for resources to continue production of compiled and evaluated data essential for nuclear technology. | |
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Radiation deep penetration calculations for the IFMIF testcell wall [Abstract] |
S.P. Simakov, J. Li, U. Fischer, Fusion Eng. Design 85 (2010) 1924-1927. doi:10.1016/j.fusengdes.2010.06.025 |
Abstract Deep radiation penetration calculations were performed for the IFMIF test cell wall on the basis of two different approaches employing the Monte-Carlo technique and a coupled Monte-Carlo-deterministic computational scheme called MCDO. For the Monte-Carlo calculations, the McDeLicious code was used which is an extension to MCNP-5 with the capability to simulate the d-Li neutron source on the basis of tabulated d-Li cross-section data. Use was made of a three dimensional geometry model of the IFMIF test cell representing in detail its interior and the shielding 3 m thick heavy concrete walls. The interface program MCDO, which couples McDeLicious and the 3D discrete ordinate code TORT, was used to transport the neutrons and photons through the wall and to obtain spatial distributions of the doses in the adjacent rooms. These coupled calculations have revealed hot spots of the radiation doses in the access room neighbouring the test cell in the d-beam downstream direction. The dose rate there exceeds several times the limit of 100 mikro-Sv/h for the work personnel. | |
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Analysis of proton-induced reactions by using simulation [Abstract] |
H. Iwamoto, Y. Iwamoto, Y. Hirata, N. Otuka, K. Niita, JAEA-Conf 2010-005 pp. 81-86. doi:10.11484/jaea-conf-2010-005 |
Abstract Energy spectrum of proton, neutron, composite particles (deuteron, triton, 3He, 4He for p(175 MeV) +
58Ni and p(62.9 MeV) + 208Pb reactions are analyzed by using the Bertini and ISOBAR models
implemented in PHITS and the INC-FRG model. | |
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Development of Web-based user interface for evaluated covariance data files [Abstract] |
T. Togashi, K. Kato, R. Suzuki, N. Otuka, JAEA-Conf. 2010-005, pp. 69-74. doi:dx.doi.org/10.11484/jaea-conf-2010-005 |
Abstract We develop a web-based interface which visualizes cross sections with their covariance compiled in
the ENDF format in order to support evaluated covariance data users who do not have experience of
NJOY calculation. A package of programs has been constructed without aid of any existing program
libraries. | |
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Study of neutron-induced fission cross sections of U, Am, and Cm at n_TOF [Abstract] |
P.M. Milazzo, R. Capote, et al., (the n_TOF Collaboration), Procs. VIII Latin American Symposium on Nuclear Physics and Applications, Eds. R. Alcaron, H.F. Arellano, P.L. Cole, A.J. Kreiner, AIP Conf. Procs. 1265 (2010) pp. 477-482. doi:10.1063/1.3480244 |
Abstract Neutron induced fission cross sections of several isotopes have been measured at the CERN n_TOF spallation neutron facility. Between them some measurements involve isotopes (233U, 241Am, 243Am, 245Cm) relevant for applications to nuclear technologies. The n_TOF facility delivers neutrons with high instantaneous flux and in a wide energy range, from thermal up to 250 MeV. The experimental apparatus consists of an ionization chamber that discriminates fission fragments and α particles coming from natural radioactivity of the samples. All the
measurements were performed referring to the standard cross section of 235U. | |
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Astrophysics at n_TOF facility [Abstract] |
G. Tagliente, R. Capote, et al., (the n_TOF Collaboration), Procs. VIII Latin American Symposium on Nuclear Physics and Applications, Eds. R. Alcaron, H.F. Arellano, P.L. Cole, A.J. Kreiner, AIP Conf. Procs. 1265 (2010) pp. 160-165. doi:10.1088/1742-6596/312/4/042024 |
Abstract The neutron time of flight (n_TOF) facility at CERN is a spallation neutron source with white neutron energy spectrum (from thermal to several GeV), covering the full energy range of interest for nuclear astrophysics, in particular for measurements of the neutron capture cross section required in s-process nucleosynthesis. This contribution presents an overview on the astrophysical program carried on at the n_TOF facility, the main results and their implications. | |
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Elastic Scattering of 7Li + 27Al at Several Angles in the 7 - 11 MeV Energy Range [Abstract] |
D. Abriola, et. al. 19th Int. Conf. on Ion Beam Analysis, 7-11 September 2009, Nucl. Instr. Meth. Phys. Res. B268 (2010) pp. 1793-1796. doi:10.1063/1.3480140 |
Abstract We have measured elastic excitation functions for the 7Li + 27Al system, in an energy range close to its Coulomb barrier (Elab = 8.4 MeV) in steps of 0.25 MeV. For this purpose, an array of eight surface-barrier detectors was used. To get an insight on the background composition (mainly α particles), a telescope-detector was used for atomic-number identification. Identical measurements for the 6Li + 27Al system are planned for the near future. | |
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Radiative recombination rate coefficients for highly-charged tungsten ions [Abstract] |
M.B. Trzhaskovskayaa, V.K. Nikulin, R.E.H. Clark, Atomic Data and Nuclear Data Tables 96 (2010) 1-25. doi:10.1016/j.adt.2009.08.004 |
Abstract Partial and total radiative recombination rate coefficients are presented for highly-charged ions of tungsten with closed shells, W28+, W38+, W46+, W56+, W64+, W70+, and W72+, as well as for the H-like ion W73+ and the bare nucleus W74+. The temperature range 103�??1010K is considered. Calculations have been performed in the framework of the fully relativistic Dirac�??Fock treatment of photoionization and radiative recombination processes taking into account all significant multipoles of the radiation field. We assess the influence of multipole effects on recombination rate coefficients as compared with the commonly used dipole approximation. For the first time, we show that the relativistic Maxwell�??Boltzmann distribution of continuum electrons should be used at high temperature. This decreases the rate coefficient significantly compared to the nonrelativistic distribution. | |
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Measurements of emission spectra from hot, dense germanium plasma in short pulse laser experiments [Abstract] |
D.J. Hoarty, S.F. James, C.R.D. Brown, B.M. Williams, H.-K. Chung, J.W.O. Harris, L. Upcraft, B.J.B. Crowley, C.C. Smith, R.W. Lee, High Energy Density Physics 6 (2010) pp.105-108. doi:10.1016/j.hedp.2009.05.019 |
Abstract Heating of thin foil targets by an high power laser at intensities of 1017�??1019 W/cm2 has been studied as a method for producing high temperature, high density samples to investigate X-ray opacity and equation
of state. The targets were plastic (parylene-N) foils with a microdot made of a mixture of germanium and
titanium buried at depth of 1.5 mm. The L-shell spectra from the germanium and theK-shell spectra from the
titanium were taken using crystal spectrometers recording onto film and an ultra fast X-ray streak camera
coupled to a conical focussing crystal with a time resolution of 1 ps. The conditions in the microdot were
inferred by comparing the measured spectra to synthetic spectra produced by the time-dependent collisional�??
radiative (CR) models FLY and FLYCHK. The data were also compared to simulated spectra from
a number of opacity codes assuming local thermodynamic equilibrium (LTE). Temperature and density
gradients were taken into account in the comparisons. The sample conditions were inferred from the CR
modelling using FLYCHK to be 800 100 eV and 1.5 0.5 g/cc. The best fit to the LTE models was at
a temperature 20% lower than with the CR model. Though the sample departs from LTE significantly useful
spectral comparisons can still be made. The results and comparisons are discussed along with improvements
to the experimental technique to achieve conditions closer to LTE. | |
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ERRORF - A code to calculate covariance of self-shielding factor and its temperature gradient [Abstract] |
N. Otuka, A. Zukeran, H. Takano, G. Chiba, M. Ishikawa, JAEA-Data/Code 2008-012, Japan Atomic Energy Agency, June 2008. doi:10.11484/jaea-data-code-2008-012 |
Abstract A computer code, ERRORF, was developed for calculation of covariance of self-shielding factor and its temperature gradient. This code is based on several modules. With this code, covariance of self-shielding factor and its temperature gradient can be calculated from evaluated nuclear library in the ENDF format. | |
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Covarancies of resonance self-shielding factor and its temperature gradient for uncertainty evaluation of Doppler reactivity [Abstract] |
A. Zukeran, G. Chiba, N. Otuka, M. Ishikawa, H. Takano, JAEA-Research 2008-091, Japan Atomic Energy Agency, February 2009.
doi:10.11484/jaea-research-2008-091 |
Abstract Uncertainty of Doppler reactivity is theoretically formulated and then uncertainties of self-shielding factor and its temperature gradient due to errors of resonance parameters were evaluated from NJOY output. Sensitivity analysis was made for 235U, 238U, 239Pu and 240Pu of JENDL-3.3 based on JFS-3 70 group structure. Resultant sensitivity coefficients are provided for the uncertainty evaluation of Doppler reactivity. | |
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Neutron-induced activation cross sections on hafnium isotopes from the threshold to 20 MeV [Abstract] |
V. Semkova, R. J. Tornin, N. Janeva, N. Koyumdjieva, A. Moens, A.J.M. Plompen, K. Volev, Procs. of Scientific Workshop on Neutron Measurements, Theory and Applications Nuclear Data for Sustainable Nuclear Energy, 28-30 April 2009, Geel, Belgium, Ed. F. J. Hambsch, JRC Scientific and Technical Reports, EUR 23883 EN-2010, pp. 155-159, ISBN 978-92-79-11705-3, ISSN 1018-5593. |
Abstract Here in we report on 174Hf(n,2n)173Hf, 176Hf(n,2n)175Hf, 177Hf(n,3n)175Hf, 177Hf(n,p)177gLu, 178Hf(n,x)177gLu reaction cross section measurements using the activation technique. The irradiations were carried out at the 7-MV Van de Graaff accelerator at IRMM, Geel. Quasi-monoenergetic neutrons with energies between 14.8 and 20.5 MeV were produced via the 3H(d,n)4He reaction at Ed = 1, 1.4, 2, 3, and 4 MeV. Both natural and samples enriched in 177Hf and 178Hf were used to account for the interference between reactions leading to the same product. The radioactivity of the samples was determined by gamma-ray spectrometry using a HPGe detector. The current measurements are compared with the data from other authors and evaluated nuclear data files. Cross sections for three of the studied reactions are reported for the first time. | |
|
Nuclear Data Sheets for A = 72 [Abstract] |
D. Abriola and A.A. Sonzogni, Nuclear Data Sheets 111 (2010) 1-140 doi:10.1016/j.nds.2009.12.001 |
Abstract Experimental data on ground�?? and excited�??state properties for all known nuclei with mass number A=72 have been compiled and evaluated. States populated in radioactive decay, as well as in nuclear reactions, have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties, are given. This work supersedes the 1994 evaluation by W.�??T. Chow and M.M. King (1994Ch45). | |
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Cyclotron production of the 105,106mAg, 100,101Pd, 100,101m,105Rh radionucldies by natPd(p,x) nuclear processes [Abstract] |
M.U. Khandaker, K. Kim, G. Kim, N. Otuka, Nucl. Instr. Meth. Phys. Res. B 268 (2010) pp. 2303-2311. doi:10.1016/j.nimb.2010.04.002 |
Abstract Production cross-sections of the 105g+m,106mAg, 100,101Pd, and 100g+m,101m,105g+mRh radionuclides through
proton-induced reactions on natural palladium were measured up to 40 MeV by using a stacked-foil activation
technique combined with high-resolution c-ray spectrometry. The production cross-sections of
101Pd and 100g+m,105g+mRh radionuclides have been reported here for the first time from the natPd(p,x)
nuclear processes. The present results are compared with the available literature values as well as the
theoretical data calculated by the TALYS and the ALICE-IPPE computer codes. A quantitative comparison
of the present results with the theoretical data has also been done with several deviation factor definitions.
Optimal production pathways of the therapeutic 105gRh radionuclide with minimal contamination
using cyclotrons are discussed elaborately. | |
|
The 235U(n,f) prompt fission neutron spectrum at 100 K input neutron energy |
N. Kornilov, F.-J. Hambsch, I. Fabry, S. Oberstedt, T. Belgya, Z. Kis, L. Szentmiklosi, S. Simakov, Nucl. Sci. Eng. 165 (2010) pp.117-127. |
|
Neutron activation cross sections for zirconium isotopes [Abstract] |
V. Semkova, E. Bauge, A.J.M. Plompen, D.L. Smith, Nucl. Phys. A832 (2010) pp.149 169. doi:10.1016/j.nuclphysa.2009.10.133 |
Abstract New experimental cross sections are presented for 90Zr(n,α)87mSr, 90Zr(n,x)89mY, 90Zr(n,p)90mY, 90Zr(n,2n)89Zr, 90Zr(n,2n)89mZr, 91Zr(n,nα)87mSr, 91Zr(n,x)90mY, 91Zr(n,p)91mY, 92Zr(n,x)91mY, 92Zr(n,p)92Y, 94Zr(n,alpha)91Sr, 94Zr(n,x)93Y and 94Zr(n,p)94Y reactions. These have been obtained with the activation technique using gamma-ray spectrometry and irradiations at the IRMM Van de Graaff laboratory. The new data were obtained in the energy range from 14 to 21 MeV. In nearly all cases this work provides the first data above 15 MeV and for the 92Zr(n,x)91mY and 91Zr(n,nalpha)87mSr reactions no earlier data were reported. The experimental results are compared with model calculations using the TALYS code to obtain a first indication of the impact of the new data on modeling of n +Zr reactions. | |
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High resolution measurements of the 241Am(n,2n) reaction cross section [Abstract] |
C. Sage, V. Semkova, O. Bouland, P. Dessagne, A. Fernandez, F. Gunsing, C. N�stren, G. Nogu�re, H. Ottmar, A.J.M. Plompen, P. Romain, G. Rudolf, J. Somers, F. Wastin, Phys. Rev. C81 (2010) 064604. doi:10.1103/PhysRevC.81.064604 |
Abstract Measurements of the 241Am(n,2n) reaction cross section have been performed at the Joint Research Centre (JRC) Geel in the frame of a collaboration between the European Commission (EC) JRC and French laboratories from CNRS and the Commissariat `a L�??Energie Atomique (CEA) Cadarache. Raw material coming from the Atalante facility of CEA Marcoule has been transformed by JRC Karlsruhe into suitable 241AmO2 samples embedded in Al2O3 matrices specifically designed for these measurements. The irradiations were carried out at the 7-MV Van de Graaff accelerator. The 241Am(n,2n) reaction cross section was determined relative to the 27Al(n,alpha)24Na standard cross section. The measurements were performed in four sessions, using quasi-monoenergetic neutrons with energies ranging from 8 to 21 MeV produced via the 2H(d,n)3He and the 3H(d,n)4He reactions. The induced activity was measured by standard gamma-ray spectrometry using a high-purity germanium detector. Below 15 MeV, the present results are in agreement with data obtained earlier. Above 15 MeV, these measurements allowed the experimental investigation of the 241Am(n,2n) reaction cross section for the first time. The present data are in good agreement with predictions obtained with the TALYS code that uses an optical and fission model developed at CEA. | |
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Neutron physics of the Re/Os clock. I. Measurement of the (n,?) cross sections of 186,187,188Os at the CERN n_TOF facility |
M. Mosconi, A. Mengoni, R. Capote, et al., (the n_TOF Collaboration), Phys. Rev. C 82 (2010) 015802.
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Neutron physics of the Re/Os clock. II. The (n,n') cross section of 187Os at 30 keV neutron energy |
M. Mosconi, M. Heil, F. K?eler, R. Plag. A. Mengoni, Phys. Rev. C 82 (2010) 015803.
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Neutron physics of the Re/Os clock. III. Resonance analyses and stellar (n,gamma) cross sections of 186,187,188Os |
A. Mengoni, R. Capote, et al., (the n_TOF Collaboration), Phys. Rev. C 82 (2010) 015804.
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IFMIF test facilities - 3 years of EVEDA |
F. Arbeiter, U. Fischer, P. Garin, R. Heidinger, V. Heinzel, A. Klix, A. M?ng, St. Simakov, K. Tian, P. Vladimirov, Jahrestagung Kerntechnik (Berlin 2010): INFORUM GmbH (2010) compact 810.
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Comparative study of the tungsten irradiation conditions in IFMIF and DEMO |
S.P. Simakov, P. Pereslavtsev, U. Fischer, A. Moeslang, Jahrestagung Kerntechnik (Berlin 2010): INFORUM GmbH (2010) compact 811.
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Assessment of the tritium production in the HFTM specimen cells of IFMIF |
A. Klix, U. Fischer, S.P. Simakov, IEEE Transactions on Plasma Science 38 (2010) pp. 259 264.
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Measurement of Capture Cross Sections of 90,91,92,94,96Zr Isotopes at n_TOF |
C. Moreau, R. Capote, et al., Proc. Int. Conf. on Nucl. Data for Sci. and Technol. AIP Conference Proceedings 769 (2005) 880. doi:10.1063/1.1945146 |
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Measurements of X- and gamma-ray emission probabilities in the beta- decay of 233Pa |
F.G. Kondev, I. Ahmad, J.P. Greene, M.A. Kellett, A.L. Nichols, Appl. Radiat. Isot. 68 (2010) pp. 2382-2386.
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Nuclear data evaluation methodology including estimates of covariances |
R. Capote, D.L. Smith, A. Trkov, EPJ Web of Conferences 8 (2010) 04001.
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Nuclear reaction data file for astrophysics (NRDF/A) in Hokkaido University Nuclear Reaction Data Center [Abstract] |
K. Kato, M. Kimura, N. Furutachi, T. Togashi, A. Makinaga, N. Otuka, Procs. Tours Symp. Nuclear Physics and Astrophysics - VII, Kobe, Japan, 16-20 November 2009, AIP Conf. Proc. 1238 (2010) pp. 199-204.
doi:10.1063/1.3455928 |
Abstract The activities of the Japan Nuclear Reaction Data Centre is explained. The main task of the centre is data compilation of Japanese nuclear reaction data in collaboration of the International Network of Nuclear Reaction Data Centres. As one of recent activities, preparation of a new database (NRDF/A) and evaluation of astronuclear reaction data are reported. Collaboration in the nuclear data activities among Asian countries is proposed. | |
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High temperature, high density opacity measurements using short pulse lasers |
D.J. Hoarty, S.F. James, C.R.D. Brown, B.M. Williams, T. Guymer, M. Hill, J. Morton, D. Chapman, R. Shepherd, J. Dunn, G. Brown, M. Schneider, P. Beiersdorfer, H. K. Chung, J.W.O. Harris, L .Upcraft, C.C. Smith, R.W. Lee, J. Physics: Conference Series 244 (2010) 012002.
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Depression of reactivity by the collision energy in the single barrier H+CD4 HD+CD3 reaction |
Weiqing Zhang, Yong Zhou, Guorong Wu, Yunpeng Lu, Huilin Pan, Bina Fu, Quan Shuai, Lan Liu, Shu Liu, Liling Zhang, Bo Jiang, Dongxu Dai, Soo-Ying Lee, Zhen Xie, B.J. Braams, J.M. Bowman, M.A. Collins, Dong H. Zhang, Xueming Yang, Procs. Nat. Acad. Sci. 107 29 (2010) pp. 12782-12785.
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Evidence for vinylidene production in the photodissociation of the allyl radical |
Chao Chen, B. Braams, D.Y. Lee, J.M. Bowman, P.L. Houston, D. Stranges, Phys. Chem. Letters 1 12 (2010) pp. 1875-1880.
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Ab-Initio-based potential energy surfaces for complex molecules and molecular complexes |
J.M. Bowman, B.J. Braams, S. Carter, C. Chen, G. Czako, B. Fu, X. Huang, E. Kamarchik, A.R. Sharma, B.C. Shepler, Y. Wang, Z. Xie, Phys. Chem. Letters 1 12 (2010) pp. 1866-1874.
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Shared-proton mode lights up the infrared spectrum of fluxional cations H5+ and D5+ |
T.C. Cheng, B. Bandyopadyay, Yimin Wang, S. Carter, B.J. Braams, J.M. Bowman, M.A. Duncan, Phys. Chem. Letters 1 4 (2010) pp.758-762.
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Global potential energy surfaces for O(3P) + H2O(1A1) collisions |
P.F. Conforti, M. Braunstein, B.J. Braams, J. M. Bowman, Chem. Phys. 133 16 (2010) 164312.
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197Au(n,gamma) cross section in the resonance region |
C. Massimi, R. Capote, A. Mengoni, et al., (the n_TOF Collaboration), Phys. Rev. C81 (2010) 044616.
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The 92Zr(n,gamma) reaction and its implications for stellar nucleosynthesis |
G. Tagliente, R. Capote, A. Mengoni, et al., (the n_TOF Collaboration), Phys. Rev. C81 (2010) 055801.
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Neutron-induced fission cross section of 234U and 237Np measured at the CERN Neutron Time-of-Flight (n_TOF) facility |
C.Paradela, R. Capote, A. Mengoni, et al., (the n_TOF Collaboration), Phys. Rev. C82 (2010) 034601.
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Description of analysing power and (p,n) reaction by a global dispersive coupled-channel optical model potential |
W.L. Sun, L.J. Hao, E.Sh. Soukhovitskii, R. Capote, J.M. Quesada, Nucl. Phys. Trends: The 7th China-Japan Joint Nuclear Physics Symposium, Tsukuba (Japan), 9-13 November 2009, Eds. A. Ozawa, W. Liu, AIP Conf. Procs. 1235, ISBN: 978-0-7354-0780-0.
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Neutron cross-sections for next generation reactors: New data from n_TOF |
N. Colonna, R. Capote, A. Mengoni, et al., (the n_TOF Collaboration), Appl. Radiat. Isot. 68 (2010) pp. 643-646.
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Spectrum of prompt fission neutrons from 235U(n,F) |
V.M. Maslov, N.A. Tetereva, V.G. Pronyaev, A.B. Kagalenko, K.I. Zolotarev, R. Capote, T. Granier, B. Morillon, F.-J. Hambsch, J.-C. Sublet, Atomic Energy 108 6 (2010) pp. 432-443.
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Status of the problem of nuclear cross section data for IBA |
A. Gurbich , I. Bogdanovic-Radovic, M. Chiari , C. Jeynes, M. Kokkoris, O. Schwerer, A.R. Ramos, M. Mayer, E. Rauhala, Shi Liqun, I. Vickridge, J. Nucl. Instrum. Methods Phys. Res. B266 (2008) pp. 1198-1202. |
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Measurements of the Zr-90,91,92,93,94,96(n,γ) cross-sections at n_TOF |
P.M. Milazzo, R. Capote, A. Mengoni,et al., (the n_TOF collaboration), Proc. 2nd Int. Conf., Current Problems in Nuclear Physics and Atomic Energy (NPAE-Kyiv2008), 9-15 June 2009, Kiev, Ukraine, pp.500-503. |
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Permutationally invariant potential energy surfaces in high dimensionality |
B.J. Braams, J.M. Bowman, Int. Reviews in Physical Chemistry 28 (2009) pp. 577-606. |
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Full-dimensional ab initio potential energy surface and vibrational configuration interaction calculations for vinyl |
A.R. Sharma, B.J. Braams, S. Carter, B.C. Shepler, J.M. Bowman, J. Chem. Phys. 130 (2009) 174301. |
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Ab initio modeling of molecular IR spectra of astrophysical interest: application to CH4 |
R. Warmbier, R. Schneider, A.R. Sharma, B.J. Braams, J.M. Bowman, P.H. Hauschildt, J. Astronomy and Astrophysics 495 (2009) pp. 655-661. |
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Ab Initio Calculation of the Photoelectron Spectra of the Hydroxycarbene Diradicals |
L. Koziol, V.A. Mozhayskiy, B.J. Braams, J.M. Bowman, A.I. Krylov, J. Phys. Chem. A113 (2009) pp. 7802-7809. doi:10.1021/jp903476w |
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Applications of NLTE population kinetics |
H.-K. Chung, R.W. Lee, J. High Energy Density Physics 5 (2009) pp. 1-14. |
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X-ray spectroscopy of buried layer foils irradiated at laser intensities in excess of 1020 W/cm2 |
S.N. Chen, P.K. Patel, H.-K. Chung, A.J. Kemp, S. Le Pape, B.R. Maddox, S.C. Wilks, R.B. Stephens, F.N. Beg, J. Phys. Plasmas 16 (2009) 062701. |
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Multi-Code Ab Initio Calculation of Ionization Distributions and Radiation Losses for Tungsten in Tokamak Plasmas |
Yu. Ralchenko, J. Abdallah, Jr., A. Bar-Shalom, J. Bauche, C. Bauche-Arnoult, C. Bowen, H.-K. Chung, J. Colgan, G. Faussurier, C.J. Fontes, M. Foster, F. de Gaufridy de Dortar, I. Golovkin, S.B. Hansen, R.W. Lee, V. Novikov, J. Oreg, O. Peyrusse, M. Poirier, A. Sasaki, H. Scott, H.L. Zhang, AIP Conf. Proc.?Atomic Processes in Plasmas: Procs. of 16th Int. Conf. on Atomic Processes in Plasmas, Ed. K.B. Fournier, 1161 (2009) pp. 242-250, AIP, Melville, New York, ISBN: 978-0-7354-0661-2. |
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Radiative recombination and photoionization cross sections for heavy element impurities in plasmas: II. Ions of Si, Cl, Ar, Ti, Cr, Kr, and Xe |
M.B. Trzhaskovskayaa, V.K. Nikulin, R.E.H. Clark, Atomic Data and Nuclear Data Tables 95 (2009) pp. 987-1050. |
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Development of new standards for exchange of atomic and molecular data |
Yu. Ralchenko, R.E.H. Clark, M.-L. Dubernet, S. Gagarin, D. Humbert, P.A. Loboda, N. Moreau, E. Roueff, D.R. Schultz, AIP Conf. Proc. - ICAMDATA-2008: 6th Int. Conf. on Molecular Data and Their Applications, Eds. Shaoping Zhu, Jun Yan, 1125 (2009) pp. 207-216, AIP, Melville, New York, ISBN: 978-0-7354-0661-2. |
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Atomic, Molecular and Plasma-Surface Interaction Data for Fusion Energy Research |
R.E.H. Clark, D. Humbert, AIP Conf. Proc. - ICAMDATA-2008: 6th Int. Conf. on Molecular Data and Their Applications, Eds. Shaoping Zhu, Jun Yan, 1125 (2009) pp. 197 206, AIP, Melville, New York, ISBN: 978-0-7354-0661-2. |
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Recent advances on hydrogenic retention in ITER's plasma-facing materials: Beryllium, Carbon, and Tungsten |
C.H. Skinner, A.A. Haasz, V.Kh. Alimov, N. Bekris, R.A. Causey, R.E.H. Clark, J.P. Coad, J.W. Davis, R.P. Doerner, M. Mayer, A. Pisarev, J. Roth, T. Tanabe, J. Fusion Science and Technology 54 (2008) pp. 891-945. |
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n_TOF Experiment: Past, Present and Future |
S. Marrone, R. Capote, A. Mengoni, (the n_TOF Collaboration), AIP Conf. Proc. - Nuclear Physics and Applications: 1st Ulaanbaatar Conf. on Nuclear Physics and Applications, Eds. D. Dashdorj, U. Agvaanluvsan, G.E. Mitchell, 1109 (2009) pp. 78-83, AIP, Melville, New York, ISBN: 978-0-7354-0646-9. |
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The n_TOF Total Absorption Calorimeter for neutron capture measurements at CERN |
C. Guerrero. R. Capote, et. al., (the n_TOF Collaboration), J. Nucl. Instr. Meth. Physics Research, Section A:Accelerators, spectrometers, detectors and associated equipment, 608 (2009) pp. 424-433. |
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High-accuracy U-233(n, f) cross-section measurement at the white-neutron source n_TOF from near-thermal to 1 MeV neutron energy |
M. Calviani, R. Capote, et. al., Phys. Rev. C80 (2009) 044064. |
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Evaluation and use of the prompt fission neutron spectrum and spectra covariance matrices in criticality and shielding [Abstract] |
I. Kodeli, A. Trkov, R. Capote, Y. Nagaya, V. Maslov, J. Nucl. Instr. Meth. Physics Research, Section A:Accelerators, spectrometers, detectors and associated equipment 610 (2009) pp. 540-552. doi:10.1016/j.nima.2009.08.076 |
Abstract The prompt fission neutron spectra covariance matrices of 235U, 238U and 239Pu were evaluated using
the Monte Carlo method for two empirical spectra formulations, Watt and Kornilov, and compared to
the existing evaluations such as JENDL-3.3. The fission spectra, together with the covariance matrices
and the methods for the calculation of the corresponding sensitivity profiles were validated on several
applications, including shielding (VENUS-3 benchmark, pressure vessel dosimetry) as well as on fast
and thermal reactor systems (KRITZ and SNEAK critical experiments). A new set of parameters for a
Kornilov model is proposed that improve both benchmark performance and the agreement with
recently measured differential spectra. A recommendation to use constrained sensitivity coefficients
was confirmed for the case of the fission spectrum induced uncertainty in the effective multiplication
factor ðkeff �? and in the detector responses, in order to assure the proper normalisation of the
corresponding covariance matrices. | |
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The determination of beam quality correction factors: Monte Carlo simulations and measurements |
D.M. Gonzalez-Castano, G.H. Hartmann, F, Sanchez-Doblado, F. Gomez, R.P. Kapsch, J. Pena, R. Capote, Physics in Medicine and Biology 54 (2009) pp. 4723-4741. |
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Cross sections of the reaction Pa-231(d,3n)U-230 for the production of U-230/Th-226 for targeted alpha therapy |
A. Morgenstern, O. Lebeda, J. Stursa, R. Capote, M. Sin, F. Bruchertseifer, B. Zielinska, C. Apostolidis, Phys. Rev. C80 (2009) 054612. |
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Nuclear Data Sheets for A = 84 |
D. Abriola, et. al., Nucl. Data Sheets, 110 (2009) pp. 2815-2944. |
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R. Capote Noy, et. al., Nucl. Data Sheets, 110 (2009) pp. 3108-3214. |
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The JEFF-3.1/-3.1.1 Radioactive Decay Data and Fission Yields Sub-libraries |
M.A. Kellett, O. Bersillon, R.W. Mills, OECD Data Bank 2009 - JEFF Report 20, ISBN 978-92-64-99087-6, NEA no. 6287. |
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Current status of Nuclear reaction Data File for Astrophysics (NRDF/A) [Abstract] |
T. Yoshida, N. furutachi, M. Kimura, M. Asano. T. Togashi, H. Murakami, K. Kato, N Otuka, published in proceedings of the 2008 Annual Symposium on Nuclear Data, 20 - 21 November 2008, Ricotti, Tokai, Japan, (JAEA-Conf 2009-004) pp. 79-82. doi:10.11484/jaea-conf-2009-004 |
Abstract Recent activities in JCPRG for compilations of EXFOR and Nuclear Reaction Data File (NRDF)
have been introduced. As an extension of such activities, a preparation of new nuclear data libraries:
Nuclear Reaction Data File for Astrophysics (NRDF/A) has been planned. The framework of the
data table has been almost built. As the next step, evaluations by using cluster models have been
planned. | |
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A Dispersive, Lane-consistent Optical Potential, Coupled-channel Optical Model Code OPTMAN and its Application |
E.Sh. Soukhovitski, S. Chiba, R. Capote, J.M. Quesada, published in proceedings of the 2008 Annual Symposium on Nuclear Data, 20 - 21 November 2008, Ricotti, Tokai, Japan, (JAEA-Conf 2009-004) pp. 51-57. |
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Low and medium energy deuteron-induced reactions on Al-27 [Abstract] |
R. Bem, E. Simeckova, M. Honusek, U. Fischer, S.P. Simakov, R.A. Forrest, M. Avrigeanu, A.C. Obreja, F.L. Roman, V. Avrigeanu, Phys. Rev. C79 (2009) 044610. doi:10.1103/PhysRevC.79.044610 |
Abstract The activation cross sections of (d,p), (d,2p), and (d,p) reactions on 27Al were measured in the energy
range from 4 to 20 MeV using the stacked-foils technique. Following a previous extended analysis of elastic
scattering, breakup, and direct reaction of deuterons on 27Al, for energies from 3 to 60 MeV, the preequilibrium
and statistical emissions are considered in the same energy range. Finally, all deuteron-induced reactions on 27Al
including the present data measured up to 20 MeV deuteron energy are properly described due to a simultaneous
analysis of the elastic scattering and reaction data.
| |
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Deformation-dependent Tamura-Udagawa-Lenske multistep direct model |
H. Wienke, R. Capote, M. Herman, M. Sin, Phys. Rev. C78 (2008) 064611. |
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Towards a prediction of fission cross sections on the basis of microscopic nuclear inputs |
S. Goriely, S. Hilaire, A.J. Koning, M. Sin, R. Capote, Phys. Rev. C79 (2009) 024612. |
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Multipole and relativistic effects in radiative recombination process in hot plasmas |
M.B. Trzhaskovskaya, V.K. Nikulin, R.E.H. Clark, Phys. Rev. E78 (2008) 035401. |
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Radiative Recombination and Photoionization Cross Sections for Heavy Element Impurities in Plasmas |
M.B. Trzhaskovskaya, V.K. Nikulin, R.E.H. Clark, Atomic Data and Nucl. Data Tables 94 (2008) pp.71-139. |
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Nuclear Data Sheets for A=96 |
D. Abriola and A.A. Sonzogni, Nucl. Data Sheets 109 (2008) pp.2501-2655. |
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JENDL Actinoid File 2008 [Abstract] |
O. Iwamoto, T. Nakagawa, N. Otuka, S. Chiba, K. Okumura, G. Chiba, T. Ohsawa, K. Furutaka, J. Nucl. Sci. Technol. 46 (2009) pp. 510-528. doi:10.3327/jnst.46.510 |
Abstract JENDL Actinoid File 2008 (JENDL/AC-2008) was released in March 2008. It includes nuclear data for neutron-induced reactions for 79 nuclides from Ac (Z=89) to Fm (Z=100). The neutron energy range is 10�??5 eV to 20 MeV. Almost all data for 62 actinoids in JENDL-3.3 were revised. New evaluations were performed for 17 nuclides, which have half-lives longer than one day. A new comprehensive theoretical model code CCONE was widely used for the evaluation of cross sections and neutron emission spectra. Thermal cross sections for many nuclides were revised based on experimental data. Resonance parameters were readjusted to reproduce them. Simultaneous evaluations of fission cross sections were performed for six important nuclei. The least-squares fitting code GMA was used for the evaluation of fission cross sections for minor actinoids. In this paper, we present the evaluation methods and results of the JENDL/AC-2008. | |
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Neutron capture cross section of C-14 of astrophysical interest studied by Coulomb breakup of C-15 |
T. Nakamura, N. Fukuda, N. Aoi, N. Imai, M. Ishihara, H. Iwasaki, T. Kobayashi, T. Kubo, A. Mengoni, T. Motobayashi, M. Notani, H. Otsu, H. Sakurai, S. Shimoura, T. Teranishi, Y. X. Watanabe, and K. Yoneda, Phys. Rev. C79 (2009) 035805. |
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JENDL Actinoid File 2008 and Plan of Covariance Evaluation [Abstract] |
O. Iwamoto, T. Nakagawa, N. Otuka, S. Chiba, K. Okumura, Nucl. Data Sheets 109 (2008) pp. 2885-2889. doi:10.1016/j.nds.2008.11.028 |
Abstract JENDL Actinoid File 2008 (JENDL/AC-2008), which is one of JENDL special purpose files, was
released in March 2008. It provides nuclear data for neutron induced nuclear reactions for actinoid
nuclides from Ac (Z=89) to Fm (Z=100). The data for 62 nuclides in JENDL-3.3 were revised and
newly evaluated data were added for 17 nuclides that have a half-life longer than 1 day. The energy
range of incident neutrons is from 10�??5 eV to 20 MeV. The nuclear reaction model code CCONE
was widely used for the evaluation of cross sections and energy-angular distributions of secondary
neutrons in the fast energy region. Covariance data for the fission and capture cross sections and
the number of neutrons per fission will be evaluated for important nuclides in JENDL/AC-2008.
The evaluation methods and the preliminary results of estimated covariances are presented. | |
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The measurement of the Pb-206(n,γ) cross section and stellar implications |
C Domingo-Pardo, R Capote, A Mengoni, et al., J. Phys. G: Nucl. Part. Phys. 35 (2008) 014020. |
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Neutron capture cross section of Zr-90: Bottleneck in the s-process reaction flow |
G. Tagliente, R. Capote, A. Mengoni, et al., Phys. Rev. C77 (2008) 035802. |
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Experimental study of the Zr-91(n,γ) reaction up to 26 keV |
G. Tagliente, R. Capote, A. Mengoni, et al., Phys. Rev. C78 (2008) 045804. |
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Investigation of new reaction cross-section evaluations in order to update and extend the IRDF-2002 reactor dosimetry library |
E.M. Zsolnay, H.J. Nolthenius and A.L. Nichols. Presented at 13th Int. Symp. Reactor Dosimetry, 25-30 May 2008, Akersloot, near Alkmaar, the Netherlands; Reactor Dosimetry State of the Art 2008, Proc. 13th Int. Symp., W. Voorbraak, L. Debarberis, P. D Hondt and J. Wagemans (Eds), World Scientific, Singapore, 2009, ISBN 981-4271-10-1. |
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Nuclear Structure activities at the IAEA-NDS |
D. Abriola, poster presentation at Nuclear Structure Conference 2008, East Lansing, Michigan, USA, 3-6 June 2008. |
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An ENDF-6 compatible evaluation for neutron induced reactions of Th-232 in the unresolved resonance region [Abstract] |
I. Sirakov, R. Capote, F. Gunsing, P. Schillebeeckx and A. Trkov, Annals Nucl. Energy 35 (2008) pp. 1223-1231. doi:10.1016/j.anucene.2007.12.008 |
Abstract An evaluation for neutron induced reactions of 232Th has been performed in the unresolved resonance region from 4 to 100 keV. A
generalized single-level representation compatible with the energy-dependent options of the ENDF-6 format has been used. The average
partial cross sections have been expressed in terms of transmission coefficients by applying the Hauser�??Feschbach statistical reaction
theory including width-fluctuations. The evaluation is based on a combined analysis of experimental average cross section data (including
the most recent capture cross section data obtained at the time-of-flight facilities GELINA and n_TOF), and results of dispersive
coupled-channel optical model calculations. Experimental data on transmission and self-indication measurements as well as integral
benchmark calculations have been used for validation. The evaluation also includes covariance information | |
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A new formalism for reference dosimetry of small and nonstandard fields |
R. Alfonso, P. Andreo, R. Capote, M. Saiful Huq, W. Kilby, P. Kjall, T.R Mackie, H. Palmans, K. Rosser, J. Seuntjens, W. Ullrich and S. Vatnitsky, Med Phys. 35 2008, pp. 5179-5186. |
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Progress in Evaluated Nuclear Data for Tungsten with Covariances [Abstract] |
A. Trkov, R. Capote, I. Kodeli, L. Leal, Proc. PHYSOR 2008: Int. Conf. Physics of Reactors: A Sustainable Resource, Interlaken, Switzerland, 14-19 September 2008, CD-ROM, 2008 (ISBN 978-3-9521409-5-6). |
Abstract New evaluations for the tungsten isotopes 180,182,183,184,186W in the neutron energy range up to 150 MeV were
produced, including the covariance information. Minor adjustments to the existing resonance parameters were
made. Evaluations in the fast energy region were based on nuclear model calculations using the EMPIRE-2.19
code; covariance data were generated with the Monte Carlo technique to produce a prior estimate for the
covariance matrix. Experimental data were introduced through the GANDR system. The evaluated files were
tested on selected fusion neutronics benchmarks and fast reactor benchmarks. Marked improvement in
predicting measured integral parameters was observed, compared to the ENDF/B-VII library | |
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Evaluation of the covariance matrix of the U-235 neutron induced prompt fission spectrum [Abstract] |
I. Kodeli, A. Trkov, R. Capote, Proc. PHYSOR 2008: Int. Conf. Physics of Reactors: A Sustainable Resource, Interlaken, Switzerland, 14-19 September 2008, CD-ROM, 2008 (ISBN 978-3-9521409-5-6). |
Abstract The new Monte Carlo (MC) method has been applied to produce the covariance matrix of the prompt
fission neutron spectra (PFNS) for 235U neutron induced fission. Parameters of the model describing the PFNS
were sampled randomly within the given uncertainty intervals, assuming normal distribution. The covariance
matrix for the Watt spectrum generated by the MC method was validated by comparison with the matrix derived
analytically. Analytical derivation is appropriate in case of linear dependence of the spectra on the underlying
parameters, whereas in the MC approach the extension to more complex models is straightforward: PFNS
covariance matrices were obtained both for the Watt model and for the phenomenological parameterization of
the fission neutron spectra proposed by Kornilov et al. Derived covariance data were used in the cross section
sensitivity and uncertainty analyses of several KRITZ UO2 and MOX critical configurations performed in the
scope of the OECD international benchmark exercise. Two different approaches to calculate the sensitivity
coefficients of keff relative to the fission spectra were used as a means to check and assure the mathematical
correctness of the matrices. | |
|
Decay studies of minor actinide nuclides, and future opportunities for improving the decay data of neutron-rich fission products |
F.G. Kondev, M.A. Kellett, A.L. Nichols, et al., Proc. PHYSOR 2008: Int. Conf. Physics of Reactors: A Sustainable Resource, Interlaken, Switzerland, 14-19 September 2008, CD-ROM, 2008 (ISBN 978-3-9521409-5-6). |
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International efforts to measure, model and evaluate nuclear data for the minor actinides |
A. Mengoni, R. Capote, M.A. Kellett, A.L. Nichols, Proc. PHYSOR 2008: Int. Conf. Physics of Reactors: A Sustainable Resource, Interlaken, Switzerland, 14-19 September 2008, CD-ROM, 2008 (ISBN 978-3-9521409-5-6). |
|
Transmission through multi-humped fission barriers with absorption: A recursive approach |
M. Sin and R. Capote, Phys. Rev. C77 054601 (2008). |
|
Evaluation of Tungsten Nuclear Reaction Data with Covariances [Abstract] |
A. Trkov, R. Capote, I. Kodeli, L. Leal, Nucl. Data Sheets 109 (12) (2008) pp. 2905-2909. |
Abstract As a follow-up of the work presented at the ND-2007 conference in Nice, additional fast reactor benchmarks were analyzed. Adjustment to the cross sections in the keV region was necessary. Evaluated neutron cross section data files for 180,182,183,184,186W isotopes were produced. Covariances were generated for all isotopes except 180W. In the resonance range the retro-active method was used. Above the resolved resonance range the covariance prior was generated by the Monte Carlo technique from nuclear model calculations with the Empire-II code. Experimental data were taken into account through the GANDR system using the generalized least-squares technique. Introducing experimental data results in relatively small changes in the cross sections, but greatly constrains the uncertainties. The covariance files are currently undergoing testing. | |
|
Covariances of Prompt Fission Neutron Spectra [Abstract] |
I. Kodeli, R. Capote and A. Trkov, Nucl. Data Sheets 109 (12) (2008) pp. 2840-2845. |
Abstract Following the outcomes and the recommendations of the Working Party on Evaluation Cooperation
(WPEC) SG-26 the impact of the uncertainties and energy correlations in the prompt neutron
fission spectra (PFNS) was studied in several critical benchmarks, both thermal and fast. Two
different approaches to calculate the sensitivity of keff with respect to the fission neutron spectra,
including the new so-called normalized sensitivity method, were used as a means to check and
assure the mathematical correctness of the derived fission spectrum covariance matrices. A new
Monte Carlo (MC) method has been proposed and applied to produce the covariance matrices of
the PFNS for the neutron induced fission on 235U, 238U and 239Pu nuclei. The MC method was
validated by comparison with the matrix derived analytically using the so-called File-30 formalism
in ENDF terminology. Several sets of covariance matrices of the PFNS of 235U, 238U and 239Pu
nuclei were derived from the uncertainties assigned to the model parameters of the Watt and the
recently proposed Kornilov PFNS parameterizations. | |
|
An Investigation of the Performance of the Unified Monte Carlo Method of Neutron Cross Section Data Evaluation |
R. Capote and D.L. Smith, Nucl. Data Sheets 109 (12) (2008) pp. 2768-2773. |
|
Development of Covariance Capabilities in EMPIRE Code |
M. Herman, M.T. Pigni, P. Obložinský, S.F. Mughabghab, C.M. Mattoon, R. Capote, Young Sik Cho and A. Trkov, Nucl. Data Sheets, 109 (12) (2008) pp. 2752-2761. |
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Measurements of fission cross-sections of actinides at n_TOF |
N. Colonna, A. Mengoni, et al., published in proceedings CANDIDE workshop, 16-18 October 2007, NEMEA-4 Conference: Neutron Measurements, Evaluations and Applications, Nuclear data needs for Generation-IV and accelerator driven systems, pp. 65-70, Ed: A. Plompen, EUR 23235 EN?2008. |
|
Nuclear Data Activities at the International Atomic Energy Agency |
M.A. Kellett, published in book prepared for 50th Anniversary of the Karlsruhe Nuclide Chart, pp. 214-220, European Commission JRC Report, Eds: G. Pfennig, C. Normand, J. Magill, Th. Fanghaenel, EUR 23420 EN - 2008. |
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Production of U-230/Th-226 for Targeted Alpha therapy via Proton Irradiation of Pa-231 |
A. Morgenstern, O. Lebeda, J. Stursa, F. Bruchertseifer, R. Capote, J. McGinley, G. Rasmussen, M. Sin, B. Zielinska and C. Apostolidis, Anal. Chem. 80 (2008) pp. 8763-8770. |
|
Exploring the reactor heat problem: Study of the beta decay of Tc-104,105 using the TAS technique |
A. Algora, J.L. Tain, B. Rubio, A.L. Nichols, et al., Eur. Phys. J. Special Topics 150 (2007) pp. 383-384. |
|
Mass Chain Evaluations for the Evaluated Nuclear Structure Data File (ENSDF) - An Urgent Appeal for European Participation |
F.G. Kondev, A.L. Nichols and J.K. Tuli (invited paper), Nuclear Physics News, Vol. 17 No. 4, 2007, published on behalf of the Nuclear Physics European Collaboration Committee (NuPECC). |
|
Cross-sections of the reactions Th-232(p,3n)Pa-230 for production of U-230 for targeted alpha therapy |
A. Morgenstern, C. Apostolidis, F. Bruchertseifer, R. Capote, T. Gouder, F. Simonelli, M. Sin and K. Abbas, App. Radiat. Isot., 66 (2008) pp. 1275-1280. |
|
Measurement of the stellar cross sections for the reactions Be-9(n,?)Be-10 and C-13(n,?)C-14 via AMS |
A. Wallner, A. Mengoni et al., J. Phys. G: Nucl. Part. Phys 35 (2008) 014018.164. |
|
Maintaining the quality and credibility of a large nuclear database through extended multinational initiatives |
A.L. Nichols, S. Dunaeva, A. Trkov and V. Zerkin, , Proc. 2nd Int. Conf. Current Problems in Nuclear Physics and Atomic Energy (NPAE-Kyiv2008), 9?15 June 2009, Kiev, Ukraine, pp. 28-35. |
|
Towards predictions of neutron-induced fission cross section |
S. Goriely, S. Hilaire, A.J. Koning, M. Sin, R. Capote. Presented at 13th International Symposium on Capture Gamma-ray Spectroscopy and Related Topics (CGS-13), 25 ? 29 August 2008, Cologne, Germany; Proc. 13th Int. Symp. Capture Gamma-ray Spectroscopy and Related Topics, J. Jolie, A. Zilges, N. Warr and A. Blazhev (Eds), AIP Conference Proceedings Vol. 1090 (2009) 621 - 622, American Institute of Physics, Melville, New York, ISBN 978-0-7354-0623-0. |
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Applications of the total absorption technique to reactor decay heat calculations: Study of the beta decay of Tc-102,104,105 |
A. Algora, D. Jordan, J.L. Tain, B. Rubio, J. Agramunt, A.B. Perez-Cerdan, L. Caballero, E. N?cher, A. Krasznahorkay, M.D. Hunyadi, J. Guly?s, A. Vit?z, M. Czatl?s, L. Csige, J. ?yst?, H. Penttil?, S. Rinta-Antila, I. Moore, T. Eronen, A. Jokinen, A. Nieminen, J. Hakala, P. Karvonen, A. Kankainen, U. Hager, T. Sonoda, A. Saastamoinen, J. Rissanen, T. Kessler, C. Weber, J. Ronkainen, S. Rahaman, V. Elomaa, K. Burkard, W. H?ller, L. Batist, W. Gelletly, T. Yoshida, A.L. Nichols, A. Sonzogni and K. Per?j?rvi (invited paper), presented at 13th International Symposium on Capture Gamma-ray Spectroscopy and Related Topics (CGS-13), 25 ? 29 August 2008, Cologne, Germany; Proc. 13th Int. Symp. Capture Gamma-ray Spectroscopy and Related Topics, J. Jolie, A. Zilges, N. Warr and A. Blazhev (Eds), AIP Conference Proceedings Vol. 1090 (2009) pp. 207-214, American Institute of Physics, Melville, New York, ISBN 978-0-7354-0623-0. |
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Studies of Nuclear Structure and Decay Data Properties of Actinide Nuclei |
F.G. Kondev, I. Ahmad, M.P. Carpenter, C. Chiara, J.P. Greene, R.V.F. Janssens, T.L. Khoo, T. Lauritsen, C.J. Lister, E.F. Moore, D. Seweryniak, S. Zhu, S.W. Yates, Z.M. Koening, A.L. Nichols, M.A. Kellett, C.E. Porter and L.K. Felker (invited paper), presented at 13th International Symposium on Capture Gamma-ray Spectroscopy and Related Topics (CGS-13), 25 ? 29 August 2008, Cologne, Germany; Proc. 13th Int. Symp. Capture Gamma-ray Spectroscopy and Related Topics, J. Jolie, A. Zilges, N. Warr and A. Blazhev (Eds), AIP Conference Proceedings Vol. 1090 (2009) pp. 199-206, American Institute of Physics, Melville, New York, USA, ISBN 978-0-7354-0623-0. |
|
Development of JENDL actinoid file [Abstract] |
O. Iwamoto, T. Nakagawa, N. Otuka, S. Chiba, K. Okamura, G. Chiba, Proc. PHYSOR 2008: Int. Conf. Physics of Reactors: A Sustainable Resource, Interlaken, Switzerland, 14-19 September 2008, CD-ROM, 2008 (ISBN 978-3-9521409-5-6). |
Abstract Nuclear data for neutron induced reactions with actinides from Ac to Fm have been evaluated for JENDL Actinoid File (JENDL/AC). Almost all data in JENDL-3.3 have been updated based on available experimental data and using the newly developed theoretical model code CCONE. Integral benchmark tests for fission reactors are in progress using preliminary versions of JENDL/AC. The JENDL/AC will be released in 2008. | |
|
Nuclear physics of the s process |
I. Dillmann, C. Domingo Pardo, F. Kaeppeler, A. Mengoni, K. Sonnabend, Pub. Astro. Soc. of Australia, 25 (2008) pp. 18-29; www.publish.csiro.au/journals/pasa |
|
A global dispersive coupled-channel optical model potential for actinides |
R. Capote, S. Chiba, E.Sh. Soukhovitskii, J.M. Quesada, E. Bauge, J. Nucl. Sci. Technol. 45 (2008) pp. 333-340. |
|
Covariance analyses of self-shielding factor and its temperature gradient for Uranium-238 neutron capture reaction [Abstract] |
N. Otuka, A. Zukeran, H. Takano, G. Chiba, M. Ishikawa, J. Nucl. Sci. Technol. 45 (2008) pp. 195-210. doi:10.3327/jnst.45.195 |
Abstract Covariances of the self-shielding factor and its temperature gradient for the uranium-238 neutron capture reaction have been evaluated from the resonance parameter covariance matrix and the sensitivity of the self-shielding factor and its temperature gradient to the resonance parameters. The resonance parameters and their covariance matrix for uranium-238 were taken from JENDL-3.3, while the sensitivity coefficients were calculated by varying resonance parameters and temperature. A set of computer code modules has been developed for the calculation of the sensitivity coefficients at numerous resonance levels. The present result shows that the correlation among resonance parameters yields a substantial contribution to the standard deviations of the self-shielding factor and its temperature gradient. In addition to the standard deviations of these quantities, their correlation matrices in the JFS-3 70 group structure are also obtained. | |
|
Nuclear physics for the Re/Os clock |
M. Mosconi, R. Capote, A. Mengoni, et al., J. Phys. G: Nucl. Part Phys. 35 (2008) 014015. |
|
Status and outlook of the neutron time-of-flight facility n_TOF at CERN |
F. Gunsing, R. Capote, A. Mengoni, et al., Nucl. Instrum. Methods Phys. Res. B261 (2007) pp. 925-929. |
|
Neutron reactions and nuclear cosmo-chronology |
M. Mosconi, M. Heil, F. Kaeppeler, R. Capote, A. Mengoni, et al., Prog. Part. Nucl. Phys. 59 (2007) pp. 165-173. |
|
The C-14(n,gamma) cross section between 10 keV and 1 MeV |
R. Reifarth, M. Heil, C. Forssen, U. Besserer, A. Couture, S. Dababneh, L. Dorr, J. Gorres, R.C. Haight, F. Kappeler, A. Mengoni, S. O?Brien, N. Patronis, R. Plag, R.S. Rundberg, M. Wiescher, J.B. Wilhelmy, Phys. Rev. C77 (2008) 015804. |
|
The n_TOF facility at CERN |
D. Cano-Ott, R. Capote, A. Mengoni, et al., Proc. 8th Int. Topical Meeting Nucl. Applications and Utilization of Accelerators (ACCAPP '07 2007) pp. 821-826, American Nuclear Society, La Grange Park, USA. |
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Measurement of the radiative neutron capture cross section of Pb-206 and its astrophysical implications |
C. Domingo Pardo, A. Mengoni, et al., (the n_TOF collaboration), Phys. Rev. C76 (2007) 045805. |
|
Measurement of the neutron induced fission cross section on transuranic (TRU) elements at the n_TOF facility at CERN |
A. Mengoni, et al. (n_TOF collaboration), presented at VII Latin American Symposium on Nuclear Physics and Applications, published in AIP 978-0-7354-0461-8/07, Eds: R. Alarcon, P.L. Cole C. Djalali and F. Umeres. |
|
Measurement of La-139(n,γ) cross section at n_TOF |
A. Mengoni, et al. (n_TOF collaboration), pp. 551-553 in AIP conference proceedings, Vol. 831, Eds: by S. V. Harissopulos, P. Demetriou and R. Julin, College Park, American Institute of Physics, 2006. |
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Pulse shape analysis of signals from BaF2 and CeF3 scintillators for neutron capture experiments |
S. Marrone, E. Berthomieux, F. Becvar, D. Cano-Ott, N. Colonna, C. Domingo-Pardo, F. Gunsing, R.C. Haight, M. Heil, F. Kappeler, M. Krticka, P. Mastinu, A. Mengoni, P.M. Milazzo, J. O Donnell, R. Plag, P. Schillebeeckx, G. Tagliente, J.L. Tain, R. Terlizzi and J.L. Ullmann, Nucl. Instrum. Methods Phys. Res. A568 (2006) pp. 904-911. |
|
Measurement of the neutron capture cross section of the s-only isotope Pb-204 from 1 eV to 440 keV |
C. Domingo-Pardo, U. Abbondanno, G. Aerts, et al. (n_TOF collaboration), Phys. Rev. C75 (2007) 015806. |
|
Angular distributions of protons scattered by Ar-40 nuclei with excitation of the 2+(1.46 MeV) and 3-(3.68 MeV) collective levels for incident energies of 25.1, 32.5, and 40.7 MeV |
N.T. Okumusoglu, F. Korkmaz Gorur, E.Sh. Soukhovitski, R. Capote, J.M. Quesada and S. Chiba, Phys. Rev. C75 (2007) 034616. |
|
The La-139(n,?) cross section: Key for the onset of the s-process |
R. Terlizzi, U. Abbondanno, G. Aerts, et al. (n_TOF collaboration), Phys. Rev. C75 (2007) 035807. |
|
Neutron cross section measurements at n_TOF for ADS related studies |
R. Capote, A. Mengoni, et al., J. Phys. 41 (2006) pp. 352-360. |
|
Stellar neutron capture cross section of the unstable s-process branching point Sm-151 |
K. Wisshak, F. Voss, F. Kaeppeler, M. Krticka, S. Raman, A. Mengoni and R. Gallino, Phys. Rev. C73 (2006) 015802. |
|
Resonance capture cross section of Pb-207 |
C. Domingo-Pardo, U. Abbondanno, G. Aerts, et al. (n_TOF collaboration), Phys. Rev. C74 (2006) 055802. |
|
Letter to the editor |
A.L. Nichols, Ann. Nucl. Energy 32 (2005) pp. 1605-1607. |
|
Rare gases transition probabilities for plasma diagnostics |
K. Katsonis, R. E. H. Clark, M. Cornille, A. Siskos and A. Ndiaye, J. Abdallah, pp. 415-418 in AIP conference proceedings, v. 812, Eds: M. J. Sadowski, M. Dudek, H.-J. Hartfuss and E. Pawelec, College Park, American Institute of Physics, 2006. |
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Implications of Sm-151(n,?) cross section at n_TOF |
S. Marrone, A. Mengoni, et al. (n_TOF Collaboration), pp. 502-504 in AIP Conference Proceedings, Vol. 831, Eds: by S. V. Harissopulos, P. Demetriou and R. Julin, College Park, American Institute of Physics (2006), ISBN 0-7354-0323-6. |
|
EMPIRE: Nuclear Reaction Model Code System for Data Evaluation |
M. Herman, R. Capote, B.V. Carlson, P. Obložinský, M. Sin, M. Trkov, H. Wienke and V. Zerkin, Nuclear Data Sheets (2007) 0090-3752. |
|
Approximated lane consistency of the dispersive coupled channel potential for actinides |
J.M. Quesada, R. Capote, E.Sh. Soukhovitskii and S. Chiba; Phys. Rev. C76 (2007) 057602. |
|
Uncertainty estimation in intensity-modulated radiotherapy absolute dosimetry verification |
F. S�nchez-Doblado, G.H. Hartmann, J. Pena, R. Capote, M. Paiusco, B. Rhein, A. Leal and J.I. Lagares, Int. J. Radiation Oncology Biol. Phys. 68 (2007) pp. 301-310. |
|
IAEA Coordinated Research Project: updated decay data library for actinides |
M.A. Kellett, F.G. Kondev and A.L. Nichols, presented at 16th Int. Conf. on Radionuclide Metrology and its Applications (ICRM 2007), 3-7 September 2007, Cape Town, South Africa; also published in Appl. Radiat. Isot. 66 (2008) pp. 694-700. |
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Heavy element and actinide decay data: UKHEDD2.5 |
A.L. Nichols and R.J. Perry, Serco Assurance report SA/NST/18923/W002, Issue 1; UKNSF (2007) p. 213, JEF/DOC-1166, February 2007. |
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Activation product decay data: UKPADD6.7 |
A.L. Nichols and R.J. Perry, Serco Assurance report SA/NST/18923/W001, Issue 1; UKNSF (2007) p. 212, JEF/DOC-1165, February 2007. |
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Recent advances in the JENDL project [Abstract] |
K. Shibata, T. Nakagawa, T. Fukahori, O. Iwamoto, A. Ichihara, N. Iwamoto, S. Kunieda, N. Otuka, J. Katakura, Y. Watanabe, K. Kosako, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 727-732. doi:10.1051/ndata:07743 |
Abstract General- and special-purpose JENDL data files are being produced in cooperation with the Japanese Nuclear Data Committee. Nuclear model codes have been developed in order to raise the reliability of the fourth version of JENDL General-Purpose File (JENDL-4). MA and FP data have been evaluated for JENDL-4. The capture cross section of 235U was examined in the energy region from 2 keV to 1 MeV. As a follow-up action on the previous library JENDL-3.3, covariances of several nuclei were estimated for a study on ADS. The evaluation for the 2007 versions of JENDL High Energy File (JENDL/HE) and JENDL Photonuclear Data File (JENDL/PD), which are regarded as special-purpose files, is in the final stage. Analyses of neutron transmission experiments reveal the reliability of JENDL/HE. | |
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Beta-decay data requirements for reactor decay heat calculations: Study of the possible source of the gamma-ray discrepancy in reactor heat summation calculations |
A. Algora, A.L. Nichols, et al., in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.43-46. |
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Neutron resonance spectroscopy at n_TOF at CERN |
F. Gunsing, R. Capote, A. Mengoni, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.537-542. |
|
IAEA coordinated research programme: Nuclear data for the production of therapeutic radionuclides |
R. Capote, E. Betak, B.V. Carlson, et al., in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.1367-1370. |
|
The U-234 neutron capture cross section measurement at the n_TOF facility |
C. Lampoudis, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.595-598. |
|
Inelastic neutron scattering cross section of Os-187 at 30 keV |
M. Mosconi, M. Heil, F. Kappeler, A. Mengoni, R. Plag, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 1307-1310. |
|
Design study for a new spallation target of the n_TOF facility at CERN |
C. Carrapico, S. Andriamonje, E. Berthoumieux, I. F. Goncalves, F. Gunsing, A. Mengoni, P. Vaz, V. Vlachoudis (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.445-448. |
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New cross section measurements for neutron-induced reactions on Cr, Ni, Cu, Ta and W isotopes obtained with the activation technique |
V. Semkova, R. Capote, R. Jaime Tornin, A.J. Koning, A. Moens, A.J.M. Plompen, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.559-562. |
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Measurement of neutron induced fission of U-235, U-233 and Cm-245 with the FIC detector at the CERN n_TOF facility |
M. Calviani, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.335-338. |
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Measurement of the Zr-90,91,92,93,94,96(n,γ) and La-139(n,γ) cross sections at n_TOF |
G. Tagliente, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp.1303-1306. |
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Neutron-induced fission cross sections measurements at n_TOF |
L. Audouin, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 421-424. |
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Simultaneous measurement of the neutron capture and fission yields of U-233 |
E. Berthoumieux, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 571-574. |
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Measurement of the Au-197 (n,γ) cross section at n_TOF: towards a new standard |
C. Massimi, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 537-542. |
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Capture cross section measurements of Os-186,187,188 at n_TOF. The resolved resonance region |
K. Fujii, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 599-602. |
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The neutron capture cross sections of Np-237(n,γ) and Pu-240(n,γ) and its relevance in the transmutation of nuclear waste |
C. Guerrero, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 627-630. |
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Improved lead and bismuth (n,γ) cross sections and their astrophysical impact |
C. Domingo-Pardo, A. Mengoni, R. Capote, et al. (n_TOF Collaboration), in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 1311-1314. |
|
Extension of the nuclear reaction model code EMPIRE to actinides' nuclear data evaluation |
R. Capote, M. Sin, A. Trkov, M. Herman, B.V. Carlson, P. Obložinský, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 255-258. |
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Lane consistency of the dispersive coupled-channel optical model potential |
R. Capote, E. Soukhovitskii, J.M. Quesada, S. Chiba, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 239-242. |
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Development of IAEA nuclear reaction databases and services |
V. Zerkin, A. Trkov, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 769-772. |
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Experimental studies to improve specific actinide decay data |
F.G. Kondev, M.A. Kellett, I. Ahmad, J.P. Greene, A.L. Nichols, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 93-96. |
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The Global Assessment of Nuclear Data, GANDR |
D.W. Muir, A. Trkov, I. Kodeli, R. Capote, V. Zerkin, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 717-720. |
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Deformation dependent TUL multi-step direct model |
H. Wienke, R. Capote, M. Herman, M. Sin, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 171-174. |
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Evaluation of the Rh-103 neutron cross-section data in the unresolved resonance region for improved criticality safety |
L.C. Mihailescu, I. Sirakov, R. Capote, et al., in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 649-652. |
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EMPIRE ultimate expansion: resonances and covariances |
M. Herman, S.F. Mughabghab, R. Capote, et al., in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 207-210. |
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Neutron-induced fission cross section on actinides using microscopic fission energy surfaces |
M. Sin, R. Capote, S. Goriely, S. Hilaire, A.J. Koning, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 313-316. |
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Evaluation of tungsten isotopes in the fast neutron range including cross section covariance estimation |
R. Capote, A. Trkov, I. Kodeli, E. Soukhovitskii, L.C. Leal, M. Herman, D.W. Muir, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 689-692. |
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The art of collecting experimental data internationally: EXFOR, CINDA and the NRDC network [Abstract] |
H. Henriksson, O. Schwerer, D. Rochman, M.V. Mikhaylyukova, N. Otuka, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 737-740. doi:10.1051/ndata:07290 |
Abstract The world-wide network of nuclear reaction data centres (NRDC) has, for about 40 years, provided data services to the scientific community. This network covers all types of nuclear reaction data, including neutron-induced, charged-particle-induced, and photonuclear data, used in a wide range of applications, such as fission reactors, accelerator driven systems, fusion facilities, nuclear medicine, materials analysis, environmental monitoring, and basic research. The now 13 nuclear data centres included in the NRDC are dividing the efforts of compilation and distribution for particular types of reactions and/or geographic regions all over the world. A central activity of the network is the collection and compilation of experimental nuclear reaction data and the related bibliographic information in the EXFOR and CINDA databases. Many of the individual data centres also distribute other types of nuclear data information, including evaluated data libraries, nuclear structure and decay data, and nuclear data reports. The network today ensures the world-wide transfer of information and coordinated evolution of an important source of nuclear data for current and future nuclear applications. | |
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The JEFF evaluated nuclear data project [Abstract] |
A.J. Koning, R.A. Forrest, M.A. Kellett, A.L. Nichols, et al., in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 721-726. doi:10.1051/ndata:07476 |
Abstract The status of the Joint Evaluated Fission and Fusion file (JEFF) is described. JEFF-3.1 comprises a significant update of actinide evaluations, materials evaluations that have emerged from various European nuclear data projects, the activation library JEFF-3.1/A, the decay data and fission yield sub-libraries, and fusion-related data files from the EFF project. The revisions were motivated by the availability of new measurements, modelling capabilities and trends from integral experiments. Validations have been performed, mainly for criticality, reactivity temperature coefficients, fuel inventory and shielding of thermal and fast systems. Compared with earlier releases, JEFF-3.1 provides improved performance with respect to a variety of scientific and industrial applications. Following on from the public release of JEFF-3.1, the French nuclear power industry has selected this suite of nuclear applications libraries for inclusion in their production codes. | |
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Status and future work of the NEA Working Party on international nuclear data Evaluation Cooperation |
A.J. Koning, J. Katakura, P. Obložinský, A.L. Nichols, C. Nordborg, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 741-746. |
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The aims and activities of the International Network of Nuclear Structure and Decay Data Evaluators |
A.L. Nichols and J.K. Tuli, in Proceedings of the International Conference on Nuclear Data for Science and Technology, April 22-27, 2007, Nice, France, Eds: O.Bersillon, F.Gunsing, E.Bauge, R.Jacqmin, and S.Leray, EDP Sciences, 2008, pp. 37-42. |
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IAEA fusion activities and nuclear data support for innovative concepts |
R.E.H. Clark. A. Malaquias, G. Mank, A.L. Nichols, Fusion Sci. Technol. 51 (2007) pp. 7-10. |
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Measurement of the Pu-240 half-life |
I. Ahmad, F.G. Kondev, J.P. Green, M.A. Kellett and A.L. Nichols, Nucl. Instrum. Methods Phys. Res. A579 (2007) pp. 458-460. |
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Measurement of the half-life of Cm-246 and the ?-decay emission probabilities of Cm-246 and Cf-250 |
F.G. Kondev, I. Ahmad, J.P. Greene, M.A. Kellett and A.L. Nichols, Appl. Radiat. Isot. 65 (2007) pp. 335-340. |
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Atomic and nuclear data services of the International Atomic Energy Agency |
A.L. Nichols, O. Schwerer and S. Dunaeva, presented to 56th Int. Conf. "Nucleus 2006", 4-8 September 2006, Sarov, Russia (also to be published in proceedings). |
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Uncertainty estimation in intensity-modulated radiotherapy absolute dosimetry verification |
F. Sánchez-Doblado, G.H. Hartmann, J. Pena, R. Capote, M. Paiusco. B. Rhein, A. Leal and J.I. Lagares, Int. J. Radiation Oncology Biol. Phys. 68 (2007) pp. 301-310. |
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Measurement of La-139(n,?) Cross Section |
R. Terlizzi, R. Capote, A. Mengoni, et al., presented at 12th Int. Symposium on Capture Gamma-Ray Spectroscopy and Related Topics, 4-9 September 2005, University of Notre Dame, USA, also published in AIP 819, Eds: A. Woehr and A. Aprahamian (2006) pp. 283-287. |
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Measurement of the resonance capture cross section of Pb-204,206 and termination of the s -process |
C. Domingo-Pardo, R. Capote, A. Mengoni, et al., presented at 12th Int. Symposium on Capture Gamma-Ray Spectroscopy and Related Topics, 4-9 September 2005, University of Notre Dame, USA, also published in AIP 819, Eds: A. Woehr and A. Aprahamian (2006) pp. 288-292. |
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Neutron Capture Cross Section Measurements at n_TOF of Np-237, Pu-240 and Am-243 for the Transmutation of Nuclear Waste |
D. Cano-Ott, R. Capote, A. Mengoni, et al., presented at 12th Int. Symposium on Capture Gamma-Ray Spectroscopy and Related Topics, 4-9 September 2005, University of Notre Dame, USA, also published in AIP 819, Eds: A. Woehr and A. Aprahamian (2006) pp. 318-322. |
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Monte Carlo correction factors for a Farmer 0.6 cm³ ion chamber dose measurement in the build-up region of the 6MV clinical beam |
J. Pena, F. Sánchez-Doblado, R. Capote, J.A. Terrón and F. Gómez, Phys. Med. Biol. 51 (2006) pp. 1523-1532. |
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Measurement of the Sm-151(n,?) cross section from 0.6 eV to 1 MeV via the neutron time-of-flight technique at the CERN n_Tof facility |
S. Marrone, R. Capote, A. Mengoni, et al.,Phys. Rev. C73 (2006) 034604:1-18. |
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Neutron capture cross section of Th-232 measured at the n_TOF facility at CERN in the unresolved resonance region up to 1 MeV |
G. Aerts, R. Capote, A. Mengoni, et al., Phys. Rev. C73 (2006) 054610:1 10. |
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Fission of light actinides: Th-232(n,f) and Pa-231(n,f) reactions |
M. Sin, R. Capote, A. Ventura, M. Herman and P. Obložinský, Phys. Rev. C74 (2006) 014608 pp. 1-13. |
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New measurement of neutron capture resonances in Bi-209 |
C. Domingo-Pardo, R. Capote, A. Mengoni, et al., Phys. Rev. C74 (2006) 025807:1-10. |
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Isospin dependent dispersive coupled channel optical model potential for actinides |
R. Capote, E.Sh. Soukhovitski, J.M. Quesada and S. Chiba, presented at Workshop on Nuclear Data for the Next Decade, 26-28 September 2005, CEA-DIF Bruyeres-le-Châtel, France; also published in NEA Workshop Proc. - Perspectives on Nuclear Data for the Next Decade, Ed.: E. Bauge (2006) pp. 43-55. |
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International Atomic Energy Agency: Dedicated nuclear databases |
A.L. Nichols, presented at a plenary session on ‘Advances in Nuclear Data Libraries’, PHYSOR-2006, ANS Topical Meeting on Advances in Nuclear Analysis and Simulation, 10-14 September 2006, Vancouver, British Columbia, Canada, also published in proceedings PHYSOR-2006, ANS, Inc. topical Meeting on Reactor Physics, ISBN: 0-89448-697-7. |
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Measurement of the Neutron Capture Cross Section of U-236 |
F. Gunsing, R. Capote, A. Mengoni, et al., presented at PHYSOR-2006, ANS Topical Meeting on "Advances in Nuclear Analysis and Simulation", 10-14 September 2006, Vancouver, British Columbia, Canada, also published in proceedings PHYSOR-2006, ANS, Inc. Topical Meeting on Reactor Physics, ISBN: 0-89448-697-7. |
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Measurement at n_TOF of the Np-237(n,γ) and Pu-240(n,γ) Cross Sections for the Transmutation of Nuclear Waste |
A. Guerrero, R. Capote, A. Mengoni, et al. presented at PHYSOR-2006, ANS Topical Meeting on "Advances in Nuclear Analysis and Simulation", 10-14 September 2006, Vancouver, British Columbia, Canada, also published in proceedings PHYSOR-2006, ANS, Inc. Topical Meeting on Reactor Physics, ISBN: 0-89448-697-7. |
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Measurement of the Neutron Capture Cross Section of U-234 in n_TOF at CERN |
W. Dridi, R. Capote, A. Mengoni, et al. presented at PHYSOR-2006, ANS Topical Meeting on "Advances in Nuclear Analysis and Simulation", 10-14 September 2006, Vancouver, British Columbia, Canada, also published in proceedings PHYSOR-2006, ANS, Inc. Topical Meeting on Reactor Physics, ISBN: 0-89448-697-7. |
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n_TOF fission data of interest to GEN-IV and ADS |
C. Paradela, R. Capote, A. Mengoni, et al. presented at PHYSOR-2006, ANS Topical Meeting on "Advances in Nuclear Analysis and Simulation", 10-14 September 2006, Vancouver, British Columbia, Canada, also published in proceedings PHYSOR-2006, ANS, Inc. Topical Meeting on Reactor Physics, ISBN: 0-89448-697-7. |
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Validation of Th-232 Evaluated Nuclear Data Through Benchmark Experiments [Abstract] |
A. Trkov and R. Capote presented at Nuclear Energy for New Europe, 18-21 September 2006, Portoro?,Slovenia, also published in proceedings of the Int. Conf. Nuclear Energy for New Europe, 2006, pp. 110.1-110.7. |
Abstract Evaluated nuclear data files for nuclides of the thorium-uranium cycle were released as a result of a coordinated research project of the International Atomic Energy Agency. To validate the data a series of benchmark test cases were analysed, with emphasis on the most important nuclides 232Th and 233U. Remaining nuclides appearing in the benchmarks were taken from the ENDF/B-VII beta-2 library, except for a few sensitivity studies where the data were taken from other sources. The results show marked improvement in the agreement with measurements, much of it coming from the new evaluations | |
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Evaluation of neutron cross section data in the unresolved resonance region with a link to the optical model |
I. Sirakov, P. Schillebeeckx and R. Capote, presented to Wonder2006 – Workshop on Nuclear Data Evaluation for Reactor Applications, 9-11 October 2006, Chateau de Cadarache, Saint-Paul-lez-Durance, France (also to be published in proceedings). |
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Highlights from the coordinated research project on the thorium-uranium fuel cycle |
A. Trkov and R. Capote, 3rd Workshop on Neutron Measurements, Evaluations and Applications, NEMEA-3, 25-28 October 2006, Borovets, Bulgaria, EUR22794EN(2006), pp. 43-48. Ed: A.J.M. Plompen, Luxembourg, ISBN 978-92-79-06158-5. |
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Modelling of nuclear data in the fast neutron region |
R. Capote, M. Sin and A. Trkov, 3rd Workshop on Neutron Measurements, Evaluations and Applications, NEMEA-3, 25-28 October 2006, Borovets, Bulgaria, EUR22794EN(2006), pp. 13-18. Ed: A.J.M. Plompen, Luxembourg, ISBN 978-92-79-06158-5. |
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Achievements of and perspectives for the n_TOF facility at CERN |
A. Mengoni,3rd Workshop on Neutron Measurements, Evaluations and Applications, NEMEA-3, 25-28 October 2006, Borovets, Bulgaria, EUR22794EN(2006), Ed: A.J.M. Plompen, Luxembourg, ISBN 978-92-79-06158-5. |
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International Efforts to Improve Atomic and Nuclear Databases for Energy and Non-Energy Applications |
A.L. Nichols (invited paper), presented at the BARC Golden Jubilee DAE-BRNS National Workshop on Nuclear Data for Advanced Nuclear Systems, 8-11 November 2006, Mangalore, India, also published in Current Science 93 (2007) pp. 26-34. |
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IAEA Co-ordinated Research Project: Update of X-ray and gamma-ray decay data standards for detector calibration and other applications |
A.L. Nichols, presented at 14th Int. Conf. on Radionuclide Metrology and its Applications (ICRM 2003), 2-6 June 2003, Dublin, Ireland; also published in Appl. Radiat. Isot.60 (2004) pp. 247-256. |
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IAEA Nuclear Data Section: Provision of atomic and nuclear databases for user applications |
D.P. Humbert, A.L. Nichols and O. Schwerer, presented at 14 th Int. Conf. on Radionuclide Metrology and its Applications (ICRM 2003), 2-6 June 2003, Dublin, Ireland; also published in Appl. Radiat. Isot.60 (2004) pp. 311-316. |
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Table of radionuclides, Vol. 1 – A = 1 to 150 |
M.-M. Bé, V. Chisté, C. Dulieu, E. Browne, V. Chechev, N. Kuzmanko, R. Helmer, A. Nichols, E. Schönfeld and R. Dersch, Monographie BIPM-5 (2004) Bureau International des Poids et Mesures. |
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Table of radionuclides, Vol. 2 – A = 151 to 242 |
M.-M. Bé, V. Chisté, C. Dulieu, E. Browne, V. Chechev, N. Kuzmanko, R. Helmer, A. Nichols, E. Schönfeld and R. Dersch, Monographie BIPM-5 (2004) Bureau International des Poids et Mesures. |
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Microionization chamber for reference dosimetry in IMRT verification: clinical implications on OAR dosimetric errors |
F. Sánchez-Doblado, R. Capote, A. Leal, J.V. Roselló, J.I. Lagares, R. Arráns and G.H. Hartmann, presented at Advanced Workshop on Current Topics in Monte Carlo Treatment Planning, 3-5 May 2004, McGill University, Medical Physics Unit, Montréal, Québec, Canada; published in Phys. Med. Biol. 50 (2005) pp. 959-970. |
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An EGSnrc photon cross section sensitivity study in low energy photon transport |
R. Capote, R. Linares and F. Sánchez-Doblado, presented at Advanced Workshop on Current Topics in Monte Carlo Treatment Planning, 3-5 May 2004, McGill University, Medical Physics Unit, Montréal, Québec, Canada. |
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On the thermal scattering law data for reactor lattice calculations [Abstract] |
A. Trkov and M. Mattes, Eds.: I. Jencic and M. Tkavc, Proc. Int. Conf. Nuclear Energy for New Europe 2004, Portoro?, Slovenia, 6-9 September 2004, pp. 201.1-201.8, Nuclear Society of Slovenia (2004). |
Abstract Thermal scattering law data for hydrogen bound in water, hydrogen bound in zirconium
hydride and deuterium bound in heavy water have been re-evaluated. The influence of the
thermal scattering law data on critical lattices has been studied with detailed Monte Carlo
calculations and a summary of results is presented for a numerical benchmark and for the
TRIGA reactor benchmark. Systematics for a large sequence of benchmarks analysed with the
WIMS-D lattice code are also presented. | |
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Nuclear Reaction Data Centre Network: A success story |
O. Schwerer, V. McLane, H. Henriksson and S. Maev, presented at International Conference on Nuclear Data for Science and Technology, 27 September - 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 83-86, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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NEA Working Party on International Nuclear Data Cooperation – Recent achievements and plans |
P. Obložinský, J. Katakura, A.J. Koning, A.L. Nichols and C. Nordborg, presented at International Conference on Nuclear Data for Science and Technology, 27 September – 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 128-131, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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Nuclear decay data: On-going studies to address and improve radionuclide decay characteristics |
A.L. Nichols (invited paper), presented at International Conference on Nuclear Data for Science and Technology, 27 September – 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 242-251, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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Neutron cross-section evaluations for Ge-70,72,73,74,76 [Abstract] |
O. Iwamoto, M. Herman, S.F. Mughabghab, P. Oblo?insk� and A. Trkov, presented at International Conference on Nuclear Data for Science and Technology, 27 September ? 1 October 2004, Santa F�, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 434-437, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
Abstract Entirely new evaluations have been performed for neutrons on all isotopes of Ge, from a thermal energy up to
20 MeV, with a focus on photon production. The resonance parameters were considerably improved compared to earlier
evaluations. The fast-neutron region has been evaluated using the EMPIRE-2.19 code. The results were validated against
photon data on Fe and Nb. Isotopic evaluations for Ge were summed up and compared with available measurements on natural
Ge. Various quantities related to photon production, showing strong dependence on neutron incident energy, are discussed | |
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Review of neutron cross-section evaluations for fission products |
P. Obložinský, M. Herman, S. Mughabghab, I. Sirakov, J. Chang, T. Nakagawa, K. Shibata, M. Kawai, A. V. Ignatyuk, V. G. Pronyaev, V. Zerkin, S. Qingbiao and Z. Youxiang, presented at International Conference on Nuclear Data for Science and Technology, 27 September - 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 438-441, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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SIGACE code for generating high-temperature ACE files; validation and benchmarking [Abstract] |
A.R. Sharma, S. Ganesan and A. Trkov, presented at International Conference on Nuclear Data for Science and Technology, 27 September ? 1�October 2004, Santa F�, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P.�Talou, Vol. 769, Part 1 (2005) pp.�499-502, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
Abstract A code named SIGACE has been developed as a tool for MCNP users within the scope of a research contract
awarded by the Nuclear Data Section of the International Atomic Energy Agency (IAEA) (Ref: 302-F4-IND-11566 B5-
IND-29641). A new recipe has been evolved for generating high-temperature ACE files for use with the MCNP code.
Under this scheme the low-temperature ACE file is first converted to an ENDF formatted file using the ACELST code
and then Doppler broadened, essentially limited to the data in the resolved resonance region, to any desired higher
temperature using SIGMA1. The SIGACE code then generates a high-temperature ACE file for use with the MCNP
code. A thinning routine has also been introduced in the SIGACE code for reducing the size of the ACE files. The
SIGACE code and the recipe for generating ACE files at higher temperatures has been applied to the SEFOR fast reactor
benchmark problem (sodium-cooled fast reactor benchmark described in ENDF-202/BNL-19302, 1974 document). The
calculated Doppler coefficient is in good agreement with the experimental value. A similar calculation using ACE files
generated directly with the NJOY system also agrees with our SIGACE computed results. The SIGACE code and the
recipe is further applied to study the numerical benchmark configuration of selected idealized PWR pin cell
configurations with five different fuel enrichments as reported by Mosteller and Eisenhart. The SIGACE code that has
been tested with several FENDL/MC files will be available, free of cost, upon request, from the Nuclear Data Section of
the IAEA | |
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Data dissemination and international collaboration |
T. Fukahori, A.V. Ignatyuk, F.G. Kondev, K.-L. Kratz, V. McLane, A.L. Nichols, A. Nouri, O. Schwerer, A.A. Sonzogni and D.F. Winchell, presented at International Conference on Nuclear Data for Science and Technology, 27 September - 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 539-544, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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EXFOR-CINDA-ENDF: Migration of databases to give higher quality nuclear data services |
V.V. Zerkin, V. McLane, M.W. Herman and C.L. Dunford, presented at International Conference on Nuclear Data for Science and Technology, 27 September - 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Editors: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 586-589, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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Status of the international neutron cross-section standards file |
V.G. Pronyaev, S.A. Badikov, C. Zhenpeng, A.D. Carlson, E.V. Gai, G.M. Hale, F.J. Hambsch, H.M. Hofmann, N.M. Larson, D.L. Smith. S.Y. Oh, S. Tagesen and H. Vonach, presented at International Conference on Nuclear Data for Science and Technology, 27 September – 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 1 (2005) pp. 808-815, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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Recent developments of the nuclear reaction model code EMPIRE [Abstract] |
M. Herman, P.�Oblo?insk�, R. Capote, M. Sin, A. Trkov, A. Ventura and V. Zerkin, presented at International Conference on Nuclear Data for Science and Technology, 27�September ? 1�October 2004, Santa F�, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick, T. Kawano and P.�Talou, Vol. 769, Part 2 (2005) pp. 1184-1187, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
Abstract Recent extensions and improvements of the EMPIRE code system are outlined. They add to the code new
capabilities such as fission of actinides, preequilibrium emission of clusters, photo-nuclear reactions, and reactions on excited
targets. These features, along with improved ENDF formatting, exclusive spectra, and recoils make the forthcoming 2.19
release a complete tool for evaluation of nuclear data at incident energies above the resonance region | |
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Improvement of the fission channel in the EMPIRE code [Abstract] |
M. Sin, R. Capote, M. Herman, P. Oblo?insk�, A. Ventura and A. Trkov, presented at International Conference on Nuclear Data for Science and Technology, 27 September ? 1�October 2004, Santa F�, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Eds.: R.C. Haight, M.B. Chadwick,T. Kawano and P.�Talou, Vol. 769, Part 2 (2005) pp. 1249-1252, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
Abstract The new fission formalism implemented in EMPIRE-2.19 is presented along with several examples of applications
to neutron- and photon-induced fission. | |
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Review of experimental data on alpha-induced reactions on some nuclei (Mg-24, Si-28, S-32, Ar-36, Ca-40) in terms of astrophysical applications |
S.A. Dunaeva, V. McLane, M. Savin and S. Taova, presented at International Conference on Nuclear Data for Science and Technology, 27 September - 1 October 2004, Santa Fé, USA; also published in AIP Conf. Proc. - Int. Conf. on Nuclear Data for Science and Technology, Editors: R.C. Haight, M.B. Chadwick, T. Kawano and P. Talou, Vol. 769, Part 2 (2005) pp. 1386-1389, AIP, Melville, New York, ISBN 0-7354-0254-X, ISSN 0094-243X. |
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IAEA nuclear data for applications: cross section standards and the reference input parameter library (RIPL) |
R. Capote Noy, A.L. Nichols and V.G. Pronyaev, presented at Enlargement Workshop on Neutron Measurements, Evaluations and Applications, NEMEA-2, Bucharest, Romania, 20-23 October 2004, EUR 22136 EN (2005), pp. 7-16, Ed.: A.J.M. Plompen, Luxembourg, ISBN 92-894-8618-X. |
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Fission of thorium isotopes |
M. Sin, R. Capote Noy, M. Herman, P. Obložinský, A. Trkov and A. Ventura, presented at Enlargement Workshop on Neutron Measurements, Evaluations and Applications, NEMEA-2, Bucharest, Romania, 20-23 October 2004, EUR 22136 EN (2005), pp. 153-156, Ed.: A.J.M. Plompen, Luxembourg, ISBN 92-984-8618-X. |
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Neutron activation cross section measurements from threshold to 20 MeV for the validation of nuclear models and their parameters |
A.J.M. Plompen, D.L. Smith, R. Capote et al., A report by the Working Party on International Evaluation Co‑operation of the NEANuclear Science Committee (WPEC-19), NEA/WPEC-19, OECD, Paris, 2005, ISBN 92-64-01070. |
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Nuclear data services of the International Atomic Energy Agency: an overview |
A.L. Nichols, L. Costello and V.V. Zerkin (invited paper), presented at DAE-BRNS National Workshop on Nuclear Data for Reactor Technology and Fuel Cycle, 7-10 March 2005, Bhabha Atomic Research Centre (BARC), Trombay, Mumbai, India. |
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Nuclear databases for energy applications: an IAEA perspective |
R. Capote-Noy, A.L. Nichols and A. Trkov, presented at Int. Workshop on Nuclear Data Needs for Generation IV Nuclear Energy Systems, Antwerp, Belgium, 5-7 April 2005; pp. 244-252 in Proc. Int. Workshop on Nuclear Data Needs for Generation IV Nuclear Energy Systems, Ed. P. Rullhusen (2006), World Scientific, Singapore, ISBN 981-256-830-1. |
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IAEA Coordinated Research Project on fission product yield data for minor actinides up to 150 MeV |
M. Lammer and A.L. Nichols, presented at 3rd International Workshop on Nuclear Fission and Fission-product Spectroscopy, Fission 2005, 11-14 May 2005, Cadarache, France; also published in AIP Conf. Proc. – 3rd Int. Workshop on Nuclear Fission and Fission-product Spectroscopy, Eds.: H. Goutte, H. Faust, G. Fioni and D. Goutte, Vol. 798 (2005) pp. 285-293, AIP, Melville, New York, ISBN 0-7354-0288-4, ISSN 0094-243X. |
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Nuclear decay data: observations and reflections |
A.L. Nichols (invited paper), presented at 15th Int. Conf. on Radionuclide Metrology and its Applications (ICRM 2005), 5-9 September 2005, Oxford, UK; also published in Appl. Radiat. Isot., 64 (2006) pp. 1384-1391. |
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Revisiting the U-238 thermal capture cross section and gamma-ray emission probabilities from Np-239 decay |
A. Trkov, G.L. Molnár, Zs. Révay, S.F. Mughabghab, R.B. Firestone, V.G. Pronyaev, A.L. Nichols and M.C. Moxon, Nucl. Sci. Eng. 150 (2005) pp. 336-348. |
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Status and perspective of nuclear data production, evaluation and validation [Abstract] |
A. Trkov (invited paper), Nucl. Eng. Technol. 37 (2005) pp. 11-24. |
Abstract A very important feature in the development of nuclear technology has been and will continue to be the flow of information
from nuclear data production to the various applications fields in nuclear technology. Both, nuclear data and this
communications flow are defined in this paper. Nuclear data result from specific technical activities including their production,
evaluation, processing, verification, validation and applications. These activities are described, focusing on nuclear
reactor calculations. Mathematical definitions of different types of nuclear data are introduced, and international forums
involved in nuclear data activities are listed. Electronic links to various sources of information available on the web are
specified, whenever possible | |
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Level densities of transitional Sm nuclei |
R. Capote, A. Ventura, F. Cannata and J. M. Quesada, Phys. Rev. C71 (2005) 064320. |
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Dispersive coupled channel analysis of nucleon scattering from Th-232 up to 200 MeV |
E.Sh. Soukhovitskii, R. Capote, J.M. Quesada and S. Chiba, Phys. Rev. C72 (2005) 024604. |
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Micro ionization chamber dosimetry in IMRT verification: clinical implications of dosimetric errors in the PTV |
F. Sánchez-Doblado, R. Capote, J.V. Roselló, A. Leal,J.I. Lagares, R. Arráns and G.H. Hartmann, Radiother. Oncol. 75 (2005) pp. 342-348. |
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Nuclear reaction and structure data services of the National Nuclear Data Center |
B. Pritychenko, A.A. Sonzogni, D.F. Winchell, V.V. Zerkin, R. Arcilla, T.W. Burrows, C.L. Dunford, M.W. Herman, V. McLane, P. Obložinský, Y. Sunborn and J.K. Tuli, Ann. Nucl. Energy 33 (2006) pp. 390-399. |
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Simulation of an end-of cycle trip transient with the LOADF code package |
M. Bo?i? and A. Trkov, Int. Conf. Nuclear Energy for New Europe 2005, Bled, Slovenia, 5-8 September 2005. |
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Neutron capture reaction rates for stellar nucleosynthesis |
A. Mengoni, published in Proc. 20th Int. Conf. on Capture Gamma-ray Spectroscopy and Related Topics, University of Notre Dame, Indiana, USA, 4-9 September 2005. |
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Is a global coupled-channel dispersive optical model potential for actinides feasible? |
R. Capote, E.Sh. Soukhovitski, J.M. Quesada and S. Chiba, Phys. Rev. C72 (2005) 064610. |
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Neutron capture cross section measurements for nuclear astrophysics at CERN n-TOF |
U. Annondanno, R. Capote, A. Mengoni et al., (the n-TOF Collaboration), Nucl. Phys. A758 (2005) pp. 501-504. |
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Measurement of the Sm-151(n,γ) cross section at n_TOF |
S. Marrone, R. Capote, A. Mengoni, et al., (the n-TOF Collaboration), Nucl. Phys. A758 (2005) pp. 533-536. |
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Measurement of the Zr-90,91,92,94,96(n,γ) cross sections at n_TOF |
G. Tagliente, R. Capote, A. Mengoni et al., (the n-TOF Collaboration), Nucl. Phys. A758 (2005) pp. 573-576. |
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Stellar neutron capture rates of C-14 |
R. Reifarth, A. Mengoni et al., Nucl. Phys. A578 (2005) pp. 787-790. |
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Nuclear data requirements for decay heat calculations |
A.L. Nichols, pp. 65-69 in Lecture Notes, Vol. 20, Workshop on Nuclear Reaction Data and Nuclear Reactors: Physics, Design and Safety, 25 February – 28 March 2002, The Abdus Salam International Centre for Theoretical Physics, Eds.: M. Herman, N. Paver, ICTP Publ., Trieste, Italy, 2005. |
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Higher Landau levels contribution to the energy of interacting electrons in a quantum dot |
A. Gonzalez, J.D. Serna, R. Capote and G. Avendaño, Physica E30 (2005) pp. 134-137. |
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Laser-generated nanosecond pulsed neutron sources: scaling from VULCAN to table-top |
T. Zagar, J. Galy, J. Magill and M. Kellett, New J. Phys.7 (2005) pp. 2-13. |
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